Thoron Activity Concentrations Research Articles

New-designed measurement device for radon and thoron activity concentration based on gas direct detection

A new-designed measurement device for radon and thoron activity concentration is developed based on gas direct measurement to support their in-situ calibration. It consists of a 2000 mm2 Passivated Implanted Planar Silicon (PIPS) detector, a Multi-Channel Analyzer (MCA), a Micro Controller Unit (MCU), and a small electrostatic chamber with a volume of nearly 23 ml. The device records those alpha particles emitted from radon and thoron gas, and the detection efficiency and the crosstalk factor of 218Po/216Po are determined by Monte Carlo simulation. Measurement results have been compared with AlphaGUARD DF2000 in pure radon and thoron environments, respectively. Results show that the measurement results of the devices and the reference monitor agree well with each other, with an average relative deviation of 0.48% for radon gas from about 3300 Bq/m3 to 38 kBq/m3 and -3.25% for thoron gas from about 25 kBq/m3 to 70 kBq/m3. Uncertainty assessment has also been done, and a relative system uncertainty of radon is about 6.8%, while that of thoron is nearly 7.3%.

Radon and thoron activity concentration in soil gas of Johor state: a statistical relationship with proxies

Radon and thoron activity concentration in soil gas of Johor state: a statistical relationship with proxies

Impact of humidity and flowrate on the thoron measurement sensitivity of electrostatic radon monitors

The accurate measurement of thoron activity concentration is an important issue in both thoron exposure evaluation and in reducing its influence on radon measurement. For radon monitors based on electrostatic collection technique and an alpha spectrometry analyser, air humidity and sampling flowrate are key factors influencing the sensitivity of thoron activity concentration measurement. For the purpose of improving thoron measurement sensitivity and stability, theoretical derivation and experimental studies were systemically performed in this study. The results show that thoron measurement sensitivity decreases as a negative exponential function with absolute humidity increasing, and the sensitivity of thoron is much lower than that of radon under the same conditions, which is mainly caused by the small value of the concentration ratio of thoron inside to outside of the chamber. When the air exchange rate of the measurement chamber (sampling flowrate/inner volume) increases, the measurement sensitivity of thoron gas first increases rapidly and then decreases slowly after reaching its maximum at the air exchange rate of 0.24 s−1. In practice, in the normal air exchange rate range (for example <0.05 s−1), increasing the sampling flowrate could greatly improve the thoron measurement sensitivity, which consequently suggests an effective way to update thoron measurement under the present conditions of the monitor.

Pilot Study of Thoron Concentration in an Underground Thorium Mine.

The Steenkampskraal mine in the Western Cape Province in South Africa provides some interesting challenges for radiation protection practitioners in view of the high thoron values encountered in this mine. The mine contains high natural thorium concentrations that lead to high thoron activity concentrations, as will be shown in this paper. The influence of ventilation has been studied, and the source term has been investigated by considering the thorium content of the rocks and the thoron exhalation. The thoron activity concentrations are around 10 kBq m -3 at a monazite seam, and the thorium exhalation is consistent with these levels. The thoron concentrations can be reduced by ventilation but not eliminated. However, the thoron progeny can probably be reduced dramatically. Issues that affect the thoron levels are also discussed. Further studies are needed, but the thoron may well not be a radiation protection problem despite the high thoron concentrations.

Thoron activity concentration in Malaysian soil gas: Geogenic impact assessment

Given the rather short half-life of thoron (220Rn), at 56 s, its contribution to radiation exposure is often overlooked. Nevertheless, in a thorium (232Th) rich environment potential hazard does exist, in particular regarding prolonged duration exposures to 220Rn and its short-lived alpha-particle emitting progeny [polonium (216Po)]. Herein, concerning the geology and major soil types in the Malaysian state of Perak, an activity concentration map has been established for 220Rn in soil gas, with the use made of a RAD7 detector and the THORON protocol for in-situ measurements. The detector has been coupled to a soil probe driven to a depth of 0.8 m. The activity concentration of 220Rn in the soil ranged from undetectable to 563 kBq m−3 with a mean value of 38 ± 11 kBq m−3. Granite and Triassic-Jurassic formations in the region showed more elevated 220Rn activity while Quaternary and Silurian formations revealed low 220Rn values. Moreover, while elevated 220Rn activity concentrations were found in peat, riverine, and granite source soils, the activity concentrations in marine and other soils were low. A primary map of 220Rn in the soil gas has been developed based on geogenic impact assessment, with a greater 220Rn activity concentration in the central part of the state.

Radiological assessment subjected to outdoor radon and thoron concentrations and terrestrial gamma radiation measurements in Perak Malaysia

The concentrations of radon, thoron and terrestrial gamma radiation were measured to evaluate the outdoor effective dose. The outdoor radon activity concentration ranged from 5.79 to 5110 ± 46.36 Bq m−3, with a mean of 320.03 Bq m−3 which is higher than the EPA level of 14.8 Bq m−3. The range of the thoron activity concentration outdoor was from 0.00 to 4226.7 ± 58.5 Bq m−3, with a mean of 226.1 Bq m−3 which was above the UNSCEAR recommended level of 10 Bq m−3. The terrestrial gamma radiation dose rates range was from 98.31 to 3769.71 nGy h−1 with a mean of 446.27 nGy h−1. The effective dose contribution from radon exposures in the study was estimated to be 3.2 ± 0.5 mSv y−1 is about 84% total annual effective dose received by the population in those areas. The estimated thoron and gamma dose contributions (15%, and 1% respectively) were not significant. The outdoor doses for thoron and gamma were lower than the ICRP (2007) value of 1 mSv. The total annual outdoor effective dose with an occupancy factor of 1825 h (5 h day−1) was estimated to be within the range of 0.30–551.41 ± 0.65 mSv, with a mean of 3.75 mSv which is a little higher than the world average of 2.4 mSv.

Long-Term Measurements of Radon and Thoron Exhalation Rates from the Ground Using the Vertical Distributions of Their Activity Concentrations.

A long-term measurement technique of radon exhalation rate was previously developed using a passive type radon and thoron discriminative monitor and a ventilated type accumulation chamber. In the present study, this technique was applied to evaluate the thoron exhalation rate as well, and long-term measurements of radon and thoron exhalation rates were conducted for four years in Gifu Prefecture. The ventilated type accumulation chamber (0.8 × 0.8 × 1.0 m3) with an open bottom was embedded 15 cm into the ground. The vertical distributions of radon and thoron activity concentrations from the ground were obtained using passive type radon-thoron discriminative monitors (RADUETs). The RADUETs were placed at 1, 3, 10, 30, and 80 cm above the ground inside the accumulation chamber. The measurements were conducted from autumn 2014 to autumn 2018. These long-term results were found to be in good agreement with the values obtained by another methodology. The radon exhalation rates from the ground showed a clearly seasonal variation. Similar to findings of previous studies, radon exhalation rates from summer to autumn were relatively higher than those from winter to spring. In contrast, thoron exhalation rates were not found to show seasonal variation.

Development and calibration of a method for direct measurement of 220Rn (thoron) activity concentration

The interest in the measurement of thoron (220Rn) activity concentration in air has recently increased, with the attention for the development of standards useful for the calibration of measuring instruments. Due to its short half-life (55.8 s), consolidated techniques for the realization and the use of controlled atmospheres of radon (222Rn) are not effective in the case of thoron. New adequate methodology are required. A method for the measurement of the thoron reference activity based on the direct detection of the alpha particles produced by the decay of 220Rn, from natural samples containing 232Th, is here proposed. The possibility of observing an acceptable spectrum is entrusted to the realization of measurement chambers small enough to reduce as much as possible the energy loss of the alpha particles before they reach the Silicon detector. Such a chamber was realized and used with a known thoron atmosphere in a controlled environment. The experimental results are compared with those obtained from the simulation with the Monte Carlo method: (i) the alpha spectra coming directly from thoron atoms exhibit similar shape with a linear trend plus an exponential trend on the left side of the 220Rn peak, depending from the distance between source and detector; (ii) the corresponding 220Rn detection efficiency values are compatible considering the uncertainties. An investigation was conducted to study the shape of the 220Rn spectra vs the different volume of chambers, through Monte Carlo simulations. The results show: (i) the linear part of the spectra shape goes to reduce with the increasing of the height of the chamber; (ii) the 220Rn detection efficiency decreases with the increasing of the height of the chamber.

Using a scale model room to assess the contribution of building material of volcanic origin to indoor radon

Abstract In the frame of Radon rEal time monitoring System and Proactive Indoor Remediation (RESPIRE), a LIFE 2016 project funded by the European Commission, the contribution of building materials of volcanic origin to indoor radon concentration was investigated. First, total gamma radiation and related outdoor dose rates of geological materials in the Caprarola area (Central Italy) were measured to define main sources of radiation. Second, 222Rn and 220Rn exhalation rates of these rocks used as building materials were measured using an accumulation chamber connected in a closed loop with a RAD7 radon monitor. Among others, the very porous “Tufo di Gallese” ignimbrite provided the highest values. This material was then used to construct a scale model room of 62 cm × 50 cm × 35 cm (inner length × width × height, respectively) to assess experimental radon and thoron activity concentration at equilibrium and study the effects of climatic conditions and different coatings on radon levels. A first test was carried out at ambient temperature to determine experimental 222Rn and 220Rn equilibrium activities in the model room, not covered with plaster or other coating materials. Experimental 222Rn equilibrium was recorded in just two days demonstrating that the room “breaths”, exchanging air with the outdoor environment. This determines a dilution of indoor radon concentration. Other experiments showed that inner covers (such as plasterboard and different kinds of paints) partially influence 222Rn but entirely cut the short-lived 220Rn. Finally, decreases in ambient temperature reduce radon exhalation from building material and, in turn, indoor activity concentration.

Radon and thoron radiation exposure of the Angolan population living in adobe houses

This study investigates radon and thoron activity concentrations in adobe houses of Angola. Activity concentrations were recorded by passive detectors in rainy and dry seasons in 40 dwellings located at three areas with different climatic and geological backgrounds (Cabinda, Huambo, Menongue). Regarding seasonal and spatial variations, radon activity concentrations are higher in the rainy than in the dry season and both radon and thoron levels are the highest in Huambo, the central part of the country. The number of adobe houses above certain radon and thoron levels were estimated and the contribution of thoron to the inhalation dose was significant.

INDOOR RADON AND THORON IN THE VICINITY OF PROPOSED URANIUM MINING SITE: A CASE STUDY AT DASARLAPALLY VILLAGE, TELANGANA STATE, INDIA

Studies are being conducted for the past few decades in and around the uranium mining sites across the globe to identify environmental nuclear radiation risk to the common public. The area near Dasarlapally village was identified for uranium exploration by the AMDER, Hyderabad. The present study was carried out to measure the indoor radon and thoron activity concentrations in the dwellings of Dasarlapally village. For this purpose different types of dwellings were chosen randomly across the village. The measured annual average concentration of radon and thoron in dwellings were found to be 141±42 and 139±77 Bqm-3, respectively, and the calculated annual effective inhalation dose due to radon was determined to be 3.5mSv. Seasonal variation and diurnal variation of radon and thoron activity concentration were investigated. The variation of radon and thoron activity concentration in different types of dwellings was also studied, and the variation was found to be statistically insignificant. The uncertainty propagated in the effective inhalation dose due to thoron was discussed.

RADON, THORON AND THEIR PROGENY DISTRIBUTION AND ESTIMATION OF ANNUAL EFFECTIVE DOSE AND EXCESS LIFETIME CANCER RISK IN PANATHADY, KASARAGOD DISTRICT, KERALA.

Radon and thoron are natural radioactive gases that tend to accumulate in the indoor environment and one of their major health implications is the ability to cause lung cancer. Present study comprises the quantification of radon and thoron activity concentrations and measurement of gamma exposure rates in different types of dwellings from the endosulfan-affected area, Panathady, Kasaragod district, Kerala. It is observed that, residents of this area were more prone to various diseases and health problems including cancer. The LR-115 type II solid state nuclear track detectors with single entry pin-hole based dosemeters have been used for the measurement of 222Radon and 220Rn activity concentrations. The assessment of radiological parameters such as annual effective doses and excess lifetime cancer risk has also been done in order to understand the dose level and the associated risk. The estimated values have been compared with the limit recommended by the United Nations Scientific Committee on the Effects of Atomic Radiation (UNSCEAR) and International Commission on Radiological Protection (ICRP). The average indoor radon and thoron activity concentrations observed in these dwellings were 134±30 and 111±28Bqm-3, respectively. The estimated activity concentrations, effective doses, etc. are found to be within the recommended level by the UNSCEAR or ICRP.

Thoron standard source

Thoron (220Rn) has been identified as a possible health concern in specific places such as monazite processing plants and (rare-earth) mines. The short half-life of thoron (55.8 s) makes thoron calibration sources and thoron chambers less common than the corresponding radon (222Rn) ones. In this paper an inexpensive and straight forward but accurate thoron source is described that can easily be set up in typical nuclear environmental laboratories. The source of thoron is a solution of Th(NO3)4 in water. Thoron is extracted by bubbling air through the solution using an aerator. The gamma rays from the solution are measured at the same time. The thoron activity concentration in the exit stream follows from the reduction in the intensity of the gamma rays from the progeny of thoron over time.

ASSESSMENT OF ANNUAL EFFECTIVE DOSE FROM EXPOSURE TO NATURAL RADIOACTIVITY SOURCES IN A CASE-CONTROL STUDY IN BIHOR COUNTY, ROMANIA.

The purpose of the article is to evaluate the annual effective dose for 80 women divided into two samples; one sample located in the former uranium Băiţa-Ştei area, hereinafter referred to as case sample, respectively for a control sample, located in the same county, but exposed in most cases to indoor radon activity concentrations <300 Bq m-3. In this regard, the homemade 'RaThoGamma' kit was used, which contained two thermoluminescent dosimeters, a CR-39 track detector (RSKS) for indoor radon activity concentration, two CR-39 track detectors (Radtrak2®/ Radtrak2T®) for radon and thoron activity concentrations as well as Direct Radon Progeny Sensors/Direct Thoron Progeny Sensors for measuring time-averaged radon and thoron progenies concentrations. In addition, a total of 80 water samples were collected in order to evaluate the ingestion dose due to radon and radium activity concentrations in drinking water. The maximum total annual effective dose in the control sample was 14.1 mSv, while in the case sample the maximum annual effective dose was 60.5 mSv. This difference is mainly due to radon progenies inhalation. Other pathways did not show a statistically significant difference between the two samples, showing a minor contribution to the annual effective dose.

The experimental study on the emanation power of a flow-through thoron source made from incandescent gas mantles

To improve the quality of the calibration of thoron concentration activity measurement, an experimental study on the emanation power of a flow-through thoron source based on incandescent gas mantles was carried out in this paper. The thoron activity concentrations of the outflowed air from the flow-through source were measured using RAD7, and the quantitative relationship between thoron concentrations and flowrates was studied through theoretical analysis, and the thoron emanation powers were obtained from the fitting of the relationship above. Results show that the thoron concentration decreased with the increasing flowrate in the gas path, and the thoron emanation powers of three batches of gas mantles obtained by fitting were 1.33% ± 0.17%, 0.77% ± 0.10% and 0.57% ± 0.07% respectively in low humidity condition. Those results were checked using the gamma spectroscopy method, and were consistent within the error range.

Indoor radon and thoron concentrations in some towns of central and South Serbia

This study presents the results of indoor radon and thoron activity concentrations of some municipalities in central and south part of Serbia: Krusevac, Brus, Blace and Kursumlija. Measurements were carried out in 60 dwellings during the winter season. Passive discriminative radon-thoron detectors known as UFO detectors were used. The mean values of indoor radon and thoron concentrations were 82 Bq m−3 and 42 Bq m−3, respectively. Population-weighted mean values were 76 Bq m−3 and 40 Bq m−3, respectively. 26.7% of dwellings had radon concentration higher than 100 Bq m−3 (one location had even more than 300 Bq m−3). There are no statistically significant correlations of indoor radon and thoron concentrations neither with the period of house construction, nor with the existence of a basement. The results of this study represent the first step of investigating radon and thoron levels in these parts of Serbia and therefore could be the basis for creating a radon map.

Study on Seasonal Variation of Indoor Radon, Thoron and their Progeny Levels in Belur and Channarayapatna Taluks of Hassan District, Karnataka State, India

Seasonal variation of indoor radon, thoron and their progeny concentrations have been measured in different types of buildings at different locations of Belur and Channarayapatna taluks using time integrated passive radon dosimeters containing LR-115 Type II solid state nuclear track detector. The average radon and thoron activity concentrations, their progeny levels, life time fatality risk and annual effective dose due to radon and thoron were estimated in summer, rainy, autumn and winter seasons. A detail analysis of radon and thoron distribution in twenty different houses with seasonal variation is presented in this paper. In general, the levels of radon and thoron concentration were observed to be highest in winter and lowest in summer

A new thoron atmosphere reference measurement system

A new thoron reference (220Rn) in air measurement system is developed at the LNE-LNHB with the collaboration of the IRSN. This measurement system is based on a reference volume with an alpha detector which is able to directly measure thoron and its decay products at atmospheric pressure. In order to improve the spectrum quality of the thoron progenies, we have applied an electric field to catch the decay products on the detector surface. The developed system is a portative device which can be used to measure reference thoron atmosphere such as the BACCARA chamber at IRSN (Picolo et al., 1999). As this system also allows the measurement of radon (222Rn) in air, it was validated using the radon primary standards made at the LNE-LNHB. This thoron measurement system will be used, at IRSN, as a reference instrument in order to calibrate the thoron activity concentration in the BACCARA facility.

Diffuse surface emanations as indicator of structural permeability in fault-controlled geothermal systems

Diffuse degassing processes provide valuable information on geothermal reservoir characteristics not only in the context of monitoring, but also for exploration purposes. Areas with increased gas emissions can be indicative of major upflow zones from the reservoir through deep-reaching, permeable fault zones. These fault zones may act as preferential target areas for geothermal production drillings. In this study it is successfully demonstrated that diffuse degassing measurements can be used for the detection and characterization of permeable structural elements. The combination of following techniques has been applied at the Brady's geothermal system in the Basin-and-Range Province (Nevada, USA): accumulation chamber method for carbon dioxide and hydrogen sulfide measurements, alpha-spectroscopic measurements of radon and thoron activity concentrations, and gamma-spectroscopic measurements of selected nuclides.

Estimation of radon and thoron caused dose at exraction and processing sites of mineral sand mining area in Vietnam (HA TINH province)

Mineral sands are mined in several countries to supply to the titanium and zircon producing industries. Coastal black mineral sands usually contain, besides ilmenite (FeTiO3) and rutile (TiO2), radioactive minerals such as zircon (ZrSiO4) and monazite (RePO4). Radon and thoron activity concentration originated from natural radioactive contents of the black mineral sand was monitored at the extraction and processing for black minerals in the coastal areas of Ha Tinh Province, one of the around 40 coastal mineral sand deposits in Vietnam. The survey was carried out with the Raduet chambers made by Radosys Ltd—Hungary. The obtained results for 25 investigated points show that the measured values are not high in the residential houses and in case of the sand extraction site as well. At the titanium processing plant the measured values were higher than outside the facility (Radon: 18–55 Bq/m3 with average of 34 Bq/3 and Thoron 33–118 Bq/m3 with average of 58 Bq/m3) but still comparable to the average concentration of the world published by UNSCEAR. The typical outdoor levels of radon and thoron gas are each of the order of 10 Bq/m3. Although the radon concentrations were low in the zircon and titanium processing plants, the thoron concentrations in the houses for separating rutile and zircon were very high. At zircon processing factory, the thoron concentration could reach 2,931 Bq/m3 and the estimated annual effective dose would be 21.4 mSv/a. Intervention has to be taken in order to reduce the thoron level in this factory since the level of thoron and its progenies corresponding to an annual occupational effective dose is beyond the action level of 6 mSv/a.