Thin Foils Research Articles

Femtosecond Dynamics of Fast Electron Pulses in Relativistic Laser-Foil Interactions.

We report the femtosecond time-resolved dynamics of relativistic electron pulses in ultraintense laser-foil interactions, by characterizing the terahertz self-radiation with single-shot ultrabroadband interferometry. Experimental measurements together with theoretical modeling reveal that the electron pulses inherit the duration of the driving laser pulse. We also visualize the electron recirculation dynamics, where electrons remain trapped inside the self-generated electrostatic potential well and rebound back and forth around the thin foil for hundreds of femtoseconds. Our results not only demonstrate an insitu, real-time metrology scheme for electron bursts, but also have important implications for understanding and manipulating the time-domain properties of laser-driven particle and radiation sources.

Curing of epoxy adhesives between thin metal foils by means of inductive heating

Metal foils are being widely used, from the chemical or electronics sector to household appliances. The joining of these foils by adhesive bonding is often the preferred method due to discolouring and warping under the thermal stresses of other joining methods, such as welding. However, long curing times are a disadvantage of adhesive bonding compared to welding. The use of electromagnetic induction is a promising solution for accelerated curing. This work investigates induction heating for accelerated curing of 1-C epoxy adhesives for bonding of thin nickel foils. Process parameters for rapid curing of the adhesives were determined based on reaction kinetics using differential scanning calorimetry measurements. According to those results peel test specimens were fabricated, and the peel resistance was evaluated using a 90° peel load.

High-temperature treatment of functional Heusler alloy Ni46Mn41In13 thin foils for microsystem devices and electronics

In this study, the high-temperature transformation in a thin foil of non-stoichiometric Heusler alloy based on Ni-Mn-In is investigated using in-situ TEM. The highly ordered cubic L21 phase undergoes decomposition upon heating, forming a phase with a composition close to Ni75Mn25, which is identified as disordered FCC-Ni3Mn and secondary phases, mainly manganese oxides and sulfides. All phases formed upon heating to a temperature of 1173 K are preserved during the in-situ cooling experiment to a temperature of 123 K.

Novel device to study double-alpha decay at the FRS Ion Catcher

A novel system has been developed to detect simultaneous double-alpha emission from purified and weightless sources. The system includes the collection of 224Ra low-energy recoils in purified helium buffer gas from the decay of 228Th. The recoil products are thermalized and collected in a cryogenic buffer gas cell and extracted into an RF-ion guide for mass selection. The mass-separated ions are implanted at low kinetic energy into a thin carbon foil placed between two large-area double-sided silicon strip detectors to observe correlated alpha-particle emission. The apparatus is described in detail, including insights into its experimental performance.

Local Heat Transfer Distribution On Thin Metal Foil Impinged by Array of Free Surface Jets

Abstract The present study focuses on the measurement of the local heat transfer distribution of a smooth flat plate impinged by an array of free surface jets on a thin metal foil. Local Nusselt number distributions are measured for a fixed jet diameter (d = 3 mm). The jet arrays consist of perfectly round apertures arranged in a square pattern, with a uniform spacing of 4d between adjacent jets in both the streamwise and spanwise direction. A wide range of Reynolds numbers varying from 1000 to 12500 are covered in this study. The nozzle to plate spacing (z/d) is varied between 1 to 10. The effect of the Reynolds number and nozzle to plate spacing on the local and spanwise average Nusselt number distributions are studied. The local Nusselt number exhibits an increase with nozzle-to-plate spacing within the low Reynolds number range (Re = 1000 to 2500). However, for Reynolds numbers exceeding 2500, the influence of nozzle-to-plate spacing on Nusselt number distributions remains negligible up to a nozzle-to-plate distance (z/d) of 5. Beyond this point, there is a gradual decrease in the Nusselt number value. The Nusselt number value gradually decreases beyond z/d of 5. At a Reynolds number of 1500, the Nusselt number increases by 71% for z/d = 10 in comparison to z/d = 1. Empirical correlations for local and spanwise average Nusselt number are proposed which satisfactory predict the local as well as spanwise average Nusselt number distributions.

Homogenization of foil windings with globally supported polynomial shape functions

In conventional finite element simulations, foil windings with thin foils and with a large number of turns require many mesh elements. This renders models quickly computationally infeasible. This paper uses a homogenized foil winding model and approximates the voltage distribution in the foil winding domain by globally supported polynomials. This way, the small-scale structure in the foil winding domain does not have to be resolved by the finite element mesh. The method is validated successfully for a stand-alone foil winding example and for a pot inductor example. Moreover, a transformer equipped with a foil winding at its primary side is simulated using a field-circuit coupled model.

Spontaneous Skyrmion Bubbles in an Iron-Silicon Alloy with Uniaxial Magnetic Anisotropy.

The magnetic skyrmions exhibit intriguing topological behaviors, holding promise for future applications in the realm of spintronic devices. Despite recent advancements, achieving spontaneous magnetic skyrmions and topological transitions in magnets featuring uniaxial magnetic anisotropy, particularly at elevated temperatures (>100 K), remains a challenging endeavor. Here, single-crystal Fe5Si3 nanorods with the central symmetry and uniaxial magnetic anisotropy were successfully synthesized on a mica substrate through chemical vapor deposition, which exhibit a high Curie temperature (TC) of about 372 K. The real-time observation, facilitated by Lorentz transmission electron microscopy, revealed the spontaneous formation of magnetic skyrmions and evolution of domains in focused ion beam-prepared Fe5Si3 thin foils. Moreover, Fe5Si3 device transport measurements expose notable magnetoresistance (MR) effects, enabling the interchange between positive and negative MR across specific temperature settings. These results offer various potential avenues for exploring diverse topological spin textures and their formation mechanisms, indicating inventive applications for iron-silicon alloy in the realm of spintronics.

In-situ formation of quasi-solid polymer electrolyte for wide-temperature applicable Li-metal batteries

As next-generation rechargeable batteries, the development of solid-state lithium-metal batteries (LMBs) in a multitude of applications is confronted with a trade-off between high energy density, safety, and wide-temperature tolerance. Especially in cold climates, their applications are challenged by insufficient dynamics in bulk electrolyte and at electrode/electrolyte interface. Herein, a flexible, highly ionic conductive, and low-temperature applicable quasi-solid polymer electrolyte (QSPE) is designed and fabricated, which achieves a stable Li-metal anode over a wide-temperature range (−20 ∼ 60 °C). The QSPEs prepared via in-situ polymerization of polyethylene glycol (PEO)-based monomers in low-melting solvent (1,3-dioxolane (DOL) or ethyl difluoroacetate (EDFA)) endow low-temperature tolerance, prominent ionic conductivity (4.5 × 10−4 S cm−1 at −20 °C) and exceptional electrochemical performance over a wide-temperature range. Consequently, with the DOL-based QSPE (D-QSPE), the Li/D-QSPE/LiFePO4 cell presents stable, long-term cycling at −20 °C (minimal capacity degradation over 550 cycles) and excellent fast-charging capacity (capacity retention of 81 % over 1300 cycles at 5 C). Even utilizing a thin lithium foil (25 μm) and a high mass loading LiFePO4 cathode (2.5 mAh cm−2), the assembled Li/LFP cell with a N/P ratio of 1.96 still exhibits good cycling performance at −20 °C. Additionally, the EDFA-based QSPE (E-QSPE) allows LMBs with NCM811 cathodes cycling over 140 cycles (capacity retention > 95 %) at −20 °C. With the capability of circumventing sluggish ion transport kinetics of quasi-solid polymer LMBs in cold climates, the developed polymer electrolyte provides new pathways for safe, high-capability, and wide-temperature operable batteries.

Cu-based thin rolled foils: relationship among alloy composition, micromechanical and antiviral properties against SARS-CoV-2

The healthcare-associated infections (HAIs) and pandemics caused by multidrug-resistant (MDR) and new-generation pathogens threaten the whole world community. Cu and its alloys have been attracting widespread interest as anti-contamination materials due to the rapid inactivation of MDR-superbugs and viruses. Applying thin Cu-based foils on pre-existing surfaces in hygiene-sensitive areas represents a quick, simple, cost-effective self-sanitising practice. However, the influence of chemical composition and microstructure should be deeply investigated when evaluating the antimicrobial capability and durability of Cu-based materials. The effect of composition on micromechanical and antiviral properties was investigated by comparing Cu15Zn and Cu18Ni20Zn (foil thickness from 13 to 27 μm) with Phosphorous High-Conductivity (PHC) Cu. The influence of recrystallisation annealing of PHC Cu was also investigated. Microstructural characterisation was carried out by optical (OM) and scanning electron (FEG-SEM) microscopy, Energy-dispersive Spectroscopy (EDS) and Electron-Backscattered Diffraction (EBSD). The micromechanical behaviour was assessed by microhardness, microscale abrasion and scratch tests. Cu-based foils were exposed to SARS-CoV-2 for different time points in quasi-dry conditions (artificial sweat solution), evaluating their antiviral capability by quantitative Reverse-Transcriptase Polymerase Chain Reaction (qRT-PCR). Surface morphology, contact angle measurements and Cu release were measured. All Cu-based surfaces completely inactivated SARS-CoV-2 in 10 min: pure Cu was the best option regarding antiviral efficiency, while Cu15Zn showed the best trade-off between micromechanical and antiviral properties.

Comparative study of ion milling techniques for the preparation of ceramic fibers in transmission electron microscopy

Sample preparation, essential to any analysis, remains an under-documented step. Preparation methods for transmission electron microscopy (TEM) are complex and lead to artifacts that need to be identified to avoid wrong conclusions about the sample's microstructure. Ion milling techniques are increasingly becoming the reference techniques to prepare thin foils. The possibilities of different ion beam processes for milling samples will be shown and compared, using ceramic carbon/carbide fibers, a material applied in many industrial applications, as a test specimen. This overview of ion milling preparation techniques will enable us to identify the advantages, disadvantages and parameters in order to best prepare these thin samples. It will be carried out for the community, and will also highlight a new preparation method for ceramic fibers to minimize the artefacts inherent in these techniques.

Feasibility analysis for the application of conduction tracks on textiles by means of laser radiation

Textiles are not only used for clothing but also have found applications in many other areas. Textiles fulfilling functional or technical properties are called “technical textiles.” Incorporation of conductive components, sensors, or materials reacting to environmental influences convert those into so-called “smart textiles.” Common methods of applying conductive tracks to textiles are embroidery, which can cause damage to the textile, or printing of a low-conductivity paste that may include toxic chemicals. A new method of applying electrical conductors to textiles for contacting is laser welding. In this process, a thin metal foil is welded on locally with an absorber placed above the metal foil to ensure that sufficient energy is applied to partially melt the textile underneath the metal foil. One variant for welding conductive tracks is the use of a globo-optics and a diode laser system with a wavelength of 975 nm. With these optics, the glass sphere focuses the laser beam and serves as a mechanical pressure tool for achieving a zero gap between fabric and foil. Parameters that are varied are the processing speed and the laser power receiving different track widths, as well as the type of textile. In this work, their influence is evaluated by microscopy, electrical resistance measurements during Martindale tests for abrasion resistance, and tensile tests. The investigations clarify the durability and utility of welded conductive tracks on textiles. It is possible to produce conductive tracks out of beaten copper joined on textiles using laser radiation showing conductivity after 10,000 abrasion cycles. The tensile strength of textiles totally made of thermoplastics is more influenced by the heat input of the laser than blended textiles, but their abrasion resistance is worse. Furthermore, an outlook on the possibility of welding using a laser source with a wavelength of 450 nm (blue laser) and a scanner as optics will be given.

Directional-sensitive wide field-of-view monitoring of high-intensity proton beams by spectral tracking of scattered particles with scattering foil and miniaturized radiation camera

Monitoring and characterization of particle beams in wide-range is often necessary in research and many applications with particle accelerators. The quantitative measurement and evaluation of composition especially of high-intensity beams are limited and can become a challenge with conventional methods especially with simplified instrumentation for ease of deployment. For this purpose, we developed a novel technique based on high-resolution spectral-sensitive tracking of single particles scattered from the beam path by a thin foil. We use a compact radiation camera equipped with the semiconductor pixel detector Timepix3 together with dedicated Monte-Carlo simulations. Particle-event type discrimination and directional information are produced by the detector spectral-tracking response together with particle-type resolving power derived from experimental calibrations. Directional- and spectral-sensitive components can be resolved in wide field-of-view. Quantification of the primary beam intensity is extrapolated by numerical calculations. Demonstration and evaluation of the technique are provided by measurements with 33 MeV protons from a light ion cyclotron accelerator.Scattered particles originating from the thin foil, the accelerator beam nozzle, and the air space along the beam path are detected and evaluated.

Generation of Terahertz Radiation by Relativistic Laser Pulses on the Surface of Thick Solid Targets and Thin Foils

Terahertz pulse generation from multiterawatt laser surface plasma near thick solid targets and thin foils has been studied. Pulses with energies up to 7 μJ were detected in the spectral region <3 THz in the direction of specular reflection from the surface of the CaF2 target. The dependence of the terahertz pulse energy \\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$${{W}_{{{\ ext{THz}}}}}$$\\end{document} on the laser pulse intensity \\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$I_{L}^{\\alpha }$$\\end{document} can be approximated by the power function \\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$${{W}_{{{\ ext{THz}}}}} \\sim I_{L}^{\\alpha }$$\\end{document}. For a fixed laser pulse duration and variable energy the power index lies in the range \\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$\\alpha \\approx 1.5{-} 2.8$$\\end{document}, while for a fixed energy and variable duration \\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$\\alpha \\approx 1$$\\end{document}.

Damage failure prediction study of carbon fiber metal laminates in hot stamping process

In addressing the difficulty of forming Fiber Metal Laminates (FMLs), a laminate composed of a 0.1 mm-thick 304 Stainless Steel Foil (SSF) and Carbon Fiber Reinforced Plastics (CFRP) as the base material is prepared using a specific process. Subsequently, forming limit diagrams are obtained through hemispherical bulge forming experiments to investigate the forming performance of FMLs laminates. The damage phenomena of various forming specimens during the thermal stamping process are analyzed. Based on different damage forms, corresponding theoretical models are established to simulate and predict the forming damage modes of FMLs through simulation. The research results indicate that the stamping formability of FMLs is influenced by the damage tolerance of the thin stainless steel foil. During the thermal stamping process, FMLs may experience delamination, fracture/crack of the thin stainless steel foil, and rupture/tearing/wrinkling of the prepreg. To address these issues, cohesive elements, GTN-M-K damage, and Hashin damage models are established, providing a reasonable simulation prediction of the stamping damage phenomena of FMLs.

Correction: Microstructure-controlled Electrodeposition of Mechanically Reliable Double-layered Thin Foils for Secondary Batteries

Correction: Microstructure-controlled Electrodeposition of Mechanically Reliable Double-layered Thin Foils for Secondary Batteries

Evaluation of surface pretreatment methods on thin austenitic stainless steel foils for adhesive bonding applications

ABSTRACT Stainless steel is used across all industries, from the chemical or construction sector to household appliances. To produce load bearing joints, a surface treatment of the passive surface of austenitic stainless steel is generally necessary. However, the treatment of thin-walled foil materials inhibits challenges concerning the deformation under thermal loads. This work investigates the effectiveness and mechanisms of different surface treatments on 50 µm thin AISI 316 L steel foil. Basic cleaning, surface finishing with an aluminum oxide abrasive, flame-pyrolytic deposition of silicon dioxide and application of a primer, etching with hydrochloric acid, treatment by atmospheric plasma, ns-pulsed laser surface cleaning, and fs-laser structuring are investigated. The effects of these treatments are analyzed in surface energy investigations by contact angle measurement, roughness measurements, and SEM-EDX. The bonding strength is tested with epoxy adhesives and a methyl methacrylate adhesive under 90° peel load. The failure mechanisms are further investigated by FTIR spectroscopy and SEM-EDX. The results show that the used coating with primer produces the strongest bonds, followed by the fs-laser treatment. In particular, sub-microscopic surface structures induced by fs-laser show promising results. SEM images show a full wetting of the capillary structures, providing the possibility of mechanical interlocking on a sub-microscopic level.

Experimental study and modeling of the wettability of fluorine graphene. Corrosion behavior of the fluorine graphene layer on a copper substrate

Fluorographene (FG) is a high-quality 2D insulator, which is effectively used as the atomically thin tunnel barrier. To date, the most common idea is that the complete fluorination of graphene (G) leads to an increase in hydrophobicity. We have shown that in reality fluorination leads to superhydrophilicity and to a significant increase in the defectiveness of the graphene layer. Without hydrocarbons, as well as due to the high defectiveness and superhydrophilicity, the corrosion current of FG is an order of magnitude higher than for pure copper and two orders of magnitude higher than for G synthesized on copper. The simulation results confirm experimental data on FG superhydrophilicity after prolonged fluorination. Thus, in order to achieve high hydrophilicity, it is not necessary to create hydroxyl groups on the surface of FG. A higher concentration of fluorine (the C/F composition ratio) is realized on a thicker copper plate with a graphene layer, compared to thin copper foil. Different fluorine concentrations are associated with different sizes of crystal grains, their orientation, as well as defectiveness and the number of graphene layers. The corrosive effect leads to a decrease in roughness and a multiple decrease in the amount of F on the FG.

A Self‐Regulated Interface Enabled by Multi‐Functional pH Buffer for Reversible Zn Electrochemistry

AbstractAqueous Zn‐ion batteries with mild acidic electrolytes are considered the promising energy storage solutions due to their outstanding merits of high energy density and cost‐effectiveness. However, the rampant dendrite growth and severe parasitic reactions caused by a series of factors such as irregular Zn2+ transport pathway and pH variation would result in poor cycling stability. Herein, a self‐regulated interface strategy implemented by ammonium persulfate ((NH4)2S2O8, denoted as APS) multifunctional additive is proposed to simultaneously address the above issues. The zincophilic NH4+ preferentially adsorbs on the Zn protuberance to exclude water molecules and shield the “tip effect,” thus inhibiting side‐reactions and inducing uniform Zn deposition. Moreover, NH4+ and S2O82− can dynamically adjust H+ and OH− concentrations in a pH self‐buffer manner, thus effectively mitigating hydrogen evolution reaction and formation of by‐products. Consequently, with the existence of APS additive, Zn anode exhibits ultrahigh coulombic efficiency (CE) of 99.9% over 9000 cycles and ultra‐long lifespan of 4300 h at 5 mA cm−2. Furthermore, even under high NH4V4O10 mass loading (9.4 mg cm−2) and thin zinc foil (10 µm), the assembled NH4V4O10//Zn pouch cell with APS additive can still maintain stably over 210 cycles, demonstrating its excellent value for application.

Spectral Characteristics of Polarization Radiation in the Water Window Range

The high-intensity and monochromatic radiation sources in the water window spectral range are desirable for many applications. One of the potential candidates of soft X-ray sources is polarization radiation produced by a charged particle passing through a thin foil. In the soft X-ray range near the absorption edges of a target material, the real part of dielectric permittivity can exceed unity, and the Tamm–Frank criterion is fulfilled. Thus, two types of radiation are produced: transition and Cherenkov radiation. In this report, we theoretically investigated the spectral characteristics of radiation produced in both cases when the Tamm–Frank criterion is met or not met. We showed the dependences of the spectrum as a function of thickness and the incidence angle. To describe the properties of polarization radiation and the complex dielectric permittivity, the polarization current approach and Henke’s model were used, respectively.

Analytical results for pitching kinematics and propulsion performance of flexible foil

Natural flyers and swimmers employ flexible wings or fins to propel. While the complex interaction between the foil with deformation and the surrounding non-steady fluid environment defines the propulsion performance of the propellers, elucidating the interaction mechanism through theoretical models earns much challenge. Based on elastokinetics and linear potential flow theory, this study proposes a simplified analytical model to clarify the kinematics and the propulsion performance of a flexible thin foil pitching in flow. The dynamical forces, including the inertial force of the foil and the non-steady fluid pressure, are used to determine the averaged deformation angle of the foil. Combining the averaged deformation angle and the prescribed driving pitching motion, the kinematics of the foil is resolved analytically. Based on the analytical expressions for the corresponding pitching motion, analytical relations among the physical parameters of the stiffness and the mass of the foil and the driving frequency are given to these critical conditions, including resonance of the flow–structure system, equal pitching amplitude between the flexible foil and the rigid counterpart, phase angle transition from ${\rm \pi}/2$ to $- {\rm \pi}/2$ . Subsequently, the performance of the foil, including the thrust, the power and the propulsive efficiency, as a function of the flexibility of the foil are derived, together with the introduction of a bluff body type offset drag to the thrust. The formulated analytical theory, which matches nicely with previous reports, will help to interpret the effect of the flexibility and regulate the propulsive performance of the flexible foil when pitching in fluid.