Thick Target Research Articles

Role of an in-house designed crucible in the fabrication of isotopically enriched 28Si target for an in-beam γ-ray spectroscopy experiment.

In the present work, an in-house designed special crucible was developed to fabricate isotopically enriched 28Si targets for a γ-ray spectroscopy experiment. Initially, the crucible was tested with natural Si and then utilized to fabricate isotopically enriched 28Si targets of thickness ∼500 μg/cm2 (∼2.15 μm). The fabricated targets were uniform in thickness and had very little contamination. In addition, one of the fabricated targets was successfully utilized in an in-beam γ-ray spectroscopy experiment. The technique employed in the present work not only facilitates the fabrication of stable and pure targets but also minimizes the wastage of the source material. As a result, these efforts pave the way for future fabrication of low-abundance isotopically enriched nuclear physics targets.

Conceptional design of photoneutralization test system for negative ion-based neutral beam injection

Neutral beam injection is one of the effective heating methods in the field of magnetic confinement fusion, and neutralization is the most crucial link in the case of negative ions. To further increase the neutral beam injection power, improve the long pulse operation capability, and optimize the efficiency of the NNBI system, further research and verification about the neutralization mode are needed. Theoretically, photoneutralization can achieve more than 90% neutralization efficiency. However, maintaining stable operation of the megawatt laser cavity over extended periods poses corresponding challenges. Additionally, the cost associated with laser target surpasses the benefit gained from increased neutralization efficiency, leading to its lack of practical application thus far. This paper proposes a solution to these issues by designing a single-channel, multi-fold photoneutralization verification system utilizing the CRAFT NNBI one-quarter and one-half size negative source test equipment. An outline of the system's test and diagnostics approach is provided. Key parameters such as laser target thickness, negative ion energy, beam shape and efficiency of the photoneutralization system are numerically calculated. Combined with the experimental data of the negative source test platform, theoretical calculations show that the neutralization efficiency can achieve 63% with the system efficiency exceeding 40%. Even by increasing the incident laser power or the number of reflections, neutralization efficiency can be increased to 95%, with a simultaneous increase in system efficiency to 60%. Maintaining efficiency while increasing incident laser power could reduce the number of reflections to approximately ten, reaching an acceptable threshold. However, this adjustment will increase the irradiation density of a single mirror from 660W/mm2 increases to 3000W/mm2. This paper methodically designs a practical laser neutralization verification platform, which is expected to substantially improve the neutralization efficiency, and facilitate practical application and validation.

Breach diameter prediction of reinforced concrete wall under contact/near-contact explosives using deep neural network

In recent years, the use of Machine Learning (ML) has been expanded to several engineering fields with applications in structural engineering. Deep Neural Network (DNN) models have been widely implemented to predict the response of structural systems under conventional loading. The accuracy of these DNN models relies on the size of the dataset used, which can vary from hundreds to thousands of data points, typically formed by images, test data, and/or finite element models built for a specific environment. Such dependency becomes a limitation when DNN models are intended to be used in blast analysis and/or design, as data are typically scarce or restricted. This paper introduces the implementation of an ML/DNN model for the prediction of breach diameter of a reinforced concrete target subjected to contact and near-contact explosions. The DNN model predicts the breach diameter using experimentally collected concrete breach data. The DNN model considers several parameters related to the charge (e.g., type, geometry, orientation, casement properties) and wall target (e.g., material properties, geometry, reinforcement, fiber content), as well as proximity between the target and explosive. It was found that charge geometry, charge placement type, target thickness, scaled distance, and fiber content in the mix were important features affecting the breach diameter prediction.

First constraints on the Lμ− Lτ explanation of the muon g-2 anomaly from NA64-e at CERN

The inclusion of an additional U(1) gauge Lμ − Lτ symmetry would release the tension between the measured and the predicted value of the anomalous muon magnetic moment: this paradigm assumes the existence of a new, light Z′ vector boson, with dominant coupling to μ and τ leptons and interacting with electrons via a loop mechanism. The Lμ − Lτ model can also explain the Dark Matter relic abundance, by assuming that the Z′ boson acts as a “portal” to a new Dark Sector of particles in Nature, not charged under known interactions. In this work we present the results of the Z′ search performed by the NA64-e experiment at CERN SPS, that collected ~ 9 × 1011 100 GeV electrons impinging on an active thick target. Despite the suppressed Z′ production yield with an electron beam, NA64-e provides the first accelerator-based results excluding the g − 2 preferred band of the Z′ parameter space in the 1 keV <mZ′\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$ {m}_{Z^{\\prime }} $$\\end{document} ≲ 2 MeV range, in complementarity with the limits recently obtained by the NA64-μ experiment with a muon beam.

Excitation functions of72Ge(p,xn)72,71As reactions from threshold up to 45 MeV for production of the non-standard positron emitter 72As

Nuclear reaction cross sections for the formation of 72As and 71As in proton-induced reactions on enriched 72Ge targets were measured up to 45 MeV utilizing three different cyclotrons at the Forschungszentrum Jülich. The stacked-thin sample activation technique in combination with high-resolution γ-ray spectrometry was used. The major γ-ray peaks of 72As and 71As formed via the 72Ge(p,n)72As and 72Ge(p,2n)71As reactions, respectively, were analyzed. The incident proton energy and flux on a foil were determined using several monitor reactions. Based on integrated counts, irradiation data and the nuclear decay data, the reaction cross sections were measured. All data describe the first measurements. Theoretical nuclear model calculations were then carried out by using the codes TALYS 1.96, EMPIRE 3.2 and ALICE-IPPE. A very good agreement between the measured data and calculated values was found. The new data enabled us to calculate the thick target yields and estimate the radionuclidic impurities for a given energy range. Over the optimum energy range Ep = 14 → 7 MeV, the calculated thick target yield of 72As amounts to 272 MBq/μAh with no 71As impurity at all. The 72Ge(p,n)72As reaction on the enriched 72Ge is thus very suitable for clinical scale production of 72As at a medical cyclotron.

Improved Production of Novel Radioisotopes with Custom Energy Cyclone® Kiube

The implementation of the Variable Energy (VE) feature in the previously fixed-energy IBA Cyclone® Kiube cyclotron is presented as an upgrade enabling the production of novel radioisotopes with improved radionuclidic purity and production yields. The possibility of easily decreasing the energy of the extracted proton beam, from 18 down to 13 MeV, allows us to avoid the use of degraders and/or thick target windows, thus preventing related beam current limitations. The immediate application of the Variable Energy feature is proven by presenting the improved results obtained for the production of 68Ga from the irradiation of liquid targets simultaneously in terms of radionuclidic purity and activity produced.

Nuclear model calculation of yield for 64Cu radionuclide produced in 65Cu(α, x)64Cu reaction at ≈ 10–40 MeV

This paper used theoretical nuclear model calculations to estimate the production yield of medically important 64Cu radionuclide produced in the interaction of α-projectile with 65Cu-target at ≈10–40 MeV. Production cross-sections were predicted using TALYS-1.9(G), EMPIRE 3.2, and ALICE/ASH reaction model codes. Generally, the TALYS-1.95(G) predicted and measured cross-sections to produce 64Cu radionuclide are in very good agreement. Further, the statistical analysis of Pearson's coefficient confirmed strong positive correlations between TALYS-1.95(G) predictions and most experimentally measured production cross-sections. The calculated thick target yields of 64Cu radionuclide showed that 65Cu(α, x)64Cu reaction resulted in a maximum yield of up to ≈ 1423 MBq/μAh at ≈ 30 MeV. Furthermore, analyzes of isotopic impurities produced during 64Cu production could only give rise to the significant yield of 66Cu impurity as much as ≈ 1988 MBq/μAh, which complicated the process of radiochemistry; however, the relatively short half-life of 66Cu isotopic impurity could only demand a waiting time of about 1.5 h to decrease its contribution to a negligible level.The yield obtained for the 64Cu radionuclide via the 65Cu(α, x)64Cu route is significant. It validates the viability of this production route and underscores its potential as a promising option for the optimized supply of 64Cu in radiopharmaceutical applications. While further investigations on quality validating parameters are necessary, the potential of the 65Cu(α, x)64Cu production route cannot be overstated.

TYtool: A software application for yield and target power optimization in charged particle induced radionuclide production

A software application useful for optimization and maximizing radionuclide production without exceeding the power limits of the target material or holder has been developed. The software (TYtool) can be used for target optimization including yield calculations vs time, thickness, and incident energy, W/mm through the target, and automated target thickness optimization with the Makkonen-Craig & Helariutta − or the novel Yield/Wapproach. TYtool also facilitates graphical representation of many basic plots such as cross section, mass stopping power, activity output, projected range and it is useful for many different particles, reactions, radionuclides via the default cross section data base or the import function for cross section and mass stopping power. The software is available for free at: https://gitlab.com/NM_Karolinska_Solna/TYtool.

Design of a multi-carrier X-ray source for communication with energy modulation information.

X-ray communication is a kind of space communication technology which uses X-ray as information carrier. In order to improve the information transmission capacity, communication rate and anti-interference ability of X-ray communication, we proposes to design a novel multi-target X-ray source. The source is composed of a fast switching module of light channels based on FPGA technology and four photoelectric X-ray tubes with different target materials: Cr, Fe, Ni, and Cu. Using Geant4 software, we determined the optimal target thickness for each material, which enabled us to fully leverage the characteristic X-rays for multi-channel signal modulation transmission. Moreover, using CST software for particle trajectory simulation and optimization of the electron beam revealed that at a tube voltage of 20 kV, the focus area measures approximately 1.2 mm×1.2 mm. The simulations show that four kinds of spectra with high distinctiveness can be generated from the Cr, Fe, Ni, and Cu targets. Within a single modulation period, these spectra can be combined in various ways to create 16 different X-ray spectra signals, thereby increasing the number of communication elements and enhancing the information transmission rate.

NEBOAS: A Neutron yiElds Based On AcceleratorS application

The web-based application NEBOAS was developed to calculate the neutron yield of the accelerator-based neutron source MONNET (MONo-energetic NEutron Tower) at JRC-Geel. Neutrons are produced with p and d-induced reactions on particular targets. NEBOAS provides double differential neutron yields, as a function of the angle of neutron emission and energy. It provides also integrated neutron yields, and neutron energy spectra. Any projectile energy may be utilized, as long as it is covered by the nuclear data available on thin targets (that just degrade the projectiles' energy) or thick targets (that stop the projectiles). The calculation employs reaction cross-section evaluations from Evaluated Nuclear Data File (ENDF) or compilations of experimental measurements from the Experimental Nuclear Reaction Data (EXFOR), and stopping powers as recommended in the National Institute of Standards and Technology (NIST) or the Stopping and Range of Ions in Matter (SRIM-2013) databases.

Investigation on the intensity contrast of Kα line emission from laser–matter interactions

The intensity contrast and its angular distribution of Kα line emission originated from the difference of angular distributions of Kα and bremsstrahlung emissions from copper foil targets bombarded by electrons similar to the hot electrons generated in laser–matter interactions are investigated by Monte Carlo simulations. For mono-energetic electron incidences, a higher contrast Kα emission is generated at large detection angles relative to the incident electron direction and for higher electron energy. The Kα emission contrast is decreased with the increase in target thickness. When the areal density of targets is fixed, the contrast is almost unchanged with the change of target density and thickness. For incident electrons with a Boltzmann energy distribution, a higher contrast Kα emission can also be generated at large detection angles and for higher electron temperatures, but the contrast is lower compared to that for mono-energetic electron incidences, and it is changed only slightly with the increase in target thickness. These results help to understand the contrast of Kα emissions in previous experiments. Suggestions are proposed for future laser–matter interaction experiments for higher contrast Kα emissions.

Determination of ballistic resistance model of finite thickness material based on Artificial Neural Network

Ballistic resistance behavior of finite thickness material is affected by factors of target thickness, projectile nose shape, and impact angle. The widely used ballistic limit velocity (BLV) model can only reflect the ballistic resistance behavior of a target in a single given impact scenario. The collected BLV from different impact scenarios can only partially reflect the effect of those factors on the ballistic resistance. A general model of BLV considering these factors simultaneously is desired.In this study, numerical impact models are first verified by a significant number of experiments. A guided random sampling method is proposed to collect numerical BLV data for training/validating usage. BLV data from experiments and simulations are then assembled by this method and subsequently trained by Artificial Neural Network (ANN). k-Folder Cross Validation (K-CV) technique designed for evaluating small sample training network is introduced to validate and test the network. The ANN-predicted results are decomposed by proper singular value decomposition methods. It is found that the Rank-1 decomposition results (with highest singular value) can fully reveal the decoupled relationship between BLV and its independent factors (MAPE < 6 %), with which analytical ballistic models are established. The results show that our proposed model can quantitatively describe the fully decoupled effect of target thickness, impact angle and projectile nose shape on the BLV with high accuracy.

Radiation safety of ultra-high dose rate electron accelerators for FLASH radiotherapy.

An ultra-high dose rate (UHDR) electron accelerator for FLASH radiotherapy (RT) produces very intense bremsstrahlung by the interaction of the electron beam with objects both inside and outside of the accelerator. The bremsstrahlung dose per pulse is typically 1-2 orders of magnitude larger than that of conventional RT x-ray treatment of the same energy, and for electron energies above 10 MeV, the bremsstrahlung produces substantially more induced radioactivity outside the accelerator than for conventional RT. Therefore, a thorough radiation safety assessment is mandatory prior to the operation of a UHDR electron accelerator. To evaluate the radiation safety of a prototype FLASH-enabled Varian TrueBeam accelerator and to develop a general framework for assessment of all key radiation safety properties of a UHDR electron accelerator for FLASH RT. Production of bremsstrahlung and induced radioactivity by a UHDR electron accelerator is modeled by various analytical methods. The analytical modeling is compared with National Institute of Standards and Technology (NIST) bremsstrahlung yield data as well as measurements of primary bremsstrahlung outside the bunker and induced radioactivity of irradiated thick targets for a FLASH-enabled 16 MeV Varian TrueBeam electron accelerator. In addition, the analytical modeling is complemented by measurements of secondary bremsstrahlung inside/outside the bunker and neutrons at the maze entrance. Calculated bremsstrahlung yields deviate maximum 8.5% from NIST data, and all measurements of primary bremsstrahlung and induced radioactivity agree with calculations, validating the analytical tools. In addition, it is found that scattering foil bremsstrahlung dominates primary bremsstrahlung and the main source of secondary bremsstrahlung is the irradiated object outside the accelerator. It follows that primary and secondary bremsstrahlung outside the bunker can be calculated using the same simple formalism as that used for conventional RT. Measured primary bremsstrahlung tenth-value layers for concrete of the simple formalism are in good agreement with NCRP and IAEA data, while measured secondary bremsstrahlung tenth-value layers for concrete are considerably lower than NCRP and IAEA data. All calculations and measurements form a general framework for assessment of all key radiation safety properties of a UHDR electron accelerator. The FLASH-enabled Varian TrueBeam accelerator is safe for normal operation (max. 99 pulses per irradiation) in a bunker designed for at least 15 MV conventional x-ray treatment unless the UHDR workload is much larger than the x-ray workload. A similar finding applies to other UHDR electron accelerators. However, during beam tuning, radiation survey, or other tests with extended irradiation time, the UHDR workload may become very large, necessitating the implementation of additional safety measures.

Enhanced laser absorption and ion acceleration by boron nitride nanotube targets and high-energy PW laser pulses

Enhancing laser energy absorption with energy transfer to fast electrons is crucial for efficient laser-driven ion acceleration. In this work, we present an experimental demonstration of volumetric laser absorption using boron nitride nanotube (BNNT) targets with an average density of 15 of the solid density. We use a PW laser system operating at a pulse duration of 1.2 ps and an energy of 1.3 kJ, reaching intensities of 2 × 1019 Wcm−2 on target with moderate nanosecond contrast (109), to generate energetic ion streams from a 250 µm thick BNNT target. To characterize laser-accelerated ions, Thomson parabola spectrometers, CR-39 nuclear track detectors, and an electron spectrometer are employed. The results are compared to those achieved using flat targets made of polystyrene (PS) of the same thickness. The comparison reveals a 1.5-fold increase in proton maximum energy and a 2.5-fold increase in the maximum energy of heavy ions (C and N) when comparing the BNNT to PS. Moreover, the high-energy ion flux recorded at CR-39 is orders of magnitude higher for the BNNT after cutting off low-energy ions with Al filters. The enhanced ion acceleration is the result of a 2.3-fold increase in the electron temperature for BNNT, as measured by the electron spectrometer. These experimental findings are further validated through two-dimensional particle-in-cell simulations, which confirm the increase in electron temperature due to enhanced laser absorption ascribable to the low density and nanostructure of the BNNT target compared to the flat foil. Published by the American Physical Society 2024

Photon and neutron dose evaluation at the Beam Test Facility of the INFN - National Laboratory of Frascati

Dose evaluation and direct measurements are fundamental for radiation protection in non-conventional accelerator facilities, both before and after the primary and secondary shielding. In this paper, we will report about the experimental setup, data acquisition and analysis, together with FLUKA modeling, of the dose measurements test carried out in the Beam Test Facility (BTF) of the INFN - Frascati’s National Laboratories (LNF), where an intense mixed field is produced and measured with thermoluminescent dosimeters. BTF is an extraction and transport line of DAΦNE LINAC (Buonomo et al. 2021; Mazzitelli et al. 2003). It is optimized for electrons and positrons production in a wide range of intensity, energy (30 MeV–800 MeV), beam spot dimensions and divergence, using both primary and secondary beam of the DAΦNE LINAC. Through the years, the BTF has gained an important role in particle detectors test and development with electron/positron beam. A small fraction of the BTF’s shifts have been dedicated to radiation damage test using LINAC electron primary beam up to 5×1010 e-/s. As radiation protection group of the LNF, we evaluated the dose when electrons impinging on a Pb target from: (i) photon Bremsstrahlung production; (ii) photoneutron production. Three dedicated tests with 503 MeV electrons impinging on a ∼16 cm thick Pb target have been carried out in February, June 2022 and in January 2023, using TLD700 and TLD600, measuring doses at several charge intervals. The aim of this study focuses on evaluating dosimetric quantities produced by the mixed field, air kerma for the photon component, and ambient dose equivalent for the neutron one, using thermoluminescence dosimeters calibrated with low-energy standards: Cs-137 and Am-Be. The approach adopted involves the use of Monte Carlo simulations of the experiment, both to benchmark against experimental measurements and to validate the results obtained for energies higher than those of calibration. The results of this comparison show excellent agreement between measured and simulated quantities in the forward direction, allowing us to conclude and confirm the validity of the calibrations themselves.

K X-ray production cross sections of transition metals induced by carbon ions impact: Influence of projectile mass

K X-ray production cross sections of Co, Ni, and Zn due to the impact of 2.48 MeV to 3.84 MeV 12C3+ and 13C3+ ions were experimentally determined using the thick target approach. It was possible to observe differences in the cross sections due to the distinct mass of the ions. A reduced variable v1/v2K, where v1 is the ion velocity and v2K is the (Bohr) electron orbital velocity, was considered to scale the ion energies. When the data were plotted as a function of the reduced variable, a single curve was obtained for all targets and both isotopes. Comparisons with several models were also made, including corrections due to electron capture and multiple ionization. It was found that the adiabatic perturbation with molecular orbitals formation, plus electron capture and multiple ionization corrections, is the theory that better describes the experimental results.

A novel hydro-elastoplastic constitutive model incorporating hydrostatic damage for predicting high-pressure performance of concrete under blast loading

The evolution of damage and failure modes of concrete under blast or impact loads are the outcomes of stress wave propagation. The stress state at a point within the concrete changes instantaneously with time and space. Establishing a constitutive model that can cover the nonlinear behavior of materials under complex loading paths and histories is an extremely challenging task. The main difficulty lies in the construction of the damage model, which has not yet been fully resolved in commonly used concrete models. This paper, based on the mechanisms of damage and failure of concrete under hydrostatic pressure, constructs a state equation that includes the description of crushing and compaction damage due to the collapse and closure of pores, as well as their interactive model, negative pressure degradation caused by hydrostatic pressure, and nonlinear volumetric behavior under loading/unloading/reloading. By introducing independent shear and tensile deviatoric damage scaling functions and a damage scaling function under isotropic tension, the coupling relationship between deviatoric and volumetric damage is considered. Corresponding strength models and element erosion criteria are developed based on the new state equation and damage models. Then, single-element numerical experiments of unconstrained uniaxial compression and tension, triaxial compression under different confining pressures, monotonic and cyclic hydrostatic compression, and isotropic tension were conducted to verify the predictive accuracy of the proposed model under single loading paths. Finally, numerical experiments of contact explosion on plain concrete thick and thin targets were carried out using the proposed model, revealing the propagation laws and failure processes of the loading compression wave, unloading tensile wave, and reflected tensile wave within the concrete target. The predicted final failure modes are consistent with the experimental results.

Activation cross sections of 7Li-induced reactions on natCu for monitor reactions

Activation cross sections of 7Li-induced reactions on natCu were measured in order to investigate suitability of some reactions for monitoring experimental parameters. Cross sections producing 69,68Ge, 67,66Ga and 69m,65Zn were determined. Physical thick target yields were experimentally measured and compared with those calculated using the measured cross sections. The measured cross sections were verified by the agreements between the directly measured thick target yields and the thick target yields deduced from the measured cross sections. The 7Li-induced reactions on natCu for the production of 67,66Ga and 65Zn are suggested as monitor reactions.

Simulating the impact of electron beam energy deposition on lead target temperature

This study delves into the thermal dynamics induced by an electron beam sourced from the CIRCE III accelerator, focusing on a lead target previously employed at the National Centre for Nuclear Science and Technology (CNSTN) in Tunisia for neutron and photon production. Leveraging FLUKA software, we simulate the intricate interplay between electrons and the target surface, analyzing variations in deposited energy across different target thicknesses. Beyond elucidating the electron-target interaction, our investigation extends to predicting crucial parameters such as the maximum operational threshold and surface temperature distribution of the target. To achieve this, a computational model harnessing the finite volume method is employed, offering insights into the thermal response dynamics and paving the way for optimized operational protocols and target design refinements. Through this comprehensive analysis, we aim to advance the understanding of thermal phenomena in electron-target interactions, thereby bolstering the efficiency and safety of particle accelerator operations in diverse scientific applications.

Measurement of nuclear interaction cross sections towards neutron-skin thickness determination

The accuracy of reaction theories used to extract properties of exotic nuclei from scattering experiments is often unknown or not quantified, but of utmost importance when, e.g., constraining the equation of state of asymmetric nuclear matter from observables as the neutron-skin thickness. In order to test the Glauber multiple-scattering model, the total interaction cross section of ▪ on carbon targets was measured at initial beam energies of 400, 550, 650, 800, and 1000 MeV/nucleon. The measurements were performed during the first experiment of the newly constructed R3B (Reaction with Relativistic Radioactive Beams) experiment after the start of FAIR Phase-0 at the GSI/FAIR facility with beam energies of 400, 550, 650, 800, and 1000 MeV/nucleon. The combination of the large-acceptance dipole magnet GLAD and a newly designed and highly efficient Time-of-Flight detector enabled a precise transmission measurement with several target thicknesses for each initial beam energy with an experimental uncertainty of ±0.4%. A comparison with the Glauber model revealed a discrepancy of around 3.1% at higher beam energies, which will serve as a crucial baseline for the model-dependent uncertainty in future fragmentation experiments.