Thermoplastic Polyurethane Films Research Articles

Evaluating a novel portable semiconductor liquid cooling garment for reducing heat stress of healthcare workers in a hot-humid environment

Limited research focused on exploring personal cooling garments (PCGs) that offer excellent portability, along with a substantial, long-lasting, and consistent cooling effect for healthcare workers exposed to extreme heat while combating the COVID-19 pandemic. To address this gap, a novel, energy-efficient, and portable semiconductor liquid cooling garment (SLCG) was introduced, which incorporates a semiconductor-powered cold source and a cooling vest crafted from a semi-transparent thermoplastic polyurethane (TPU) film that offers extensive body coverage. Its practical cooling efficacy was assessed through a human trial involving ten male participants engaging in two protocols under a hot-humid environment (i.e., 30 ± 0.5 °C, RH = 80 ± 5 %). These protocols included both low-intensity (Prot.1) and moderate-intensity (Prot.2) exercises, mimicking the physical demands faced by healthcare workers. SLCG significantly reduced the mean, torso and local skin temperatures during both Prot.1 and Prot.2 (p < 0.05), also with a notable reduction in heart rate and sweat loss during Prot.1 (p < 0.05). Rating of perceived exertion as well as thermal sensations, wetness sensations and comfort sensations in the whole-body and local-body (i.e., head & neck, trunk, arms and legs) were all remarkably improved using SLCG during Prot.1 (p < 0.05). These perceptual sensations in SLCG were only improved in the whole body during the resting stage, and in the trunk region during Prot.2 (p < 0.05). Furthermore, participants felt no significant added weight or movement restrictions with SLCG in either protocol.

Graphene-Doped Thermoplastic Polyurethane Nanocomposite Film-Based Triboelectric Nanogenerator for Self-Powered Sport Sensor.

Triboelectric nanogenerators (TENGs), as novel electronic devices for converting mechanical energy into electrical energy, are better suited as signal-testing sensors or as components within larger wearable Internet of Things (IoT) or Artificial Intelligence (AI) systems, where they handle small-device power supply and signal acquisition. Consequently, TENGs hold promising applications in self-powered sensor technology. As global energy supplies become increasingly tight, research into self-powered sensors has become critical. This study presents a self-powered sport sensor system utilizing a triboelectric nanogenerator (TENG), which incorporates a thermoplastic polyurethane (TPU) film doped with graphene and polytetrafluoroethylene (PTFE) as friction materials. The graphene-doped TPU nanocomposite film-based TENG (GT-TENG) demonstrates excellent working durability. Furthermore, the GT-TENG not only consistently powers an LED but also supplies energy to a sports timer and an electronic watch. It serves additionally as a self-powered sensor for monitoring human movement. The design of this self-powered motion sensor system effectively harnesses human kinetic energy, integrating it seamlessly with sport sensing capabilities.

Room temperature self-healing and high gas barrier properties of elastomer composites incorporated with liquid metal

Flexible electronic devices require stretchable packaging materials that provide a hermetic seal. However, conventional soft materials often exhibit strong gas permeability, making it difficult to achieve stable operation, which requires films with high deformability, self-healing capability, and gas barrier functionality. In this study, a layer by layer (LBL) method was employed to uniformly coat a controllable thickness of liquid metal (LM) onto a designed and synthesized self-healing thermoplastic polyurethane (TPU) film, successfully developing a stretchable gas barrier film (TPU/LM) with high gas barrier properties. The designed polyurethane film significantly enhanced the adhesion of the liquid metal, effectively preventing leakage. The experimental results show that the water vapor transmission rate (WVTR) of the TPU/LM composite film with a thickness of 40 μm is 4.04g/(m2·day). Compared to the film without LM, the gas barrier performance has been improved by approximately 16 times. Additionally, there is a significant enhancement in nitrogen (N2) barrier, with a permeation rate reaching 4.0*10−17 cm3 cm/(cm2·s·Pa), effectively blocking the N2 permeation. This demonstrates the universality of the TPU/LM in gas barrier applications. Furthermore, the TPU/LM film also demonstrated excellent electromagnetic shielding effectiveness. The self-healing capability of the stretchable gas barrier film allows it to recover its initial gas barrier performance after mechanical damage. Humidity-sensitive resistors encapsulated with TPU/LM exhibited stable operation in both air and 90 % humidity environments, confirming the superior barrier properties of the TPU/LM. Generally, the developed TPU/LM is suitable for packaging applications in the next generation of flexible electronic devices.

Development of stopped-flow hyper-CEST NMR method on recirculating hyperpolarization system as applied to void space analysis in polymers.

129Xe NMR spectroscopy of polymers can provide important information on void spaces, sometimes called free volume, in polymers. Unfortunately, the spectroscopy's low sensitivity has limited its widespread use in both academic and industrial research. In order to overcome such a difficult situation, hyper-CEST method which employs hyperpolarization and CEST techniques, is examined after the introduction of recirculation and subtraction modes. Alongside the incorporated stopped-flow technique, these modes were very efficient in detecting very weak hidden signals from cellulose nanofiber (CNF) and silk fibroin (SF) films and in discussing the void space in these polymers. From the analysis of detailed saturation frequency dependence in the increment of 100Hz, the chemical shifts of hidden peaks were successfully determined to give reasonable values for the size of void space in CNF and SF. Application on thermoplastic polyurethane film also supported our method of analysis. The subtraction mode was very efficient in judging the presence or absence of any peak at a fixed saturation frequency. These facts support that the mode will surely be useful in the future exploratory study of very weak hidden signals.

Secondary cleft palate correction with 3D-printed thermoplastic polyurethane film – a case report

Cleft palate is an oronasal communication that can affect the area comprehending the lips and the soft palate. Its clinical signs vary depending on the degree of the defect and the age of the animal, ranging from nasal secretion, coughing, sneezing, halitosis, respiratory difficulty, aspiration pneumonia, and loss of body condition. Its diagnosis is based on inspection of the oral cavity and imaging tests. Palatal defects must be surgically corrected as quickly as possible, using mucosal flaps, grafts, or implants. A desire to evolve alternative treatments for cleft palates drives the search for ways to manufacture customized pieces. 3D printing and biomaterials have enhanced in detail and applicability; combined with design tools and imaging exams, they allow for the making of precise implants and anatomical models for the planning and execution of surgical procedures. This report describes the case of a female, mixed-breed feline treated at a veterinary clinic; it was diagnosed with secondary cleft palate, had a history of falling, and underwent previous palatoplasties with recurrence. A surgical reintervention was performed to implant a 3D-printed TPU film to close its secondary cleft palate.

Highly-sensitive ultrathin flexible pressure sensor based on quasi-2D conductive network for human physiological signal monitoring

Ultrathin flexible pressure sensors are highly desirable for human physiological signal monitoring due to their portability and ability to conform to the body. However, existing ultrathin pressure sensors face challenges in balancing the sensitivity and their range. A spatial-dimensionally constrained strategy was proposed to construct an ultrathin active layer. In detail, multi-walled carbon nanotubes (MWCNTs) with an average length of ∼1.3 μm were intentionally spin-coated into a thin thermoplastic polyurethane (TPU) film with a thickness of 1.5 μm. By doing so, a quasi-2D MWCNTs conductive network is constructed, which enabled the sensor to have ultrahigh sensitivity of 27.04 kPa−1, a wide liner detection range of 0.2–24 kPa, ultrafast response time of 40 ms and a recovery time of 10 ms, and high durability in 1500 cycles under 0.2 kPa with loading/unloading frequency of 2 Hz. Thanks to this superior performance, the ultrathin pressure sensor can be used to monitor human movement and physiological signals, including finger touch, finger bending, wrist bending, and deep breathing. Moreover, the sensor can be attached to the side wall of the tip of the renal ureteroscope, allowing for the monitoring of renal pelvic pressure. Therefore, this spatial-dimensionally constrained strategy will open up a new way to fabricate highly sensitive ultrathin pressure sensors and have great application prospects in health monitoring.

Constructing Heterostructured MWCNT-BN Hybrid Fillers in Electrospun TPU Films to Achieve Superior Thermal Conductivity and Electrical Insulation Properties.

The development of thermally conductive polymer/boron nitride (BN) composites with excellent electrically insulating properties is urgently demanded for electronic devices. However, the method of constructing an efficient thermally conductive network is still challenging. In the present work, heterostructured multi-walled carbon nanotube-boron nitride (MWCNT-BN) hybrids were easily prepared using an electrostatic self-assembly method. The thermally conductive network of the MWCNT-BN in the thermoplastic polyurethane (TPU) matrix was achieved by the electrospinning and stack-molding process. As a result, the in-plane thermal conductivity of TPU composite films reached 7.28 W m-1 K-1, an increase of 959.4% compared to pure TPU films. In addition, the Foygel model showed that the MWCNT-BN hybrid filler could largely decrease thermal resistance compared to that of BN filler and further reduce phonon scattering. Finally, the excellent electrically insulating properties (about 1012 Ω·cm) and superior flexibility of composite film make it a promising material in electronic equipment. This work offers a new idea for designing BN-based hybrids, which have broad prospects in preparing thermally conductive composites for further practical thermal management fields.

Development of AgNPs-PVP/TPU based flexible strain sensors for structural health monitoring of composite structures

Real-time in-stu structural health monitoring (SHM) of composite structure developed through highly sensitive and flexible smart sensors based on colloidal solution of Silver Nano Particles (AgNPs). Synthesis of AgNPs through chemical reduction method by citrate and then in Haxen phase transferred by using surfactant Cetyltrimethylammonium bromide (CTAB). Colloidal solution of AgNPs-Haxen and Polyvinylpyrrolidone (PVP) - Haxen has been followed by mixed, calcined and deposited that thick paste on flexible Thermoplastic Polyurethane (TPU) film. These sensors become more sensitive than metallic foil made sensors and farther this sensor pasted on polymer composite for monotonic loading like tensile loading. The data extracted from sensors was monitored effectively by data acquisitioning technique using Keithley KUSB-3100. This research based on chemical synthesis of metallic nanoparticles like silver, its functionalization, protection of these nanoparticles from environment by capping agents and by creating inert atmosphere respectively. Then these functionalized capped nanoparticles are embedded on the surface of thermoplastic Urethane (TPU) film to make piezo resistive semi conductive strips which serve as flexible strain gauge/smart sensor. One other technique is also being used to make sensor is that colloidal solution of metallic Nanoparticles sprays over TPU substrate using Connective Self Assembly (CSA) method. The sensor then properly attached to Glass fabric reinforced polymer (GFRP) composite and calibrated using data acquisitioning (DAQ) under different mode of testing.

Characterization of mechanical, thermal and rheological properties of silica-based nanocomposite filled thermoplastic polyurethane film

Characterization of mechanical, thermal and rheological properties of silica-based nanocomposite filled thermoplastic polyurethane film

Flexible conductive polymer composite film with sandwich-like structure for ultra-efficient and high-stability electromagnetic interference shielding

Flexible electromagnetic interference (EMI) shielding films with the merits of light-weight, flexibility, and high EMI shielding performance are the essential materials for the consumer electronics and communication products. Herein, we construct a hybrid conductive network based on the electrospinning thermoplastic polyurethane (TPU) film loaded with different dimensional conductive fillers, including 0D FeCl3, 1D carbon nanotube (CNT) and 2D graphene nanosheet (GN) to achieve a flexible, light-weight, and ultra-efficient EMI shielding composite film. In specific, the electrospinning porous TPU film is firstly anchored by CNTs assisted by ultrasound to generate the porous TPU/CNT film. Thereafter, the as-prepared porous TPU/CNT film is loaded a GN/CNT/FeCl3 layer by vacuum-assisted filtration to generate a double-layer GN/CNT/FeCl3@TPU/CNT film. Finally, another porous TPU/CNT film is sealed onto the GN/CNT/FeCl3@TPU/CNT film by hot-pressing, which fabricates a sandwiched TPU/CNT@GN/CNT/FeCl3@TPU/CNT composite film. It is interesting to note that the composite film possesses the ultrahigh EMI shielding value (56.0 dB at 10.0 GHz) in the X-band (8.2–12.4 GHz) with high flexibility, excellent mechanical properties, long-term durability (acid-base environment resistance and stability after 1000 bends), as well as high thermal conductivity (6.53 W/(m.K)). This work proposes a simple but efficiency strategy to design the flexible EMI shielding film with ultra-high performance and outstanding durability.

Thermal, viscoelastic, and electrical properties of thermoplastic polyurethane films reinforced with multi-walled carbon nanotubes

Thermoplastic polyurethane (TPU) doped with multi-walled carbon nanotubes (MWCNTs) at 1, 3, 5, and 7 wt% has been studied. The effect of MWCNTs on thermal, viscoelastic, and electric properties in the TPU matrix was characterized by differential scanning calorimetry (DSC), dynamic mechanical analysis (DMA), and by impedance spectroscopy. The results show that the thermal, electrical, and viscoelastic properties, such as the glass transition temperature, shifted towards high temperatures. The melting temperature decreased, and the conductivity and the storage modulus increased by 61.5 % and 58.3 %. The previously observed behavior on the films is due to the increase in the mass percentage of carbon nanotubes (CNTs) in the TPU matrix. Also, it can be said that the CNTs were homogeneously dispersed in the TPU matrix, preventing the movement of the polymer chains, and generating channels or connections that increase the conductivity and improve the thermal properties of the material.

Development and application of a protocol for extractables profiling from central venous catheters in neonates

Peripherally inserted central catheters (PICC-lines) used in neonatology are made of thermoplastic polyurethane (TPU) or silicone. These materials usually contain substances that may leach into drug vehicles or blood. In this extractables study, we determined the optimal extraction conditions using TPU films containing defined amounts of butylhydroxytoluene (BHT) and then applied them on unused and explanted PICC-lines. Maceration and sonication tests were carried out with hexane, acetone and water as the extraction solvents. The analyses were performed using gas and liquid chromatography coupled with mass spectrometry detectors, as well as inductive coupled plasma optical emission spectroscopy to detect a wide range of extractables. We selected a limited list of substances to be sought from the usual adjuvants and monomers, related to their carcinogenic, mutagenic or reprotoxic properties and/or existence in endocrine disruptors lists. The TPU-film experiments showed that acetone was slightly better than hexane, and maceration better than sonication. When applied to PICC-lines, the extraction methods were almost similar but acetone was clearly better than hexane for TPU. From the 48 peaks initially observed in GC-MS, we ended up with 37 peaks to follow in TPU PICC-lines, among which were those of BHT and 4,4′-Methylenebis(cyclohexyl isocyanate) isomers. For silicone PICC-lines, out of 41 peaks initially observed in GC-MS, we followed 20 peaks, most of them being identified as cyclosiloxanes. Barium was the main inorganic element extracted for both PICC-lines. For TPU PICC-lines, the inter-batch variability was higher than for intra-batch, but in silicone devices both were similar. When compared to new PICC-lines, explanted TPU PICC-lines extracted peaks had a lower area under the curve (AUC), while the AUCs of the peaks were higher for the majority of silicone PICC-lines extract compounds. No identified substances were detected above their toxicological threshold, but isocyanates and cyclosiloxanes toxicity was mostly studied for other exposition routes than intravenous. The methods defined in this study were efficient in producing extractable profiles from both PICC-lines.

Printed Self-Healing Stretchable Electronics for Bio-signal Monitoring and Intelligent Packaging.

Integrating self-healing capabilities into printed stretchable electronic devices is important for improving performance and extending device life. However, achieving printed self-healing stretchable electronic devices with excellent device-level healing ability and stretchability while maintaining outstanding electrical performance remains challenging. Herein, a series of printed device-level self-healing stretchable electronic devices is achieved by depositing liquid metal/silver fractal dendrites/polystyrene-block-polyisoprene-block-polystyrene (LM/Ag FDs/SIS) conductive inks onto a self-healing thermoplastic polyurethane (TPU) film via screen printing method. Owing to the fluidic properties of the LM and the interfacial hydrogen bonding and disulfide bonds of TPU, the as-obtained stretchable electronic devices maintain good electronic properties under strain and exhibit device-level self-healing properties without external stimulation. Printed self-healing stretchable electrodes possess high electrical conductivity (1.6×105Sm-1), excellent electromechanical properties, and dynamic stability, with only a 2.5-fold increase in resistance at 200% strain, even after a complete cut and re-healing treatment. The printed self-healing capacitive stretchable strain sensor shows good linearity (R2 ≈0.9994) in a wide sensing range (0%-200%) and is successfully applied to bio-signal detection. Furthermore, the printed self-healing electronic smart label is designed and can be used for real-time environmental monitoring, which exhibits promising potential for practical application in food preservation packaging.

Development of high‐performance zinc stannate based multifunctional thermoplastic polyurethane nanocomposite films

AbstractA lot of demand exists for multifunctional TPU that can provide enhanced performance to address a variety of inflatable application needs. To develop multifunctional nanocomposite films for such uses, synthesized zinc stannate (ZnSnO3) nanoparticles are integrated for the first time in a thermoplastic polyurethane (TPU) matrix. ZnSnO3 was synthesized using hydrothermal method. The morphological analysis vividly displayed the nanocubic structures. As‐synthesized nano ZnSnO3 was added as a nanofiller at varied concentration from 2 to 10 wt% in TPU and nanocomposite films were prepared by solvent intercalation and casting method. These films were thoroughly examined for their multifunctional properties such as UV protection, helium gas barrier and infrared emissivity. Mean value of UV protection factor was improved by 75% at 10 wt% loading of ZnSnO3 whereas 23% improvement was observed in helium gas barrier. Moreover, a good correlation of experimental data with various theoretical models of gas permeability was obtained at lower volume fraction of ZnSnO3. IR emissivity value also showed improvement from 0.802 to 0.842. Thus, the developed TPU‐ZnSnO3 nanocomposite films exhibited a significant improvement in multiple functional properties with improved tensile strength at optimized loading of 6 wt% of ZnSnO3.Highlights UPF mean value of ZnSnO3 incorporated TPU film has been improved by 67%. Helium gas barrier has been improved by approximately 23% at 6 wt% loading. TPU film exhibited improved properties at optimized loading of 6 wt% of ZnSnO3. Nanocomposite TPU film can be employed in various weathering inflatables.

Online structural health monitoring of polymer composite structure using gold nanoparticles (AuNPs)

A mechanism for online structural health monitoring of composite structure was established by developing highly sensitive strain gauges based on colloidal Gold Nano Particles (AuNPs). They were synthesized using well known Turkevich-Frens method followed by phase transfer in chloroform using surfactant Cetyltrimethylammonium bromide (CTAB). Flexible Strain gauges / smart sensors were formed by mixing colloidal AuNPs-chloroform solution in polystyrene (PS) – chloroform solution and depositing their thick paste on hand-made flexible thermoplastic polyurethane (TPU) film. These sensors were used as strain gauges on composite substrates for tensile testing. The developed AuNP based strain gauges were found to have 10 times higher sensitivity than normal metal foil strain gauges.

Application of Multilayered Blend Films as Soft, Stretchable, Self‐Adhesive, and Self‐Healing Absorption‐Dominant EMI Shielding and Microwave Absorber

AbstractSolution‐processable organic conductor–supramolecular elastomer blends are emerging materials for intrinsically stretchable and autonomously self‐healing organic electronics. Herein, the feasibility of a heterogenous multiphase polymer blend is demonstrated for soft, ultraflexible, self‐adhesive, and self‐healing multilayered film structures for electromagnetic interference (EMI) shielding and microwave absorber (MWA) purposes. The developed soft multilayered films achieve a 5–40 fold improvement in the thickness of the MWA compared to the current state‐of‐the‐art. The thickness normalized reflection loss (RL) is up to 65.26 dB mm−1 with 8.5 GHz bandwidth at 18–26.5 GHz. The maximum thickness normalized EMI shielding effectiveness peaks at up to 175 dB mm−1. The EMI shielding and MWA properties are maintainable up to 150% tensile strain with only a small decrease in the overall attenuation and RL. Furthermore, the developed films are capable of fully autonomously self‐healing and achieve a tough adhesion in temperatures of −30–145 °C, and underwater with maximum single‐lap shear adhesion strength of ≈481.5 kPa to soft thermoplastic polyurethane films. Thus, the developed multilayered films can be utilized for absorption‐dominant EMI shielding or MWA purposes as stretchable coatings. The developed materials also show considerable potential for emerging damage and puncture‐resistant organic soft electronics with autonomous material‐level self‐healing.

Self‐Powered Underwater Pressing and Position Sensing and Autonomous Object Grasping with a Porous Thermoplastic Polyurethane Film Sensor

AbstractMost flexible ionic tactile sensors can hardly be used in deep sea due to their poor antiswelling and anticompression properties under high hydrostatic pressure. To achieve pressure and position sensing under high hydrostatic pressure, a self‐powered underwater tactile sensor made of a porous thermoplastic polyurethane (TPU) film is presented in this paper. The sensor works by generating an electric current due to the different moving velocities of ions in the porous film under pressing. Experimental results show that the magnitude of the generated current signal increases with the applied pressure, the contacting area, and ion concentration of the solution. The direction and magnitude of the current signal depend on the pressing position of the film. The signal magnitude decreased with the closer to the center of the film. The maximum pressure sensitivity and positioning resolution are 0.62 kPa−1 and 1.31 mm respectively. Response time (0.19 s), 0.67 s recovery time, and 50–600 kPa pressure detection range are achieved. In addition, the signal magnitude is decreased only by 15.53% when the sensor is placed underwater at a simulated depth of 100 m. Proof of concept demonstration of underwater autonomously grasping objects of different weights with this sensor is successfully achieved.

Polyurethane composite films with self-assembled graphene fluoride: Constructing conductive pathways for thermal management with electrical insulation

Polymer composites incorporating carbon-based fillers have been demonstrated to have high thermal conductivity (TC), yet their high electrical conductivity restricts their utility in electronic devices. As a solution to this issue, we report graphene fluoride (GF) incorporated thermoplastic polyurethane (TPU) composites that are both thermally conductive and electrically insulating. The TPU composites, engineered for both high TC and electrical insulation while maintaining flexibility, were fabricated using a combination of electrospinning, dip-coating, and hot-pressing techniques. This study aimed to investigate the effects of various dip-coating cycles on the in-plane thermal conductivity (λ∥) of GF@TPU composites. Noticeably, GF@TPU composites exhibited an outstanding TC, reaching up to 13.5 W m−1 K−1 with 10 vol% GF loading, marking a 75-fold increase compared to the neat TPU films. Moreover, the GF@TPU composites exhibited an electrically insulating property of 6.5 × 1010 Ω/m. This work provides a promising strategy to make thermally conductive composites with electrical insulation for thermal management in smart electronics.

Surface Properties of a Biocompatible Thermoplastic Polyurethane and Its Anti-Adhesive Effect against E. coli and S. aureus.

Thermoplastic polyurethane (TPU) is a polymer used in a variety of fields, including medical applications. Here, we aimed to verify if the brush and bar coater deposition techniques did not alter TPU properties. The topography of the TPU-modified surfaces was studied via AFM demonstrating no significant differences between brush and bar coater-modified surfaces, compared to the un-modified TPU (TPU Film). The effect of the surfaces on planktonic bacteria, evaluated by MTT assay, demonstrated their anti-adhesive effect on E. coli, while the bar coater significantly reduced staphylococcal planktonic adhesion and both bacterial biofilms compared to other samples. Interestingly, Pearson's R coefficient analysis showed that Ra roughness and Haralick's correlation feature were trend predictors for planktonic bacterial cells adhesion. The surface adhesion property was evaluated against NIH-3T3 murine fibroblasts by MTT and against human fibrinogen and human platelet-rich plasma by ELISA and LDH assay, respectively. An indirect cytotoxicity experiment against NIH-3T3 confirmed the biocompatibility of the TPUs. Overall, the results indicated that the deposition techniques did not alter the antibacterial and anti-adhesive surface properties of modified TPU compared to un-modified TPU, nor its bio- and hemocompatibility, confirming the suitability of TPU brush and bar coater films in the biomedical and pharmaceutical fields.

A 3D-Printed Piezoelectric Microdevice for Human Energy Harvesting for Wearable Biosensors.

The human body is a source of multiple types of energy, such as mechanical, thermal and biochemical, which can be scavenged through appropriate technological means. Mechanical vibrations originating from contraction and expansion of the radial artery represent a reliable source of displacement to be picked up and exploited by a harvester. The continuous monitoring of physiological biomarkers is an essential part of the timely and accurate diagnosis of a disease with subsequent medical treatment, and wearable biosensors are increasingly utilized for biomedical data acquisition of important biomarkers. However, they rely on batteries and their replacement introduces a discontinuity in measured signals, which could be critical for the patients and also causes discomfort. In the present work, the research into a novel 3D-printed wearable energy harvesting platform for scavenging energy from arterial pulsations via a piezoelectric material is described. An elastic thermoplastic polyurethane (TPU) film, which forms an air chamber between the skin and the piezoelectric disc electrode, was introduced to provide better adsorption to the skin, prevent damage to the piezoelectric disc and electrically isolate components in the platform from the human body. Computational fluid dynamics in the framework of COMSOL Multiphysics 6.1 software was employed to perform a series of coupled time-varying simulations of the interaction among a number of associated physical phenomena. The mathematical model of the harvester was investigated computationally, and quantification of the output energy and power parameters was used for comparisons. A prototype wearable platform enclosure was designed and manufactured using fused filament fabrication (FFF). The influence of the piezoelectric disc material and its diameter on the electrical output were studied and various geometrical parameters of the enclosure and the TPU film were optimized based on theoretical and empirical data. Physiological data, such as interdependency between the harvester skin fit and voltage output, were obtained.