Superradiant Quantum Phase Transition Research Articles

Effective field theories and finite-temperature properties of zero-dimensional superradiant quantum phase transitions

The existence of zero-dimensional superradiant quantum phase transitions seems inconsistent with conventional statistical physics. This work clarifies this apparent inconsistency. We demonstrate the corresponding effective field theories and finite-temperature properties of light-matter interacting systems, and show how this zero-dimensional quantum phase transition occurs. We first focus on the Rabi model, which is a minimum model that hosts a superradiant quantum phase transition. With the path-integral method, we derive the imaginary-time action of the photon degrees of freedom. We also define a dynamical critical exponent as the rescaling between the temperature and the photon frequency, and perform dimensional analysis to the effective action. The dynamical critical exponent shows that the effective theory of the Rabi model is a free scalar field, where a true second-order quantum phase transition emerges. These results are also verified by numerical simulations of imaginary-time correlation functions of the order parameter. Furthermore, we also generalize this method to the Dicke model. Our results make the zero-dimensional superradiant quantum phase transition compatible with conventional statistical physics, and pave the way to understand it in the perspective of effective field theories. Published by the American Physical Society 2024

Quantum multicritical behavior for coupled optical cavities with driven laser fields

Quantum phase transitions with multicritical points are fascinating phenomena occurring in interacting quantum many-body systems. However, multicritical points predicted by theory have been rarely verified experimentally; finding multicritical points with specific behaviors and realizing their control remains a challenging topic. Here, we propose a system that a quantized light field interacts with a two-level atomic ensemble coupled by microwave fields in optical cavities, which is described by a generalized Dicke model. Multicritical points for the superradiant quantum phase transition are shown to occur. We determine the number and position of these critical points and demonstrate that they can be effectively manipulated through the tuning of system parameters. Particularly, we find that the quantum critical points can evolve into a Lifshitz point (LP) if the Rabi frequency of the light field is modulated periodically in time. Remarkably, the texture of atomic pseudo-spins can be used to characterize the quantum critical behaviors of the system. The magnetic orders of the three phases around the LP, represented by the atomic pseudo-spins, are similar to those of an axial next-nearest-neighboring Ising model. The results reported here are beneficial for unveiling intriguing physics of quantum phase transitions and pave the way towards to find novel quantum multicritical phenomena based on the generalized Dicke model.

Quantum chaos and thermalization in the two-mode Dicke model

We discuss the onset of quantum chaos and thermalization in the two-mode Dicke model, which describes the dipolar interaction between an ensemble of spins and two bosonic modes. The two-mode Dicke model exhibits normal to superradiant quantum phase transition with spontaneous breaking either of a discrete or continuous symmetry. We study the behaviour of the fidelity out-of-time-order correlator (FOTOC) derived from the Loschmidt echo signal in the quantum phases of the model. We show that the exponential growth of the FOTOC in the beginning of the time evolution cannot be related to a classical unstable point in the general case. Furthermore, we find that the collective spin observable in the two-mode Dicke model quickly saturates to its long-time average value, and shows very good agreement between its diagonal ensemble average and microcanonical average even for a small number of spins. We show that the temporal fluctuations of the expectation value of the collective spin observable around its average are small and decrease with the effective system size, which leads to thermalization of the spin system.

Theory of magnon polaritons in quantum Ising materials

We present a theory of magnon-polaritons in quantum Ising materials, and develop a formalism describing the coupling between light and matter as an Ising system is tuned through its quantum critical point. The theory is applied to Ising materials having multilevel single-site Hamiltonians, in which multiple magnon modes are present, such as the insulating Ising magnet LiHoF$_4$ . We find that the magnon-photon coupling strengths may be tuned by the applied transverse field, with the coupling between the soft mode present in the quantum Ising material and a photonic resonator mode diverging at the quantum critical point of the material. A fixed system of spins will not exhibit the diamagnetic response expected when light is coupled to mobile spins or atoms. Without the diamagnetic response, one expects a divergent magnon-photon coupling strength to lead to a superradiant quantum phase transition. However, this neglects the effects of damping and decoherence present in any real system. We show that damping and decoherence may block the superradiant quantum phase transition, and lead to weak coupling between the soft magnon mode and the resonator mode. The results of the theory are applied to experimental data on the model system LiHoF$_4$ in a microwave resonator.

Superradiant quantum phase transition for Landau polaritons with Rashba and Zeeman couplings

We develop a theory of cavity quantum electrodynamics for a two-dimensional electron gas in the presence of Rashba spin-orbit and Zeeman couplings and perpendicular magnetic field, coupled to a spatially nonuniform quantum photon field. We show that the superradiant quantum phase transition (SQPT), also known as photon condensation, can in principle occur through a pure in-plane Zeeman coupling, but it requires extremely small (unrealistic) quantum well widths or extremely fine tuning of the effective Land\'e factor which makes two Landau levels coincide. Landau level crossings can also be induced by the Rashba spin-orbit coupling and they promote the SQPT which can be obtained for certain values of the effective Land\'e factor and filling factors.

Understanding and Improving Critical Metrology. Quenching Superradiant Light-Matter Systems Beyond the Critical Point

We carefully examine critical metrology and present an improved critical quantum metrology protocol which relies on quenching a system exhibiting a superradiant quantum phase transition beyond its critical point. We show that this approach can lead to an exponential increase of the quantum Fisher information in time with respect to existing critical quantum metrology protocols relying on quenching close to the critical point and observing power law behaviour. We demonstrate that the Cramér-Rao bound can be saturated in our protocol through the standard homodyne detection scheme. We explicitly show its advantage using the archetypal setting of the Dicke model and explore a quantum gas coupled to a single-mode cavity field as a potential platform. In this case an additional exponential enhancement of the quantum Fisher information can in practice be observed with the number of atoms N in the cavity, even in the absence of N-body coupling terms.

Universal fluctuations and squeezing in a generalized Dicke model near the superradiant phase transition

In a view of recent proposals for the realization of anisotropic light-matter interaction in such platforms as (i) non-stationary or inductively and capacitively coupled superconducting qubits, (ii) atoms in crossed fields and (iii) semiconductor heterostructures with spin-orbital interaction, the concept of generalized Dicke model, where coupling strengths of rotating wave and counter-rotating wave terms are unequal, has attracted great interest. For this model, we study photon fluctuations in the critical region of normal-to-superradiant phase transition when both the temperatures and numbers of two-level systems are finite. In this case, the superradiant quantum phase transition is changed to a fluctuational region in the phase diagram that reveals two types of critical behaviors. These are regimes of Dicke model (with discrete $\mathbb{Z}_2$ symmetry), and that of (anti-) and Tavis-Cummings $U(1)$ models. We show that squeezing parameters of photon condensate in these regimes show distinct temperature scalings. Besides, relative fluctuations of photon number take universal values. We also find a temperature scales below which one approaches zero-temperature quantum phase transition where quantum fluctuations dominate. Our effective theory is provided by a non-Goldstone functional for condensate mode and by Majorana representation of Pauli operators. We also discuss Bethe ansatz solution for integrable $U(1)$ limits.

Resilience of the superradiant phase against A2 effects in the quantum Rabi dimer

We explore the quantum criticality of a two-site model combining quantum Rabi models with hopping interaction. Through a combination of analytical and numerical approaches, we find that the model allows the appearance of a superradiant quantum phase transition (QPT) even in the presence of strong $\mathbf{A}^2$ terms, preventing single-site superradiance. In the two-site model the effect of $\mathbf{A}^2$ terms can be surmounted by the photon delocalization from hopping, and a reversed superradiant QPT occurs as a consequence of the competition between $\mathbf{A}^2$ terms and the hopping interaction. We characterize the phase diagram and scaling functions, and extract the critical exponents in the vicinity of the critical point, thus establishing the universal behavior of the second-order phase transition. Remarkably the effective hopping strength will be enhanced if more cavities are cascaded. We also prove that the multi-qubit counterpart of the quantum Rabi dimer, i.e., the Dicke dimer, has the same properties in beating the $\mathbf{A}^2$ effect. Our work provides a way to the study of phase transitions in presence of the $\mathbf{A}^2$ terms and offers the prospect of investigating quantum-criticality physics and quantum devices in many-body systems.

Rashba Cavity QED: A Route Towards the Superradiant Quantum Phase Transition.

We develop a theory of cavity quantum electrodynamics for a 2D electron gas in the presence of Rashba spin-orbit coupling and perpendicular static magnetic field, coupled to spatially nonuniform multimode quantum cavity photon field. We demonstrate that the lowest polaritonic frequency of the full Hamiltonian can vanish for realistic parameters, achieving the Dicke superradiant quantum phase transition. This singular behavior originates from soft spin-flip transitions possessing a nonvanishing dipole moment at nonzero wave vectors and can be viewed as a static paramagnetic instability.

Single-Photon-Triggered Quantum Phase Transition

We propose a hybrid quantum model combining cavity QED and optomechanics, which allows the occurrence of equilibrium superradiant quantum phase transition (QPT) triggered by a single photon. This single-photon-triggered QPT exists both in the cases of ignoring and including the so-called $A^2$ term, i.e., it is immune to the no-go theorem. It originally comes from the photon-dependent quantum criticality featured by the proposed hybrid quantum model. Moreover, a reversed superradiant QPT is induced by the competition between the introduced $A^2$ term and the optomechanical interaction. This work offers an approach to manipulate QPT with a single photon, which should inspire the exploration of single-photon quantum-criticality physics and the engineering of new single-photon quantum devices.

Superradiant phase transition with graphene embedded in one dimensional optical cavity

We theoretically investigate the cavity QED of graphene embedded in an optical cavity under perpendicular magnetic field. We consider the coupling of cyclotron transition and a multimode cavity described by a multimode Dicke model. This model exhibits a superradiant quantum phase transition, which we describe exactly in an effective Hamiltonian approach. The complete excitation spectrum in both the normal phase and superradiant phase regimes is given. In contrast to the single mode case, multimode coupling of cavity photon and cyclotron transition can greatly reduce the critical vacuum Rabi frequency required for quantum phase transition, and dramatically enhance the superradiant emission by fast modulating the Hamiltonian. Our work paves a way to experimental explorations of quantum phase transitions in solid state systems.

Ultrastrong-coupling quantum-phase-transition phenomena in a few-qubit circuit QED system

We study ultrastrong-coupling quantum-phase-transition phenomena in a few-qubit system. In the one-qubit case, three second-order transitions occur and the Goldstone mode emerges under the condition of ultrastrong-coupling strength. Moreover, a first-order phase transition occurs between two different superradiant phases. In the two-qubit case, a two-qubit Hamiltonian with qubit-qubit interactions is analyzed fully quantum mechanically. We show that the quantum phase transition is inhibited even in the ultrastrong-coupling regime in this model. In addition, in the three-qubit model, the superradiant quantum phase transition is retrieved in the ultrastrong-coupling regime. Furthermore, the N-qubit model with U(1) symmetry is studied and we find that the superradiant phase transition is inhibited or restored with the qubit-number parity.

Nonergodicity in the Anisotropic Dicke Model.

We study the ergodic-nonergodic transition in a generalized Dicke model with independent corotating and counterrotating light-matter coupling terms. By studying level statistics, the average ratio of consecutive level spacings, and the quantum butterfly effect (out-of-time correlation) as a dynamical probe, we show that the ergodic-nonergodic transition in the Dicke model is a consequence of the proximity to the integrable limit of the model when one of the couplings is set to zero. This can be interpreted as a hint for the existence of a quantum analogue of the classical Kolmogorov-Arnold-Moser theorem. In addition, we show that there is no intrinsic relation between the ergodic-nonergodic transition and the precursors of the normal-superradiant quantum phase transition.

Probing the Dynamics of a Superradiant Quantum Phase Transition with a Single Trapped Ion.

We demonstrate that the quantum phase transition (QPT) of the Rabi model and critical dynamics near the QPT can be probed in the setup of a single trapped ion. We first demonstrate that there exists equilibrium and nonequilibrium scaling functions of the Rabi model by finding a proper rescaling of the system parameters and observables, and show that those scaling functions are representative of the universality class to which the Rabi model belongs. We then propose a scheme that can faithfully realize the Rabi model in the limit of a large ratio of the effective atomic transition frequency to the oscillator frequency using a single trapped ion and, therefore, the QPT. It is demonstrated that the predicted universal functions can indeed be observed based on our scheme. Finally, the effects of realistic noise sources on probing the universal functions in experiments are examined.

Collectively induced many-vortices topology via rotatory Dicke quantum phase transition

We examine the superradiance of a Bose–Einstein condensate pumped with a Laguerre–Gaussian laser of high winding number, e.g., . The laser beam transfers its orbital angular momentum (OAM) to the condensate at once due to the collectivity of the superradiance. An ℓ-fold rotational symmetric structure emerges with the rotatory superradiance. ℓ number of single-charge vortices appear at the arms of this structure. Even though the pump and the condensate profiles initially have cylindrical symmetry, we observe that it is broken to ℓ-fold rotational symmetry at the superradiance. Breaking of the cylindrical symmetry into the ℓ-fold symmetry and OAM transfer to the condensate become significant after the same critical pump strength. Reorganization of the condensate resembles the ordering in the experiment by Esslinger and colleagues (2010 Nature 264 1301). We numerically verify that the critical point for the onset of the reorganization, as well as the properties of the emitted pulse, conform to the characteristics of superradiant quantum phase transition.

Field-dependent superradiant quantum phase transition of molecular magnets in microwave cavities

We study a superradiant quantum phase transition in the model of triangular molecular magnets coupled to the electric component of a microwave cavity field. The transition occurs when the coupling strength exceeds a critical value, dc, which, in sharp contrast to the standard two-level emitters, can be tuned by an external magnetic field. In addition to emitted radiation, the molecules develop an in-plane electric dipole moment at the transition. We estimate that the transition can be detected in state-of-the-art microwave cavities if their electric field couples to a crystal containing a sufficient number of oriented molecules.

Dicke coupling by feasible local measurements at the superradiant quantum phase transition.

We address characterization of many-body superradiant systems and establish a fundamental connection between quantum criticality and the possibility of locally estimating the coupling constant, i.e., extracting its value by probing only a portion of the whole system. In particular, we consider Dicke-like superradiant systems made of an ensemble of two-level atoms interacting with a single-mode radiation field at zero effective temperature, and address estimation of the coupling by measurements performed only on radiation. At first, we obtain analytically the quantum Fisher information (QFI) and show that optimal estimation of the coupling may be achieved by tuning the frequency of the radiation field to drive the system toward criticality. The scaling behavior of the QFI at the critical point is obtained explicitly upon exploiting the symplectic formalism for Gaussian states. We then analyze the performances of feasible detection schemes performed only on the radiation subsystem, namely homodyne detection and photon counting, and show that the corresponding Fisher informations (FIs) approach the global QFI in the critical region. We thus conclude that criticality is a twofold resource. On the one hand, global QFI diverges at the critical point, i.e., the coupling may be estimated with the arbitrary precision. On the other hand, the FIs of feasible local measurements (which are generally smaller than the QFI out of the critical region), show the same scaling of the global QFI; i.e., optimal estimation of coupling may be achieved by locally probing the system, despite its strongly interacting nature.

Variational treatment of entanglement in the Dicke model

We introduce a variational ansatz for the Dicke model that extends mean-field theory through the inclusion of spin–oscillator correlations. The correlated variational state is obtained from the mean-field product state via a unitary transformation. The ansatz becomes correct in the limit of large oscillator frequency and in the limit of a large spin, for which it captures the leading quantum corrections to the classical limit exactly including the spin–oscillator entanglement entropy. We explain the origin of the unitary transformation before we show that the ansatz improves substantially upon mean-field theory, giving near exact results for the ground state energy and very good results for other observables. We then discuss why the ansatz still encounters problems in the transition regime at moderate spin lengths, where it fails to capture the precursors of the superradiant quantum phase transition faithfully. This observation illustrates the principal limits of semi-classical formulations, even after they are extended with correlations and entanglement.

Influence of Virtual Photon Process on the Generation of Squeezed Light from Atoms in an Optical Cavity

We show that a collection of two-level atoms in an optical cavity beyond the rotating wave approximation and in the dispersive-adiabatic and non-dispersive adiabatic regime constitutes a nonlinear medium and is capable of generating squeezed state of light. It is found that squeezing produced in the non-dispersive adiabatic regime is significantly high compared to that produced in the dispersive-adiabatic limit. On the other hand, we also show that it could be possible to observe the Dicke superradiant quantum phase transition in the dispersive-adiabatic regime where the Ã2 term is negligible. Such a system can be an essential component of a larger quantum-communication system.

Time-delayed feedback control of the Dicke–Hepp–Lieb superradiant quantum phase transition

We apply the time-delayed Pyragas control scheme to the dissipative Dicke model via a modulation of the atom-field-coupling. The feedback creates an infinite sequence of non-equilibrium phases with fixed points and limit cycles in the primary superradiant regime. We analyse this Hopf bifurcation scenario as a function of delay time and feedback strength and determine analytical conditions for the phase boundaries.