Superfluid Spin Transport Research Articles

Excitonic density wave and spin-valley superfluid in bilayer transition metal dichalcogenide

Artificial moiré superlattices in 2d van der Waals heterostructures are a new venue for realizing and controlling correlated electronic phenomena. Recently, twisted bilayer WSe2 emerged as a new robust moiré system hosting a correlated insulator at moiré half-filling over a range of twist angle. In this work, we present a theory of this insulating state as an excitonic density wave due to intervalley electron–hole pairing. We show that exciton condensation is strongly enhanced by a van Hove singularity near the Fermi level. Our theory explains the remarkable sensitivity of the insulating gap to the vertical electric field. In contrast, the gap is weakly reduced by a perpendicular magnetic field, with quadratic dependence at low field. The different responses to electric and magnetic field can be understood in terms of pair-breaking versus non-pair-breaking effects in a BCS analog of the system. We further predict superfluid spin transport in this electrical insulator, which can be detected by optical spin injection and spatial-temporal imaging.

Superfluid spin transport in magnetically ordered solids (Review article)

The paper reviews the theory of the long-distance spin superfluid transport in solid ferro- and antiferromagnets based on the analysis of the topology, the Landau criterion, and phase slips. Experiments reporting evidence of the existence of spin superfluidity are also overviewed.

Topological transport of vorticity in Heisenberg magnets

We study a robust topological transport carried by vortices in a thin film of an easy-plane ferromagnetic insulator between two metal contacts. A vortex, which is a nonlocal topological spin texture in two-dimensional magnets, exhibits some beneficial features as compared to skyrmions, which are local topological defects. In particular, the total topological charge carried by vorticity is robust against local fluctuations of the spin order-parameter magnitude. We show that an electric current in one of the magnetized metal contacts can pump vortices into the insulating bulk. Diffusion and nonlocal Coulomb-like interaction between these vortices will establish a steady-state vortex flow. Vortices leaving the bulk produce an electromotive force at another contact, which is related to the current-induced vorticity pumping by the Onsager reciprocity. The voltage signal decays algebraically with the separation between two contacts, similarly to a superfluid spin transport. Finally, the vorticity and closely related skyrmion type topological hydrodynamics are generalized to arbitrary dimensions, in terms of nonsingular order-parameter vector fields.

Superfluid spin transport in ferro- and antiferromagnets

This paper focuses on spin superfluid transport, observation of which was recently reported in antiferromagnet Cr$_2$O$_3$ [Yuan et al., Sci. Adv. 4, eaat1098 (2018)]. This paper analyzes the role of dissipation in transformation of spin current injected with incoherent magnons to a superfluid spin current near the interface where spin is injected. The Gilbert damping parameter in the Landau-Lifshitz-Gilbert theory does not describe dissipation properly, and the dissipation parameters are calculated from the Boltzmann equation for magnons scattered by defects. The two-fluid theory is developed similar to the two-fluid theory for superfluids. This theory shows that the influence of temperature variation in bulk on the superfluid spin transport (bulk Seebeck effect) is weak at low temperatures. The scenario that the results of Yuan et al. are connected with the Seebeck effect at the interface between the spin detector and the sample is also discussed. The Landau criterion for an antiferromagnet put in a magnetic field is derived from the spectrum of collective spin modes. The Landau instability starts in the gapped mode earlier than in the Goldstone gapless mode, in contrast to easy-plane ferromagnets where the Goldstone mode becomes unstable. The structure of the magnetic vortex in the geometry of the experiment is determined. The vortex core has the skyrmion structure with finite magnetization component normal to the magnetic field. This magnetization creates stray magnetic fields around the exit point of the vortex line from the sample, which can be used for experimental detection of vortices.

Spin hydrodynamics in amorphous magnets

Spin superfluidity, i.e., coherent spin transport mediated by topologically stable textures, is limited by parasitic anisotropies rooted in relativistic interactions and spatial inhomogeneities. Since structural disorder in amorphous magnets can average out the effect of these undesired couplings, we propose this class of materials as platforms for superfluid spin transport. We establish nonlinear equations describing the hydrodynamics of spin in insulating amorphous magnets, where the currents are defined in terms of coherent rotations of a noncollinear texture. Our theory includes dissipation and nonequilibrium torques at the interface with metallic reservoirs. This framework allows us to determine different regimes of coherent dynamics and their salient features in nonlocal magneto-transport measurements. Our work paves the way for future studies on macroscopic spin dynamics in materials with frustrated interactions.

Spin supercurrent and effect of quantum phase transition in the two-dimensional XY model

We have verified the influence of quantum phase transition on spin transport in the spin-1 two-dimensional XY model on the square lattice, with easy plane, single ion and exchange anisotropy. We analyze the effect of the phase transition from the Néel phase to the paramagnetic phase on the AC spin conductivity. Our results show a bit influence of the quantum phase transition on the conductivity. We also obtain a conventional spin transport for ω > 0 and an ideal spin transport in the limit of DC conductivity and therefore, a superfluid spin transport for the DC current in this limit. We have made the diagrammatic expansion for the Green-function with objective to include the effect exciton–exciton scattering on the results.

Magnetic Domain Walls as Hosts of Spin Superfluids and Generators of Skyrmions.

A domain wall in a magnet with easy-axis anisotropy is shown to harbor spin superfluid associated with its spontaneous breaking of the U(1) spin-rotational symmetry. The spin superfluid is shown to have several topological properties, which are absent in conventional superfluids. First, the associated phase slips create and destroy Skyrmions to obey the conservation of the total Skyrmion charge, which allows us to use a domain wall as a generator and detector of Skyrmions. Second, the domain wall engenders the emergent magnetic flux for magnons along its length, which are proportional to the spin supercurrent flowing through it, and thereby provides a way to manipulate magnons. Third, the spin supercurrent can be driven by the magnon current traveling across it owing to the spin transfer between the domain wall and magnons, leading to the magnonic manipulation of the spin superfluid. The theory for superfluid spin transport within the domain wall is confirmed by numerical simulations.

Spin superfluidity in the anisotropic XY model in the triangular lattice

Abstract We use the SU(3) Schwinger׳s boson theory to study the spin transport properties in the two-dimensional anisotropic frustrated Heisenberg model in the triangular lattice at T=0. We have investigated the behavior of the spin conductivity for this model which presents an single-ion anisotropy. We study the spin transport in the Bose-Einstein condensation regime where we have that the tz bosons are condensed and the following condition is valid: 〈 t z 〉 = 〈 t z † 〉 = t . Our results show a metallic spin transport for ω > 0 and a superfluid spin transport in the limit of DC conductivity, ω → 0 , where σ ( ω ) tends to infinity in this limit of ω.

Topological Effects on Quantum Phase Slips in Superfluid Spin Transport

We theoretically investigate effects of quantum fluctuations on superfluid spin transport through easy-plane quantum antiferromagnetic spin chains in the large-spin limit. Quantum fluctuations result in the decaying spin supercurrent by unwinding the magnetic order parameter within the easy plane, which is referred to as phase slips. We show that the topological term in the nonlinear sigma model for the spin chains qualitatively differentiates the decaying rate of the spin supercurrent between the integer versus half-odd-integer spin chains. An experimental setup for a magnetoelectric circuit is proposed, in which the dependence of the decaying rate on constituent spins can be verified by measuring the nonlocal magnetoresistance.

Thermally activated phase slips in superfluid spin transport in magnetic wires

We theoretically study thermally-activated phase slips in superfluid spin transport in easy-plane magnetic wires within the stochastic Landau-Lifshitz-Gilbert phenomenology, which runs parallel to the Langer-Ambegaokar-McCumber-Halperin theory for thermal resistances in superconducting wires. To that end, we start by obtaining the exact solutions for free-energy minima and saddle points. We provide an analytical expression for the phase-slip rate in the zero spin-current limit, which involves detailed analysis of spin fluctuations at extrema of the free energy. An experimental setup of a magnetoeletric circuit is proposed, in which thermal phase slips can be inferred by measuring nonlocal magnetoresistance.

Topological spin transport by Brownian diffusion of domain walls

We propose thermally-populated domain walls (DWs) in an easy-plane ferromagnetic insulator as robust spin carriers between two metals. The chirality of a DW, which serves as a topological charge, couples to the metal spin accumulation via spin-transfer torque and results in the chirality-dependent thermal nucleation rates of DWs at the interface. After overpopulated DWs of a particular (net) chirality diffuse and leave the ferromagnet at the other interface, they reemit the spin current by spin pumping. The conservation of the topological charge supports an algebraic decay of spin transport as the length of the ferromagnet increases; this is analogous to the decaying behavior of superfluid spin transport but contrasts with the exponential decay of magnon spin transport. We envision that similar spin transport with algebraic decay may be implemented in materials with exotic spin phases by exploiting topological characteristics and the associated conserved quantities of their excitations.

Nonlocal Magnetoresistance Mediated by Spin Superfluidity.

The electrical response of two diffusive metals is studied when they are linked by a magnetic insulator hosting a topologically stable (superfluid) spin current. We discuss how charge currents in the metals induce a spin supercurrent state, which in turn generates a magnetoresistance that depends on the topology of the electrical circuit. This magnetoresistance relies on phase coherence over the entire magnet and gives direct evidence for spin superfluidity. We show that driving the magnet with an ac current allows coherent spin transport even in the presence of U(1)-breaking magnetic anisotropy that can preclude dc superfluid transport. Spin transmission in the ac regime shows a series of resonance peaks as a function of frequency. The peak locations, heights, and widths can be used to extract static interfacial properties, e.g., the spin-mixing conductance and effective spin Hall angle, and to probe dynamic properties such as the spin-wave dispersion. Thus, ac transport may provide a simpler route to realizing nonequilbrium coherent spin transport and a useful way to characterize the magnetic system, serving as a precursor to the realization of dc superfluid spin transport.

Superfluid spin transport through antiferromagnetic insulators

A theoretical proposal for realizing and detecting spin supercurrent in an isotropic antiferromagnetic insulator is reported. Superfluid spin transport is achieved by inserting the antiferromagnet between two metallic reservoirs and establishing a spin accumulation in one reservoir such that a spin bias is applied across the magnet. We consider a class of bipartite antiferromagnets with Neel ground states, and temperatures well below the ordering temperature, where spin transport is mediated essentially by the condensate. Landau-Lifshitz and magneto-circuit theories are used to directly relate spin current in different parts of the heterostructure to the spin-mixing conductances characterizing the antiferromagnet|metal interfaces and the antiferromagnet bulk damping parameters, quantities all obtainable from experiments. We study the efficiency of spin angular-momentum transfer at an antiferromagnet|metal interface by developing a microscopic scattering theory for the interface and extracting the spin-mixing conductance for a simple model. Within the model, a quantitative comparison between the spin-mixing conductances obtained for the antiferromagnet|metal and ferromagnet|metal interfaces is made.

Superfluid spin transport through easy-plane ferromagnetic insulators.

Superfluid spin transport-dissipationless transport of spin-is theoretically studied in a ferromagnetic insulator with easy-plane anisotropy. We consider an open geometry where the spin current is injected into the ferromagnet from one side by a metallic reservoir with a nonequilibrium spin accumulation and ejected into another metallic reservoir located downstream. Spin transport is studied using a combination of magnetoelectric circuit theory, Landau-Lifshitz-Gilbert phenomenology, and microscopic linear-response theory. We discuss how spin superfluidity can be probed in a magnetically mediated negative electron-drag experiment.