Superconducting Tunnel Junctions Research Articles

Phase-tunable thermoelectricity in a Josephson junction

Superconducting tunnel junctions constitute the units of superconducting quantum circuits and are massively used both for quantum sensing and quantum computation. In previous works, we predicted the existence of a nonlinear thermoelectric effect in a electron-hole symmetric system, namely, a thermally biased tunnel junction between two different superconductors, where the Josephson effect is suppressed. In this paper we investigate the impact of the phase-coherent contributions on the thermoelectric effect, by tuning the size of the Josephson coupling changing the flux of a direct-current Superconducting Quantum Interference Device (dc-SQUID). For a suppressed Josephson coupling, the system generates a finite average thermoelectric signal, combined to an oscillation due to the standard ac Josephson phenomenology. At large Josephson couplings, the thermoelectricity induces an oscillatory behaviour with zero average value of the current/voltage with an amplitude and a frequency associated to the Josephson coupling strength, and ultimately tuned by the dc-SQUID magnetic flux. In conclusion, we demonstrate to be able to control the dynamics of the spontaneous breaking of the electron-hole symmetry. Furthermore, we compute how the flux applied to the dc-SQUID and the lumped elements of the circuit determine the frequency of the thermoelectric signal across the structure, and we envision a frequency modulation application.

The Influence of LO Power Heating of the Tunnel Junction on the Performance of THz SIS Mixers

We describe the performance of a superconductor- insulator-superconductor (SIS) mixer operating in the frequency range of 780-950 GHz. Unlike most SIS mixers, the tunnel junction employs two different superconductors, a niobium nitride top and a niobium bottom electrode sandwiching an aluminum nitride barrier layer, fabricated on a niobium titanium nitride ground plane. The mixer was tested in a pulse tube cryostat, with all the optical components, in the signal path, mounted inside the vacuum environment to avoid attenuation of the RF signal as it propagates from the hot/cold loads to the mixer. With this setup, we have measured an RF-corrected noise temperature of ~220 K. In this article, we focus on investigating the influence of local oscillator (LO) power heating on the performance of the terahertz mixer. The increase in the junction's physical temperature can be observed experimentally by noting the suppression of the gap voltage in the pumped current-voltage (I-V ) curve as the LO pumping level is increased. Similar observation has already been reported, and attempts were made to estimate the effective temperature of the device using equations of heat transfer between the mixer chip layers. Here, we present an experimental method of quantifying this effect by recovering the effective temperature of the junction through comparing the pumped I-V curves at different pumping levels and fixed bath temperature, with the unpumped I-V curves obtained at varying bath temperatures. We also estimate, for the first time, the effect of heating on the noise temperature as a function of bath temperature and frequency. We show that for typical experimental parameters, the LO heating can increase the double-sideband receiver noise temperature by as much as 20%, and that in the frequency range of the measurements, the effective temperature of the junction at fixed LO power increases linearly with frequency at a rate of 0.5 K/100 GHz.

A Compact Superconducting Heterodyne Focal Plane Array Implemented With HPI (Hybrid Planar Integration) Scheme

The article is concerned with the experimental evidence that proves technical feasibility of the hybrid planar integration (HPI) scheme that has been proposed to construct superconductor–insulator–superconductor (SIS) mixer focal plane arrays of unprecedented compactness. The scheme is characterized by the adoption of silicon membrane-based waveguide probes, which allows superconducting monolithic microwave integrated circuits to couple signal, and local oscillator (LO) from (computer numerical control)-machined waveguides through multiple paths. A $2\times 2$ dual-polarization balanced SIS mixer array has been implemented with this scheme, and assessed in $125 - \text{163}\,\text{GHz}$ RF band. This compact array has demonstrated uniform LO distribution, and low crosstalk between pixels. The RF performance of component pixels has been confirmed to be little affected by the high-degree integration. The potential implementation of the HPI scheme at THz frequencies is also discussed.

Superconductor-insulator transition in capacitively coupled superconducting nanowires.

We investigate superconductor–insulator quantum phase transitions in ultrathin capacitively coupled superconducting nanowires with proliferating quantum phase slips. We derive a set of coupled Berezinskii–Kosterlitz–Thouless-like renormalization group equations demonstrating that interaction between quantum phase slips in one of the wires gets modified due to the effect of plasma modes propagating in another wire. As a result, the superconductor–insulator phase transition in each of the wires is controlled not only by its own parameters but also by those of the neighboring wire as well as by mutual capacitance. We argue that superconducting nanowires with properly chosen parameters may turn insulating once they are brought sufficiently close to each other.

Quasi-Optical Characterization of Low-Loss Polymers at 300 GHz for Vacuum Window Applications

We report on the measurements of the complex refractive index of a number of low-loss polymers using a quasi-optical vector network analyzer operating in the frequency range of 210–370 GHz. The process of extracting both the real and imaginary parts of the refractive indexes is presented in this article, along with the method of error estimation. The measured refractive indexes of 25 different material samples, as well as the estimated error and the loss tangents of thicker samples, are tabulated. For selected materials, loss tangents have also been confirmed using the method of intersecting lines, which measures the additional input noise to a superconductor–insulator–superconductor receiver due to the dielectric sample. The data obtained from this work will be useful for the design of low-loss vacuum windows for cryogenic receivers operating in the 300-GHz range.

Distribution of Magnetic Field Strength along the Stationary Josephson Vortex in a Dirty S–I–S Junction

The results are presented from a numerical study of the joint effect of random quantum short circuits in a disordered layer of an insulator and nonzero temperatures $$0 \leqslant T < {{T}_{{\text{c}}}}$$ on the distribution of the magnetic field strength along the stationary Josephson vortex in a dirty superconductor–insulator–superconductor junction with nonmagnetic impurities in the insulator layer.

Quantum Response of a Bolometer Based on the SINIS Structure with a Suspended Absorber

Bolometers based on the superconductor–insulator–normal-metal–insulator–superconductor (SINIS) structure with an absorber suspended above the substrate are developed, fabricated, and experimentally studied in the terahertz frequency range. In contrast to the previously studied bolometers with an absorber located directly on the substrate, the real bolometric mode of operation is achieved, i.e., there is more than one excited electron per quantum of electromagnetic radiation (the quantum efficiency is larger than 1). A quantum efficiency of fifteen electrons per quantum of radiation with a frequency of 350 GHz was achieved in the studied bolometers.

SINIS Bolometer with Microwave Readout

A bolometer, which is based on a superconductor–insulator–normal metal–insulator–superconductor (SINIS) structure, integrated into a twin-slot antenna with a central frequency of 90 GHz, and connected with a superconducting microwave readout resonator, has been designed, fabricated, and experimentally studied. Such an elementary cell is designed for the multi-element array of a high-sensitive radioastronomic receiver, in which the readout from a great number of channels is performed by a single coaxial cable instead of separate wires and amplifier in each channel.

Demonstration of a wideband submillimeter-wave low-noise receiver with 4–21 GHz IF output digitized by a high-speed 32 GSps ADC

We report on a 275–500 GHz heterodyne receiver system in combination with a wideband intermediate-frequency (IF) backend to realize 17 GHz instantaneous bandwidth. The receiver frontend implements a heterodyne mixer module that integrates a superconductor-insulator-superconductor (SIS) mixer chip and a cryogenic low-noise preamplifier. The SIS mixer is developed based on high-current-density junction technologies to achieve a wideband radio frequency (RF) and IF bandwidth. The IF backend comprises an IF chain divided into two channels for 4.0–11.5 GHz and 11.3–21.0 GHz and an analog-to-digital converter (ADC) module that is capable of high-speed sampling at 32 Giga samples per second with 12.5 GHz bandwidth per channel and an effective number of bits of 6.5. The IF backend allows us to simultaneously cover the full 4–21 GHz IF range of the receiver frontend. The measured noise temperature of the receiver frontend was below three times the quantum noise (hf/kB) over the entire RF band. A dual-polarization sideband-separating receiver based on this technique could provide up to 64 GHz of instantaneous bandwidth, which demonstrates the possibility of future wideband radio astronomical observations with advanced submillimeter-wave heterodyne receivers.

Electronic Evolution from the Parent Mott Insulator to a Superconductor in Lightly Hole-Doped Bi2Sr2CaCu2O8 + δ**Supported by the National Natural Science Foundation of China (Grant Nos. 11888101, 11922414, and 11534007), the National Key Research and Development Program of China (Grant Nos. 2016YFA0300300 and 2017YFA0302900), the Strategic Priority Research Program (B) of the Chinese Academy of Sciences (Grant No. XDB25000000), the

High temperature superconductivity in cuprates is realized by doping the Mott insulator with charge carriers. A central issue is how such an insulating state can evolve into a conducting or superconducting state when charge carriers are introduced. Here, by in situ vacuum annealing and Rb deposition on the Bi2Sr2Ca0.6Dy0.4Cu2O8 + δ (Bi2212) sample surface to push its doping level continuously from deeply underdoped (Tc = 25 K, doping level p ∼ 0.066) to the near-zero doping parent Mott insulator, angle-resolved photoemission spectroscopy measurements are carried out to observe the detailed electronic structure evolution in the lightly hole-doped region for the first time. Our results indicate that the chemical potential lies at about l eV above the charge transfer band for the parent state at zero doping, which is quite close to the upper Hubbard band. With increasing hole doping, the chemical potential moves continuously towards the charge transfer band and the band structure evolution exhibits a rigid band shift-like behavior. When the chemical potential approaches the charge transfer band at a doping level of ∼0.05, the nodal spectral weight near the Fermi level increases, followed by the emergence of the coherent quasiparticle peak and the insulator–superconductor transition. Our observations provide key insights in understanding the insulator–superconductor transition in doping the parent cuprate compound and for establishing related theories.

Resonant Andreev reflections probed by photon-assisted tunnelling at the atomic scale

Tunneling across superconducting junctions proceeds by a rich variety of processes, which transfer single electrons, Cooper pairs, or even larger numbers of electrons by multiple Andreev reflections. Photon-assisted tunneling combined with the venerable Tien-Gordon model has long been a powerful tool to identify tunneling processes between superconductors. Here, we probe superconducting tunnel junctions including an impurity-induced Yu-Shiba-Rusinov (YSR) state by exposing a scanning tunneling microscope with a superconducting tip to microwave radiation. We find that a simple Tien-Gordon description describes tunneling of single electrons and Cooper pairs into the bare substrate, but breaks down for tunneling via YSR states by resonant Andreev reflections. We develop an improved theoretical description which is in excellent agreement with the data. Our results establish photon-assisted tunneling as a powerful tool to analyze tunneling processes at the atomic scale which should be particularly informative for unconventional and topological superconductors.

Stanene: A good platform for topological insulator and topological superconductor

Two dimensional (2D) topological insulators (TIs) and topological superconductors (TSCs) have been intensively studied for recent years due to its great potential for dissipationless electron transportation and fault-tolerant quantum computing, respectively. Here we focus on stanene, the tin analogue of graphene, to give a brief review of its development as a candidate for both 2D TI and TSC. Stanene is proposed to be a TI with a large gap of 0.3 eV, and its topological properties are sensitive to various factors, e.g., the lattice constants, chemical functionalization and layer thickness, which offer various methods for phase tunning. Experimentally, the inverted gap and edge states are observed recently, which are strong evidence for TI. In addition, stanene is also predicted to be a time reversal invariant TSC by breaking inversion symmetry, supporting helical Majorana edge modes. The layer-dependent superconductivity of stanene is recently confirmed by both transport and scanning tunneling microscopy measurements. This review gives a detailed introduction to stanene and its topological properties and some prospects are also discussed.

Superconducting X-ray detectors

Owing to their high sensitivity and low noise, superconducting detectors are used for photon detection from microwave to high-energy particles. X-ray detection plays an important role in materials analysis, astronomy, and medical radiography, which require high efficiency as well as high energy resolution. However, traditional semiconducting detectors cannot fulfill these requirements. In this article, we review superconducting quantum detectors for X-ray detection, including transition-edge sensor (TES), superconducting tunneling junctions (STJs), kinetic inductance detectors (KIDs) and superconducting nanowire single-photon detectors (SNSPDs), and introduce the physical structures, working mechanisms, and device behaviors of these detectors. We also review their performances regarding X-ray detection and analyze their respective characteristics. According to recent progress and the requirements of various applications, possible improvement of superconducting detectors for X-rays are discussed.

Direct Measurement of the Be7 L/K Capture Ratio in Ta-Based Superconducting Tunnel Junctions

We report a high-statistics measurement of the L/K orbital electron capture ratio in ^{7}Be embedded in cryogenic Ta. The thin Ta film formed part of a high-resolution superconducting tunnel junction radiation detector that was used to identify the signals from different decay channels. The measured L/K capture ratio of 0.070(7) is significantly larger than the only previous measurement of this quantity and the theoretical predictions that include in-medium effects. This value is a uniquely sensitive probe of the 1s and 2s orbital overlaps with the nucleus and is of relevance to nuclear and atomic physics, as well as Li production in novae and other astrophysical scenarios. This is the first experiment that uses superconducting tunnel junctions for nuclear-recoil detection, opening a new experimental avenue for low-energy precision measurements with rare isotopes.

Improved critical temperature of superconducting plasma-enhanced atomic layer deposition of niobium nitride thin films by thermal annealing

The efficiency of the superconducting radio frequency cavities composed of Nb required the deposition of thickness-controlled multilayer coatings of superconductor-insulator-superconductor (S-I-S) on the internal surfaces of the cavities. Herein, we report the plasma-enhanced atomic layer deposition of carbon-free NbN (50 µm thick), followed by a thermal treatment, to obtain the superconducting layer in the S-I-S structure. Using (tert-butylimido)-tris(diethylamino)-niobium as the niobium precursor and H2 and NH3 plasma as reactive gasses, the deposition and annealing parameters were optimized by studying their effects on the film properties (crystallinity, density, and composition). We demonstrated that the superconducting critical temperature (Tc) can be improved after thermal annealing up to 13.8 K, a value compatible with the targeted application. In addition to the expected densified layers and increased grain size, we observed a partial transformation of the oxide present in the as-deposited layer into niobium oxynitride, which could indicate the origin of the improvement of the superconducting properties. With low carbon and oxygen impurity concentrations in the films, this study contributes to the understanding of the relationship between the structure, composition, and superconductivity in NbN.

Feasibility of Laboratory-Based EXAFS Spectroscopy with Cryogenic Detectors.

Extended X-ray Absorption Fine Structure (EXAFS) spectroscopy is a powerful technique that gives element-specific information about the structure of molecules. The development of a laboratory EXAFS spectrometer capable of measuring transmission spectra would be a significant advance as the technique is currently only available at synchrotron radiation lightsources. Here, we explore the potential of cryogenic detectors as the energy resolving component of a laboratory transmission EXAFS instrument. We examine the energy resolution, count-rate, and detector stability needed for good EXAFS spectra and compare these to the properties of cryogenic detectors and conventional X-ray optics. We find that superconducting tunnel junction (STJ) detectors are well-suited for this application.

Development of embedded STJ for large format array X-ray detector

We have been developing an embedded superconducting tunnel junction (e-STJ) for a large-format array X-ray detector. Compared with the conventional STJ array, the e-STJ array is suitable for enlarging the detection area effectively because the e-STJ detector utilizes a three-dimensional packaging technology. To investigate the relationship between the fabrication method and the electric characteristics of the e-STJ, we designed and fabricated three types of simplified e-STJ and measured their subgap leakage current in the temperature range from 4.2 K to 0.3 K. We found that the roughness of the embedding hole on the Si substrate and the contact part between the embedded STJ and the side of the embedding hole affected the subgap leakage current.

Achieving μeV tunneling resolution in an in-operando scanning tunneling microscopy, atomic force microscopy, and magnetotransport system for quantum materials research.

Research in new quantum materials requires multi-mode measurements spanning length scales, correlations of atomic-scale variables with a macroscopic function, and spectroscopic energy resolution obtainable only at millikelvin temperatures, typically in a dilution refrigerator. In this article, we describe a multi-mode instrument achieving a μeV tunneling resolution with in-operando measurement capabilities of scanning tunneling microscopy, atomic force microscopy, and magnetotransport inside a dilution refrigerator operating at 10 mK. We describe the system in detail including a new scanning probe microscope module design and sample and tip transport systems, along with wiring, radio-frequency filtering, and electronics. Extensive benchmarking measurements were performed using superconductor-insulator-superconductor tunnel junctions, with Josephson tunneling as a noise metering detector. After extensive testing and optimization, we have achieved less than 8 μeV instrument resolving capability for tunneling spectroscopy, which is 5-10 times better than previous instrument reports and comparable to the quantum and thermal limits set by the operating temperature at 10 mK.

Signatures of the Higgs mode in transport through a normal-metal–superconductor junction

A superconductor subject to electromagnetic irradiation in the terahertz range can show amplitude oscillations of its order parameter. However, coupling this so-called Higgs mode to the charge current is notoriously difficult. We propose to achieve such a coupling in a particle-hole-asymmetric configuration using a DC-voltage-biased normal-metal--superconductor tunnel junction. Using the quasiclassical Green's function formalism, we demonstrate three characteristic signatures of the Higgs mode: (i) The AC charge current exhibits a pronounced resonant behavior and is maximal when the radiation frequency coincides with the order parameter. (ii) The AC charge current amplitude exhibits a characteristic nonmonotonic behavior with increasing voltage bias. (iii) At resonance for large voltage bias, the AC current vanishes inversely proportional to the bias. These signatures provide an electric detection scheme for the Higgs mode.

Tunneling spectroscopy of c -axis epitaxial cuprate junctions

Atomically precise epitaxial structures are unique systems for tunneling spectroscopy that minimize extrinsic effects of disorder. We present a systematic tunneling spectroscopy study, over a broad doping, temperature, and bias range, in epitaxial c-axis La$_{2-x}$Sr$_{x}$CuO$_{4}$/La$_{2}$CuO$_{4}$/La$_{2-x}$Sr$_{x}$CuO$_{4}$ heterostructures. The behavior of these superconductor/insulator/superconductor (SIS) devices is unusual. Down to 20 mK there is complete suppression of c-axis Josephson critical current with a barrier of only 2 nm of La$_{2}$CuO$_{4}$, and the zero-bias conductance remains at 20-30% of the normal-state conductance, implying a substantial population of in-gap states. Tunneling spectra show greatly suppressed coherence peaks. As the temperature is raised, the superconducting gap fills in rather than closing at $T_{c}$. For all doping levels, the spectra show an inelastic tunneling feature at $\sim$ 80 meV, suppressed as $T$ exceeds $T_{c}$. These nominally simple epitaxial cuprate junctions deviate markedly from expectations based on the standard Bardeen-Cooper-Schrieffer (BCS) theory.