Sum-frequency Mixing Process Research Articles

Picojoule-level supercontinuum generation in thin-film lithium niobate on sapphire.

We demonstrate ultraviolet-to-mid-infrared supercontinuum generation (SCG) inside thin-film lithium niobate (TFLN) on sapphire nanowaveguides. This platform combines wavelength-scale confinement and quasi-phasematched nonlinear interactions with a broad transparency window extending from 350 to 4500 nm. Our approach relies on group-velocity-matched second-harmonic generation, which uses an interplay between saturation and a small phase-mismatch to generate a spectrally broadened fundamental and second harmonic using only a few picojoules of in-coupled fundamental pulse energies. As the on-chip pulse energy is increased to tens of picojoules, these nanowaveguides generate harmonics up to the fifth order by a cascade of sum-frequency mixing processes. For in-coupled pulse energies in excess of 25 picojoules, these harmonics merge together to form a supercontinuum spanning 360-2660 nm. We use the overlap between the first two harmonic spectra to detect f-2f beatnotes of the driving laser directly at the waveguide output, which verifies the coherence of the generated harmonics. These results establish TFLN-on-sapphire as a viable platform for generating ultra-broadband coherent light spanning from the ultraviolet to mid-infrared spectral regions.

Single-shot fourth-order autocorrelator

The temporal contrast is one of the most important parameters of an ultra-high intense laser pulse. Third-order auto-correlator or cross-correlator have been widely used to characterize the temporal contrast of an ultra-intense laser pulse in the past decades. Here, a novel and simple single-shot fourth-order auto-correlator to characterize the temporal contrast with higher time resolution and better pulse contrast fidelity in comparison to third-order correlators is proposed. The single-shot fourth-order autocorrelation consists of a frequency degenerate four-wave mixing process and a sum-frequency mixing process. The proof-of-principle experiments show that a dynamic range of approximately 10^11 compared with the noise level, a time resolution of approximately 160 fs, and a time window of 65 ps can be successfully obtained using the novel single-shot fourth-order auto-correlator, which is the highest dynamic range with simultaneous high time resolution for single-shot temporal contrast measurement so far. Furthermore, the temporal contrast of laser pulse from a PW laser system is successfully measured in single-shot with a dynamic range of about 2*10^10 and simultaneous a time resolution of 160 fs.

Picosecond high-power 355-nm UV generation in CsLiB6O10 crystal.

We report third-harmonic generation (THG) at 355 nm in CsLiB6O10 (CLBO) by using sum-frequency mixing process. As a fundamental laser source, we employ a hybrid master oscillator power amplifier (MOPA) system seeded by a gain-switched laser diode (GS-LD) at 1064 nm to produce narrow spectral picosecond pulses. Both CLBO and walk-off compensated prism-coupled CLBO device generate over 30-W output of 355-nm UV lights, which means walk-off effect in CLBO is negligible in the picosecond laser system. The maximum THG conversion efficiency from the fundamental reaches about 48%, which is 1.2 times higher than that of LiB3O5 (LBO). Theoretical THG outputs with CLBO and LBO are numerically calculated in order to verify the validity of these experimental results in detail.

Tuning visible light generation based on multi-channel quasi-periodically poled LiTaO 3

We demonstrate broadband tuning visible light generation based on a multi-channel quasi-periodically poled LiTaO 3 crystal, in which a quasi-phase matched optical parametric generation process and a quasi-phase matched sum-frequency mixing process were achieved simultaneously. The conversion characters on spectrum and energy were studied by using a nanosecond pulse laser at 1.064 μm as pump light. We could tune the visible light over ~ 26 nm by means of changing the crystal's channel and temperature. The ratio of the output wavelength variation to that of temperature was ~ 0.07 nm/°C. The single-pass slope efficiency was 6.3% with the maximum output energy of 25 μJ.

Compact, passively Q-switched, all-solid-state master oscillator-power amplifier-optical parametric oscillator (MOPA-OPO) system pumped by a fiber-coupled diode laser generating high-brightness, tunable, ultraviolet radiation

We report on a compact, tunable ultraviolet laser system that consists of an optical parametric oscillator (OPO) and a longitudinally diode-pumped Nd:YAG master oscillator-power amplifier (MOPA). The pump energy for the whole laser system is supplied via a single delivery fiber. Nanosecond pulses are produced by an oscillator that is passively Q-switched by a Cr(4+):YAG crystal. The OPO is pumped by the second harmonic of the Nd:YAG MOPA. Continuously tunable radiation is generated by an intracavity sum-frequency mixing process within the OPO in the range of 245-260 nm with high beam quality. Maximum pulse energies of 1.2 mJ were achieved, which correspond to an optical efficiency of 3.75%, relating to the pulse energy of the MOPA at 1064 nm.

Cascaded third-harmonic generation in a single short-range-ordered nonlinear photonic crystal

Collinear third-harmonic generation at 526.7 nm was realized by the simultaneous phase matching of two second-order processes in a single quadratic crystal: second-harmonic generation (SHG) and sum-frequency mixing (SFM). The measured conversion efficiency was 12%. As a nonlinear medium a LiNbO(3) nonlinear photonic crystal with short-range order was used that allowed simultaneous phase matching by use of discrete reciprocal vector (for the SHG process) and continuous reciprocal vectors (for the SFM process). It was demonstrated that the third harmonic could be generated efficiently in such a crystal even if the intermediate process of SHG was not perfectly phase matched.

Investigation of passively synchronized dual-wavelength Q-switched lasers based on V:YAG saturable absorber

In this paper the results of a theoretical and experimental investigation of synchronized passive Q-switching of two Nd:YVO4-based solid-state lasers operating at two different wavelengths, is described. A V:YAG saturable absorbing material was used as a passive Q-switch performing the synchronization of the two laser fields. This material provides Q-switching operation at both 1064 and 1342 nm wavelengths simultaneously, saturating the same energy level. By adjusting the pump power of both lasers, it was possible to optimize the overlap of the two pulse trains and to switch between different states of synchronization. A theoretical model based on rate equations, which has been developed in order to investigate optical performance of the laser system, is in a good agreement with the experimental results. The principle of synchronized Q-switching can lead to new, pulsed all-solid-state light sources at new wavelengths based on sum-frequency mixing processes.

Efficient generation of green and UV light in a single PP-KTP waveguide pumped by a compact all-fiber system

We present simultaneous efficient second- (SHG) and third-harmonic generation (THG) in a single periodically-poled KTP waveguided crystal pumped by a compact femtosecond Yb-based laser in a condition of exactly phase-matched frequency doubling and nonphase-matched sum-frequency mixing processes. Internal conversion efficiency as high as 33% for SHG (532nm) and ∼2% for the cascaded THG (355nm) is reported. We believe this to be a clear experimental demonstration that strong third-harmonic can be generated in frequency doubling crystals through a nonphase-matched sum-frequency mixing process.

Multistep cascading in periodically poled directional couplers

We suggest a novel scheme for multistep cascaded parametric processes based on a periodically poled nonlinear directional coupler and derive the conditions for simultaneous phase matching of the second-harmonic generation and sum-frequency mixing processes. We predict an efficient wavelength conversion by the cascaded third-harmonic generation from the third optical communication window (1.53-1.56 microm) to visible in a LiNbO3 poled waveguide coupler.

Combustion exhaust measurements of nitric oxide with an ultraviolet diode-laser-based absorption sensor

A diode-laser-based sensor has been developed for ultraviolet absorption measurements of the nitric oxide (NO) molecule. The sensor is based on the sum-frequency mixing (SFM) of the output of a tunable, 395-nm external-cavity diode laser and a 532-nm diode-pumped, frequency-doubled Nd:YAG laser in a beta-barium borate crystal. The SFM process generates 325 +/- 75 nW of ultraviolet radiation at 226.8 nm, corresponding to the (v' = 0, v" = 0) band of the A2Sigma+-chi2II electronic transition of NO. Results from initial laboratory experiments in a gas cell are briefly discussed, followed by results from field demonstrations of the sensor for measurements in the exhaust streams of a gas turbine engine and a well-stirred reactor. It is demonstrated that the sensor is capable of fully resolving the absorption spectrum and accurately measuring the NO concentration in actual combustion environments. Absorption is clearly visible in the gas turbine exhaust even for the lowest concentrations of 9 parts per million (ppm) for idle conditions and for a path length of 0.51 m. The sensitivity of the current system is estimated at 0.23%, which corresponds to a detection limit of 0.8 ppm in 1 m for 1000 K gas. The estimated uncertainty in the absolute concentrations that we obtained using the sensor is 10%.

Quasi-phase-matched generation of tunable blue light in a quasi-periodic structure.

We present what is to our knowledge a new approach to generating tunable blue light by cascaded nonlinear frequency conversion in a single LiTaO3 crystal. Simultaneous quasi-phase matching of an optical parametric generation process and a sum-frequency mixing process is achieved by means of structuring the crystal with a quasi-periodic optical superlattice. The spectral (wavelength tuning and bandwidth) and power characteristics of the blue-light generation are studied with a fixed-wavelength 532-nm picosecond laser and a wavelength-tunable nanosecond optical parametric oscillator (OPO) as the pump sources. By tuning the OPO wavelength, we could tune the blue output over approximately 20 nm. Temperature tuning of the blue output at a fixed pump wavelength of 532 nm was limited to approximately 1.5 nm. A maximum blue power of 15 microW was generated at a pump power of 0.5 mW, corresponding to an efficiency of 3%.

Polarization properties of coherent VUV light at 125 nm generated by sum-frequency four-wave mixing in mercury

The polarization of the VUV light generated by four-wave sum-frequency mixing process ω4=2ω1+ω2 in mercury vapor at room temperature is analyzed in detail. Due to the specific two-photon transition used to enhance the nonlinear process, the polarization of the VUV wave is shown to be identical to the polarization of the wave at the frequency ω2. In particular, circularly polarized VUV is observed with degree of circular polarization exceeding 0.99.

Cross-phase modulation caused by cascading of third-order processes

The evolution of the phase of a weak signal wave (ω2) copropagating with a strong gate wave (ω1) in a centrosymmetric medium is studied analytically and numerically for the case when the two waves are involved in a nearly phase-matched third-order process that generates a third wave (ω3=2ω1+ω2). It is shown that the signal wave collects, in addition to the phase shift that is due to the ω2=ω1+ω2-ω1 process, an extra nonlinear phase shift caused by cascading of two third-order nonlinear processes, ω3=2ω1+ω2 and ω2=ω3-2ω1. The attractive feature of this new type of cross-phase modulation is the fact that one can control its magnitude and sign by changing the wave-vector mismatch of the sum-frequency mixing process and the gate intensity.

Effect of cubic nonlinearities on the sum-frequency generation process in asymmetric quantum wells

The effect of third-order nonlinear polarization on the sum-frequency mixing process has been theoretically investigated in an asymmetric InGaAs-AlAs quantum well. The effect of doping on the interband mixing process is considered. The cubic nonlinearities induced by a strong intersubband coupling field significantly modify the sum-frequency absorption process in doped structures.

Effect of cubic nonlinearities on the sum-frequency generation process in asymmetric quantum wells

The effect of third-order nonlinear polarization on the sum-frequency mixing process has been theoretically investigated in an asymmetric InGaAs-AlAs quantum well. The effect of doping on the interband mixing process is considered. The cubic nonlinearities induced by a strong intersubband coupling field significantly modify the sum-frequency absorption process in doped structures.

Spectrally compensated sum-frequency mixing scheme for generation of broadband radiation at 193 nm

A dispersively compensated scheme for sum-frequency mixing of broadband ultrashort laser pulses is reported. An increase of the bandwidth of the sum-frequency mixing process by 12 times compared with the noncompensated bandwidth of the given crystal has been demonstrated. Mixing radiation at 266 and 707 nm in a 1-mm-thick beta-barium metaborate crystal by using the compensated scheme results in an output bandwidth of 0.6 nm at 193 nm, which corresponds to a minimum output pulse duration of 90 fs.

Twice sum-frequency mixing of a dual-wavelength Nd:YALO3 laser to get 413.7-nm violet coherent radiation in LiIO3 crystal

A new method to obtain 413.7-nm violet coherent radiation by second-order sum-frequency mixing of the outputs (1341.4 and 1079.5 nm) of a double-wavelength Nd:YALO3 (Nd:YAP) laser in two LiIO3 crystals is reported. First, a 598.1-nm orange coherent radiation is obtained by sum-frequency mixing (SFM) of 1341.4- and 1079.5-nm radiations in a LiIO3 crystal, and then the 598.1- and 1341.4-nm radiations are mixed again in a second LiIO3 crystal to get 413.7-nm radiation. The phase-matching angles are obtained for both SFM processes. The experimental results agree well with calculated results.