States Of Open Quantum Systems Research Articles

Efficient steady-state solver for hierarchical quantum master equations.

Steady states play pivotal roles in many equilibrium and non-equilibrium open system studies. Their accurate evaluations call for exact theories with rigorous treatment of system-bath interactions. Therein, the hierarchical equations-of-motion (HEOM) formalism is a nonperturbative and non-Markovian quantum dissipation theory, which can faithfully describe the dissipative dynamics and nonlinear response of open systems. Nevertheless, solving the steady states of open quantum systems via HEOM is often a challenging task, due to the vast number of dynamical quantities involved. In this work, we propose a self-consistent iteration approach that quickly solves the HEOM steady states. We demonstrate its high efficiency with accurate and fast evaluations of low-temperature thermal equilibrium of a model Fenna-Matthews-Olson pigment-protein complex. Numerically exact evaluation of thermal equilibrium Rényi entropies and stationary emission line shapes is presented with detailed discussion.

A general framework for complete positivity

Complete positivity of quantum dynamics is often viewed as a litmus test for physicality, yet it is well known that correlated initial states need not give rise to completely positive evolutions. This observation spurred numerous investigations over the past two decades attempting to identify necessary and sufficient conditions for complete positivity. Here we describe a complete and consistent mathematical framework for the discussion and analysis of complete positivity for correlated initial states of open quantum systems. This formalism is built upon a few simple axioms and is sufficiently general to contain all prior methodologies going back to Pechakas, PRL (1994). The key observation is that initial system-bath states with the same reduced state on the system must evolve under all admissible unitary operators to system-bath states with the same reduced state on the system, in order to ensure that the induced dynamical maps on the system are well-defined. Once this consistency condition is imposed, related concepts like the assignment map and the dynamical maps are uniquely defined. In general, the dynamical maps may not be applied to arbitrary system states, but only to those in an appropriately defined physical domain. We show that the constrained nature of the problem gives rise to not one but three inequivalent types of complete positivity. Using this framework we elucidate the limitations of recent attempts to provide conditions for complete positivity using quantum discord and the quantum data-processing inequality. The problem remains open, and may require fresh perspectives and new mathematical tools. The formalism presented herein may be one step in that direction.

A Perturbative Method for Nonequilibrium Steady State of Open Quantum Systems

We develop a method of calculating the nonequilibrium steady state (NESS) of an open quantum system that is weakly coupled to reservoirs in different equilibrium states. We describe the system using a Redfield-type quantum master equation (QME). We decompose the Redfield QME into a Lindblad-type QME and the remaining part $\mathcal{R}$. Regarding the steady state of the Lindblad QME as the unperturbed solution, we perform a perturbative calculation with respect to $\mathcal{R}$ to obtain the NESS of the Redfield QME. The NESS thus determined is exact up to the first order in the system-reservoir coupling strength (pump/loss rate), which is the same as the order of validity of the QME. An advantage of the proposed method in numerical computation is its applicability to systems larger than those in methods of directly solving the original Redfield QME. We apply the method to a noninteracting fermion system to obtain an analytical expression of the NESS density matrix. We also numerically demonstrate the method in a nonequilibrium quantum spin chain.

Environmental dynamics, correlations, and the emergence of noncanonical equilibrium states in open quantum systems

Quantum systems are invariably open, evolving under surrounding influences rather than in isolation. Standard open quantum system methods eliminate all information on the environmental state to yield a tractable description of the system dynamics. By incorporating a collective coordinate of the environment into the system Hamiltonian, we circumvent this limitation. Our theory provides straightforward access to important environmental properties that would otherwise be obscured, allowing us to quantify the evolving system-environment correlations. As a direct result, we show that the generation of robust system-environment correlations that persist into equilibrium (heralded also by the emergence of non-Gaussian environmental states) renders the canonical system steady state almost always incorrect. The resulting equilibrium states deviate markedly from those predicted by standard perturbative techniques and are instead fully characterized by thermal states of the mapped system-collective coordinate Hamiltonian. We outline how noncanonical system states could be investigated experimentally to study deviations from canonical thermodynamics, with direct relevance to molecular and solid-state nanosystems.

Equilibrium states of open quantum systems in the strong coupling regime

In this work we investigate the late-time steady states of open quantum systems coupled to a thermal reservoir in the strong coupling regime. In general such systems do not necessarily relax to a Boltzmann distribution if the coupling to the thermal reservoir is nonvanishing or equivalently if the relaxation time scales are finite. Using a variety of nonequilibrium formalisms valid for non-Markovian processes, we show that starting from a product state of the closed system = system+environment, with the environment in its thermal state, the open system which results from coarse graining the environment will evolve towards an equilibrium state at late times. This state can be expressed as the reduced state of the closed system thermal state at the temperature of the environment. For a linear (harmonic) system and environment, which is exactly solvable, we are able to show in a rigorous way that all multitime correlations of the open system evolve towards those of the closed system thermal state. Multitime correlations are especially relevant in the non-Markovian regime, since they cannot be generated by the dynamics of the single-time correlations. For more general systems, which cannot be exactly solved, we are able to provide a general proof that all single-time correlations of the open system evolve to those of the closed system thermal state, to first order in the relaxation rates. For the special case of a zero-temperature reservoir, we are able to explicitly construct the reduced closed system thermal state in terms of the environmental correlations.

State transfer based on decoherence-free target state by Lyapunov-based control

We propose a Lyapunov-based control approach for state transfer based on the decoherence-free target state. The expected target state is constructed to be a decoherence-free state in a decoherence-free subspace (DFS) by an external laser field I, so that the system state can be decoupled from the environment, and no more decoherence process will occur. With the decoherence-free target state, we design a Lyapunov-based control field II to steer the given initial state to the decoherence-free state of open quantum systems as completely as possible, and decouple the system state from the environment at the same time. In the end, it is verified that the state transfer control designed comes true on a Λ-type four-level atomic system, and the system can stay on the decoherence-free target state without coupling to environment.

Avoiding dark states in open quantum systems by tailored initializations

We study the transport of excitations on a network of three coupled two-level systems that are subjected to an environment that induces incoherent hopping between the nodes. The two end nodes are coupled to a source while the central node is coupled to a drain. A common feature of these networks is the existence of a dark state that blocks the transport to the drain. Here we propose a means to avoid this state by a suitable initialization of the system, induced by a source that is common to both coupled nodes.

Equivalence of the effective Hamiltonian approach and the Siegert boundary condition for resonant states

AbstractTwo theoretical methods of finding resonant states in open quantum systems, namely the approach of the Siegert boundary condition and the Feshbach formalism, are reviewed and shown to be algebraically equivalent to each other for a simple model of the T‐type quantum dot. It is stressed that the seemingly Hermitian Hamiltonian of an open quantum system is implicitly non‐Hermitian outside the Hilbert space. The two theoretical approaches extract an explicitly non‐Hermitian effective Hamiltonian in a contracted space out of the seemingly Hermitian (but implicitly non‐Hermitian) full Hamiltonian in the infinite‐dimensional state space of an open quantum system.

Pointer states via engineered dissipation

Pointer states are long-lasting high-fidelity states in open quantum systems. We show how any pure state in a non-Markovian open quantum system can be made to behave as a pointer state by suitably engineering the coupling to the environment via open-loop periodic control. Engineered pointer states are constructed as approximate fixed points of the controlled open-system dynamics, in such a way that they are guaranteed to survive over a long time with a fidelity determined by the relative precision with which the dynamics is engineered. We provide quantitative minimum-fidelity bounds by identifying symmetry and ergodicity conditions that the decoherence-inducing perturbation must obey in the presence of control, and develop explicit pulse sequences for engineering any desired set of orthogonal states as pointer states. These general control protocols are validated through exact numerical simulations as well as semi-classical approximations in realistic single and two qubit dissipative systems. We also examine the role of control imperfections, and show that while pointer-state engineering protocols are highly robust in the presence of systematic pulse errors, the latter can also lead to unintended pointer-state generation in dynamical decoupling implementations, explaining the initial-state selectivity observed in recent experiments.

Stationary states of two-level open quantum systems

A problem of finding stationary states of open quantum systems is addressed. We focus our attention on a generic type of open system: a qubit coupled to its environment. We apply the theory of block operator matrices and find stationary states of two-level open quantum systems under certain conditions applied on both the qubit and the surrounding.

Resonant States of Open Quantum Systems

We first show that quantum resonant states observe particle number conservation and hence are consistent with the probabilistic interpretation of quantum mechanics. We then present for a class of quantum open systems, a resonant-state expansion of the sum of the retarded and advanced Green's functions. The expansion is given purely in terms of all discrete eigenstates and does not contain any background integrals. Using the expansion, we argue that the Fano asymmetry of resonance peaks is interpreted as interference between discrete eigenstates. We microscopically derive the Fano parameters for several cases.

Quantum-to-Classical Crossover of Quasibound States in Open Quantum Systems

In the semiclassical limit of open ballistic quantum systems, we demonstrate the emergence of instantaneous decay modes guided by classical escape faster than the Ehrenfest time. The decay time of the associated quasibound states is smaller than the classical time of flight. The remaining long-lived quasibound states obey random-matrix statistics, renormalized in compliance with the recently proposed fractal Weyl law for open systems [W.T. Lu, S. Sridhar, and M. Zworski, Phys. Rev. Lett. 91, 154101 (2003)]. We validate our theory numerically for a model system, the open kicked rotator.

Stationary states of relaxed open systems

Several different first-principle theories that are all potentially able to determine the long-time limit of states of open quantum systems are examined and critically compared in the formal second-order approximation. Because of a big parameter of the problem (increasing time), formal mathematical solution behind this second order exists just in the form of practically inapplicable formulae. Fortunately, in the second order, physical arguments could be given leading to a unique conclusion.

Pure stationary states of open quantum systems.

Using Liouville space and superoperator formalism we consider pure stationary states of open and dissipative quantum systems. We discuss stationary states of open quantum systems, which coincide with stationary states of closed quantum systems. Open quantum systems with pure stationary states of linear oscillator are suggested. We consider stationary states for the Lindblad equation. We discuss bifurcations of pure stationary states for open quantum systems which are quantum analogs of classical dynamical bifurcations.

Regularization of Quantum Relative Entropy in Finite Dimensions and Application to Entropy Production

The fundamental concept of relative entropy is extended to a functional that is regular-valued also on arbitrary pairs of nonfaithful states of open quantum systems. This regularized version preserves almost all important properties of ordinary relative entropy such as joint convexity and contractivity under completely positive quantum dynamical semigroup time evolution. On this basis a generalized formula for entropy production is proposed, the applicability of which is tested in models of irreversible processes. The dynamics of the latter is determined by either Markovian or non-Markovian master equations and involves all types of states.

Transitions between stationary states during a self-organization process of open quantum systems

A theoretical-informational description of self-organization processes during transitions between stationary states in open quantum systems is given. The S- and I-theorems about the change in quantum measures of the entropy and of the Kullbach discrimination information during the self-organization process are formulated. A nonparametric criterium of the ordering of states of a system is given. New extremal properties of mixed states of a self-organizing system are considered.