The tribological behavior of an addendum modified altered tooth sum optimized spur gear set were experimentally compared with that of the standard spur gear under several loading conditions including the wear morphology study and wear debris analysis. The temperature, viscosity, elastohydrodynamic oil film thickness, specific film thickness, and combined surface roughness variation under increasing operating load were analyzed experimentally. Finally, the performance impact of addendum shifted altered tooth sum optimized gear was examined. Results show that the tribological improvement strongly depends on the addendum alteration and modified tooth sum condition. The modification of the addendum in gears with a negatively altered tooth sum facilitates the transition from single-tooth contact to two-tooth contact, broadening the lubrication range while preserving optimal film thickness and improving wear resistance. However, it is reverse to decrease the film thickness and increase wear for standard and profile-modified positively altered tooth sum gear. The gear tribological performance can be significantly improved by profile modification and negatively altered tooth sum approach with a lower rate of degradation of oil and damage on the tooth contacting surface.