Spin Gas Research Articles

Many-body effects on second-order phase transitions in spinor Bose-Einstein condensates and breathing dynamics

We unravel the correlation effects of the second-order quantum phase transitions emerging on the ground state of a harmonically trapped spin-1 Bose gas, upon varying the involved Zeeman terms, as well as its breathing dynamics triggered by quenching the trapping frequency. It is found that the boundaries of the associated magnetic phases are altered in the presence of interparticle correlations for both ferromagnetic and anti-ferromagnetic spin-spin interactions, an effect which becomes more prominent in the few-body scenario. Most importantly, we unveil a correlation-induced shrinking of the anti-ferromagnetic and broken-axisymmetry phases implying that ground states with bosons polarized in a single spin-component are favored. Turning to the dynamical response of the spinor gas it is shown that its breathing frequency is independent of the system parameters while correlations lead to the formation of filamentary patterns in the one-body density of the participating components. The number of filaments is larger for increasing spin-independent interaction strengths or for smaller particle numbers. Each filament maintains its coherence and exhibits an anti-correlated behavior while distinct filaments show significant losses of coherence and are two-body correlated. Interestingly, we demonstrate that for an initial broken-axisymmetry phase an enhanced spin-flip dynamics takes place which can be tuned either via the linear Zeeman term or the quench amplitude.

Quantum Quench and Nonequilibrium Dynamics in Lattice-Confined Spinor Condensates.

We present an experimental study on nonequilibrium dynamics of a spinor condensate after it is quenched across a superfluid to Mott insulator (MI) phase transition in cubic lattices. Intricate dynamics consisting of spin-mixing oscillations at multiple frequencies are observed in time evolutions of the spinor condensate localized in deep lattices after the quantum quench. Similar spin dynamics also appear after spinor gases in the MI phase are suddenly moved away from their ground states via quenching magnetic fields. We confirm these observed spectra of spin-mixing dynamics can be utilized to reveal atom number distributions of an inhomogeneous system, and to study transitions from two-body to many-body dynamics. Our data also imply the nonequilibrium dynamics depend weakly on the quench speed but strongly on the lattice potential. This enables precise measurements of the spin-dependent interaction, a key parameter determining the spinor physics.

Preparing the spin-singlet state of a spinor gas in an optical cavity

We propose a method to prepare the spin singlet in an ensemble of integer-spin atoms confined within a high-finesse optical cavity. Using a cavity-assisted Raman transition to produce an effective Tavis-Cummings model, we show that a high fidelity spin singlet can be produced probabilistically, although with low efficiency, heralded by the \emph{absence} of photons escaping the cavity. In a different limit, a similar configuration of laser and cavity fields can be used to engineer a model that emulates spinor collisional dynamics. Borrowing from techniques used in spinor Bose-Einstein condensates, we show that adiabatic transformation of the system Hamiltonian (via a time-dependent, effective quadratic Zeeman shift) can be used to produce a low fidelity spin singlet. Then, by following this method with the aforementioned heralding technique, we show that it is possible to prepare the singlet state with both high fidelity and good efficiency for a large ensemble.

Mesoscopics of half-quantum vortex pair deconfinement in a trapped spin-one condensate

Motivated by a recent experiment in an antiferromagnetic spin-1 Bose-Einstein condensate of ${}^{23} \textrm{Na}$ atoms, we study the energetical stability of a singly quantum vortex injected into the center of a quasi-two-dimensional gas with zero total spin against dissocation into a pair of half-quantum vortices. We find that the critical dissociation point of this confinement-deconfinement type phase transition can be expressed in terms of the ratio of density-density ($c_0$) and spin-spin ($c_2$) coupling constants. The transition of bound to unbound vortices, in particular, sensitively depends on (1) the ratio of system size ($R$) to density healing length ($\xi_d$), and (2) the trap potential. Specifically, the critical ratio $(c_2 / c_0)_{\textrm{cr}}$ increases when $R / \xi_d$ decreases, and is relatively larger in a harmonic trap than in a box trap. Dissociation is energetically generally favored for $c_2 / c_0 < (c_2 / c_0)_{\textrm{cr}}$, which as a corollary implies that vortex dissociation is observed as well for negative $c_2 < 0$, e.g., in a rubidium spin-1 BEC, whereas in a sodium spin-1 BEC ($c_2>0$) it is energetically blocked above the critical ratio $(c_2 / c_0)_{\textrm{cr}}$. Tuning the coupling ratio $c_2/c_0$ by using microwave control techniques, the dependence of the deconfinement phase transition on coupling parameters, density, and system size we predict, can be verified in experiments with ultracold spinor gases.

Cavity QED Engineering of Spin Dynamics and Squeezing in a Spinor Gas.

We propose a method for engineering spin dynamics in ensembles of integer-spin atoms confined within a high-finesse optical cavity. Our proposal uses cavity-assisted Raman transitions to engineer a Dicke model for integer-spin atoms, which, in a dispersive limit, reduces to effective atom-atom interactions within the ensemble. This scheme offers a promising and flexible new avenue for the exploration of a wide range of spinor many-body physics. As an example of this, we present results showing that this method can be used to generate spin-nematic squeezing in an ensemble of spin-1 atoms. With realistic parameters, the scheme should enable substantial squeezing on time scales much shorter than current experiments with spin-1 Bose-Einstein condensates.

Phase Transitions in Definite Total Spin States of Two-Component Fermi Gases.

Second-order phase transitions have no latent heat and are characterized by a change in symmetry. In addition to the conventional symmetric and antisymmetric states under permutations of bosons and fermions, mathematical group-representation theory allows for non-Abelian permutation symmetry. Such symmetry can be hidden in states with defined total spins of spinor gases, which can be formed in optical cavities. The present work shows that the symmetry reveals itself in spin-independent or coordinate-independent properties of these gases, namely as non-Abelian entropy in thermodynamic properties. In weakly interacting Fermi gases, two phases appear associated with fermionic and non-Abelian symmetry under permutations of particle states, respectively. The second-order transitions between the phases are characterized by discontinuities in specific heat. Unlike other phase transitions, the present ones are not caused by interactions and can appear even in ideal gases. Similar effects in Bose gases and strong interactions are discussed.

Functions of State for Spinor Gas in General Relativity

The energy momentum tensor of perfect fluid is a simplified but successful model in astrophysics. In this paper, assuming the particles driven by gravity and moving along geodesics, we derived the functions of state in detail. The results show that, these functions have a little correction for the usual thermodynamics. The new functions naturally satisfy the causal condition and consist with relativity. For the self potentials of the particles we introduce an extra function $W$, which acts like negative pressure and can be used to describe dark matter. The results are helpful to understand the relation and interaction between space-time and matter.

Nonlinear Spinors as the Candidate of Dark Matter

In this paper, we discuss the equation of state for nonlinear spinor gases in the context of cosmology. The mean energy momentum tensor is similar to that of the prefect fluid, but an additional function of state $W$ is introduced to describe the nonlinear potential. The equation of state $w(a)\lesssim -1$ in the early universe is calculated, which provides a natural explanation for the negative pressure of dark matter and dark energy. $W$ may be also the main origin of the cosmological constant $\Lambda$. So the nonlinear spinor gases may be a candidate for dark matter and dark energy.

Bose-Fermi mapping and a multibranch spin-chain model for strongly interacting quantum gases in one dimension: Dynamics and collective excitations

We show that the wave function of a one dimensional spinor gas with contact $s$-wave interaction, either bosonic or fermionic, can be mapped to the direct product of the wave function of a spinless Fermi gas with short-range $p$-wave interaction and that of a spin system governed by spin parity projection operators. Applying this mapping to strongly interacting spinor gases, we obtain a generalized spin chain model that captures both the static and dynamics properties of the system. Using this spin chain model, we investigate the breathing mode frequency and the quench dynamics of strongly interacting harmonically trapped spinor gases.

Momentum distributions and numerical methods for strongly interacting one-dimensional spinor gases

One-dimensional spinor gases with strong $\ensuremath{\delta}$ interaction fermionize and form a spin chain. The spatial degrees of freedom of this atom chain can be described by a mapping to spinless noninteracting fermions and the spin degrees of freedom are described by a spin-chain model with nearest-neighbor interactions. Here, we compute momentum and occupation-number distributions of up to 16 strongly interacting spinor fermions and bosons as a function of their spin imbalance, the strength of an externally applied magnetic field gradient, the length of their spin, and for different excited states of the multiplet. We show that the ground-state momentum distributions resemble those of the corresponding noninteracting systems, apart from flat background distributions, which extend to high momenta. Moreover, we show that the spin order of the spin chain---in particular antiferromagnetic spin order---may be deduced from the momentum and occupation-number distributions of the system. Finally, we present efficient numerical methods for the calculation of the single-particle densities and one-body density matrix elements and of the local exchange coefficients of the spin chain for large systems containing more than 20 strongly interacting particles in arbitrary confining potentials.

Upper bound of one-magnon excitation and lower bound of effective mass for ferromagnetic spinor Bose and Fermi gases

Using a variational method, we derive an exact upper bound for one-magnon excitation energy in ferromagnetic spinor gases, which limits the quantum corrections to the effective mass of a magnon to be positive. We also derive an upper bound for one-magnon excitation energy in lattice systems. The results hold for both Bose and Fermi systems in $d$ dimensions as long as the interaction is local and invariant under spin rotation.

Quantum magnetism without lattices in strongly interacting one-dimensional spinor gases

We show that strongly interacting multicomponent gases in one dimension realize an effective spin chain, offering an alternative simple scenario for the study of one-dimensional (1D) quantum magnetism in cold gases in the absence of an optical lattice. The spin-chain model allows for an intuitive understanding of recent experiments and for a simple calculation of relevant observables. We analyze the adiabatic preparation of antiferromagnetic and ferromagnetic ground states, and show that many-body spin states may be efficiently probed in tunneling experiments. The spin-chain model is valid for more than two components, opening the possibility of realizing SU(N) quantum magnetism in strongly interacting 1D alkaline-earth-metal or ytterbium Fermi gases.

Density-functional theory for the spin-1 bosons in a one-dimensional harmonic trap

We propose the density-functional theory for one-dimensional harmonically trapped spin-1 bosons in the ground state with repulsive density-density interaction and anti-ferromagnetic spin-exchange interaction. The density distributions of spin singlet paired bosons and polarized bosons with different total polarization for various interaction parameters are obtained by solving the Kohn-Sham equations which are derived based on the local density approximation and the Bethe ansatz exact results for homogeneous system. Non-monotonicity of the central densities is attributed to the competition between the density interaction and spin-exchange. The results reveal the phase separation of the paired and polarized bosons, the density profiles of which respectively approach the Tonks-Girardeau gases of Bose-Bose pairs and scalar bosons in the case of strong interaction. We give the R-P phase diagram at strong interaction and find the critical polarization, which paves the way to direct observe the exotic singlet pairing in spinor gas experimentally.

Antiferromagnetic Spatial Ordering in a Quenched One-Dimensional Spinor Gas

We have experimentally observed the emergence of spontaneous antiferromagnetic spatial order in a sodium spinor Bose-Einstein condensate that was quenched through a magnetic phase transition. For negative values of the quadratic Zeeman shift, a gas initially prepared in the F=1, m(F)=0 state collapsed into a dynamically evolving superposition of all three spin projections, m(F)=0, ±1. The quench gave rise to rich, nonequilibrium behavior where both nematic and magnetic spin waves were generated. We characterized the spatiotemporal evolution through two particle correlations between atoms in each pair of spin states. These revealed dramatic differences between the dynamics of the spin correlations and those of the spin populations.

Coherent multi-flavour spin dynamics in a fermionic quantum gas

Microscopic spin interaction processes are fundamental for global static and dynamical magnetic properties of many-body systems. Quantum gases as pure and well isolated systems offer intriguing possibilities to study basic magnetic processes including non-equilibrium dynamics. Here, we report on the realization of a well-controlled fermionic spinor gas in an optical lattice with tunable effective spin ranging from 1/2 to 9/2. We observe long-lived intrinsic spin oscillations and investigate the transition from two-body to many-body dynamics. The latter results in a spin-interaction driven melting of a band insulator. Via an external magnetic field we control the system's dimensionality and tune the spin oscillations in and out of resonance. Our results open new routes to study quantum magnetism of fermionic particles beyond conventional spin 1/2 systems.

Long-time-scale dynamics of spin textures in a degenerateF=187Rb spinor Bose gas

We investigate the long-term dynamics of spin textures prepared by cooling unmagnetized spinor gases of $F=1$ ${}^{87}$Rb to quantum degeneracy, observing domain coarsening and a strong dependence of the equilibration dynamics on the quadratic Zeeman shift $q$. For small values of $|q|$, the textures arrive at a configuration independent of the initial spin-state composition, characterized by large length-scale spin domains and the establishment of easy-axis (negative $q$) or easy-plane (positive $q$) magnetic anisotropy. For larger $|q|$, equilibration is delayed as the spin-state composition of the degenerate spinor gas remains close to its initial value. These observations support the mean-field equilibrium phase diagram predicted for a ferromagnetic spinor Bose-Einstein condensate and also illustrate that equilibration is achieved under a narrow range of experimental settings, making the $F=1$ ${}^{87}$Rb gas more suitable for studies of nonequilibrium quantum dynamics.

Bilinear-biquadratic spin-1 chain undergoing quadratic Zeeman effect

The Heisenberg model for spin-1 bosons in one dimension presents many different quantum phases, including the famous topological Haldane phase. Here we study the robustness of such phases in front of a SU(2) symmetry-breaking field as well as the emergence of unique phases. Previous studies have analyzed the effect of such uniaxial anisotropy in some restricted relevant points of the phase diagram. Here we extend those studies and present the complete phase diagram of the spin-1 chain with uniaxial anisotropy. To this aim, we employ the density-matrix renormalization group together with analytical approaches. The complete phase diagram can be realized using ultracold spinor gases in the Mott insulator regime under a quadratic Zeeman effect.

Polar phase of one-dimensional bosons with large spin

Spinor ultracold gases in one dimension (1D) represent an interesting example of strongly correlated quantum fluids. They have a rich phase diagram and exhibit a variety of quantum phase transitions. We consider a 1D spinor gas of bosons with a large spin S. A particular example is the gas of chromium atoms (S=3), where the dipolar collisions efficiently change the magnetization and make the system sensitive to the linear Zeeman effect. We argue that in 1D the most interesting effects come from the pairing interaction. If this interaction is negative, it gives rise to a (quasi)condensate of singlet bosonic pairs with an algebraic order at zero temperature, and for (2S+1)≫1 the saddle point approximation leads to physically transparent results. Since in 1D one needs a finite energy to destroy a pair, the spectrum of spin excitations has a gap. Hence, in the absence of a magnetic field, there is only one gapless mode corresponding to phase fluctuations of the pair quasicondensate. Once the magnetic field exceeds the gap, another condensate emerges, namely the quasicondensate of unpaired bosons with spins aligned along the magnetic field. The spectrum then contains two gapless modes corresponding to the singlet-paired and spin-aligned unpaired Bose condensed particles, respectively. At T=0, the corresponding phase transition is of the commensurate–incommensurate type.

Universal Thermometry for Quantum Simulation

Quantum simulation is a highly ambitious program in cold atom research currently being pursued in laboratories worldwide. The goal is to use cold atoms in optical lattices to simulate models for unsolved strongly correlated systems, so as to deduce their properties directly from experimental data. An important step in this effort is to determine the temperature of the system, which is essential for deducing all thermodynamic functions. This step, however, remains difficult for lattice systems at the moment. Here, we propose a method based on a generalized fluctuation-dissipation theorem. It does not rely on numerical simulations and gives a universal thermometry scheme for quantum gas systems including mixtures and spinor gases, provided that the local density approximation is valid.

Ground states of a mixture of two species of spinor Bose gases with interspecies spin exchange

We consider a mixture of two species of spin-1 atoms with interspecies spin exchange, which may cooperate or compete with intraspecies spin exchanges and thus dramatically affect the ground state. It represents a new class of bosonic gases differing from single-species spinor gases. We determine the exact ground states in several parameter regimes and study the composite structures using the generating function method generalized here to be applicable to a mixture of two species of spinor gases. The most interesting phase is the so-called entangled Bose-Einstein condensation (BEC), which is fragmented BEC with quantum entanglement between the two species and with both interspecies and intraspecies singlet pairs. For comparison, we also apply the generating function method to a mixture of two species of pseudospin-$\frac{1}{2}$ atoms, for which the total spin quantum number of each species is fixed as half of the atom number, in contrast with the case of spin $1$, for which it is a variable determined by energetics. Consequently, singlet pairs in entangled BEC of a pseudospin-$\frac{1}{2}$ mixture are all interspecies. Interspecies spin exchange leads to novel features beyond those of spinor BEC of a single species of atoms as well as mixtures without interspecies spin exchange.