Spin-rotation Symmetry Research Articles

Spin Hall effect emerging from a noncollinear magnetic lattice without spin–orbit coupling

The spin Hall effect (SHE), which converts a charge current into a transverse spin current, has long been believed to be a phenomenon induced by spin–orbit coupling. Here, we identify an alternative mechanism to realize the intrinsic SHE through a noncollinear magnetic structure that breaks the spin rotation symmetry. No spin–orbit coupling is needed even when the scalar spin chirality vanishes, different from the case of the topological Hall effect and topological SHE reported previously. In known noncollinear antiferromagnetic compounds Mn3X (X = Ga, Ge, and Sn), for example, we indeed obtain large spin Hall conductivities based on ab initio calculations.

Persistent spin helix manipulation by optical doping of a CdTe quantum well

Time-resolved Kerr-rotation microscopy explores the influence of optical doping on the persistent spin helix in a [001]-grown CdTe quantum well at cryogenic temperatures. Electron spin diffusion dynamics reveal a momentum-dependent effective magnetic field providing SU(2) spin-rotation symmetry, consistent with kinetic theory. The Dresselhaus and Rashba spin-orbit coupling parameters are extracted independently from rotating the spin helix with external magnetic fields applied parallel and perpendicular to the effective magnetic field. Most importantly, a non-uniform spatiotemporal precession pattern is observed. The kinetic theory framework of spin diffusion allows for modeling of this finding by incorporating the photocarrier density into the Rashba ($\alpha$) and the Dresselhaus ($\beta_3$) parameters. Corresponding calculations are further validated by an excitation-density dependent measurement. This work shows universality of the persistent spin helix by its observation in a II-VI compound and the ability to fine-tune it by optical doping.

Symmetry enriched U(1) quantum spin liquids

We classify and characterize three dimensional $U(1)$ quantum spin liquids (deconfined $U(1)$ gauge theories) with global symmetries. These spin liquids have an emergent gapless photon and emergent electric/magnetic excitations (which we assume are gapped). We first discuss in great detail the case with time reversal and $SO(3)$ spin rotational symmetries. We find there are 15 distinct such quantum spin liquids based on the properties of bulk excitations. We show how to interpret them as gauged symmetry-protected topological states (SPTs). Some of these states possess fractional response to an external $SO(3)$ gauge field, due to which we dub them "fractional topological paramagnets". We identify 11 other anomalous states that can be grouped into 3 anomaly classes. The classification is further refined by weakly coupling these quantum spin liquids to bosonic Symmetry Protected Topological (SPT) phases with the same symmetry. This refinement does not modify the bulk excitation structure but modifies universal surface properties. Taking this refinement into account, we find there are 168 distinct such $U(1)$ quantum spin liquids. After this warm-up we provide a general framework to classify symmetry enriched $U(1)$ quantum spin liquids for a large class of symmetries. As a more complex example, we discuss $U(1)$ quantum spin liquids with time reversal and $Z_2$ symmetries in detail. Based on the properties of the bulk excitations, we find there are 38 distinct such spin liquids that are anomaly-free. There are also 37 anomalous $U(1)$ quantum spin liquids with this symmetry. Finally, we briefly discuss the classification of $U(1)$ quantum spin liquids enriched by some other symmetries.

Topological Z2 resonating-valence-bond spin liquid on the square lattice

A one-parameter family of long-range resonating valence bond (RVB) state on the square lattice was previously proposed to describe a critical spin liquid (SL) phase of the spin-$1/2$ frustrated Heisenberg model. We provide evidence that this RVB state in fact also realises a topological (long-range entangled) $\mathbb{Z}_2$ SL, limited by two transitions to critical SL phases. The topological phase is naturally connected to the $\mathbb{Z}_2$ gauge symmetry of the local tensor. This work shows that, on one hand, spin-$1/2$ topological SL with $C_{4v}$ point group symmetry and $SU(2)$ spin rotation symmetry exists on the square lattice and, on the other hand, criticality and nonbipartiteness are compatible. We also point out that, strong similarities between our phase diagram and the ones of classical interacting dimer models suggest both can be described by similar Kosterlitz-Thouless transitions. This scenario is further supported by the analysis of the one-dimensional boundary state.

Pauli metallic ground state in Hubbard clusters with Rashba spin-orbit coupling

We study the ``phase diagram'' of a Hubbard plaquette with Rashba spin-orbit coupling. We show that the peculiar way in which Rashba coupling breaks the spin-rotational symmetry of the Hubbard model allows a mixing of singlet and triplet components in the ground state that slows down and changes the nature of the Mott transition and of the Mott insulating phases.

Prediction of a magnetic Weyl semimetal without spin-orbit coupling and strong anomalous Hall effect in the Heusler compensated ferrimagnet Ti2MnAl

We predict a magnetic Weyl semimetal in the inverse Heusler Ti2MnAl, a compensated ferrimagnet with a vanishing net magnetic moment and a Curie temperature of over 650 K. Despite the vanishing net magnetic moment, we calculate a large intrinsic anomalous Hall effect (AHE) of about 300 S/cm. It derives from the Berry curvature distribution of the Weyl points, which are only 14 meV away from the Fermi level and isolated from trivial bands. Different from antiferromagnets Mn3X (X= Ge, Sn, Ga, Ir, Rh, and Pt), where the AHE originates from the non-collinear magnetic structure, the AHE in Ti2MnAl stems directly from the Weyl points and is topologically protected. The large anomalous Hall conductivity (AHC) together with a low charge carrier concentration should give rise to a large anomalous Hall angle. In contrast to the Co-based ferromagnetic Heusler compounds, the Weyl nodes in Ti2MnAl do not derive from nodal lines due to the lack of mirror symmetries in the inverse Heusler structure. Since the magnetic structure breaks spin-rotation symmetry, the Weyl nodes are stable without SOC. Moreover, because of the large separation between Weyl points of opposite topological charge, the Fermi arcs extent up to 75% of the reciprocal lattice vectors in length. This makes Ti2MnAl an excellent candidate for the comprehensive study of magnetic Weyl semimetals. It is the first example of a material with Weyl points, large anomalous Hall effect and angle despite a vanishing net magnetic moment.

Fermionic Spinon Theory of Square Lattice Spin Liquids near the Néel State

Quantum fluctuations of the N\'eel state of the square lattice antiferromagnet are usually described by a $\mathbb{CP}^1$ theory of bosonic spinons coupled to a U(1) gauge field, and with a global SU(2) spin rotation symmetry. Such a theory also has a confining phase with valence bond solid (VBS) order, and upon including spin-singlet charge 2 Higgs fields, deconfined phases with $\mathbb{Z}_2$ topological order possibly intertwined with discrete broken global symmetries. We present dual theories of the same phases starting from a mean-field theory of fermionic spinons moving in $\pi$-flux in each square lattice plaquette. Fluctuations about this $\pi$-flux state are described by 2+1 dimensional quantum chromodynamics (QCD$_3$) with a SU(2) gauge group and $N_f=2$ flavors of massless Dirac fermions. It has recently been argued by Wang et al. (arXiv:1703.02426) that this QCD$_3$ theory describes the N\'eel-VBS quantum phase transition. We introduce adjoint Higgs fields in QCD$_3$, and obtain fermionic dual descriptions of the phases with $\mathbb{Z}_2$ topological order obtained earlier using the bosonic $\mathbb{CP}^1$ theory. We also present a fermionic spinon derivation of the monopole Berry phases in the U(1) gauge theory of the VBS state. The global phase diagram of these phases contains multi-critical points, and our results imply new boson-fermion dualities between critical gauge theories of these points.

Topology and symmetry of surface Majorana arcs in cyclic superconductors

We study the topology and symmetry of surface Majorana arcs in superconductors with nonunitary "cyclic" pairing. Cyclic $p$-wave pairing may be realized in a cubic or tetrahedral crystal, while it is a candidate for the interior $^3P_2$ superfluids of neutron stars. The cyclic state is an admixture of full gap and nodal gap with eight Weyl points and the low-energy physics is governed by itinerant Majorana fermions. We here show the evolution of surface states from Majorana cone to Majorana arcs under rotation of surface orientation. The Majorana cone is protected solely by an accidental spin rotation symmetry and fragile against spin-orbit coupling, while the arcs are attributed to two topological invariants: the first Chern number and one-dimensional winding number. Lastly, we discuss how topologically protected surface states inherent to the nonunitary cyclic pairing can be captured from surface probes in candidate compounds, such as U$_{1-x}$Th$_{x}$Be$_{13}$. We examine tunneling conductance spectra for two competitive scenarios in U$_{1-x}$Th$_{x}$Be$_{13}$---the degenerate $E_u$ scenario and the accidental scenario.

Two Topologically Distinct Dirac-Line Semimetal Phases and Topological Phase Transitions in Rhombohedrally Stacked Honeycomb Lattices

Three-dimensional topological semimetals can support band crossings along one-dimensional curves in the momentum space (nodal lines or Dirac lines) protected by structural symmetries and topology. We consider rhombohedrally (ABC) stacked honeycomb lattices supporting Dirac lines protected by time-reversal, inversion and spin rotation symmetries. For typical band structure parameters there exists a pair of nodal lines in the momentum space extending through the whole Brillouin zone in the stacking direction. We show that these Dirac lines are topologically distinct from the usual Dirac lines which form closed loops inside the Brillouin zone. In particular, an energy gap can be opened only by first merging the Dirac lines going through the Brillouin zone in a pairwise manner so that they turn into closed loops inside the Brillouin zone, and then by shrinking these loops into points. We show that this kind of topological phase transition can occur in rhombohedrally stacked honeycomb lattices by tuning the ratio of the tunneling amplitudes in the directions perpendicular and parallel to the layers. We also discuss the properties of the surface states in the different phases of the model.

Ising order in a magnetized Heisenberg chain subject to a uniform Dzyaloshinskii-Moriya interaction

We report a combined analytical and density matrix renormalized group study of the antiferromagnetic XXZ spin-1/2 Heisenberg chain subject to a uniform Dzyaloshinskii-Moriya (DM) interaction and a transverse magnetic field. The numerically determined phase diagram of this model, which features two ordered Ising phases and a critical Luttinger liquid one with fully broken spin-rotational symmetry, agrees well with the predictions of Garate and Affleck [Phys. Rev. B 81, 144419 (2010)]. We also confirm the prevalence of the N z N\'eel Ising order in the regime of comparable DM and magnetic field magnitudes.

Emergent Ising degrees of freedom above a double-stripe magnetic ground state

Double-stripe magnetism $[\mathbf{Q}=(\pi/2, \pi/2)]$ has been proposed as the magnetic ground state for both the iron-telluride and BaTi$_2$Sb$_2$O families of superconductors. Double-stripe order is captured within a $J_1-J_2-J_3$ Heisenberg model in the regime $J_3 \gg J_2 \gg J_1$. Intriguingly, besides breaking spin-rotational symmetry, the ground state manifold has three additional Ising degrees of freedom associated with bond-ordering. Via their coupling to the lattice, they give rise to an orthorhombic distortion and to two non-uniform lattice distortions with wave-vector $(\pi, \pi)$. Because the ground state is four-fold degenerate, modulo rotations in spin space, only two of these Ising bond order parameters are independent. Here we introduce an effective field theory to treat all Ising order parameters, as well as magnetic order, and solve it within a large-$N$ limit. All three transitions, corresponding to the condensations of two Ising bond order parameters and one magnetic order parameter are simultaneous and first order in three dimensions, but lower dimensionality, or equivalently weaker interlayer coupling, and weaker magnetoelastic coupling can split the three transitions, and in some cases allows for two separate Ising phase transitions above the magnetic one.

Topological spinon bands and vison excitations in spin-orbit coupled quantum spin liquids

Spin liquids are exotic quantum states characterized by the existence of fractional and deconfined quasiparticle excitations, referred to as spinons and visons. Their fractional nature establishes topological properties such as a protected ground-state degeneracy. This work investigates spin-orbit coupled spin liquids where, additionally, topology enters via non-trivial band structures of the spinons. We revisit the $Z_2$ spin-liquid phases that have recently been identified in a projective symmetry-group analysis on the square lattice when spin-rotation symmetry is maximally lifted [Phys. Rev. B 90, 174417 (2014)]. We find that in the case of nearest neighbor couplings only, $Z_2$ spin liquids on the square lattice always exhibit trivial spinon bands. Adding second neighbor terms, the simplest projective symmetry-group solution closely resembles the Bernevig-Hughes-Zhang model for topological insulators. Assuming that the emergent gauge fields are static we investigate vison excitations, which we confirm to be deconfined in all investigated spin phases. Particularly, if the spinon bands are topological, the spinons and visons form bound states consisting of several spinon-Majorana zero modes coupling to one vison. The existence of such zero modes follows from an exact mapping between these spin phases and topological $p+ip$ superconductors with vortices. We propose experimental probes to detect such states in real materials.

Unification of bosonic and fermionic theories of spin liquids on the kagome lattice

Recent numerical studies have provided strong evidence for a gapped $Z_2$ quantum spin liquid in the kagome lattice spin-1/2 Heisenberg model. A special feature of spin liquids is that symmetries can be fractionalized, and different patterns of symmetry fractionalization imply distinct phases. The symmetry fractionalization pattern for the kagome spin liquid remains to be determined. A popular approach to studying spin liquids is to decompose the physical spin into partons obeying either bose (Schwinger bosons) or fermi (Abrikosov fermions) statstics, which are then treated within the mean-field theory. A longstanding question has been whether these two approaches are truly distinct, or describe the same phase in complementary ways. Here we show that all 8 $Z_2$ spin liquid phases in Schwinger-boson mean-field (SBMF) construction can also be described in terms of Abrikosov fermions, unifying pairs of theories that seem rather distinct. The key idea is that for $Z_2$ spin liquid states that admit a SBMF description on kagome lattice, the symmetry fractionalization of visions is uniquely fixed. Two promising candidate states for kagome Heisenberg model, Sachdev's $Q_{1}=Q_{2}$ SBMF state and Lu-Ran-Lee's $Z_2[0,\pi]\beta$ Abrikosov fermion state, are found to describe the same symmetric spin liquid phase. We expect these results to aid in a complete specification of the numerically observed spin liquid phase. We also discuss a set of $Z_2$ spin liquid phases in fermionic parton approach, where spin rotation and lattice symmetries protect gapless edge states, that do not admit a SBMF description.

Chiral quantum spin liquid on the repulsive Haldane–Hubbard model in square lattices

In this paper, we present a study on the repulsive Haldane–Hubbard model with spin-rotation symmetry in square lattices by deriving non-linear σ model for magnetic states. It is found that a chiral spin liquid state as the ground state of the correlated system exists in the topological spin-density wave proposed by Wu et al (2016 J. Phys.: Condens. Matter 28 115602), of which the low energy physics can be determined by the Chern–Simons–Hopf gauge field theory.

Nematic superconductivity in CuxBi2Se3 : Surface Andreev bound states

We study theoretically the topological surface states (TSSs) and the possible surface Andreev bound states (SABSs) of Cu$_{x}$Bi$_{2}$Se$_{3}$ which is known to be a topological insulator at $x=0$. The superconductivity (SC) pairing of this compound is assumed to have the broken spin-rotation symmetry, similar to that of the A-phase of $^{3}$He as suggested by recent nuclear-magnetic resonance experiments. For both spheroidal and corrugated cylindrical Fermi surfaces with the hexagonal warping terms, we show that the bulk SC gap is rather anisotropic; the minimum of the gap is negligibly small as comparing to the maximum of the gap. This would make the fully-gapped pairing effectively nodal. For a clean system, our results indicate the bulk of this compound to be a topological superconductor with the SABSs appearing inside the bulk SC gap. The zero-energy SABSs which are Majorana fermions, together with the TSSs not gapped by the pairing, produce a zero-energy peak in the surface density of states (SDOS). The SABSs are expected to be stable against short-range nonmagnetic impurities, and the local SDOS is calculated around a nonmagnetic impurity. The relevance of our results to experiments is discussed.

Observation of spin-orbit effects with spin rotation symmetry

The spin–orbit interaction enables interconversion between a charge current and a spin current. It is usually believed that in a nonmagnetic metal (NM) or at a NM/ferromagnetic metal (FM) bilayer interface, the symmetry of spin–orbit effects requires that the spin current, charge current, and spin orientation are all orthogonal to each other. Here we demonstrate the presence of spin–orbit effects near the NM/FM interface that exhibit a very different symmetry, hereafter referred to as spin-rotation symmetry, from the conventional spin Hall effect while the spin polarization is rotating about the magnetization. These results imply that a perpendicularly polarized spin current can be generated with an in-plane charge current simply by use of a FM/NM bilayer with magnetization collinear to the charge current. The ability to generate a spin current with arbitrary polarization using typical magnetic materials will benefit the development of magnetic memories.

Persistence of the flat band in a kagome magnet with dipolar interactions

The weathervane modes of the classical Heisenberg antiferromagnet on the kagome lattice constitute possibly the earliest and certainly the most celebrated example of a flat band of zero-energy excitations. Such modes arise from the underconstraint that has since become a defining criterion of strong geometrical frustration. We investigate the fate of this flat band when dipolar interactions are added. These change the nearest-neighbor model fundamentally as they remove the Heisenberg spin-rotational symmetry while also introducing a long-range component to the interaction. We explain how the modes continue to remain approximately dispersionless, while being lifted to finite energy as well as being squeezed: they change their ellipticity described by the ratio of the amplitudes of the canonically conjugate variables comprising them. This phenomenon provides interesting connections between concepts such as constraint counting and self-screening underpinning the field of frustrated magnetism. Moreover, this property is found to be remarkably stable to a wide range of additional interactions.

Magnon Spin-Momentum Locking: Various Spin Vortices and Dirac magnons in Noncollinear Antiferromagnets.

We generalize the concept of the spin-momentum locking to magnonic systems and derive the formula to calculate the spin expectation value for one-magnon states of general two-body spin Hamiltonians. We give no-go conditions for magnon spin to be independent of momentum. As examples of the magnon spin-momentum locking, we analyze a one-dimensional antiferromagnet with the Néel order and two-dimensional kagome lattice antiferromagnets with the 120° structure. We find that the magnon spin depends on its momentum even when the Hamiltonian has the z-axis spin rotational symmetry, which can be explained in the context of a singular band point or a U(1) symmetry breaking. A spin vortex in momentum space generated in a kagome lattice antiferromagnet has the winding number Q=-2, while the typical one observed in topological insulator surface states is characterized by Q=+1. A magnonic analogue of the surface states, the Dirac magnon with Q=+1, is found in another kagome lattice antiferromagnet. We also derive the sum rule for Q by using the Poincaré-Hopf index theorem.

Magnetic Domain Walls as Hosts of Spin Superfluids and Generators of Skyrmions.

A domain wall in a magnet with easy-axis anisotropy is shown to harbor spin superfluid associated with its spontaneous breaking of the U(1) spin-rotational symmetry. The spin superfluid is shown to have several topological properties, which are absent in conventional superfluids. First, the associated phase slips create and destroy Skyrmions to obey the conservation of the total Skyrmion charge, which allows us to use a domain wall as a generator and detector of Skyrmions. Second, the domain wall engenders the emergent magnetic flux for magnons along its length, which are proportional to the spin supercurrent flowing through it, and thereby provides a way to manipulate magnons. Third, the spin supercurrent can be driven by the magnon current traveling across it owing to the spin transfer between the domain wall and magnons, leading to the magnonic manipulation of the spin superfluid. The theory for superfluid spin transport within the domain wall is confirmed by numerical simulations.

Nuclear Magnetic Resonance Signature of the Spin-Nematic Phase in LiCuVO_{4} at High Magnetic Fields.

We report a ^{51}V nuclear magnetic resonance investigation of the frustrated spin-1/2 chain compound LiCuVO_{4}, performed in pulsed magnetic fields and focused on high-field phases up to 56T. For the crystal orientations H∥c and H∥b, we find a narrow field region just below the magnetic saturation where the local magnetization remains uniform and homogeneous, while its value is field dependent. This behavior is the first microscopic signature of the spin-nematic state, breaking spin-rotation symmetry without generating any transverse dipolar order, and is consistent with theoretical predictions for the LiCuVO_{4} compound.