Anisotropic Spectrum Research Articles

Quasinormal scale elimination theory of the anisotropic energy spectra of atmospheric and oceanic turbulence

Quasinormal scale elimination theory of rotating turbulence offers a new explanation of physics governing atmospheric and oceanic spectra including the well-known Nastrom and Gage spectra observed in the upper troposphere and lower stratosphere. The terrestrial circulations may be characterized as flows with ``compactified dimensionality'' (spatial dimension between 2 and 3). Such flows may have both inverse and direct cascades in the same inertial range (dual cascade) and their spectral amplitudes may be determined not by energy/enstrophy fluxes, but by the magnitude of the Coriolis parameter.

The transverse magnetic surface plasmon in anisotropic black phosphorene

Using the Kubo formalism, the intraband optical conductivity of black phosphorene (BP) with an anisotropic energy spectrum is obtained. The presence of BP in an infinite sandwich between two dielectric media supports the transverse magnetic (TM) BP surface plasmon polariton (SPP) wave. Thereby, the effective indices neff for TM BP SPP mode exhibits a linear relation with the incident frequency, which can be tuned by the chemical potential as well as by the dielectric medium surrounding the BP layer. The sublinear dependence of the reciprocal of neff on the chemical potential indicates the effective masses in the armchair and zigzag directions are dependent on the carrier wave vector. Moreover, the effective mass in the armchair direction is more dispersive. The anisotropic optoelectronic features in BP offer more tunability in the design and application of optoelectronic devices as an isotropic system like graphene.

Coherence properties of high-frequency wave field propagating through inhomogeneous ionosphere with anisotropic random irregularities of electron density: 1. Theoretical background

Rigorous analytic solution is constructed for the first of 2 s-order space position and frequency coherence function (which is alternatively also termed as symmetric) of the high-frequency wave field propagating through the stochastic transionospheric channel with the inhomogeneous layer of the background ionosphere and anisotropic fluctuations of the electron density in the approximation of the appropriate Markov equation. It is obtained employing the anisotropic parabolic model of the effective structure function of the fractional electron density fluctuations with two different scales along and across the Earth's magnetic field. The explicit analytic solution is presented, which is capable of describing the coherence properties of the field for any given inhomogeneous distribution of the electron density in the background ionosphere along a path of propagation. The procedure of calibrating the spatial scales of the anisotropic parabolic model of the electron density fluctuations along and across the Earth's magnetic field lines in order to provide the adequate solution to correspond to the realistic anisotropic inverse power law spectrum of the electron density fluctuations is presented in the companion paper.

Chromaticity-tunable white random lasing based on a microfluidic channel.

The color and/or chromaticity controllability of random lasing is a key factor to promote practical applications of random lasers as high luminance sources for speckle-free imaging. Here, white coherent random lasing with tunable chromaticity is obtained by using broadband enhancement Au-Ag nanowires as scatterers and the resonance energy transfer process between different dyes in the capillary microfluidic channel. Red, green and blue random lasers are separately fabricated with low thresholds, benefiting from the plasmonic resonance of the nanogaps and/or nanotips with random distribution and sizes within Au-Ag nanowires and positive optical feedback provided by the capillary wall. A white random laser system is then designed through reorganizing the three random lasers. And, the chromaticity of the white random laser is flexibly tunable by adjusting pump power density. In addition, the white random laser has anisotropic spectra due to the coupling role between the lasers. This characteristic is then utilized to obtain different random lasing with different chromaticity over a broad visible range. The results may provide a basis for applying random laser in the field of high brightness illumination, biomedical imaging, and sensors.

Probing of Higher Excited States of Merocyanine Derivatives of Azaazulene and Indandione by Fluorescence Excitation Anisotropy Spectra

This paper is dedicated to the spectral and quantum-chemical studies of higher excited states of merocyanine derivatives of azaazulene and indandione. A particular attention is paid to the analysis of fluorescence excitation anisotropy spectra of the mentioned compounds. The long-wave shift by ≈ 50 nm of a deep clear minimum in the fluorescence excitation anisotropy spectrum due to an elongation of the polymethine dye chromophore is established. Such shift is close in a value to the bathochromic shift of the first minimum in the anisotropy spectrum of symmetric ionic polymethine dyes, in which this minimum corresponds to the second electronic transition. The parallel spectral study and quantum-chemical calculations allowed us to correctly interpret the fluorescence excitation anisotropy spectra of merocyanines and relate the first clear minimum with the seventh electronic transition. The last resembles the second electronic transition between delocalized molecular orbitals (MO) in polymethine dyes.

Constraining dark photons and their connection to 21 cm cosmology with CMB data

In the inhomogeneous Universe, the cosmological conversion of dark photons into ordinary photons (and vice versa) may happen at a great number of resonance redshifts. This alters the CMB observed energy spectrum and degree of small-scale anisotropies. We utilize results from the EAGLE simulation to obtain the conversion probability along random line-of-sights to quantify these effects. We then apply our results to the case where dark photons are sourced by dark matter decay and their high-redshift conversion into ordinary photons modify the global 21 cm signal expected from the cosmic dawn era. Concretely, we show that a significant portion of the parameter space for which a converted population of photons in the Rayleigh-Jeans tail of the CMB explains the absorption strength observed by EDGES, is ruled out from the brightness temperature measurements of COBE/FIRAS and the CMB anisotropy measurements of Planck and SPT.

Eumelanin Adsorption on Silicon: Optical Properties of Si(001)-Adsorbed Eumelanin Tetrameric Protomolecules

We predict the optical properties (in particular optical absorbance and reflectance anisotropy spectra (RAS)) of the silicon(001) surface organically functionalized by the adsorption of chosen tetr...

Spectral tuning of light-harvesting complex II in the siphonous alga Bryopsis corticulans and its effect on energy transfer dynamics

Light-harvesting complex II (LHCII) from the marine green macroalga Bryopsis corticulans is spectroscopically characterized to understand the structural and functional changes resulting from adaptation to intertidal environment. LHCII is homologous to its counterpart in land plants but has a different carotenoid and chlorophyll (Chl) composition. This is reflected in the steady-state absorption, fluorescence, linear dichroism, circular dichroism and anisotropic circular dichroism spectra. Time-resolved fluorescence and two-dimensional electronic spectroscopy were used to investigate the consequences of this adaptive change in the pigment composition on the excited-state dynamics. The complex contains additional Chl b spectral forms – absorbing at around 650 nm and 658 nm – and lacks the red-most Chl a forms compared with higher-plant LHCII. Similar to plant LHCII, energy transfer between Chls occurs on timescales from under hundred fs (mainly from Chl b to Chl a) to several picoseconds (mainly between Chl a pools). However, the presence of long-lived, weakly coupled Chl b and Chl a states leads to slower exciton equilibration in LHCII from B. corticulans. The finding demonstrates a trade-off between the enhanced absorption of blue-green light and the excitation migration time. However, the adaptive change does not result in a significant drop in the overall photochemical efficiency of Photosystem II. These results show that LHCII is a robust adaptable system whose spectral properties can be tuned to the environment for optimal light harvesting.

Anisotropic turbulence-induced statistical properties evolution of a radially polarized partially coherent pulsed beam on propagation

In this study, we introduce a new kind of partially coherent vector beam with Gaussian distribution in the spatial, temporal and correlation components named a radially polarized partially coherent Gaussian Schell-model pulsed (GSMP) beam as a natural extension of scalar Gaussian Schell-model pulsed beam. Analytical formulas for the two-frequency cross-spectral density matrix elements of this beam are derived based on the extended Huygens–Fresnel theory. Within the frame of extend anisotropic non-Kolmogorov spectrum, the effects of asymmetry anisotropic turbulence eddies on the statistical properties of a radially polarized partially coherent GSMP beam are investigated numerically. Our work improves the classical theory of stochastic electromagnetic beams on propagation and may be useful for applications involving free-space optical communications.

Assessing non-linear models for galaxy clustering – II. Model validation and forecasts for Stage IV surveys

ABSTRACT Accurate modelling of non-linear scales in galaxy clustering will be crucial for data analysis of Stage IV galaxy surveys. A selection of competing non-linear models must be made based on validation studies. We provide a comprehensive set of forecasts of two different models for the halo redshift space power spectrum, namely the commonly applied TNS model and an effective field theory of large-scale structure (EFTofLSS) inspired model. Using simulation data and a least-χ2 analysis, we determine ranges of validity for the models. We then conduct an exploratory Fisher analysis using the full anisotropic power spectrum to investigate parameter degeneracies. We proceed to perform an MCMC analysis utilizing the monopole, quadrupole, and hexadecapole spectra, with a restricted range of scales for the latter in order to avoid biasing our growth rate, f, constraint. We find that the TNS model with a Lorentzian damping and standard Eulerian perturbative modelling outperforms other variants of the TNS model. Our MCMC analysis finds that the EFTofLSS-based model may provide tighter marginalized constraints on f at z = 0.5 and z = 1 than the TNS model, despite having additional nuisance parameters. However this depends on the range of scales used as well as the fiducial values and priors on the EFT nuisance parameters. Finally, we extend previous work to provide a consistent comparison between the Fisher matrix and MCMC forecasts using the multipole expansion formalism, and find good agreement between them.

User’s guide to extracting cosmological information from line-intensity maps

Line-intensity mapping (LIM) provides a promising way to probe cosmology, reionization and galaxy evolution. However, its sensitivity to cosmology and astrophysics at the same time is also a nuisance. Here we develop a comprehensive framework for modelling the LIM power spectrum, which includes redshift space distortions and the Alcock-Paczynski effect. We then identify and isolate degeneracies with astrophysics so that they can be marginalized over. We study the gains of using the multipole expansion of the anisotropic power spectrum, providing an accurate analytic expression for their covariance, and find a 10%-60% increase in the precision of the baryon acoustic oscillation scale measurements when including the hexadecapole in the analysis. We discuss different observational strategies when targeting other cosmological parameters, such as the sum of neutrino masses or primordial non-Gaussianity, finding that fewer and wider bins are typically more optimal. Overall, our formalism facilitates an optimal extraction of cosmological constraints robust to astrophysics.

Stochastic gravitational wave background anisotropies in the mHz band: astrophysical dependencies

ABSTRACT We show that the anisotropies of the astrophysical stochastic gravitational wave background in the mHz band have a strong dependence on the modelling of galactic and sub-galactic physics. We explore a wide range of self-consistent astrophysical models for stellar evolution and for the distribution of orbital parameters, all calibrated such that they predict the same number of resolved mergers to fit the number of detections during LIGO/Virgo O1 + O2 observations runs. We show that different physical choices for the process of black hole (BH) collapse and cut-off in the BH mass distribution give fractional differences in the angular power spectrum of anisotropies of up to 50 per cent on all angular scales. We also point out that the astrophysical information which can be extracted from anisotropies is complementary to the isotropic background and individual mergers. These results underline the interest in the anisotropies of the stochastic gravitational wave background as a new and potentially rich field of research, at the cross-road between astrophysics and cosmology.

Super-sample tidal modes on the celestial sphere

The super-sample tidal effect carries information on long-wavelength fluctuations that we cannot measure directly. It arises from the mode-coupling between short-wavelength and long-wavelength perturbations beyond a finite region of a galaxy survey and violates statistical isotropy of observed galaxy power spectra. In this paper, we propose the use of bipolar spherical harmonic (BipoSH) decomposition formalism to characterize statistically anisotropic power spectra. Using the BipoSH formalism, we perform a comprehensive study of the effect of the super-sample tides on measurements of other cosmological distortions such as the redshift-space distortion (RSD) and Alcock-Paczy\'{n}ski (AP) effects by means of the Fisher information matrix formalism. We find that the BipoSH formalism can break parameter degeneracies among the super-sample tidal, RSD and AP effects, indicating that the super-sample tides have little impact on the measurements of the RSD and AP effects. We also show that the super-sample tides are detectable with an accuracy better than the $\Lambda$CDM prediction without impairing the accuracy of measurements of other anisotropies assuming a SPHEREx-like galaxy survey.

Estimating the angular power spectrum of the gravitational-wave background in the presence of shot noise

There has been much recent interest in studying anisotropies in the astrophysical gravitational-wave (GW) background, as these could provide us with interesting new information about galaxy clustering and large-scale structure. However, this information is obscured by shot noise, caused by the finite number of GW sources that contribute to the background at any given time. We develop a new method for estimating the angular spectrum of anisotropies, based on the principle of combining statistically-independent data segments. We show that this gives an unbiased estimate of the true, astrophysical spectrum, removing the offset due to shot noise power, and that in the limit of many data segments, it is the most efficient (i.e. lowest-variance) estimator possible.

Temporal Frequency Spread of Plane Wave Propagation through Moderate to Strong Turbulence

In this study, we derive new expressions for the atmospheric-brought on frequency unfold of plane waves propagating thru slight to strong turbulence in a horizontal direction based on the modified anisotropic non-Kolmogorov electricity spectrum as antagonistic to conventional Kolmogorov electricity spectrum. The energy regulation price varies from three to 4 instead of the traditional Kolmogorov power law price; the general amplitude price differs from the conventional Kolmogorov regular cost 0.033. these new expressions are based on slight to robust fluctuation vicinity and anisotropic non-Kolmogorov turbulence. The simulation results show that temporal frequency unfold will decrease even as the anisotropic component   2  is increasing

Properties of the stochastic astrophysical gravitational wave background: Astrophysical sources dependencies

This article explores the properties (amplitude and shape) of the angular power spectrum of the anisotropies of the astrophysical gravitational wave background (AGWB) focusing on the signatures of the astrophysical models describing subgalactic physics. It demonstrates that while some parameters have negligible impact, others, and in particular the stellar evolution models, the metallicity and the merger time delay distribution can result in relative differences of order 40% in the angular power spectrum of anisotropies in both the LIGO/Virgo and LISA frequency bands. It is also shown that the monopole and the anisotropic components of the AGWB are complementary and sensitive to different astrophysical parameters. It follows that AGWB anisotropies are a new observable with the potential to provide new astrophysical information that cannot be accessed otherwise.

In-depth investigation of the binding of flavonoid taxifolin with bovine hemoglobin at physiological pH: Spectroscopic and molecular docking studies.

The use of bioactive flavonoids as drugs has long mesmerized the scientific world. Their small size and planar structure enables them to interact with limitless substrates especially biomolecules. Taxifolin is a flavonoid well known for its anti-oxidizing and metal chelating properties. Its interaction with a few biomolecules has been studied so far to exploit its pharmacological activities. Hemoglobin, an iron containing macromolecule acts as a major carrier protein and is also associated with the occurrence of many diseases. Our present study lays emphasis on the interaction of flavanonol taxifolin with bovine hemoglobin at physiological pH. This was achieved by monitoring the changes in the absorbance, fluorescence, anisotropic, lifetime and circular dichroic spectra. Benesi-Hildebrand plot determined a binding constant value of 20.0 × 103 M-1 at 25 °C. Stern-Volmer quenching studies reveal that the binding is associated with a static mode of quenching. The complexation is thermodynamically favored as indicated by the negative value of enthalpy and positive value of entropy changes seen from the van't Hoff plot. Theoretical DFT calculations were used to find out an optimized geometry and HOMO-LUMO energy gap for taxifolin. Molecular docking studies revealed the location of taxifolin inside the hemoglobin moiety.

Electronic Nature of Neutral and Charged Two-Photon Absorbing Squaraines for Fluorescence Bioimaging Application

The electronic properties of neutral 2,4-bis(4-bis(2-hydroxyethyl) amino-2-hydroxy-6-(2-(2-(2-methoxyethoxy)ethoxy)ethoxy)phenyl)squaraine (1) and charged 2-((3-octadecylbenzothiazol-2(3H)-ylidene)methyl)-3-oxo-4-((3-(4-(pyridinium-1-yl)butyl)benzo-thiazol-3-ium-2-yl)methylene)cyclobut-1-enolate iodide (2) squaraine derivatives were analyzed based on comprehensive linear photophysical, photochemical, nonlinear optical studies (including two-photon absorption (2PA) and femtosecond transient absorption spectroscopy measurements), and quantum chemical calculations. The steady-state absorption, fluorescence, and excitation anisotropy spectra of these new squaraines revealed the values and mutual orientations of the main transition dipoles of 1 and 2 in solvents of different polarity, while their role in specific nonlinear optical properties was shown. The degenerate 2PA spectra of 1 and 2 exhibited similar shapes, with maximum cross sections of ∼300–400 GM, which were determined by the open aperture Z-scan method over a broad spectral range. The nature of the time-resolved excited-state absorption spectra of 1 and 2 was analyzed using a femtosecond transient absorption pump–probe technique and the characteristic relaxation times of 4–5 ps were revealed. Quantum chemical analyses of the electronic properties of 1 and 2 were performed using the ZINDO/S//DFT theory level, affording good agreement with experimental data. To demonstrate the potential of squaraines 1 and 2 as fluorescent probes for bioimaging, laser scanning fluorescence microscopy images of HeLa cells incubated with new squaraines were obtained.

The space station based detector HERD: precise high energy cosmic rays physics and multimessenger astronomy

The High Energy cosmic-Radiation Detection (HERD) facility is one of several scientific payloads planned to go onboard China's Space Station, which is planned to be operational starting in around 2025 for about 10 years. The main scientific objectives of HERD are the search for signals of dark matter annihilation products, precise cosmic electron/positron spectrum and measurements of anisotropy up to 10 TeV, precise cosmic ray spectrum and composition measurements up to the knee energy, and high energy γ-ray monitoring and survey. HERD consists of a 3-D cubic calorimeter (CALO) surrounded by microstrip silicon trackers (STKs) from five sides except the bottom. CALO is made of about 7,500 cubes of LYSO crystals, corresponding to about 55 radiation lengths and 3 nuclear interaction lengths, respectively. The top STK microstrips of six X-Y layers are sandwiched with tungsten converters to measure with high efficiency incoming γ-rays. In the baseline design, each of the four side STKs is made of only three layers of microstrip detectors. All STKs will also be used for measuring the charge and incoming directions of electrons/positrons and cosmic rays, as well as identifying back scattered tracks. With this design, HERD can achieve the following performance: energy resolution of 1% for electrons and γ-rays beyond 100 GeV and 20% for protons from 100 GeV to 1 PeV; electron/proton separation power better than 10−5; effective geometrical factors of > 3 m2sr for electrons and gamma-rays, > 2 m2sr for cosmic ray nuclei. Substantial activity is ongoing to optimize the detector parameters.

Electromagnetic scattering characteristics of foil in hypersonic plasma turbulence

To investigate the electromagnetic scattering problem related to a foil in a turbulent hypersonic plasma environment, the scattering field formulas for hypersonic plasma turbulence were improved by applying the anisotropic power spectrum. Using the theory of electromagnetic scattering of a conducting object, the second moment of a conducting object's scattering field is obtained in the hypersonic plasma turbulence. Finally, the backscattering cross-section of the foil surrounded by the hypersonic plasma turbulence was calculated. The results showed that the fractal dimension led to an increase in the complexity of the hypersonic turbulent structure, and thus had a greater influence on the electromagnetic wave scattering. The scattering cross-section of the foil in the hypersonic turbulence decreases rapidly. Meanwhile, the anisotropic parameters in the model represent scale-dependent stretching of the turbulent eddy. As the anisotropic parameters of the turbulence increase, there will be less scattering of the hypersonic turbulence. At this point, the total scattering cross-section of the foil in hypersonic plasma turbulence increases gradually. By improving the aerodynamic shape of the aircraft, it can produce a large number of anisotropic turbulent eddies which can effectively improve the passive jamming capability when the foil is cast.