Isotopically pure /sup 233/U samples, with only 3 x 10/sup -3/ ppm /sup 232/U content, were prepared by thermal neutron irradiation of thoria and subsequent chemical processing. The /sup 233/U sample thus obtained was reirradiated with a fisaion neutron spectrum in the core of the Kyoto University Reactor (KUR), and measurements were made of the fission spectrum average cross section for the /sup 233/U(n 2n)/sup 232/U reaction. A value of 4.08 plus or minus 0.30 mb was obtained for this cross section, in agreement with the renormalized value of Halperin et al., ithin the limits of experimental error. In order to asaess the energy-dependent cross section from the value of this integral measurement, the /sup 233/U(n,2n) cross section was calculated assuming a Maxwellian-type fisaion spectrum and adopting the energydependent evaluated cross sections of ENDF/B-III and other authors. The values of the cross section thus determined were found to be about 32 to 91% larger than the measured cross section given above. The result of Pearlstein's calculation of the /sup 233/ U(n,2n) cross section by the statistical model, again assuming the Maxwellian distribution, is smaller than the measured crosss section by about 19%. (auth)
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