This paper presents a novel methodology for designing high-capacity frequency domain chipless RFID tags based on the backscattering principle. The tag consists of multiple square open-loop resonators loaded with a varying number of square metallic patches to form a mesh structure. Thus, in contrast to conventional designs, the overall physical size of each resonator remains fixed and does not change with respect to its operating resonant frequency. The RCS response of the proposed tag can be easily manipulated by varying the loading factor of each resonator. The tag size is further miniaturized by placing resonators on both sides of the substrate used. The tag configuration with resonators arranged in the form of a single row (4 × 1) printed on both sides of the substrate is finally chosen for maximum robustness and efficiency. The frequency shift coding (FSC) technique is used to encode more than one bit per resonator by using segments within sub-bands. The proposed tag encodes 16-bit data in a frequency band from 5.9 to 10.5 GHz and has a very high code density of 23.51 bits/cm2 and a spectral efficiency of 3.47 bits/GHz. The design methodology is novel and leads to a very efficient chipless RFID tag that can be used in a variety of high-data-capacity applications.