Advanced aircraft with thrust vectoring/aerodynamic rudder layout have significant control coupling problems. The traditional single-loop control parameter design method cannot take into account the performance of multiple control loops in this scenario. Therefore, a control law parameter optimization method based on the singular value of the hysteresis matrix is proposed. First, the control parameter optimization interval is determined using the time domain control performance index. Then, the singular value method is used to measure the stability margin of the multiple-input multiple-output (MIMO) system on this basis, and the corresponding optimal objective function is established to optimize the controller parameters. The feasibility of this method is verified by numerical simulation. The results show that the designed control parameter optimization algorithm has better time domain control performance and larger system stability margin than the traditional single-loop control parameter design method.