We reported a high-power 915 nm Pr3+:LiYF4 (Pr:YLF) laser dual-ended pumped by laser diodes (LDs). The maximum output power of the laser was 3.39 W with a slope efficiency of 19.8 %. The fluctuation range of the laser wavelength was less than 0.58 nm. As far as we know, this is the highest power at 915 nm for LD-pumped Pr:YLF lasers to date. To eliminate the power saturation phenomenon and further improve the laser output power, we proposed a simple and effective method, i.e., laser energy levels cascade. Based on the experimental data, we calculated the populations of 3P0 and 1G4 energy levels in Pr:YLF crystal during laser cascading and developed two different models to verify the feasibility of the laser cascade mechanism. Moreover, the laser cascade could be realized merely by designing the lens film without introducing other devices, which provided a simple and effective solution for developing high-performance lasers.