One new phenylpropanoid glycoside, pedicularioside H, and five known glycosides, gardoside methyl ester, shanzhiside methyl ester, 5-deoxypulchelloside I, verbascoside and pedicularioside A, were isolated from whole plants of Pedicularis spicata. On the basis of the spectral data, chemical evidence and comparison with authentic samples, pedicularioside H was determined to be 1′- O-β- d-(3-methoxy-4-hydroxy-β-phenyl)-ethyl-4′- O-feruloyl-β- d-apiosyl(1→3′)-α- l-rhamnosyl-(1→6′)-glucopyranoside.