This paper presents the design of a precise “ball-column” device to efficiently and accurately measure the geometric error terms of both rotary axes of the five-axis machine tool. A geometric error measurement method of spherical contact was proposed based on the influence of the geometric error term from a five-axis machine tool rotating axis on the integrated geometric error of the machine tool. A multiple degree of freedom, step-by-step contact method based on on-machine measure for measuring the spherical center point is proposed, and the solution formula of each geometric error term of the rotating axis is established, respectively. This method can identify 12 geometric errors based on the influence of one rotating axis on another rotating axis after long term operation. The spatial error field of the five-axis machine tool was constructed by analyzing the error law of the two rotating axes of machine tools based on various positions and postures. Finally, after the comparison of the experiment, the results showed that the accuracy of the developed error measurement device reached 91.8% and the detection time was as short as 30–40 min.
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