Resonant THz Research Articles

Observation of THz surface waves escaping from metal gratings through a dielectric substrate.

Extensive research has been conducted on generating THz waves using Smith-Purcell radiation, yet a portion of the electron bunch's interaction energy with the gratings is confined to the metal gratings' surface, leading to a low THz radiation power. This paper experimentally demonstrates that metal gratings with a dielectric substrate can emit the resonant modes in surface waves when excited by relativistic femtosecond electron bunches. The observed spectra of the resonant THz waves align well with the theoretical estimations derived from the configuration's dispersion relation and 3D simulations. In comparison to traditional Smith-Purcell radiation generated by the grating, these resonant THz waves exhibit significantly higher intensity and improved orientation. Additionally, we investigated the radiation characteristics of the resonant THz waves, including radiation angle, beam-grating distance, beam energy, and bunch length. This innovative approach presents a novel method for generating high-power coherent terahertz radiation.

Resonant THz detection by periodic multi-gate plasmonic FETs

Resonant THz detection by periodic multi-gate plasmonic FETs

Mapping LiNbO_{3} Phonon-Polariton Nonlinearities with 2D THz-THz-Raman Spectroscopy.

Two-dimensional terahertz-terahertz-Raman spectroscopy can provide insight into the anharmonicities of low-energy phonon modes-knowledge of which can help develop strategies for coherent control of material properties. Measurements on LiNbO_{3} reveal THz and Raman nonlinear transitions between the E(TO_{1}) and E(TO_{3}) phonon polaritons. Distinct coherence pathways are observed with different THz polarizations. The observed pathways suggest that the origin of the third-order nonlinear responses is due to mechanical anharmonicities, as opposed to electronic anharmonicities. Further, we confirm that the E(TO_{1}) and E(TO_{3}) phonon polaritons are excited through resonant one-photon THz excitation.

Anion-water hydrogen bond vibration revealed by the terahertz Kerr effect.

The microscopic mechanism for ionic influence on the hydrogen bond network of water has not been fully understood. Here we employ the terahertz Kerr effect (TKE) technique to map the intermolecular hydrogen bond dynamics in a series of aqueous halide solutions at the sub-picosecond scale. Compared with pure water, the significantly enhanced bipolar TKE response associated with polarization anisotropy in an ionic aqueous solution is successfully captured. We decompose the measured TKE response into different molecular motion modes and demonstrate that the obviously increasing positive polarity response is mainly due to the anion-water hydrogen bond vibration mode with the resonant THz electric field excitation. Our measurement results provide an experimental basis for further insight into the effects of ions on the structure and dynamics of a hydrogen bond in water.

Major reshaping of narrow beams by resonant multilayer structures.

Major reshaping of electromagnetic MM-wave beams transmitted at resonant frequencies through high-quality multilayer structures is demonstrated. Beam reshaping emerges due to efficient excitation of intrinsic quasi-optical modes with complex spatial profiles by an incident beam. This leads to a significant increase of width and distortion of shape of transmitted beams, which grow with increasing likelihood of excitation of higher-order modes. The beam shape is extremely sensitive to imperfections of real structures and can become complex and asymmetric even at the normal-angle transmission of symmetric incident beams. The effect is of importance for the resonant MM-wave and THz spectroscopy of low-loss dielectric materials.

Broadband THz amplification and superradiant spontaneous emission in a guided FEL.

While significant progress has been made to fill the "THz gap", critical applications requiring powerful and energy efficient THz sources and amplifiers, from high frequency communications to medical and security imaging and nonlinear spectroscopy, continue to drive research on new methods of THz generation. Here we demonstrate a Free Electron Laser (FEL) THz source based on a novel interaction regime where broadband THz pulses can be phase and group velocity matched to the electron beam in a magnetic undulator via dispersion in a waveguide. Using < 10 pC, 6 MeV electron beams we show amplification of broadband THz pulses and demonstrate THz generation via both stimulated emission and spontaneous coherent superradiant emission, due to the short bunch length (< 200 fs rms) relative to resonant THz frequency (0.8 THz). A newly developed multifrequency simulation, designed to model the special case of guided FEL interaction, is benchmarked with the experiments and then used to extrapolate the capabilities of this "zero-slippage" FEL to efficient, tunable generation of > 100 μJ THz pulses when using higher (200 pC) beam charges and a tapered resonant condition.

AlGaN/GaN field effect transistor with two lateral Schottky barrier gates towards resonant detection in sub-mm range

We report on the investigations of AlGaN/GaN field effect transistors with two lateral Schottky barrier gates on the sides of the two-dimensional electron gas. This kind of ‘EdgeFET’ allowed us to efficiently control the current flow in the 2DEG conduction channel. Moreover, due to depletion, regions at a certain range of reverse biasing form a nanowire, which is beneficial for the adjustable resonant THz detection. Our studies of DC characteristics and photoresponse in the sub-terahertz frequency confirm the validity of the approach.

Direct observation of mode-specific phonon-band gap coupling in methylammonium lead halide perovskites

Methylammonium lead iodide perovskite is an outstanding semiconductor for photovoltaics. One of its intriguing peculiarities is that the band gap of this perovskite increases with increasing lattice temperature. Despite the presence of various thermally accessible phonon modes in this soft material, the understanding of how precisely these phonons affect macroscopic material properties and lead to the peculiar temperature dependence of the band gap has remained elusive. Here, we report a strong coupling of a single phonon mode at the frequency of ~ 1 THz to the optical band gap by monitoring the transient band edge absorption after ultrafast resonant THz phonon excitation. Excitation of the 1 THz phonon causes a blue shift of the band gap over the temperature range of 185 ~ 300 K. Our results uncover the mode-specific coupling between one phonon and the optical properties, which contributes to the temperature dependence of the gap in the tetragonal phase.

Tunable terahertz radiation generation by nonlinear photomixing of cosh-Gaussian laser pulses in corrugated magnetized plasma

AbstractThis paper presents a scheme of THz generation by nonlinear photomixing of two cosh-Gaussian lasers pulses having different frequencies (ω1, ω2) and wave numbers $(\vec k_1, \vec k_2 )$ and same electrical field amplitude in a corrugated plasma embedded with transverse static magnetic field. Cosh-Gaussian laser pulses have steep gradient in intensity profile along with wider cross-section, which exerts a stronger nonlinear ponderomotive force at ω1 − ω2 and $\vec k_1 - \vec k_2 $ on plasma electrons imparting a nonlinear oscillatory velocity to plasma electrons. Oscillatory plasma electrons couple with the density ripple n′ = nα0eiαx to produce a nonlinear current, which is responsible for resonant THz radiation at frequency $\sim\left( {{\rm \omega} _{\rm c}^2 + {\rm \omega} _{\rm p}^2} \right)^{1/2} $. The amplitude, efficiency and beam quality of THz radiation can be optimized by choosing proper corrugation factor (α of the plasma), applied magnetic field (ωc), decentered parameter (b), and beam width parameter a0 of cosh-Gaussian lasers. An efficiency of $\sim\!10^{ - 2} - 10^{ - 1} $ is achieved for laser electric field E = 3.2 × 109 V/cm.

A Graphene-Based THz Ring Resonator for Label-Free Sensing

In this paper, we report on a novel resonant THz sensor for label-free analysis. The structure consists of a silicon nitride dielectric ring resonator vertically coupled to a thin layer of graphene strip ring resonator on top. The cladding is assumed to be porous alumina on the top of the graphene strip, which enhances the interaction of the surface plasmon wave and the target molecules. Finite difference time domain analysis is used to systematically design the structure and to investigate the performance of the sensor. Our simulations show that the proposed structure has larger refractive index sensitivity and lower intrinsic quality factor with respect to the similar optical structure. It is also shown that the overall performance of the proposed structure in terms of figures of merit is superior to the performance of a similar optical structure. The proposed structure can be used for lab-on-a-chip sensing applications due to its compactness and is capable of being spectrally or spatially multiplexed for multi-analytic sensing.

High-Field High-Repetition-Rate Sources for the Coherent THz Control of Matter.

Ultrashort flashes of THz light with low photon energies of a few meV, but strong electric or magnetic field transients have recently been employed to prepare various fascinating nonequilibrium states in matter. Here we present a new class of sources based on superradiant enhancement of radiation from relativistic electron bunches in a compact electron accelerator that we believe will revolutionize experiments in this field. Our prototype source generates high-field THz pulses at unprecedented quasi-continuous-wave repetition rates up to the MHz regime. We demonstrate parameters that exceed state-of-the-art laser-based sources by more than 2 orders of magnitude. The peak fields and the repetition rates are highly scalable and once fully operational this type of sources will routinely provide 1 MV/cm electric fields and 0.3 T magnetic fields at repetition rates of few 100 kHz. We benchmark the unique properties by performing a resonant coherent THz control experiment with few 10 fs resolution.

Tunable Terahertz Hybrid Metal–Graphene Plasmons

We report here a new type of plasmon resonance that occurs when graphene is connected to a metal. These new plasmon modes offer the potential to incorporate a tunable plasmonic channel into a device with electrical contacts, a critical step toward practical graphene terahertz optoelectronics. Through theory and experiments, we demonstrate, for example, anomalously high resonant absorption or transmission when subwavelength graphene-filled apertures are introduced into an otherwise conductive layer. These tunable plasmon resonances are essential yet missing ingredients needed for terahertz filters, oscillators, detectors, and modulators.

Observation of Thermoelectric Voltages from the Two-Dimensional Electron Gas of a HgTe Quantum Well Due to Resonant THz Laser Heating

HgTe quantum wells (QWs) have shown a number of interesting phenomena, recently the first two-dimensional topological insulating state. We have studied thermoelectric photovoltages of two-dimensional electrons in a 6.1 nm wide HgTe QW induced by cyclotron resonance absorption (B = 2 to 5 T) of a THz laser beam. We have estimated thermopower coefficients by detailed analysis of the photovoltage signals developed across various contacts of a large Hall bar structure at a bath temperature of 1.6 K. The photovoltage signals are washed out at bath temperature of 18 K.

High-Q resonant cavities for terahertz quantum cascade lasers.

We report on the realization and characterization of two different designs for resonant THz cavities, based on wire-grid polarizers as input/output couplers, and injected by a continuous-wave quantum cascade laser (QCL) emitting at 2.55 THz. A comparison between the measured resonators parameters and the expected theoretical values is reported. With achieved quality factor Q ≈ 2.5 × 10(5), these cavities show resonant peaks as narrow as few MHz, comparable with the typical Doppler linewidth of THz molecular transitions and slightly broader than the free-running QCL emission spectrum. The effects of the optical feedback from one cavity to the QCL are examined by using the other cavity as a frequency reference.

Split ring resonator based THz-driven electron streak camera featuring femtosecond resolution.

Through combined three-dimensional electromagnetic and particle tracking simulations we demonstrate a THz driven electron streak camera featuring a temporal resolution on the order of a femtosecond. The ultrafast streaking field is generated in a resonant THz sub-wavelength antenna which is illuminated by an intense single-cycle THz pulse. Since electron bunches and THz pulses are generated with parts of the same laser system, synchronization between the two is inherently guaranteed.

Resonant THz sensor for paper quality monitoring using THz fiber Bragg gratings

We report fabrication of THz fiber Bragg gratings (TFBG) using CO(2) laser inscription on subwavelength step-index polymer fibers. A fiber Bragg grating with 48 periods features a ~4 GHz-wide stop band and ~15 dB transmission loss in the middle of a stop band. The potential of such gratings in the design of resonant sensors for the monitoring of paper quality is demonstrated. Experimental spectral sensitivity of the TFBG-based paper thickness sensor was found to be ~-0.67 GHz/10 μm. A 3D electromagnetic model of a Bragg grating was used to explain experimental findings.

Optimal structure for resonant THz detection of plasmons–polaritons in the 2D quantum wells

We investigate terahertz plasmon-polariton (PP) resonances for hetero-structures (AlGaN/GaN, SiGe/Si/SiGe, AlGaAs/GaAs and InAlN/GaN) with grating coupler in order to find the optimal structure. We show a modeling work devoted to a parametric study (influence of geometry, temperature…) that the resonances are tunable in frequency allowing a control of the terahertz detection. The modeling shows that AlGaN/GaN and InAlN/GaN heterostructures present the highest PP resonances at 300K. Then we compare modeling with room temperature and cryogenic temperature FTIR measurements on group III-N heterostructures which are indeed the most promising.

Carrier transport in THz quantum cascade lasers: Are Green's functions necessary?

We have applied two different simulation models for the stationary carrier transport and optical gain analysis in resonant phonon depopulation THz Quantum Cascade Lasers (QCLs), based on the semiclassical ensemble Monte Carlo (EMC) and fully quantum mechanical non-equilibrium Green's functions (NEGF) method, respectively. We find in the incoherent regime near and above the threshold current a qualitative and quantitative agreement of both methods. Therefore, we show that THz-QCLs can be successfully optimized utilizing the numerically efficient EMC method.

Limiting factors for high temperature operation of THz quantum cascade lasers

AbstractWe theoretically investigate the temperature performance of GaAs‐based resonant phonon depopulation THz quantum cascade lasers, using an ensemble Monte Carlo simulation which includes both carrier‐carrier and carrier‐phonon scattering. By evaluating the temperature dependence of the different carrier transport paths, we identify the factors restricting high temperature operation. As a major detrimental effect, a strongly increased occupation of the lower laser level is found due to a less efficient depletion at elevated temperatures, which can mainly be attributed to the resonant nature of the depletion process. (© 2008 WILEY‐VCH Verlag GmbH &amp; Co. KGaA, Weinheim)

Asynchronous optical sampling for high-speed characterization of integrated resonant terahertz sensors

Two femtosecond Ti:sapphire lasers with slightly different repetition rates near 1 GHz are coupled to implement high-speed asynchronous optical sampling. The application of this technique is successfully demonstrated in the field of terahertz time-domain spectroscopy (TDS). A time delay of 1 ns is scanned at a frequency of 5 kHz without moving mechanical parts. Compared with that of conventional TDS schemes based on lock-in detection and moving mirrors, the readout time of integrated resonant THz sensors is reduced by a factor of 20, opening the way for high-throughput THz sensing in marker-free DNA analysis.