Textile-reinforced cementitious composites have great potential to offer novel design opportunities for thin-section structures thanks to their superior material capabilities. In this work, new cementitious composites with novel reinforcement configurations are developed, which have superior mechanical properties. The cementitious composites contain inclined through-the-thickness reinforcements, and their enhanced performance on thin-section material hardening under flexural loading is demonstrated. Furthermore, a new practical FE modeling approach is proposed that involves the combined use of multiple cohesive regions and 1D reinforcement elements that pass through these regions with a bilinear material law. This approach provides a new computationally efficient modelling framework whereby reinforcement pull-out during hardening is readily captured without resorting to computationally demanding interface laws between the reinforcement and the cementititous matrix. The model can model enhanced hardening of new configurations and provides comparable results with the experimental findings. The model can be used in the modelling and design of novel cementitious composites with engineered reinforcement configurations. Overall, this study aims to open up new avenues for the smart material design of cementitious composites with novel structural reinforcements.