Decoherence Rate Research Articles

Long Electron Spin Coherence Times of Atomic Hydrogen Trapped in Silsesquioxane Cages.

Encapsulated atomic hydrogen in cube-shaped octasilsesquioxane (POSS) cages of the Si8O12R8 type (where R is an organic group) is one of the simplest alternative stable systems to paramagnetic endofullerenes that have been regarded as key elements of spin-based quantum technologies. Apart from common sources of decoherence such as nuclear spin and spectral diffusion, all H@POSS species studied so far suffer from additional shortening of T2 at low temperatures due to methyl group rotations. Here we eliminate this factor for the first time by studying the smallest methyl-free derivative with R = H, namely, H@T8H8. By applying dynamical decoupling methods, we measure electron spin coherence times T2 up to 280 ± 76 μs at T = 90 K and observe a linear dependence of the decoherence rate 1/T2 on trapped hydrogen concentrations, which we attribute to the spin dephasing mechanism of instantaneous diffusion and a nonuniform spatial distribution of encapsulated H atoms.

Characterization and Coherent Control of Spin Qubits with Modulated Electron Beam and Resonator

AbstractThe coherent dynamics and control of spin qubits are fundamental requirements for the development and implementation of quantum technology. However, controlling a single spin qubit within a set of qubits is challenging due to the spatial extent of the applied magnetic field, which can negatively impact the coherent dynamics of neighboring qubits. In this study, a scheme is proposed for characterizing and controlling the coherent dynamics of spin qubits. The proposed scheme comprises a resonator that encloses the desired quantum system and a modulated electron beam that passes through the resonator in close proximity to the qubit of interest. The scheme involves solving the quantum master equation with Lindblad terms to obtain the system's dynamics. Reliability of the proposed model is validated by testing it on a potassium atom, 41K, and an NV‐ center in diamond. The results demonstrate that by controlling the parameters of the resonator and electron beam, the coherence and decoherence rates of these quantum systems can be enhanced. The proposed scheme has the potential to characterize various types of spin‐based quantum systems and implement quantum logic gates for quantum computation .

Strong coupling dynamics of driven quantum systems with permanent dipoles

Many optically active systems possess spatially asymmetric electron orbitals. These generate permanent dipole moments, which can be stronger than the corresponding transition dipole moments, significantly affecting the system dynamics and creating polarized Fock states of light. We derive a master equation for these systems with an externally applied driving field by employing an optical polaron transformation that captures the photon mode polarization induced by the permanent dipoles. This provides an intuitive framework to explore their influence on the system dynamics and emission spectrum. We find that permanent dipoles introduce multiple-photon processes and a photon sideband, which causes substantial modifications to single-photon transition dipole processes. In the presence of an external drive, permanent dipoles lead to an additional process that we show can be exploited to control the decoherence and transition rates. We derive the emission spectrum of the system, highlighting experimentally detectable signatures of optical polarons, and measurements that can identify the parameters in the system Hamiltonian, the magnitude of the differences in the permanent dipoles, and the steady-state populations of the system.

The weak field limit of quantum matter back-reacting on classical spacetime

Consistent coupling of quantum and classical degrees of freedom exists so long as there is both diffusion of the classical degrees of freedom and decoherence of the quantum system. In this paper, we derive the Newtonian limit of such classical-quantum (CQ) theories of gravity. Our results are obtained both via the gauge fixing of the recently proposed path integral theory of CQ general relativity and via the CQ master equation approach. In each case, we find the same weak field dynamics. We find that the New-tonian potential diffuses by an amount lower bounded by the decoherence rate into mass eigenstates. We also present our results as an unraveled system of stochastic differential equations for the trajectory of the hybrid classical-quantum state and provide a series of kernels for constructing figures of merit, which can be used to rule out part of the parameter space of classical-quantum theories of gravity by experimentally testing it via the decoherence-diffusion trade-off. We compare and contrast the weak field limit to previous models of classical Newtonian gravity coupled to quantum systems. Here, we find that the Newtonian potential and quantum state change in lock-step, with the flow of time being stochastic.

Effects of intrinsic decoherence on quantum coherence and correlations between spins within a two-dimensional honeycomb lattice graphene layer system

This research delves into the influence of intrinsic decoherence on the behavior of quantum correlations and coherence between two interacting qubits in a graphene-based system. To evaluate the amount of nonclassical correlations in the system, we employ local quantum uncertainty (LQU), and to assess quantum coherence we use the relative entropy of coherence [Formula: see text] and [Formula: see text]-norm [Formula: see text]. We assume that the system is initially prepared in an extended-Werner-like (EWL) state, and we investigate how these quantifiers evolve over time and examine their sensitivity to various graphene layer system parameters, mixture parameter of the initial state and the intrinsic decoherence rate. Our results indicate that by adjusting the wave number operators, decreasing the intrinsic decoherence rate, and increasing the initial state mixing parameter, it is possible to enhance both quantum correlations and coherence within the two-dimensional honeycomb lattice system. In addition, we found that quantum coherence is more resilient to intrinsic decoherence than LQU, moreover, the [Formula: see text]-norm is more robust than the relative entropy of coherence.

Coherent memory for microwave photons based on long-lived mechanical excitations

Mechanical resonators, due to their capability to host ultralong-lived phonon modes, are particularly attractive for quantum state storage and as memory elements in conjunction with quantum computing and communication networks. Here we demonstrate absorptive-type coherent memory based on long-lived mechanical excitations. The itinerant coherent microwave field is captured, stored, and retrieved from a mechanical memory oscillator which is pre-cooled to the ground state. The phase space distribution allows us to distinguish between coherent and thermal components and study their evolution as a function of storage time. Our device exhibits attractive functions with an energy decay time of T1 = 15.9 s, a thermal decoherence rate of Γth = 2.85 Hz, and acquires less than one quantum noise during the τcoh = 55.7 ms storage period. We demonstrate that both the amplitude and phase information of microwave coherent states can be recovered, indicating the coherence of our memory device. These results suggest that high-Q mechanical resonators and long coherence time phonons could be ideal candidates for the construction of long-lived and on-demand microwave quantum memories.

Active-feedback quantum control of an integrated low-frequency mechanical resonator

Preparing a massive mechanical resonator in a state with quantum limited motional energy provides a promising platform for studying fundamental physics with macroscopic systems and allows to realize a variety of applications, including precise sensing. While several demonstrations of such ground-state cooled systems have been achieved, in particular in sideband-resolved cavity optomechanics, for many systems overcoming the heating from the thermal bath remains a major challenge. In contrast, optomechanical systems in the sideband-unresolved limit are much easier to realize due to the relaxed requirements on their optical properties, and the possibility to use a feedback control schemes to reduce the motional energy. The achievable thermal occupation is ultimately limited by the correlation between the measurement precision and the back-action from the measurement. Here, we demonstrate measurement-based feedback cooling on a fully integrated optomechanical device fabricated using a pick-and-place method, operating in the deep sideband-unresolved limit. With the large optomechanical interaction and a low thermal decoherence rate, we achieve a minimal average phonon occupation of 0.76 when pre-cooled with liquid helium and 3.5 with liquid nitrogen. Significant sideband asymmetry for both bath temperatures verifies the quantum character of the mechanical motion. Our method and device are ideally suited for sensing applications directly operating at the quantum limit, greatly simplifying the operation of an optomechanical system in this regime.

GRAPE optimization for open quantum systems with time-dependent decoherence rates driven by coherent and incoherent controls

The GRadient Ascent Pulse Engineering (GRAPE) method is widely used for optimization in quantum control. GRAPE is gradient search method based on exact expressions for gradient of the control objective. It has been applied to various coherently controlled closed and open quantum systems. In this work, we adopt the GRAPE method for optimizing objective functionals in open quantum systems driven by both coherent and incoherent controls. In our case, a tailored or engineered environment acts on the controlled system as control via time-dependent decoherence rates or, equivalently, via spectral density of the environment. To develop the GRAPE approach for this problem, we compute gradient of various objectives for general N-level open quantum systems for the piecewise constant class of control. The case of a single qubit is considered in details and solved analytically. For this case, an explicit analytical expression for evolution and objective gradient is obtained via diagonalization of a matrix determining the system’s dynamics in the Bloch ball. The diagonalization is obtained by solving a cubic equation via Cardano’s method. The efficiency of the algorithm is demonstrated through numerical simulations for the state-to-state transition problem and its complexity is estimated. Robustness of the optimal controls is also studied.

Dynamics of molecular rotors in bulk superfluid helium.

Molecules immersed in liquid helium are excellent probes of superfluidity. Their electronic, vibrational, and rotational dynamics provide valuable clues about the superfluid at the nanoscale. Here we report on the experimental study of the laser-induced rotation of helium dimers inside the superfluid 4He bath at variable temperature. The coherent rotational dynamics of [Formula: see text] is initiated in a controlled way by ultrashort laser pulses and tracked by means of time-resolved laser-induced fluorescence. We detect the decay of rotational coherence on the nanosecond time scale and investigate the effects of temperature on the decoherence rate. The observed temperature dependence suggests a nonequilibrium evolution of the quantum bath, accompanied by the emission of the wave of second sound. The method offers ways of studying superfluidity with molecular nanoprobes under variable thermodynamic conditions.

Tunable phononic coupling in excitonic quantum emitters.

Engineering the coupling between fundamental quantum excitations is at the heart of quantum science and technologies. An outstanding case is the creation of quantum light sources in which coupling between single photons and phonons can be controlled and harnessed to enable quantum information transduction. Here we report the deterministic creation of quantum emitters featuring highly tunable coupling between excitons and phonons. The quantum emitters are formed in strain-induced quantum dots created in homobilayer WSe2. The colocalization of quantum-confined interlayer excitons and terahertz interlayer breathing-mode phonons, which directly modulates the exciton energy, leads to a uniquely strong phonon coupling to single-photon emission, with a Huang-Rhys factor reaching up to 6.3. The single-photon spectrum of interlayer exciton emission features a single-photon purity >83% and multiple phonon replicas, each heralding the creation of a phonon Fock state in the quantum emitter. Due to the vertical dipole moment of the interlayer exciton, the phonon-photon interaction is electrically tunable to be higher than the exciton and phonon decoherence rate, and hence promises to reach the strong-coupling regime. Our result demonstrates a solid-state quantum excitonic-optomechanical system at the atomic interface of the WSe2 bilayer that emits flying photonic qubits coupled with stationary phonons, which could be exploited for quantum transduction and interconnection.

Decoherence and nonclassicality of photon-added and photon-subtracted multimode Gaussian states

Photon addition and subtraction render Gaussian states non-Gaussian. We provide a quantitative analysis of the change in nonclassicality produced by these processes by analyzing the Wigner negativity and quadrature coherence scale (QCS) of the resulting states. The QCS is a recently introduced measure of nonclassicality [Phys. Rev. Lett. 122, 080402 (2019); Phys. Rev. Lett. 124, 090402 (2020)], which we show to undergo a relative increase under photon addition and subtraction that can be as large as 200%. This implies that the degaussification and the concomitant increase of nonclassicality come at a cost. Indeed, the QCS is proportional to the decoherence rate of the state so that the resulting states are considerably more prone to environmental decoherence. Our results are quantitative and rely on explicit and general expressions for the characteristic and Wigner functions of photon-added and -subtracted single- and multimode Gaussian states for which we provide a simple and straightforward derivation. These expressions further allow us to certify the quantum non-Gaussianity of the photon-subtracted states with positive Wigner function.

Decoherence of cosmological perturbations from boundary terms and the non-classicality of gravity

We note that the decoherence of inflationary curvature perturbation ζ is dominated by a boundary term of the gravity action. Although this boundary term cannot affect cosmological correlators 〈ζn〉, it induces much faster decoherence for ζ than that of previous calculations. The gravitational origin of inflationary decoherence sheds light on the quantum (or non-classical) nature of gravity. By comparing with a Schrödinger-Newton toy model of classical gravity, we show that gravity theories of classical or quantum origins can be distinguished by comparing their different impacts on decoherence rate of ζ. Our calculation also indicates that density fluctuation δρ better preserves quantum information than ζ for the purpose of constructing cosmological Bell-like experiments.

Circuit quantum electrodynamics with a quadruple quantum dot

In this theoretical work, we describe a mechanism for the coupling between a plane structure consisting of four quantum dots and a resonator. We systematically study the dependence of the quadruple coupling strength and the qubit decoherence rate and point out the optimized operating position of the hybrid system. According to the transmission given by the input–output theory, the signatures in the resonator spectrum are predicted. Furthermore, based on the parameters already achieved in previous works, we prove that the device described in this paper can achieve the strong coupling limit, i.e., this approach can be used for system extension under the existing technical conditions. Our results show an effective and promotable approach to couple quantum dot structures in plane with the resonator and propose a meaningful extension method.

Optical-density enhanced quantum entanglement via four-wave mixing process.

We theoretically propose a scheme to generate a strong continuous-variable quantum entangled light source in four-wave mixing (FWM) process by increasing the optical density of atomic medium. By properly choosing the input coupling field Rabi frequency and detuning, the optimized entanglement can be achieved to be better than -17 dB at an optical density of approximately 1, 000, which has been realized in atomic media. Besides, with the optimized one-photon detuning and coupling Rabi frequency, the optimum entanglement degree can be greatly enhanced with the increment of optical density. We also examine the effects of atomic decoherence rate and two-photon detuning on entanglement in a realistic setting, and evaluate the experimental feasibility. We find that the entanglement can be further improved by considering two-photon detuning. In addition, with optimum parameters the entanglement is robust against the decoherence. The strong entanglement provides a promising applications in continuous-variable quantum communications.

Controlled-Controlled-Phase Gates for Superconducting Qubits Mediated by a Shared Tunable Coupler

Applications for noisy intermediate-scale quantum computing devices rely on the efficient entanglement of many qubits to reach a potential quantum advantage. Although entanglement is typically generated using two-qubit gates, direct control of strong multiqubit interactions can improve the efficiency of the process. Here, we investigate a system of three superconducting transmon-type qubits coupled via a single flux-tunable coupler. Tuning the frequency of the coupler by adiabatic flux pulses enables us to control the conditional energy shifts between the qubits and directly realize multiqubit interactions. To accurately adjust the resulting controlled relative phases, we describe a gate protocol involving refocusing pulses and adjustable interaction times. This enables the implementation of the full family of pairwise controlled-phase and controlled-controlled-phase gates. Numerical simulations result in fidelities around 99% and gate times below 300 ns using currently achievable system parameters and decoherence rates.

Decoherence and thermalization of Unruh-DeWitt detector in arbitrary dimensions

We study the decoherence and thermalization of an Unruh-DeWitt detector linearly coupled to the free massless scalar field in flat spacetime with arbitrary dimensions d ≥ 2. The initial state of the detector is chosen to be a pure state consisting of a linear superposition of ground and excited states, and we calculate the time evolution of reduced density matrix of the detector. Using perturbation method, we analytically derive the transition rate of the detector (the rate of change of the diagonal elements in the density matrix) and the decoherence rate (the rate of change of the off-diagonal elements in the density matrix). We find that the results are not the same in odd and even dimensional spacetimes, but the unitarity of the qubit is preserved in both cases. The real part of the decoherence rate is related to the transition rate, while the imaginary part may contain different forms of divergence terms in different dimensions due to the temporal order product operator and the singularities of the Wightman function for quantum field theory. We derive the recurrence formula to obtain the divergence terms in each dimension and analyze the renormalization problem.

Lévy models for collapse of the wave function

Recently there has been much progress in the development of stochastic models for state reduction in quantum mechanics. In such models, the collapse of the wave function is a physical process, governed by a nonlinear stochastic differential equation that generalizes the Schrödinger equation. The present paper considers energy-based stochastic extensions of the Schrödinger equation. Most of the work carried out hitherto in this area has been concerned with models where the process driving the stochastic dynamics of the quantum state is Brownian motion. Here, the Brownian framework is broadened to a wider class of models where the noise process is of the Lévy type, admitting stationary and independent increments. The properties of such models are different from those of Brownian reduction models. In particular, for Lévy models the decoherence rate depends on the overall scale of the energy. Thus, in Lévy reduction models, a macroscopic quantum system will spontaneously collapse to an eigenstate even if the energy level gaps are small.

Strong coupling between a photon and a hole spin in silicon.

Spins in semiconductor quantum dots constitute a promising platform for scalable quantum information processing. Coupling them strongly to the photonic modes of superconducting microwave resonators would enable fast non-demolition readout and long-range, on-chip connectivity, well beyond nearest-neighbour quantum interactions. Here we demonstrate strong coupling between a microwave photon in a superconducting resonator and a hole spin in a silicon-based double quantum dot issued from a foundry-compatible metal-oxide-semiconductor fabrication process. By leveraging the strong spin-orbit interaction intrinsically present in the valence band of silicon, we achieve a spin-photon coupling rate as high as 330 MHz, largely exceeding the combined spin-photon decoherence rate. This result, together with the recently demonstrated long coherence of hole spins in silicon, opens a new realistic pathway to the development of circuit quantum electrodynamics with spins in semiconductor quantum dots.

Greedy versus map-based optimized adaptive algorithms for random-telegraph-noise mitigation by spectator qubits

In a scenario where data-storage qubits are kept in isolation as far as possible, with minimal measurements and controls, noise mitigation can still be done using additional noise probes, with corrections applied only when needed. Motivated by the case of solid-state qubits, we consider dephasing noise arising from a two-state fluctuator, described by random telegraph process, and a noise probe which is also a qubit, a so-called spectator qubit (SQ). We construct the theoretical model assuming projective measurements on the SQ, and derive the performance of different measurement and control strategies in the regime where the noise mitigation works well. We start with the Greedy algorithm; that is, the strategy that always maximizes the data qubit coherence in the immediate future. We show numerically that this algorithm works very well, and find that its adaptive strategy can be well approximated by a simpler algorithm with just a few parameters. Based on this, and an analytical construction using Bayesian maps, we design a one-parameter ($\mathrm{\ensuremath{\Theta}}$) family of algorithms. In the asymptotic regime of high noise sensitivity of the SQ, we show analytically that this $\mathrm{\ensuremath{\Theta}}$ family of algorithms reduces the data qubit decoherence rate by a divisor scaling as the square of this sensitivity. Setting $\mathrm{\ensuremath{\Theta}}$ equal to its optimal value, ${\mathrm{\ensuremath{\Theta}}}^{★}$, yields the Map-based Optimized Adaptive Algorithm for Asymptotic Regime (MOAAAR). We show, analytically and numerically, that MOAAAR outperforms the Greedy algorithm, especially in the regime of high noise sensitivity of SQ.

Scanning qubit probe of edge states in a topological insulator

In this work, we propose a novel qubit-based sensor with the ability to characterize topological edge states in low-dimensional systems. A composite system is studied, consisting of a qubit coupled to a topologically nontrivial Su-Schrieffer-Heeger chain between semi-infinite lead channels. This qubit probe utilizes decoherence dynamics which, under a weak-coupling framework, are related to the environment's local density of states. Qubit decoherence rate measurements along a sample therefore provide the means to extract edge state profiles. The environment's influence on the qubit's subspace is captured by an effective projective treatment, leading to an analytical decoherence rate expression. We demonstrate that the scanning qubit probe identifies and yields a complete spatial characterization of the topological edge states within the composite system.