Rare Isotope Accelerator Research Articles

Simulation studies for beam commissioning at FRIB Advanced Rare Isotope Separator

The Facility for Rare Isotope Beams (FRIB) includes a powerful superconducting driver accelerator and an Advanced Rare Isotope Separator (ARIS). The ARIS collects and purifies the rare isotope fragments of interest for experiments in nuclear physics, nuclear astrophysics, fundamental symmetries, etc. ARIS consists of a vertical pre-separator and downstream horizontal separator section (C-Bend). Each section can provide a high-resolution separation alternatively. The resolution reduction due to the emittance induced by momentum compression can be avoided by isotope separation in different dispersive planes. Beam commissioning of ARIS for the first experiments was completed and demonstrated particle identification of fragments. The beam tuning in ARIS largely relies on numerical simulations since the limited space for diagnostics. We report the result of the beam trajectory correction, transverse matching, and beam-based misalignment studies at ARIS.

Recent progress in the construction of KoBRA for low-energy nuclear physics experiments

A multi-purpose experimental instrument, called as KoBRA (Korea Broad acceptance Recoil spectrometer and Apparatus), has been constructed for low-energy nuclear physics experiments at RAON (Rare Isotope Accelerator complex for ON-line experiments), and is being prepared in order to produce rare isotope beams at an energy of about 20 MeV/nucleon during the first beam commissioning phase. A test was performed to measure the positions of 4He ions at the dispersive and achromatic foci of KoBRA using an 241Am α-source placed at the production target position, so as to examine the momentum dispersion and ion beam transport. We report on the results of the test and the detailed design of KoBRA including ion optics, together with the status of detectors for particle identification of rare isotopes.

LISE[formula omitted], the latest generation of the LISE[formula omitted] package, to simulate rare isotope production with fragment-separators

The LISE++ software for fragment separator simulations has undergone a major update. The package, widely used at rare isotope beam facilities, can be used to predict intensities and purities of rare isotope beams and for planning and running of experiments using in-flight separators. It is especially useful for radioactive beam production as its results can be quickly compared to on-line data. The LISE++ package has been ported to the Qt-framework in order to support modern compilers and computing methods. The benefits include 64-bit operation and LISE++ availability on three different platforms: Windows, MacOS and Linux. In addition, the porting provides the ability to take advantage of future computational improvements. The updated package is named LISEcute++ to indicate a major step forward from the previous Borland-based versions. In addition to porting to the new platform, new main features and modifications have been added, mostly devoted to improving models and implementing other codes involved in rare isotope production at FRIB. A summary of modifications completed to improve the functionality of the code are discussed in this work, as well as future plans.

Perspectives on Few-Body Cluster Structures in Exotic Nuclei

It is a fascinating phenomenon in nuclear physics that states with a pronounced few-body structure can emerge from the complex dynamics of many nucleons. Such halo or cluster states often appear near the boundaries of nuclear stability. As such, they are an important part of the experimental program beginning at the Facility for Rare Isotope Beams (FRIB). A concerted effort of theory and experiment is necessary both to analyze experiments involving effective few-body states, as well as to constrain and refine theories of the nuclear force in light of new data from these experiments. As a contribution to exactly this effort, this paper compiles a collection of ``perspectives'' that emerged out of the Topical Program ``Few-body cluster structures in exotic nuclei and their role in FRIB experiments'' that was held at FRIB in August 2022 and brought together theorists and experimentalists working on this topic.

Commissioning of the Advanced Rare Isotope Separator ARIS at FRIB

The Facility for Rare Isotope Beams (FRIB) at Michigan State University (MSU) consists of a newly constructed linear accelerator and fragment separator that are designed for enhanced production rates of rare isotopes for use in research and other societal applications. Recent activities through to August 2022 took place to commission the Advanced Rare Isotope Separator (ARIS) and carry out the first experiments. This followed commissioning of the newly constructed linac that is designed to provide orders of magnitude higher beam power than the previously coupled cyclotrons. This required that more advanced target, beam dump, and collimation systems of the new separator be designed and constructed to sustain unprecedented conditions by heavy ion beams. Commissioning with ∼1 kW beams began recently and results from activities that began in late 2021 are reported here. Comparisons between the previous and current facilities are provided.

Optical potentials for the rare-isotope beam era

We review recent progress and motivate the need for further developments in nuclear optical potentials that are widely used in the theoretical analysis of nucleon elastic scattering and reaction cross sections. In regions of the nuclear chart away from stability, which represent a frontier in nuclear science over the coming decade and which will be probed at new rare-isotope beam facilities worldwide, there is a targeted need to quantify and reduce theoretical reaction model uncertainties, especially with respect to nuclear optical potentials. We first describe the primary physics motivations for an improved description of nuclear reactions involving short-lived isotopes, focusing on its benefits for fundamental science discoveries and applications to medicine, energy, and security. We then outline the various methods in use today to build optical potentials starting from phenomenological, microscopic, and ab initio methods, highlighting in particular, the strengths and weaknesses of each approach. We then discuss publicly-available tools and resources facilitating the propagation of recent progresses in the field to practitioners. Finally, we provide a set of open challenges and recommendations for the field to advance the fundamental science goals of nuclear reaction studies in the rare-isotope beam era. This paper is the outcome of the Facility for Rare Isotope Beams Theory Alliance (FRIB-TA) topical program ‘Optical Potentials in Nuclear Physics’ held in March 2022 at FRIB. Its content is non-exhaustive, was chosen by the participants and reflects their efforts related to optical potentials.

RF power coupling of RAON RFQ

A radio frequency quadrupole (RFQ) has been constructed as a front accelerator for a rare isotope accelerator facility. The RFQ has two power couplers that are operated simultaneously for high power operation to accelerate from proton to uranium. Coaxial transmission lines have been adopted to connect each power coupler to the 80 kW solid state power amplifier(SSPA) which is consisted with combiners, circulators and 5 kW unit amplifiers. In this study, the coupling to the cavity with two power couplers was investigated for the failure of RF power units. Moreover, the operation scenario of the RFQ linac was also presented in considering the availability.

Search prospects for axionlike particles at rare nuclear isotope accelerator facilities

We propose a novel experimental scheme, called DAMSA (Dump-produced Aboriginal Matter Searches at an Accelerator), for searching for dark-sector particles, using rare nuclear isotope accelerator facilities that provide high-flux proton beams to produce a large number of rare nuclear isotopes. The high-intensity nature of their beams enables the investigation of dark-sector particles, including axion-like particles (ALPs) and dark photons. By contrast, their typical beam energies are not large enough to produce the backgrounds such as neutrinos resulting from secondary charged particles. The detector of DAMSA is then placed immediate downstream of the proton beam dump to maximize the prompt decay signals of dark-sector particles, which are often challenging to probe in other beam-dump-type experiments featuring a longer baseline, at the expense of an enormous amount of the beam-related neutron (BRN) background. We demonstrate that BRN can be significantly suppressed if the signal accompanies multiple, correlated visible particles in the final state. As an example physics case, we consider ALPs interacting with the Standard Model photon and their diphoton decay signal at DAMSA implemented at a rare nuclear isotope facility similar to the Rare isotope Accelerator complex for ON-line experiment under construction in South Korea. We show that the close proximity of the detector to the ALP production dump makes it possible to probe a high-mass region of ALP parameter space that the existing experiments have never explored.

Commissioning preparation of RAON rare isotope accelerator facility

Commissioning preparation of RAON rare isotope accelerator facility

Search for CP-Violation in ortho-Positronium Decay

We report here on the design and development of a new apparatus aiming at a 10-fold improved search for CP-violation in ortho-Positronium decay to be performed at the Facility for Rare Isotope Beams.

A Problem in the Statistical Description of Beta-Delayed Neutron Emission

Reaction measurements on fission products are being planned at both Argonne National Lab and at the Facility for Rare Isotope Beams. These indirect experiments produce specific short-lived nuclei via beta decay, and the subsequent neutron and gamma emission are studied. Some initial experiments found a surprising overabundance of gamma emission, which theory has yet to explain. To remedy this, we are developing an integrated nuclear data workflow that connects advanced nuclear shell model codes for describing the beta decay with a contemporary nuclear reaction model code.

Identification of a potential ultralow- Q -value electron-capture decay branch in Se75 via a precise Penning trap measurement of the mass of As75

Background: Low energy $\beta$ and electron capture (EC) decays are important systems in neutrino mass determination experiments. An isotope with an ultra-low Q value $\beta$-decay to an excited state in the daughter with Qes < 1 keV could provide a promising alternative candidate for future experiments. $^{75}$Se EC and $^{75}$Ge $\beta$-decay represent such candidates, but a more precise determination of the mass of the common daughter, $^{75}$As, is required to evaluate whether their potential decay branches are energetically allowed and ultra-low. Purpose: Perform a precise atomic mass measurement of $^{75}$As and combine the result with the precisely known atomic masses of $^{75}$Se and $^{75}$Ge, along with nuclear energy level data for $^{75}$As to evaluate potential ultra-low Q value decay branches in the EC decay of $^{75}$Se and the $\beta$-decay of $^{75}$Ge. Method: The LEBIT Penning trap mass spectrometer at the Facility for Rare Isotope Beams was used to perform a high-precision measurement of the atomic mass of $^{75}$As via cyclotron frequency ratio measurements of $^{75}$As$^{+}$ to a $^{12}$C$_{6}^{+}$ reference ion. Results: The $^{75}$As mass excess was determined to be ME($^{75}$As)= -73 035.98(43) keV, from which the ground-state to ground-state Q values for $^{75}$Se EC and $^{75}$Ge $\beta$-decay were determined to be 866.50(44) keV and 1179.01(44) keV, respectively. These results were compared to energies of excited states in $^{75}$As at 865.4(5) keV and 1172.0(6) keV to determine Q values of 1.1(7) keV and 7.0(7) keV for the potential ultra-low EC and $\beta$-decay branches of $^{75}$Se and $^{75}$Ge, respectively. Conclusion: The $^{75}$Se EC decay to the 865.4 keV excited state in $^{75}$As is potentially ultra-low with Qes $\approx$ 1 keV. However, a more precise determination of the 865.4(5) keV level in $^{75}$As is required.

Design and construction of a novel energy-loss optical scintillation system (ELOSS) for heavy-ion particle identification.

We present the development of a novel heavy-ion particle-identification (PID) device based on an energy-loss measurement to be implemented in the focal plane of the S800 spectrograph of the Facility for Rare Isotope Beams (FRIB). The new instrument consists of a multi-segmented optical detector [energy-loss optical scintillation system (ELOSS)] that is filled with xenon at pressures ranging from 400 to 800 Torr. The gas volume is surrounded by arrays of photomultiplier tubes and placed along the direction of the beam for recording the prompt scintillation light. The number of detected photons, which is proportional to the energy deposited by the beam particle along its track in the detector volume, allows one to identify the corresponding atomic number (Z). The ELOSS technology is expected to provide high-resolution ΔE measurements (≤0.6% σ) at a high counting rate (>50kHz). In addition, it has the capability of providing timing information with around 150ps resolution (σ) compared to the lack of useable timing information of the conventional ionization chamber relying on drifting charges. The development of fast, accurate ΔE measurement techniques for present and future nuclear science facilities will have a high impact on the design and implementation of rare-isotope beam experiments at FRIB and their scientific outcome. As such, ELOSS also represents a prototype for the development of PID detector systems of other planned and future spectrometers, such as the high rigidity spectrometer at FRIB.

Crossing N=28 Toward the Neutron Drip Line: First Measurement of Half-Lives at FRIB

New half-lives for exotic isotopes approaching the neutron drip-line in the vicinity of N∼28 for Z=12-15 were measured at the Facility for Rare Isotope Beams (FRIB) with the FRIB decay station initiator. The first experimental results are compared to the latest quasiparticle random phase approximation and shell-model calculations. Overall, the measured half-lives are consistent with the available theoretical descriptions and suggest a well-developed region of deformation below ^{48}Ca in the N=28 isotones. The erosion of the Z=14 subshell closure in Si is experimentally confirmed at N=28, and a reduction in the ^{38}Mg half-life is observed as compared with its isotopic neighbors, which does not seem to be predicted well based on the decay energy and deformation trends. This highlights the need for both additional data in this very exotic region, and for more advanced theoretical efforts.

Design of the High Rigidity Spectrometer at FRIB

A High Rigidity Spectrometer (HRS) has been designed for experiments at the Facility for Rare-Isotope Beams (FRIB) at Michigan State University (MSU). The HRS will allow experiments to be performed with the most exotic neutron-rich isotopes at high beam energies (≳100MeV/u). The HRS consists of an analysis beamline called the High-Transmission Beamline (HTBL) and the spectrometer proper called the Spectrometer Section. The maximum magnetic rigidity of the HRS is 8Tm, which corresponds to the rigidities at which rare-isotope beams are optimally produced at FRIB. The resolving power, angular acceptance, and momentum acceptance are set to match the anticipated scientific program. An ion-optical design developed for the HRS is described in detail, along with the specifications of the associated magnet and detector systems.

Solid-phase isotope harvesting of 88Zr from a radioactive ion beam facility

During routine operation of the Facility for Rare Isotope Beams (FRIB), radionuclides will accumulate in both the aqueous beam dump and along the beamline in the process of beam purification. These byproduct radionuclides, many of which are far from stability, can be collected and purified for use in other scientific applications in a process called isotope harvesting. In this work, the viability of 88Zr harvesting from solid components was investigated at the National Superconducting Cyclotron Laboratory. A secondary 88Zr beam was stopped in a series of collectors comprised of Al, Cu, W, and Au foils. This work details irradiation of the collector foils and the subsequent radiochemical processing to isolate the deposited 88Zr (and its daughter 88Y) from them. Total average recovery from the Al, Cu, and Au collector foils was (91.3 ± 8.9) % for 88Zr and (95.0 ± 5.8) % for 88Y, respectively, which is over three times higher recovery than in a previous aqueous-phase harvesting experiment. The utility of solid-phase isotope harvesting to access elements such as Zr that readily hydrolyze in near-neutral pH aqueous conditions has been demonstrated for application to harvesting from solid components at FRIB.

Recent progress in two-proton radioactivity

During the last few decades, rare isotope beam facilities have provided unique data for studying the properties of nuclides located far from the beta-stability line. Such nuclei are often accompanied by exotic structures and radioactive modes, which represent the forefront of nuclear research. Among them, two-proton (2p) radioactivity is a rare decay mode found in a few highly proton-rich isotopes. The 2p decay lifetimes and properties of emitted protons hold invaluable information regarding the nuclear structures in the presence of a low-lying proton continuum; as such, they have attracted considerable research attention. In this review, we present some of the recent experimental and theoretical progress regarding the 2p decay, including technical innovations for measuring nucleon–nucleon correlations and developments in the models that connect their structural aspects with their decay properties. This impressive progress should play a significant role in elucidating the mechanism of these exotic decays, probing the corresponding components inside nuclei, and providing deep insights into the open quantum nature of dripline systems.

A Model for Radiolysis in a Flowing-Water Target during High-Intensity Proton Irradiation.

At the Facility for Rare Isotope Beams (FRIB), interactions between heavy-ion beams and beam-dump water will create a wide variety of radionuclides which can be accessed by a technique known as “isotope harvesting”. However, irradiation of water is always accompanied by the creation of numerous radical, ionic, and molecular radiolysis products. Some of the radiolysis products have sufficiently long lifetimes to accumulate in the irradiated water and affect the harvesting chemistry. Here we investigate the formation of hydrogen peroxide, molecular hydrogen, and molecular oxygen during a high-intensity proton irradiation of a flowing-water isotope-harvesting target and compare the experimental results to simulations. The simulations kinetically model the chemical reactions occurring in the homogeneous phase of radiolysis in flowing water and establish an “effective yield”. In both the experiment and simulations, the bulk quantities of H2, H2O2, and O2 are considerably lower than predicted by primary radiolysis yields (escape yields), meaning that in the high beam intensity regime the homogeneous phase reactions have a considerable impact on the overall chemical composition of the water. Further, it could be shown that for radiation which is characterized by a limited linear energy transfer, such as the here applied protons, the bulk outcome of the microscopic kinetic modeling could be estimated by a simplified steady-state model.

Moment constraints in beams with discrete and continuous rotational symmetry

This study presents a general analysis of how the transverse rotational symmetry of a beam imposes equality constraints among transverse beam moments. Efficient analytic methods are developed to derive symmetry-imposed constraints among $k$th order moments in beams with continuous or $n$-fold rotational symmetry for arbitrary $k$ and $n$. The formalism also enables one to construct symmetry arguments based on how discrete and continuous rotational symmetries manifest themselves differently in terms of beam moments. Three case studies on beams with continuous, twofold, and threefold rotational symmetries are conducted. We prove that, regardless of their triangulation, beams with threefold rotational symmetry (e.g., from electron cyclotron resonance ion source) always have the same rms properties as beams with cylindrical symmetry. These counterintuitive results derived purely from symmetry considerations have clarified beam dynamics at the Facility for Rare Isotope Beams.

Electromagnetic Investigation on a Sextupole HTS Magnet for RAON

The rare isotope accelerator complex for online experiments (RAON) is a heavy-ion accelerator equipped with an in-flight fragment separator (IF) system and isotope separation online technique in South Korea. Six quadrupole and a sextupole high-temperature superconducting (HTS) magnets are installed in the hot cell of the IF system, which is a high radiation region, to arrange the ion beams and correct the chromatic aberrations of the ion beams. The magnets are developed and installed for RAON at the Institute for Basic Science (IBS), South Korea. Superconducting magnet systems should be capable of a stable operation against high radiation heating and thermally and electromagnetically robust in the intense radioactive hot cell region. In this paper, we describe the design, fabrication, and evaluation of a sextupole HTS magnet. Electromagnetic designs are conducted considering the position of the HTS magnets and the angle of the yoke pole tip <italic xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">et al.</i> The required design specifications are proposed as a part of RAON of IBS considering the following electromagnetic performance: 1) a magnetic field gradient of <inline-formula xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink"><tex-math notation="LaTeX">$ \geq $</tex-math></inline-formula> 3.9 T/m <sup xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">2</sup> , 2) magnetic field uniformity of <inline-formula xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink"><tex-math notation="LaTeX">$ &lt; $</tex-math></inline-formula> 0.5%, 3) effective length of 450 ± 1 mm, and 4) operating temperature of ∼ 45 K.