Radiochemical analyses of aerosols and precipitation collected along the slopes of Mauna Loa volcano in Hawaii show that the concentration of radioactivity in aerosols generally increases with height across the trade wind inversion. The time variations of the vertical distribution of radioactivity concentration and moisture mixing ratio were inversely correlated; intrusions of dry air having higher concentrations of radioactivity accompanied vertical oscillations in the upper boundary of the moist surface layer. The concentration of Sr90 in rain along the slopes generally decreased with altitude above the cloud base. This decrease is attributed to the continuous depletion of condensation nuclei through rainout while remaining droplets in the air parcels continue to grow as they move upslope.
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