Radioactive Cesium Research Articles

Estimation of water seepage rate in the active crater lake system of Kusatsu-Shirane volcano, Japan, using FDNPP-derived radioactive cesium as a hydrological tracer

We describe here a first attempt to estimate the water seepage rate of an active crater lake using radioactive cesium dispersed into the environment by the Fukushima Dai-ichi Nuclear Power Plant accident in March 2011 as a hydrological tracer. Kusatsu-Shirane volcano is one of the most active volcanoes in Japan and has an active crater lake named Yugama. There is no outflow such as a river from Yugama crater lake. The content level of stable cesium (133Cs) in Yugama water was almost constant at 15–20 nM during the sampling period of Nov. 2011 to Nov. 2014. In contrast to 133Cs, however, the radioactive cesium (134Cs and 137Cs) concentrations in Yugama water decreased at a more rapid rate than expected by radioactive decay. Based on the decreasing rates of activity concentrations of 134Cs and 137Cs in Yugama water during the three years between 2012 and 2014, it is estimated that 700–800 m3 of the Yugama water, which corresponds approximately to 0.1% of the total volume, leaks through the lakebed per day. In the estimation, balance between leakage of radioactive cesium contaminated water though lake bed and geothermal inflow of radioactive cesium-free water in the volcano was taken into account. Consequently, the water seepage rate of the Yugama crater lake was calculated to be 8.1–9.3 L s−1.

COMPARATIVE STUDY OF THE CESIUM UPTAKE ABILITY BETWEEN HEU-TYPE (CLINOPTILOLITE-HEULANDITE) ZEOLITIC TUFF AND PURE HEULANDITE

Specific continuous layers of zeolitic tuff in Ntrista stream location of Petrota area of Evros region (NA11) and pure natural crystals of heulandite (HEU1) from the collection of the Department of Mineralogy-Petrology-Economic Geology, School of Geology, Aristotle University of Thessaloniki, have been investigated. The X-Ray Diffraction analyses showed that the sample NA11 consists of 86 wt% HEU-type zeolite, 4 wt% micas+ clay-minerals, 4 wt% quartz, 2 wt% christobalite and 4 wt% feldspars, while the sample HEU1 is pure heulandite crystal. The mineral-chemistry was determined by SEM-EDS microanalyses. The zeolite of the NA11 sample is Ca-rich clinoptilolite and its chemical formulae is Ca1.8K1.0Mg0.7Na0.5Al6.4 Si29.5O72·21H2O, while the zeolite of the sample HEU1 is heulandite and its chemical formulae is Ca3.6Na1.0Κ0.2Sr0.2Ba0.1Al8.1Si27.6O72·21H2O. The uptake ability of the samples was measured by the AMAS method (Ammonium Acetate Saturation). The two examined materials show high uptake ability. The measured value for the zeolitic tuff NA11 is 231 meq/100g, while for the heulandite crystal (HEU1) is 296 meq/100g. For the determination of the cesium sorption a CsNO3 solution (concentration 500 mg/L), labelled with small activity of 137Cs, and pH 2-12 was used. The sorption of the cesium by the two materials, was determined by measuring the gamma radiation emitted by the 137Cs tracer. The zeolitic tuff presents higher uptake ability of radioactive cesium than the pure heulandite crystal, whereas the sorption of radioactive cesium is not significantly affected by the pH values of the initial solutions in the range pH 2-12.The clinoptilolitic zeolitic tuff NA11 is suitable material for various environmental, agricultural and industrial applications.

Radiation Dose Assessment Model for Terrestrial Flora and Fauna and Its Application to the Environment near Fukushima Accident

Background: To investigate radiological effects on biota, it is necessary to assess radiation dose for flora and fauna living in a terrestrial ecosystem. This paper presents a dynamic model to assess radioactivity concentration and radiation dose of terrestrial flora and fauna after a nuclear accident. Materials and Methods: Litter, organic soil, mineral soil, trees, wild crops, herbivores, omnivores, and carnivores are considered the major components of a terrestrial ecosystem. The model considers the physicochemical and biological processes of interception, weathering, decomposition of litter, percolation, root uptake, leaching, radioactive decay, and biological loss of animals. The predictive capability of the model was investigated by comparison of its predictions with field data for biota measured in the Fukushima forest area after the Fukushima nuclear accident. Results and Discussion: The predicted radioactive cesium inventories for trees agreed well with those for evergreens and deciduous trees sampled in the Fukushima area. The predicted temporal radioactivity concentrations for animals were within the range of the measured radioactivity concentrations of deer, wild boars, and black bears. The radiation dose for the animals were, for the whole simulation time, estimated to be much smaller than the lower limit (0.1 mGy∙ d-1) of the derived consideration reference level given by the International Commission on Radiological Protection for terrestrial flora and fauna. This suggested that the radiation effect of the accident on the biota in the Fukushima forest would be insignificant. Conclusion: The present dynamic model can be used effectively to investigate the radiological risk to terrestrial ecosystems following a nuclear accident.

Application of linear minimum variance estimation to the multi-model ensemble of atmospheric radioactive Cs-137 with observations

Abstract. Great efforts have been made to simulate atmospheric pollutants, but their spatial and temporal distributions are still highly uncertain. Observations can measure their concentrations with high accuracy but cannot estimate their spatial distributions due to the sporadic locations of sites. Here, we propose an ensemble method by applying a linear minimum variance estimation (LMVE) between multi-model ensemble (MME) simulations and measurements to derive a more realistic distribution of atmospheric pollutants. The LMVE is a classical and basic version of data assimilation, although the estimation itself is still useful for obtaining the best estimates by combining simulations and observations without a large amount of computer resources, even for high-resolution models. In this study, we adopt the proposed methodology for atmospheric radioactive caesium (Cs-137) in atmospheric particles emitted from the Fukushima Daiichi Nuclear Power Station (FDNPS) accident in March 2011. The uniqueness of this approach includes (1) the availability of observed Cs-137 concentrations near the surface at approximately 100 sites, thus providing dense coverage over eastern Japan; (2) the simplicity of identifying the emission source of Cs-137 due to the point source of FDNPS; (3) the novelty of MME with the high-resolution model (3 km horizontal grid) over complex terrain in eastern Japan; and (4) the strong need to better estimate the Cs-137 distribution due to its inhalation exposure among residents in Japan. The ensemble size is six, including two atmospheric transport models: the Weather Research and Forecasting – Community Multi-scale Air Quality (WRF-CMAQ) model and non-hydrostatic icosahedral atmospheric model (NICAM). The results showed that the MME that estimated Cs-137 concentrations using all available sites had the lowest geometric mean bias (GMB) against the observations (GMB =1.53), the lowest uncertainties based on the root mean square error (RMSE) against the observations (RMSE =9.12 Bq m−3), the highest Pearson correlation coefficient (PCC) with the observations (PCC =0.59) and the highest fraction of data within a factor of 2 (FAC2) with the observations (FAC2 =54 %) compared to the single-model members, which provided higher biases (GMB =1.83–4.29, except for 1.20 obtained from one member), higher uncertainties (RMSE =19.2–51.2 Bq m−3), lower correlation coefficients (PCC =0.29–0.45) and lower precision (FAC2 =10 %–29 %). At the model grid, excluding the measurements, the MME-estimated Cs-137 concentration was estimated by a spatial interpolation of the variance used in the LMVE equation using the inverse distance weights between the nearest two sites. To test this assumption, the available measurements were divided into two categories, i.e. learning and validation data; thus, the assumption for the spatial interpolation was found to guarantee a moderate PCC value (> 0.4) within an approximate distance of at least 70 km. Extra sensitivity tests for several parameters, i.e. the site number and the weighting coefficients in the spatial interpolation, the time window in the LMVE and the ensemble size, were performed. In conclusion, the important assumptions were the time window and the ensemble size; i.e. a shorter time window (the minimum in this study was 1 h, which is the observation interval) and a larger ensemble size (the maximum in this study was six, but five is also acceptable if the members are effectively selected) generated better results.

Hollandites’ crystal chemistry, properties, and processing: a review

ABSTRACT This review provides a broad overview of the structural characteristics, compositional flexibility, and structure–property relationships of hollandite materials. Hollandites have a general formula AxB 8O16, x ≤ 2, with ‘A’ cations located in one-dimensional tunnels formed by a framework of ‘B’–O octahedra. With numerous possibilities for chemical and structural modifications, hollandite family provides many opportunities to manipulate its properties for specific applications. First, we review the chemistry, structure–property relationship, and processing techniques for various applications. The primary focus is on the cumulative effects of A- and B-cation interaction, and the resultant parameters including unit cell symmetry, cation order–disorder, electronic and/or magnetic coupling, that dictate the material's applicability. Then, selected applications, such as crystalline hosts for radioactive caesium disposal, electrode material for Li-ion batteries, and ferromagnetic materials, are outlined from a structure–property relationship perspective. Finally, processing strategies in correlation with structural evolution and applications are briefly addressed.

Magnetic zeolite synthesis for efficient removal of cesium in a lab-scale continuous treatment system

Radioactive cesium was resealed to the environment as a result of many nuclear incidents. An effective treatment system is urgently needed to safely handle radioactive cesium-contaminated waters. Based on nanoscale zerovalent iron (nZVI) and zeolite, nine adsorbents were synthesized and applied to remove cesium from aqueous solutions. Magnetic zeolite composite (Ze/Fe0) was selected as the ideal adsorbent for treating cesium contaminated waters in a lab-scale continuous treatment system (LSCTS). The optimization process of the (Ze/Fe0) composite revealed that 1:1 is the optimum mass ratio between zeolite and nZVI. Furthermore, the optimization process proved that the initial pH and temperature have no significant effect on the adsorption of cesium by (Ze/Fe0) composite and the optimum dosage of (Ze/Fe0) composite is 5 g L−1. XRD and SEM results showed that the (Ze/Fe0) composite has an irregular shape with a poor crystalline structure. Kinetic and equilibrium data were best described by pseudo second order and Freundlich isotherm models. Seawater and groundwater experiments illustrated that the removal of cesium by (Ze/Fe0) composite was inhibited due to the existence of competing cations. Eight cycles of LSCTS were performed to examine the performance of (Ze/Fe0) composite in treating continuous streams of cesium contaminated waters. In all cycles except the cycle of treating contaminated seawater, LSCTS succeed to treat continuous flows of 1 mg L−1 cesium contaminated water with 100% overall removal efficiency. For treating contaminated seawater, pre-treatment unit is required to reduce the salinity of the contaminated seawater before staring the treatment process.

Variations in radioactive cesium accumulation in wheat germplasm from fields affected by the 2011 Fukushima nuclear power plant accident

Decreasing the transfer of radioactive cesium (RCs) from soil to crops has been important since the deposition of RCs in agricultural soil owing to the Fukushima nuclear power plant accident of 2011. We investigated the genotypic variation in RCs accumulation in 234 and 198 hexaploid wheat (Triticum spp.) varieties in an affected field in 2012 and 2013, respectively. The effects of soil exchangeable potassium (ExK) content to RCs accumulation in wheat varieties were also evaluated. A test field showed fourfold differences in soil ExK contents based on location, and the wheat varieties grown in areas with lower soil ExK contents tended to have higher grain RCs concentrations. RCs concentrations of shoots, when corrected by the soil ExK content, were positively significantly correlated between years, and RCs concentrations of shoots were significantly correlated with the grain RCs concentration corrected by the soil ExK content. These results indicated that there were genotypic variations in RCs accumulation. The grain to shoot ratio of RCs also showed significant genotypic variation. Wheat varieties with low RCs accumulations were identified. They could contribute to the research and breeding of low RCs accumulating wheat and to agricultural production in the area affected by RCs deposition.

Efficiently remove of Cs(I) by metals hexacyanoferrate modified magnetic Fe3O4-chitosan nanoparticles

In order to remove radioactive cesium from wastewater and realize recycling of cesium meanwhile, biopolymer: chitosan functionalized Fe3O4 nanoparticles were synthesized. Chitosan covalently functionalized particles were well dispersed, superparamagnetic and had good stability. Sodium-copper hexacyanoferrate as ion exchanger modified the particles through metal coordination for cesium adsorption. The particles showed good selectivity for Cs(I) and high adsorption capacity (161.3 mg/g). And the desorption rate of Cs(I) could reach up to 99.5%. The relative adsorption capacity still remained 96.6% after the 5th reuse. The results showed the particles were promising for removal of Cs(I) from large-scale waste water.

Isotopic ratios of uranium and caesium in spherical radioactive caesium-bearing microparticles derived from the Fukushima Dai-ichi Nuclear Power Plant

Spherical radioactive caesium (Cs)-bearing microparticles (CsMPs) were emitted during the Fukushima Dai-ichi Nuclear Power Plant (FDNPP) accident in March, 2011. The emission source (timing) and formation process of these particles remain unclear. In this study, the isotopic ratios of uranium (235U and 238U) and caesium (133Cs, 134Cs, 135Cs, and 137Cs) isotopes in the five spherical CsMPs (ca. 2 μm in size) sampled at 50 km west of the FDNPP were determined using secondary ion mass spectrometry and laser ablation-ICPMS, respectively. Results showed that the 235U/238U ratios of CsMPs were homogeneous (1.93 ± 0.03, N = 4) and close to those estimated for the fuel cores in units 2 and 3, and that the Cs isotopic ratios of CsMP were identical to those of units 2 and 3. These results indicated that U and Cs in the spherical CsMPs originated exclusively from the fuel melt in the reactors. Based on a thorough review of literatures related to the detailed atmospheric releases of radionuclides, the flow of plumes from the FDNPP reactor units during the accident and the U and Cs isotopic ratio results in this study, we hereby suggest that the spherical CsMPs originate only from the fuel in unit 2 on the night of 14 March to the morning of 15 March. The variation range of the analysed 235U/238U isotopic ratios for the four spherical particles was extremely narrow. Thus, U may have been homogenised in the source through the formation of fuel melt, which ultimately evaporating and taken into CsMPs in the reactor and was released from the unit 2.

Influence of Soil Characteristics and Land Use Type on Existing Fractions of Radioactive 137Cs in Fukushima Soils

Radioactive cesium (137Cs) in distinct soil fractions provides key information to its bioavailability, and therefore determining the effect of soil characteristics and land use types on existing fractions of 137Cs in soils is important for predicting future 137Cs mobility in Fukushima. Thus, the objective of this study was to investigate the influence of soil characteristics and land use types on sequentially extracted fractions of 137Cs in Fukushima. In this study, five coniferous forest soils, eight arable soils, and eight paddy rice soils were sampled in 2012 and 2013. The 137Cs in the soils were separated into four fractions; water-soluble, exchangeable, organic matter-bound and residual fractions. More than 90% of the soil 137Cs fraction for arable and paddy rice soils was found in the residual fraction, implying significantly reduced bioavailable 137Cs with higher fixation. In contrast, forest soils measured higher exchangeable and organic matter-bound fractions of 5%–33% and 9%–44%, respectively, implying future 137Cs mobility in the forest ecosystem. Correlation analysis showed a significant negative correlation (p < 0.05) between the organic matter fraction and residual fraction in both arable and paddy rice soils. There was a significant positive correlation (p < 0.05) for both exchangeable and residual fractions with cation exchange capacity (CEC), total carbon (TC) and total nitrogen (TN) values in arable soils. Organic matter content influenced both exchangeable and residual fractions. It was not clear whether organic matter played a direct role in 137Cs fixation or mobility in the agricultural soils. In paddy rice soils, the organic matter fraction showed a significant negative correlation with TC and TN values. Soil pH was significantly negatively correlated (p < 0.05) with both water-soluble and residual fractions in forest soils but positively (p < 0.1) with the organically bound 137Cs fraction.

Effective removal of cesium from wastewater via adsorptive filtration with potassium copper hexacyanoferrate-immobilized and polyethyleneimine-grafted graphene oxide

As an attractive alternative to radioactive cesium removal, we introduced an adsorptive filtration method using a composite membrane consisting of potassium copper hexacyanoferrate (KCuHCF) and graphene-based support. Polyethyleneimine-grafted reduced graphene oxide (PEI-rGO), used as an immobilizing matrix, was effective not only in distributing KCuHCF inside the composite with the aid of abundant amino-functionality, but also in achieving high water flux by increasing the interlayer spacing of the laminar membrane structure. Due to the rapid and selective cesium adsorption properties of KCuHCF, the fabricated membrane was found to be effective in achieving complete removal of cesium ions under a high flux (over 500 L m−2 h−1), which is difficult in a conventional membrane utilizing the molecular sieving effect. This approach offers strong potential in the field of elimination of radionuclides that require rapid and complete decontamination.

Radioactive contaminants binding on pillared layered clays

The selective sorption of radioactive cesium and strontium on Pillared Layered Clays was investigated. Two reference samples were initially used in experiments, both in vitro and in vivo. An improved nanocomposite-pillared clay with different organization and structural evolution of its building blocks, was constructed, characterized by several methods and employed in exchange experiments. The results derived from the improved material administration in ruminants for strontium and cesium sorption were positive and further investigation is under way.

Usefulness of the whole-body counter for infants and small children (BABYSCAN) as a risk communication tool after the Fukushima Daiichi nuclear power plant incident.

Responding to the radiation-related concerns of parents/guardians with infants/small children is an important public health issue for regional recovery after radioactive contamination. This study summarizes the results of a systematic internal contamination screening of infants/small children, aged 0–6 years, using BABYSCAN and individual counselling sessions with physicians about radiation concerns from 2014 to 2018 in Minamisoma City. Of 3,114 participants, no one was found to have internal contamination with radioactive caesium with a detection limit of 50 Bq/body. The questionnaire survey showed a decreasing trend of concerns about food contamination and playing outside as possible causes of internal contamination over time. Because people’s concerns were diverse in counselling sessions, individual responses are required. This study showed that examinations using BABYSCAN provide an opportunity for direct dialogue between the parents/guardians of infants/small children and experts. This can be considered a model case for risk communication conducted by the local government after a radioactive contamination incident.

Accumulation of radioactive caesium in the Japanese eel Anguilla japonica in Northeast Japan after the Fukushima nuclear accident

ABSTRACT The unpredicted nuclear accident by the Fukushima Daiichi Nuclear Power Plant (F1NPP) is a global concern for human health and ecosystems. In the present study, five-year fluctuations and accumulations of Cs, 134Cs and 137Cs in the Japanese eel were examined in Northeast Japan. The eel is one of the most important research subjects in fishery resources in Asia. The total radioactive Cs, 134Cs and 137Cs levels in the fish gradually decreased throughout the five-year study period after the F1NPP accident. A faster decay rate was found for 134Cs (10–15%) for five years after the F1NPP accident, and the decay of 137Cs (30–90%) was slower during the five years. The difference of decay rates between radiocaesiums might be explained by their different half-lives. The F1NPP derived 134Cs contamination might cease unless fresh input may be detected, and 137Cs might still be distributed and remain in the natural environment.

Black Wave: How Networks and Governance Shaped Japan’s 3/11 Disasters

Reviewer: James R. Elliott, Rice University Imagine being violently shook, drowned, and nuked in rapid succession. That in essence is what happened to Japanese communities at the epicenter of the triple disasters of March 11, 2011. It started with a nearby earthquake that thrust the ocean floor upward 52 feet. That violent energy then produced a tsunami 65 feet high, enough to devastate retaining walls and turn the sea’s surging waters black with debris as they pushed 6 miles inland, up local waterways. In the Fukushima Prefecture, these events triggered an automatic shutdown of nuclear reactors at the local power plant, as planned. The problem was that the huge batteries designed to cool the reactors by powering water through their cores were in the basement—a location intended to avoid outages from tornadoes in the United States, where the reactors were designed, but not from tsunamis where they were actually installed. With that backup power neutralized, radioactive fuel inside the reactors reached temperatures of 5,000 degrees Fahrenheit, melting through the 7-inch steel barriers and eventually spreading radioactive cesium and iodine over more than 5,000 sq. mi. The result was one of the costliest disasters in human history, with more than $235 billion in losses and an expected $200 billion more in costs of active decontamination and victim compensation, which is not yet complete.

Visualization of Low-Level Gamma Radiation Sources Using a Low-Cost, High-Sensitivity, Omnidirectional Compton Camera.

We present experimental protocols for visualizing various low-level gamma radiation sources in the ambient environment. Experiments were conducted by using a low-cost, high-sensitivity, omnidirectional, gamma-ray imaging Compton camera. In the laboratory, the position of a sub-MeV gamma radiation source such as 137Cs can easily be monitored via omnidirectional gamma-ray imaging obtained by the Compton camera. In contrast, a stationary, wall-mounted dose rate monitor cannot always successfully monitor such a source. Furthermore, we successfully demonstrated the possibility of visualizing the radioactivity movement in the environment, for example, the movement of a patient injected with 18F-fluorodeoxyglucose (18F-FDG) in a nuclear medicine facility. In the Fukushima field, we easily obtained omnidirectional gamma-ray images concerned with the distribution on the ground of low-level radioactive contamination by radioactive cesium released by the Fukushima Daiichi nuclear power plant accident in 2011. We demonstrate clear advantages of using our procedure with this camera to visualize gamma-ray sources. Our protocols can further be used to discover low-level gamma radiation sources, in place of stationary dose rate monitors and/or portable survey meters used conventionally.

Characterization of soluble and insoluble radioactive cesium in municipal solid waste incineration fly ash

Soluble and insoluble radioactive cesium in municipal solid waste incineration fly ash were analyzed by X-ray diffraction and gamma-ray spectrometry. A total of 60% of soluble radioactive cesium was determined using the Tessier extraction method, and it was almost same extraction rate with Japanese leaching test No.13. In addition, chloride compounds such as halite (NaCl) and sylvite (KCl) showed same behavior with soluble radioactive cesium, therefore, soluble radioactive cesium existed as a chloride (CsCl) with water solubility characteristics. Almost insoluble radioactive cesium trapped into silicate of crystalline phase or amorphous phase was eluted by hydrogen fluoride treatment. Radioactive 137Cs was released in three stages by heating treatment (untreated - 400 °C, 600 °C–800 °C, and 800 °C–1000 °C) according to decreasing amorphous content. The relationship between the concentrations of radioactive 137Cs and amorphous phase exhibited good linearity (R = 0.9278). Insoluble radioactive 137Cs was contained in inner part of the amorphous phase, and free radioactive cesium was determined from the concentration of the amorphous phase.

Decontamination of low-level contaminated water from radioactive cesium and cobalt using microalgae

This study selects microalgae suitable for the decontamination of radioactive cobalt (Co-60) in radioactive solutions based on the decontamination efficiency of Co-60 and Cs-137 by various microalgae. The biosorption rates of Co-60 in the low-level contaminated water have been measured using three different types of microalgae Haematococcus sp., Vacuoliviride crystalliferum, and Chlorella vulgaris, which are known to uptake Cs-137 and Sr-90 effectively. In the comparative experiments, Haematococcus sp. showed the highest decontamination efficiency within 48 h, and it could be a suitable bio-adsorbent out of three types of microalgae for the removal of Co-60. Haematococcus sp. also removed 88.0% of Cs-137 from contaminated water for 48 h. Our findings indicated that the low-level radioactive solution was decontaminated to a very low-level state through the biosorption process of microalgae.

Calculation of the effective external dose rate to a person staying in the resettlement zone of the Vetka district of the Gomel region of Belarus based on in situ and ex situ assessments in 2016–2018

The aim of this study was to perform a preliminary assessment of the expected effective dose rate from external exposure to an adult individual staying at that part of the radioactively contaminated territory of the Vetka district of the Gomel region of the Republic of Belarus, from where residents had been resettled after the Chernobyl accident. For this assessment, in summer 2016 and 2018 soil samples were taken from 19 sites located in forests (7 plots), virgin meadows (4 plots), cultivated meadows (6 plots) and vegetable gardens (2 plots), with the subsequent estimation of the inventory and vertical distribution of 137Cs in the soil. The values of 137Cs inventory in the soil ranged from 452 to 1620 kBq m−2 (mean = 904 kBq m−2, median = 964 kBq m−2). The results of the measurement of soil samples were used to calculate values of the air kerma rate, normalized to the inventory of radioactive caesium in the soil. On average, the normalized indicator of the air kerma rate from the man-made source was higher in forests (1.13 nGy h−1 per kBq m−2) compared to virgin meadows (0.95 nGy h−1 per kBq m−2). Normalized air kerma rate in cultivated meadows and vegetable gardens was approximately two times lower than the corresponding indicator for virgin meadows. Using a field gamma spectrometer-dosemeter, ambient dose equivalent rate of gamma radiation in the air was measured at the surveyed sites and the contributions of the technogenic and natural components to the dose rate were estimated. Additionally, such measurements were performed on asphalted surfaces (5 sites) and inside two wooden houses. The measured values of the total ambient dose equivalent rate at a height of 1 m above the ground, asphalted surface or house floor varied from 160 to 2260 nSv h−1. The lowest levels were recorded over asphalted surfaces and inside houses, and the highest ones at forest and virgin meadow sites. The contribution of the technogenic component to the total dose rate varied from 61.9% to 98.8% (mean = 88.9%; n = 26). The effective dose of anthropogenic radiation calculated from the results of in situ measurements in a forest, virgin meadow, cultivated meadow, kitchen garden, asphalted area and house was 0.59, 0.80, 0.34, 0.29, 0.06 and 0.06 μSv h−1, respectively. Similar values for land plots were calculated based on ex situ analysis of soil samples. It can be expected that, starting from 2020, the average effective external dose of a person staying in the resettlement zone of the Vetka district will not exceed 1 mSv year−1.

Accumulation of radioactive cesium released from Fukushima Daiichi Nuclear Power Plant in wild plants grown on grassy plain

Accumulation of radioactive cesium released from Fukushima Daiichi Nuclear Power Plant in wild plants grown on grassy plain