Quantum Regime Research Articles

Competing excitation quenching and charge exchange in ultracold Li-Ba+ collisions

Abstract Hybrid atom-ion systems are a rich and powerful platform for studying chemical reactions, as they feature both excellent control over the electronic state preparation and readout as well as a versatile tunability over the scattering energy, ranging from the few-partial wave regime to the quantum regime. In this work, we make use of these excellent control knobs, and present a joint experimental and theoretical study of the collisions of a single 138Ba+ ion prepared in the 5d 2D3/2,5/2 metastable states with a ground state 6Li gas near quantum degeneracy. We show that in contrast to previously reported atom-ion mixtures, several non-radiative processes, including charge exchange, excitation exchange and quenching, compete with each other due to the inherent complexity of the ion-atom molecular structure. We present a full quantum model based on high-level electronic structure calculations involving spin-orbit couplings. Results are in excellent agreement with observations, highlighting the strong coupling between the internal angular momenta and the mechanical rotation of the colliding pair, which is relevant in any other hybrid system composed of an alkali-metal atom and an alkaline-earth ion.

Nonreciprocal Photon Transport in a Chiral Optomechanical System

AbstractChiral interaction between light and quantum emitters leads to emergence development of chiral quantum optics and stimulates a wide range of practical applications in quantum regime, such as single‐photon isolation and photon unidirectional emission. Cavity optomechanics studying the interaction between optical and mechanical resonators plays an important role in the field of quantum optics. However, how to achieve the chiral interaction between light and mechanical oscillators and explore the applications of the chiral optomechanical systems are still difficult encountered in cavity optomechanics. Here, a method is proposed to achieve chiral optomechanical interaction by exploiting directional squeezed light in a multimode optomechanical system. Based on the chiral interaction between photon and phonon, the nonreciprocal photon transport at a single‐photon level can be realized. An isolation ratio of and a negligible insertion loss for the photonic isolator are obtained. This method paves the way to realize chiral optomechanical interaction for conducting chiral optomechanics and opens up the prospect of exploring and utilizing chiral photon–phonon manipulation in the quantum regime.

Driven-dissipative phases and dynamics in non-Markovian nonlinear photonics

Interactions between photons (nonlinearities) enable a powerful form of control over the state of light. This control has enabled technologies such as light sources at new wavelengths, ultra-short optical pulses, frequency-comb metrology systems, even quantum light sources. Common to a wide variety of nonlinear optical technologies is an equilibrium between an energy source, such as an external laser, and dissipation, such as radiation loss or absorption. In the vast majority of these systems, the coupling between the system and the outside world (which leads to loss) is well described as “Markovian,” meaning that the outside world has no memory of its past state. In this work, we introduce a class of driven-dissipative systems in which a nonlinear cavity experiences non-Markovian coupling to the outside world. In the classical regime, we show that these non-Markovian cavities can have extremely low thresholds for nonlinear effects, as well as self-pulsing instabilities at THz rates, and rich phase diagrams with alternating regions of stability and instability. In the quantum regime, we show how these systems, when implemented on state-of-the-art platforms, can enable generation of strongly squeezed cavity states with intensity fluctuations that can be more than 15 dB below the classical limit, in contrast to the Markovian driven-dissipative cavity, in which the limit is 3 dB. In the regime of few-photon nonlinearity, such non-Markovian cavities can enable a deterministic protocol to generate Fock states of high order, which are long-desired, but still elusive at optical frequencies. We expect that exploiting non-Markovian couplings in nonlinear optics should in the future lead to even richer possibilities than those discussed here for both classical and quantum light manipulations.

Surface acoustic wave amplification by drifting electrons in semiconducting epitaxial graphene on silicon carbide

Abstract A theory is presented for the amplification of a surface acoustic wave (SAW) due to its interaction with conduction electrons in gate-controlled epitaxial graphene (epigraphene) on a SiC substrate. It is assumed that the SAW is launched onto the substrate in the direction of an external dc electric field applied to the graphene sample and causing the conduction electrons to drift at a speed greater than the speed of the SAW. The wavelength of the SAW is assumed to be shorter than the mean free path of the electrons, so that the quantum regime of interaction of those electrons with the SAW is realized. The Green’s function method is used to calculate the SAW gain as a function of the electron concentration in epigraphene and the external dc electric field strength. It is shown that the substrate-induced band gap in the electronic spectrum of epigraphene leads to a significant (at least an order of magnitude) increase in the SAW gain as compared to the case of gapless graphene. In addition, the opening of the band gap results in a non-monotonic dependence of the SAW gain on the electron concentration, controlled by the gate voltage applied to the graphene sample. This dependence is characterized by the presence of a distinct maximum at a certain value of electron concentration (of about 2 × 10 12 cm−2 for typical values of the other parameters involved), which distinguishes it from the monotonic concentration dependence of the SAW gain in gapless graphene.

Hysteresis and self-oscillations in an artificial memristive quantum neuron

We theoretically study an artificial neuron circuit containing a quantum memristor in the presence of relaxation and dephasing. The charge transport in the quantum element is realized via tunneling of a charge through a quantum particle which shuttles between two terminals—a functionality reminiscent of classical diffusive memristors. We demonstrate that this physical principle enables hysteretic behavior in the current-voltage characteristics of the quantum device. In addition, being used in an artificial neural circuit, the quantum switcher is able to generate self-sustained current oscillations. Our analysis reveals that these self-oscillations are triggered only in quantum regimes with a moderate rate of relaxation, and cannot exist either in a purely coherent regime or at a very high decoherence. We investigate the hysteresis and instability leading to the onset of current self-oscillations and analyze their properties depending on the circuit parameters. Our results provide a generic approach to the use of quantum regimes for controlling hysteresis and generating self-oscillations. Published by the American Physical Society 2024

Characterization of a levitated sub-milligram ferromagnetic cube in a planar alternating-current magnetic Paul trap

Microscopic levitated objects are a promising platform for inertial sensing, testing gravity at small scales, optomechanics in the quantum regime, and large-mass superpositions. However, existing levitation techniques harnessing optical and electrical fields suffer from noise induced by elevated internal temperatures and charge noise, respectively. Meissner-based magnetic levitation circumvents both sources of decoherence but requires cryogenic environments. Here, we characterize a sub-milligram ferromagnetic cube levitated in an alternating-current planar magnetic Paul trap at room temperature. We show behavior in line with the Mathieu equations and quality factors of up to 2500 for the librational modes. Besides technological sensing applications, this technique sets out a path for megahertz librational modes in the micrometer-sized particle limit and can be extended by implementing superconducting traps in cryogenic environments, allowing for magnetic coupling to superconducting circuits and spin-based quantum systems.

Electrostatically Interacting Wannier Qubits in Curved Space

A derivation of a tight-binding model from Schrödinger formalism for various topologies of position-based semiconductor qubits is presented in the case of static and time-dependent electric fields. The simplistic tight-binding model enables the description of single-electron devices at a large integration scale. The case of two electrostatically Wannier qubits (also known as position-based qubits) in a Schrödinger model is presented with omission of spin degrees of freedom. The concept of programmable quantum matter can be implemented in the chain of coupled semiconductor quantum dots. Highly integrated and developed cryogenic CMOS nanostructures can be mapped to coupled quantum dots, the connectivity of which can be controlled by a voltage applied across the transistor gates as well as using an external magnetic field. Using the anti-correlation principle arising from the Coulomb repulsion interaction between electrons, one can implement classical and quantum inverters (Classical/Quantum Swap Gate) and many other logical gates. The anti-correlation will be weakened due to the fact that the quantumness of the physical process brings about the coexistence of correlation and anti-correlation at the same time. One of the central results presented in this work relies on the appearance of dissipation-like processes and effective potential renormalization building effective barriers in both semiconductors and in superconductors between not bended nanowire regions both in classical and in quantum regimes. The presence of non-straight wire regions is also expressed by the geometrical dissipative quantum Aharonov–Bohm effect in superconductors/semiconductors when one obtains a complex value vector potential-like field. The existence of a Coulomb interaction provides a base for the physical description of an electrostatic Q-Swap gate with any topology using open-loop nanowires, with programmable functionality. We observe strong localization of the wavepacket due to nanowire bending. Therefore, it is not always necessary to build a barrier between two nanowires to obtain two quantum dot systems. On the other hand, the results can be mapped to the problem of an electron in curved space, so they can be expressed with a programmable position-dependent metric embedded in Schrödinger’s equation. The semiconductor quantum dot system is capable of mimicking curved space, providing a bridge between fundamental and applied science in the implementation of single-electron devices.

From higher-spin gauge interactions to Compton amplitudes for root-Kerr

We develop massive higher-spin theory as a framework for describing dynamics of rotating compact objects, such as Kerr black holes. In this paper, we explore gauge interactions up to quartic order and corresponding Compton amplitudes of higher-spin massive objects coupled to electromagnetism and Yang-Mills theory. Their classical counterparts are known as root-Kerr gauge-theory solutions, whose amplitudes are closely related to those of Kerr black holes. We use three distinct approaches: (i) massive higher-spin gauge symmetry to introduce cubic interactions for all spins and the quartic interactions up to spin 3, which is implemented both off shell and via Ward identities; (ii) a chiral higher-spin approach to construct quartic Lagrangians with correct degrees of freedom to all spins; (iii) on-shell functional patterns before and after taking the classical limit to constrain the Compton amplitudes. As final results, we arrive at simple local formulae for the candidate root-Kerr Compton amplitudes both in the quantum regime and classical limit, to all orders in spin. This is a precursor to the gravitational Kerr case, which is presented in a follow-up paper.

Non-Abelian Transport Distinguishes Three Usually Equivalent Notions of Entropy Production

We extend entropy production to a deeply quantum regime involving noncommuting conserved quantities. Consider a unitary transporting conserved quantities (“charges”) between two systems initialized in thermal states. Three common formulas model the entropy produced. They respectively cast entropy as an extensive thermodynamic variable, as an information-theoretic uncertainty measure, and as a quantifier of irreversibility. Often, the charges are assumed to commute with each other (e.g., energy and particle number). Yet quantum charges can fail to commute. Noncommutation invites generalizations, which we posit and justify, of the three formulas. The noncommutation of charges, we find, breaks the equivalence of the formulas. Furthermore, different formulas quantify different physical effects of the noncommutation of charges on entropy production. For instance, entropy production can signal contextuality—true nonclassicality—by becoming nonreal. This work opens up stochastic thermodynamics to noncommuting—and so particularly quantum—charges. Published by the American Physical Society 2024

Attractive-repulsive interaction in coupled quantum oscillators.

We study the emergent dynamics of quantum self-sustained oscillators induced by the simultaneous presence of attraction and repulsion in the coupling path. We consider quantum Stuart-Landau oscillators under attractive-repulsive coupling and construct the corresponding quantum master equationin the Lindblad form. We discover an interesting symmetry-breaking transition from quantum limit cycle oscillation to a quantum inhomogeneous steady state. This transition is contrary to the previously known symmetry-breaking transition from a quantum homogeneous state to an inhomogeneous steady state. The result is supported by the analysis on the noisy classical model of the quantum system in the weak quantum regime. Remarkably, we find the generation of entanglement associated with the symmetry-breaking transition that has no analog in the classical domain. This study enriches our understanding of the collective behaviors shown by coupled oscillators in the quantum domain.

Thermodynamic quantum Fokker–Planck equations and their application to thermostatic Stirling engine

We developed a computer code for the thermodynamic quantum Fokker–Planck equations (T-QFPE), derived from a thermodynamic system–bath model. This model consists of an anharmonic subsystem coupled to multiple Ohmic baths at different temperatures, which are connected to or disconnected from the subsystem as a function of time. The code numerically integrates the T-QFPE and their classical expression to simulate isothermal, isentropic, thermostatic, and entropic processes in both quantum and classical cases. The accuracy of the results was verified by comparing the analytical solutions of the Brownian oscillator. In addition, we illustrated a breakdown of the Markovian Lindblad-master equation in the pure quantum regime. As a demonstration, we simulated a thermostatic Stirling engine employed to develop non-equilibrium thermodynamics [S. Koyanagi and Y. Tanimura, J. Chem. Phys. 161, 114113 (2024)] under quasi-static conditions. The quasi-static thermodynamic potentials, described as intensive and extensive variables, were depicted as work diagrams. In the classical case, the work done by the external field is independent of the system–bath coupling strength. In contrast, in the quantum case, the work decreases as the coupling strength increases due to quantum entanglement between the subsystem and bath. The codes were developed for multicore processors using Open Multi-Processing (OpenMP) and for graphics processing units using the Compute Unified Device Architecture. These codes are provided in the supplementary material.

Classical and quantum thermodynamics in a non-equilibrium regime: Application to thermostatic Stirling engine

We have developed a thermodynamic theory in the non-equilibrium regime, which we describe as a thermodynamic system–bath model [Koyanagi and Tanimura, J. Chem. Phys. 160, 234112 (2024)]. Based on the dimensionless (DL) minimum work principle, non-equilibrium thermodynamic potentials are expressed in terms of non-equilibrium extensive and intensive variables in time derivative form. This is made possible by incorporating the entropy production rate into the definition of non-equilibrium thermodynamic potentials. These potentials can be evaluated from the DL non-equilibrium-to-equilibrium minimum work principle, which is derived from the principle of DL minimum work and is equivalent to the second law of thermodynamics. We thus obtain the non-equilibrium Massieu–Planck potentials as entropic potentials and the non-equilibrium Helmholtz–Gibbs potentials as free energies. Unlike the fluctuation theorem and stochastic thermodynamics theory, this theory does not require the assumption of a factorized initial condition and is valid in the full quantum regime, where the system and bath are quantum mechanically entangled. Our results are numerically verified by simulating a thermostatic Stirling engine consisting of two isothermal processes and two thermostatic processes using the quantum hierarchical Fokker–Planck equations and the classical Kramers equation derived from the thermodynamic system–bath model. We then show that, from weak to strong system–bath interactions, the thermodynamic process can be analyzed using a non-equilibrium work diagram analogous to the equilibrium one for given time-dependent intensive variables. The results can be used to develop efficient heat machines in non-equilibrium regimes.

Direct measurement of microwave loss in Nb films for superconducting qubits

Niobium films are a key component in modern two-dimensional superconducting qubits, yet their contribution to the total qubit decay rate is not fully understood. The presence of different layers of materials and interfaces makes it difficult to identify the dominant loss channels in present two-dimensional qubit designs. In this paper, we present the study that directly correlates measurements of RF losses in such films to material parameters by investigating a high-power impulse magnetron sputtered (HiPIMS) film atop a three-dimensional niobium superconducting radio frequency (SRF) resonator. By using a 3D SRF structure, we are able to isolate the niobium film loss from other contributions. Our findings indicate that microwave dissipation in the HiPIMS-prepared niobium films, within the quantum regime, resembles that of record-high intrinsic quality factor of bulk niobium SRF cavities, with lifetimes extending into seconds. Microstructure and impurity level of the niobium film do not significantly affect the losses. These results set the scale of microwave losses in niobium films and show that niobium losses do not dominate the observed coherence times in present two-dimensional superconducting qubit designs, instead highlighting the dominant role of the dielectric oxide in limiting the performance. We can also set a bound for when niobium film losses will become a limitation for qubit lifetimes.

The shape of non-graviton operators for SU(2)

The BPS spectrum of AdS/CFT exhibits multi-gravitons at low energies, while having black hole states at higher energies. This can be studied concretely in AdS5/CFT4 in terms of classical cohomologies, even in the quantum regimes at finite 1/N. Recently, Chang and Lin found a threshold for non-graviton states in the SU(2) maximal super-Yang-Mills theory. We explicitly construct and present this threshold cohomology.

Ultracoherent Gigahertz Diamond Spin-Mechanical Lamb Wave Resonators.

We report the development of an all-optical approach that excites the fundamental compression mode in a diamond Lamb wave resonator with an optical gradient force and detects the induced vibrations via strain coupling to a silicon vacancy center, specifically, via phonon sidebands in the optical excitation spectrum of the silicon vacancy. Sideband optical interferometry has also been used for the detection of in-plane mechanical vibrations, for which conventional optical interferometry is not effective. These experiments demonstrate a gigahertz fundamental compression mode with a Q factor of >107 at temperatures near 7 K, providing a promising platform for reaching the quantum regime of spin mechanics, especially phononic cavity quantum electrodynamics of electron spins.

Observation of Pairwise Level Degeneracies and the Quantum Regime of the Arrhenius Law in a Double-Well Parametric Oscillator

By applying a microwave drive to a specially designed Josephson circuit, we have realized a double-well model system: a Kerr oscillator submitted to a squeezing force. We have observed, for the first time, the spectroscopic fingerprint of a quantum double-well Hamiltonian when its barrier height is increased: a pairwise level kissing (coalescence) corresponding to the exponential reduction of tunnel splitting in the excited states as they sink under the barrier. The discrete levels in the wells also manifest themselves in the activation time across the barrier which, instead of increasing smoothly as a function of the barrier height, presents steps each time a pair of excited states is captured by the wells. This experiment illustrates the quantum regime of Arrhenius’s law, whose observation is made possible here by the unprecedented combination of low dissipation, time-resolved state control, 98.5% quantum nondemolition single shot measurement fidelity, and complete microwave control over all Hamiltonian parameters in the quantum regime. Direct applications to quantum computation and simulation are discussed. Published by the American Physical Society 2024

Probing multi-mobility edges in quasiperiodic mosaic lattices

The mobility edge (ME) is a crucial concept in understanding localization physics, marking the critical transition between extended and localized states in the energy spectrum. Anderson localization scaling theory predicts the absence of ME in lower dimensional systems. Hence, the search for exact MEs, particularly for single particles in lower dimensions, has recently garnered significant interest in both theoretical and experimental studies, resulting in notable progress. However, several open questions remain, including the possibility of a single system exhibiting multiple MEs and the continual existence of extended states, even within the strong disorder domain. Here, we provide experimental evidence to address these questions by utilizing a quasiperiodic mosaic lattice with meticulously designed nanophotonic circuits. Our observations demonstrate the coexistence of both extended and localized states in lattices with broken duality symmetry and varying modulation periods. By single site injection and scanning the disorder level, we could approximately probe the ME of the modulated lattice. These results corroborate recent theoretical predictions, introduce a new avenue for investigating ME physics, and offer inspiration for further exploration of ME physics in the quantum regime using hybrid integrated photonic devices.

Self-Suppressed Quantum-Limited Timing Jitter and Fundamental Noise Limit of Soliton Microcombs.

Quantum-limited timing jitter of soliton microcombs has long been recognized as their fundamental noise limit. Here, we surpass such limit by utilizing dispersive wave dynamics in multimode microresonators. Through the viscous force provided by these dispersive waves, the quantum-limited timing jitter can be suppressed to a much lower level that forms the ultimate fundamental noise limit of soliton microcombs. Our findings enable coherence engineering of soliton microcombs in the quantum regime, providing critical guidelines for using soliton microcombs to synthesize ultralow-noise microwave and optical signals.

Probing coherent quantum thermodynamics using a trapped ion

Quantum thermodynamics is aimed at grasping thermodynamic laws as they apply to thermal machines operating in the deep quantum regime, where coherence and entanglement are expected to matter. Despite substantial progress, however, it has remained difficult to develop thermal machines in which such quantum effects are observed to be of pivotal importance. In this work, we demonstrate the possibility to experimentally measure and benchmark a genuine quantum correction, induced by quantum friction, to the classical work fluctuation-dissipation relation. This is achieved by combining laser-induced coherent Hamiltonian rotations and energy measurements on a trapped ion. Our results demonstrate that recent developments in stochastic quantum thermodynamics can be used to benchmark and unambiguously distinguish genuine quantum coherent signatures generated along driving protocols, even in presence of experimental SPAM errors and, most importantly, beyond the regimes for which theoretical predictions are available (e.g., in slow driving).

Nonequilibrium Transition between Dissipative Time Crystals

We show a dissipative phase transition in a driven nonlinear quantum oscillator in which a discrete time-translation symmetry is spontaneously broken in two different ways. The corresponding regimes display either discrete or incommensurate time-crystal order, which we analyze numerically and analytically beyond the classical limit, addressing observable dynamics, phenomenology in different (laboratory and rotating) frames, Liouvillian spectral features, and quantum fluctuations. Via an effective semiclassical description, we show that phase diffusion dominates in the incommensurate time crystal (or continuous time crystal in the rotating frame), which manifests as a band of eigenmodes with a lifetime growing linearly with the mean-field excitation number. Instead, in the discrete time-crystal phase, the leading fluctuation process corresponds to quantum activation with a single mode that has an exponentially growing lifetime. Interestingly, the transition between these two regimes manifests itself already in the quantum regime as a spectral singularity, namely, as an exceptional point mediating between phase diffusion and quantum activation. Finally, we discuss this transition between different time-crystal orders in the context of synchronization phenomena. Published by the American Physical Society 2024