Quantum Information Storage Research Articles

Unraveling the Spin Polarization of the ν = 5/2 Fractional Quantum Hall State

The fractional quantum Hall (FQH) effect at filling factor ν = 5/2 has recently come under close scrutiny, as its ground state may possess quasi-particle excitations obeying nonabelian statistics, a property sought for topologically protected quantum operations. However, its microscopic origin remains unknown, and candidate model wave functions include those with undesirable abelian statistics. We report direct measurements of the electron spin polarization of the ν = 5/2 FQH state using resistively detected nuclear magnetic resonance. We find the system to be fully polarized, which unambiguously rules out the most likely abelian contender and lends strong support for the ν = 5/2 state being nonabelian. Our measurements reveal an intrinsically different nature of interaction in the first excited Landau level underlying the physics at ν = 5/2.

Optical detection of a single rare-earth ion in a crystal.

Rare-earth-doped laser materials show strong prospects for quantum information storage and processing, as well as for biological imaging, due to their high-Q 4f↔4f optical transitions. However, the inability to optically detect single rare-earth dopants has prevented these materials from reaching their full potential. Here we detect a single photostable Pr3+ ion in yttrium aluminium garnet nanocrystals with high contrast photon antibunching by using optical upconversion of the excited state population of the 4f↔4f optical transition into ultraviolet fluorescence. We also demonstrate on-demand creation of Pr3+ ions in a bulk yttrium aluminium garnet crystal by patterned ion implantation. Finally, we show generation of local nanophotonic structures and cell death due to photochemical effects caused by upconverted ultraviolet fluorescence of praseodymium-doped yttrium aluminium garnet in the surrounding environment. Our study demonstrates versatile use of rare-earth atomic-size ultraviolet emitters for nanoengineering and biotechnological applications.

Strongly coupling a cavity to inhomogeneous ensembles of emitters: Potential for long-lived solid-state quantum memories

We investigate theoretically the coupling of a cavity mode to a continuous distribution of emitters. We discuss the influence of the emitters' inhomogeneous broadening on the existence and on the coherence properties of the polaritonic peaks. We find that their coherence depends crucially on the shape of the distribution and not only on its width. Under certain conditions the coupling to the cavity protects the polaritonic states from inhomogeneous broadening, resulting in a longer storage time for a quantum memory based on emitter ensembles. When two different ensembles of emitters are coupled to the resonator, they support a peculiar collective dark state, which is also very attractive for the storage of quantum information.

Topological Order at Nonzero Temperature

We propose a definition for topological order at nonzero temperature in analogy to the usual zero temperature definition that a state is topologically ordered, or "nontrivial", if it cannot be transformed into a product state (or a state close to a product state) using a local (or approximately local) quantum circuit. We prove that any two-dimensional Hamiltonian which is a sum of commuting local terms is not topologically ordered at T > 0. We show that such trivial states cannot be used to store quantum information using certain stringlike operators. This definition is not too restrictive, however, as the four dimensional toric code does have a nontrivial phase at nonzero temperature.

Intervalley coupling for interface-bound electrons in silicon: An effective mass study

Orbital degeneracy of the electronic conduction band edge in silicon is a potential roadblock to the storage and manipulation of quantum information involving the electronic spin degree of freedom in this host material. This difficulty may be mitigated near an interface between Si and a barrier material, where intervalley scattering may couple states in the conduction ground state, leading to nondegenerate orbital ground and first excited states. The level splitting is experimentally found to have a strong sample dependence, varying by orders of magnitude for different interfaces and samples. The basic physical mechanisms leading to such coupling in different systems are addressed. We expand our recent study based on an effective mass approach, incorporating the full plane-wave expansions of the Bloch functions at the conduction band minima. Physical insights emerge naturally from a simple Si/barrier model. In particular, we present a clear comparison between ours and different approximations and formalisms adopted in the literature and establish the applicability of these approximations in different physical scenarios.

Controlling quantum information processing in hybrid systems on chips

We investigate quantum information processing, transfer and storage in hybrid systems comprised of diverse blocks integrated on chips. Strong coupling between superconducting (SC) qubits and ensembles of ultracold atoms or NV-center spins is mediated by a microwave transmission-line resonator that interacts near-resonantly with the atoms or spins. Such hybrid devices allow us to benefit from the advantages of each block and compensate for their disadvantages. Specifically, the SC qubits can rapidly implement quantum logic gates, but are noisy (prone to decoherence), while collective states of the atomic or spin ensemble are quiet(protected from decoherence) and thus can be employed for storage of quantum information. To improve the overall performance (fidelity) of such devices we discuss dynamical control to optimize quantum state-transfer from a noisy qubit to the quiet storage ensemble. We propose to maximize the fidelity of transfer and storage in a spectrally inhomogeneous spin ensemble, by pre-selecting the optimal spectral portion of the ensemble. Significant improvements of the overall fidelity of hybrid devices are expected under realistic conditions. Experimental progress towards the realization of these schemes is discussed.

Laser cooling and real-time measurement of the nuclear spin environment of a solid-state qubit

Control over quantum dynamics of open systems is one of the central challenges in quantum science and engineering. Coherent optical techniques, such as coherent population trapping involving dark resonances, are widely used to control quantum states of isolated atoms and ions. In conjunction with spontaneous emission, they allow for laser cooling of atomic motion, preparation and manipulation of atomic states, and rapid quantum optical measurements that are essential for applications in metrology. Here we show that these techniques can be applied to monitor and control individual atom-like impurities, and their local environment, in the solid state. Using all-optical manipulation of the electronic spin of an individual nitrogen-vacancy colour centre in diamond, we demonstrate optical cooling, real-time measurement and conditional preparation of its nuclear spin environment by post-selection. These methods offer potential applications ranging from all-optical nanomagnetometry to quantum feedback control of solid-state qubits, and may lead to new approaches for quantum information storage and processing.

An atom–molecule platform for quantum computing

We propose a combined atom---molecule system for quantum information processing in individual traps, such as provided by optical lattices. In this platform, different species of atoms--one atom carrying a qubit and the other enabling the interaction--are used to store and process quantum information via intermediate molecular states. We show how gates, initialization, and readout operations could be implemented using this approach. In particular, we describe in some detail the implementation of a two-qubit phase gate in which a pair of atoms is transferred into the ground rovibrational state of a polar molecule with a large dipole moment, thus allowing atoms transferred into molecules to interact via their dipole-dipole interaction. We also discuss how the reverse process could be used as a non-destructive readout tool of molecular qubit states. Finally, we generalize these ideas to use a decoherence-free subspace for qubit encoding to minimize the decoherence due to magnetic field fluctuations. In this case, qubits will be encoded into field-insensitive states of two identical atoms, while a third atom of a different species will be used to realize a phase gate.

Creating nuclear spin entanglement using an optical degree of freedom

Molecular nanostructures are promising building blocks for future quantum technologies, provided methods of harnessing their multiple degrees of freedom can be identified and implemented. Due to low decoherence rates, nuclear spins are considered ideal candidates for storing quantum information, while optical excitations can give rise to fast and controllable interactions for information processing. A recent paper [M. Schaffry et al., Phys. Rev. Lett. 104, 200501 (2010)] proposed a method for entangling two nuclear spins through their mutual coupling to a transient optically excited electron spin. Building on the same idea, we present here an extended and much more detailed theoretical framework, showing that this method is in fact applicable to a much wider class of molecular structures than previously discussed in the original proposal.

Quantum computing implementations with neutral particles

We review quantum information processing with cold neutral particles, that is, atoms or polar molecules. First, we analyze the best suited degrees of freedom of these particles for storing quantum information, and then we discuss both single- and two-qubit gate implementations. We focus our discussion mainly on collisional quantum gates, which are best suited for atom-chip-like devices, as well as on gate proposals conceived for optical lattices. Additionally, we analyze schemes both for cold atoms confined in optical cavities and hybrid approaches to entanglement generation, and we show how optimal control theory might be a powerful tool to enhance the speed up of the gate operations as well as to achieve high fidelities required for fault tolerant quantum computation.

A classical oscillator takes the sideband route to the quantum ground state

The cooling and damping of a micromechanical oscillator's motion to the ground state could pave the way to storage of quantum information and generation of entangled states in ... The cooling and damping of a micromechanical oscillator's motion to the ground state could pave the way to storage of quantum information and generation of entangled states in ...

Single-Photon-Level Quantum Memory at Room Temperature

Room-temperature, easy-to-operate quantum memories are essential building blocks for future long distance quantum information networks operating on an intercontinental scale, because devices like quantum repeaters, based on quantum memories, will have to be deployed in potentially remote, inaccessible locations. Here we demonstrate controllable, broadband and efficient storage and retrieval of weak coherent light pulses at the single-photon level in warm atomic cesium vapor using the robust far off-resonant Raman memory scheme. We show that the unconditional noise floor of this technically simple quantum memory is low enough to operate in the quantum regime, even in a room-temperature environment.

Tuning Manganese Dopant Spin Interactions in Single GaN Nanowires at Room Temperature

Control of electron spins in individual magnetically doped semiconductor nanostructures has considerable potential for quantum information processing and storage. The manipulations of dilute magnetic interactions have largely been restricted to low temperatures, limiting their potential technological applications. Among the systems predicted to be ferromagnetic above room temperature, Mn-doped GaN has attracted particular attention, due to its attractive optical and electrical properties. However, the experimental data have been inconsistent, and the origin of the magnetic interactions remains unclear. Furthermore, there has been no demonstration of tuning the dopant exchange interactions within a single nanostructure, which is necessary for the design of nanoscale spin-electronic (spintronic) devices. Here we directly show for the first time intrinsic magnetization of manganese dopants in individual gallium nitride nanowires (NWs) at room temperature. Using high-resolution circularly polarized X-ray microscopy imaging, we demonstrate the dependence of the manganese exchange interactions on the NW orientation with respect to the external magnetic field. The crystalline anisotropy allows for the control of dilute magnetization in a single NW and the application of bottom-up approaches, such as in situ nanowire growth control or targeted positioning of individual NWs, for the design of networks for quantum information technologies.

Long-lived qubit from three spin-12atoms

A system of three spin-1/2 atoms allows the construction of a reference-frame-free (RFF) qubit in the subspace with total angular momentum $j=1/2$. The RFF qubit stays coherent perfectly as long as the spins of the three atoms are affected homogeneously. The inhomogeneous evolution of the atoms causes decoherence, but this decoherence can be suppressed efficiently by applying a bias magnetic field of modest strength perpendicular to the plane of the atoms. The resulting lifetime of the RFF qubit can be many days, making RFF qubits of this kind promising candidates for quantum information storage units. Specifically, we examine the situation of three $^6\textrm{Li}$ atoms trapped in a $\textrm{CO}_2$-laser-generated optical lattice and find that, with conservatively estimated parameters, a stored qubit maintains a fidelity of 0.9999 for two hours.

Screening Effect in Charge Qubit

We study the influence of screening effect on quantum decoherence for charge qubit and the process of quantum information storage. When the flux produced by the circulating current in SQUID loop is considered, screening effect is formally characterized by a LC resonator. Using large-detuning condition and Fröhlich transformation in the qubit-cavity-resonator system, we calculate the decoherence factor for charge qubit and the effective qubit-cavity Hamiltonian. The decoherence factor owns a factorized structure, it shows that screening effect is a resource of decoherence for charge qubit. The effective Hamiltonian shows that the screening effect results in a frequency shift for charge qubit and a modified qubit-cavity coupling constant induced by a LC resonator.

Two Level System Loss in Superconducting Microwave Resonators

High quality factor, i.e. low loss, microwave resonators are important for quantum information storage and addressing. In this work we study the resonance frequency and loss in superconducting coplanar waveguide resonators as a function of power and temperature. We find that there is increased loss at low power and low temperature. The increased loss is attributed to the existence of two-level systems (TLS) at the surfaces, interfaces, and in the bulk of insulators deposited on the structures. We show that both the temperature dependence of the resonant frequency and the power dependence of the loss can be used to find the TLS contribution to the loss. The TLS intrinsic loss tangent derived from the frequency shift data at high power is shown to agree well with the direct loss measurement at low power. The former allows for a relatively fast measurement of the TLS loss. As an example, we measure the properties of amorphous AlO <sub xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">X</sub> deposited on the resonators and find a TLS loss tangent of 1 × 10 <sup xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink">-3</sup> .

Entangling Moving Cavities in Noninertial Frames

An open question in the field of relativistic quantum information is how parties in arbitrary motion may distribute and store quantum entanglement. We propose a scheme for storing quantum information in the field modes of cavities moving in flat space-time and analyze it in a quantum field theoretical framework. In contrast with previous work that found entanglement degradation between observers moving with uniform acceleration, we find the quantum information in such systems is protected. We further discuss a method for establishing the entanglement in the first place and show that in principle it is always possible to produce maximally entangled states between the cavities.

Ultrabright and efficient single-photon generation based on nitrogen-vacancy centres in nanodiamonds on a solid immersion lens

Single photons are fundamental elements for quantum information technologies such as quantum cryptography, quantum information storage and optical quantum computing. Colour centres in diamond have proven to be stable single-photon sources and thus essential components for reliable and integrated quantum information technology. A key requirement for such applications is a large photon flux and a high efficiency. Paying tribute to various attempts to maximize the single-photon flux, we show that collection efficiencies of photons from colour centres can be increased with a rather simple experimental setup. To do so, we spin-coated nanodiamonds containing single nitrogen-vacancy (N-V) colour centres on the flat surface of a ZrO2 solid immersion lens. We found stable single-photon count rates of up to 853 kcts s− 1 at saturation under continuous wave excitation while having access to more than 100 defect centres with count rates from 400 to 500 kcts s− 1. For a blinking defect centre, we found count rates up to 2.4 Mcts s− 1 for time intervals of several tens of seconds. It seems to be a general feature that very high rates are accompanied by blinking behaviour. The overall collection efficiency of our setup of up to 4.2% is the highest yet reported for N-V defect centres in diamond. Under pulsed excitation of a stable emitter of 10 MHz, 2.2% of all pulses caused a click on the detector adding to 221 kcts s− 1 thus, opening the way towards diamond-based on-demand single-photon sources for quantum applications.

A single-atom quantum memory

The faithful storage of a quantum bit (qubit) of light is essential for long-distance quantum communication, quantum networking and distributed quantum computing. The required optical quantum memory must be able to receive and recreate the photonic qubit; additionally, it must store an unknown quantum state of light better than any classical device. So far, these two requirements have been met only by ensembles of material particles that store the information in collective excitations. Recent developments, however, have paved the way for an approach in which the information exchange occurs between single quanta of light and matter. This single-particle approach allows the material qubit to be addressed, which has fundamental advantages for realistic implementations. First, it enables a heralding mechanism that signals the successful storage of a photon by means of state detection; this can be used to combat inevitable losses and finite efficiencies. Second, it allows for individual qubit manipulations, opening up avenues for in situ processing of the stored quantum information. Here we demonstrate the most fundamental implementation of such a quantum memory, by mapping arbitrary polarization states of light into and out of a single atom trapped inside an optical cavity. The memory performance is tested with weak coherent pulses and analysed using full quantum process tomography. The average fidelity is measured to be 93%, and low decoherence rates result in qubit coherence times exceeding 180 microseconds. This makes our system a versatile quantum node with excellent prospects for applications in optical quantum gates and quantum repeaters.

Constructions and noise threshold of topological subsystem codes

Topological subsystem codes proposed recently by Bombin are quantum error-correcting codes defined on a two-dimensional grid of qubits that permit reliable quantum information storage with a constant error threshold. These codes require only the measurement of two-qubit nearest-neighbor operators for error correction. In this paper, we demonstrate that topological subsystem codes (TSCs) can be viewed as generalizations of Kitaev's honeycomb model to 3-valent hypergraphs. This new connection provides a systematic way of constructing TSCs and analyzing their properties. We also derive a necessary and sufficient condition under which a syndrome measurement in a subsystem code can be reduced to measurements of the gauge group generators. Furthermore, we propose and implement some candidate decoding algorithms for one particular TSC assuming perfect error correction. Our Monte Carlo simulations indicate that this code, which we call the five-square code, has a threshold against depolarizing noise of at least 2%.