Overburdened stockpiles are difficult to achieve natural stability in a short period time because of their complex and diverse composition of materials and significant differences in physical and chemical properties, causing numerous cases of water loss and soil loss events. We conducted a series of experiments at different rainfall intensities (30, 60, 90, and 120 mm h−1) and different gravel contents (0 %, 10 %, 20 %, 30 %, and 40 %) to study the runoff, soil erosion, and rill morphology characteristics and relationship among three of overburdened stockpiles in production and construction projects with simulated rainfall. The runoff rate and soil loss rate basically showed a trend of increasing and then decreasing with gravel content and lower gravel content had a certain degree of inhibition on the flow velocity. 20 %, 0 %, 0 %, and 20 % gravel contents had the most significant inhibition on the flow velocity at 30, 60, 90, and 120 mm h−1 rainfall intensities, respectively. Flow shear stress, stream power, unit energy of water cross-section, maximum rill length, width and depth all increased with increasing rainfall intensity. The stream power, unit stream power, and unit energy of water cross-section were larger at higher gravel content. The maximum rill length and depth were positively correlated with gravel content, which were the minimum at 0 % gravel content and all rainfall intensities. Gravel content played a more important role in the runoff, soil loss, and rill morphology. The relationship between runoff rate and soil loss rate, flow velocity and rill morphology parameters were all expressed as linear functions, and flow velocity and soil loss rate was quadratic function, with a correlation coefficient of 0.339. In contrast, runoff rate and rill morphology parameters, soil loss rate and rill morphology parameters, erosion dynamics parameters and rill morphology parameters were all expressed as power functions. In addition, the runoff rate can better describe the process of soil loss (R2 = 0.798, P < 0.05). The unit energy of water cross-section was more suitable to describe the development of maximum rill length and depth (with rill length was R2 = 0.781, and with rill depth was R2 = 0.723, P < 0.05). At the same time, the stream power was more suitable to describe the development of maximum rill width on the slope of overburdened stockpiles (R2 = 0.841, P < 0.05). These results contributed to preventing soil loss on overburdened stockpiles and helping the development of estimation models for soil erosion.