Pulsed Neutron Source Research Articles

Measurements of neutronic characteristics of rectangular and cylindrical coupled hydrogen moderators

ABSTRACT Extensive simulation calculations were performed in the design studies of the coupled hydrogen moderator for the pulsed spallation neutron source of the Japan Proton Accelerator Research Facility (J-PARC). It was indicated that a para-hydrogen moderator had an intensity-enhanced region at the fringe part, and that pulse shapes emitted from a cylindrical para-hydrogen moderator gave higher pulse-peak intensities with narrower pulse widths than those from a rectangular one without penalizing the time-integrated intensities. To validate the peculiar distribution and advantages in pulse shapes experimentally, some measurements were performed at the neutron source of the Hokkaido University electron linear accelerator facility. It was observed that the neutron intensity was enhanced at edges of the para-hydrogen moderators, whereas it decreased at the same part of the ortho-rich-hydrogen moderator, where the dimension of those moderators was 50 mm in thickness and 120 mm in width and height. The spatial distribution and pulse shapes were also measured for a cylindrical coupled para-hydrogen moderator that has the same dimensions as for the coupled moderator employed for J-PARC. The measured results from the cylindrical moderator were consistent with the results obtained in the design studies for the moderator for J-PARC.

Neutron Spectroscopy for pulsed beams with frame overlap using a double time-of-flight technique

A new double time-of-flight (dTOF) neutron spectroscopy technique has been developed for pulsed broad spectrum sources with a duty cycle that results in frame overlap, where fast neutrons from a given pulse overtake slower neutrons from previous pulses. Using a tunable beam at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory, neutrons were produced via thick-target breakup of 16 MeV deuterons on a beryllium target in the cyclotron vault. The breakup spectral shape was deduced from a dTOF measurement using an array of EJ-309 organic liquid scintillators. Simulation of the neutron detection efficiency of the scintillator array was performed using both GEANT4 and MCNP6. The efficiency-corrected spectral shape was normalized using a foil activation technique to obtain the energy-dependent flux of the neutron beam at zero degrees with respect to the incoming deuteron beam. The dTOF neutron spectrum was compared to spectra obtained using HEPROW and GRAVEL pulse height spectrum unfolding techniques. While the unfolding and dTOF results exhibit some discrepancies in shape, the integrated flux values agree within two standard deviations. This method obviates neutron time-of-flight spectroscopy challenges posed by pulsed beams with frame overlap and opens new opportunities for pulsed white neutron source facilities.

Application of the backward extrapolation method to pulsed neutron sources

Particle detectors operated in pulse mode are subjected to the dead-time effect. When the average of the detector counts is constant over time, correcting for the dead-time effect is simple and can be accomplished by analytical formulas. However, when the average of the detector counts changes over time it is more difficult to take into account the dead-time effect. When a subcritical nuclear assembly is driven by a pulsed neutron source, simple analytical formulas cannot be applied to the measured detector counts to correct for the dead-time effect because of the sharp change of the detector counts over time. This work addresses this issue by using the backward extrapolation method. The latter can be applied not only to a continuous (e.g. californium) external neutron source but also to a pulsed external neutron source (e.g. by a particle accelerator) driving a subcritical nuclear assembly. The backward extrapolation method allows to obtain from the measured detector counts both the dead-time value and the real detector counts.

Setup for polarized neutron imaging using in situ 3He cells at the Oak Ridge National Laboratory High Flux Isotope Reactor CG-1D beamline.

In the present study, we report a new setup for polarized neutron imaging at the ORNL High Flux Isotope Reactor CG-1D beamline using an in situ 3He polarizer and analyzer. This development is very important for extending the capabilities of the imaging instrument at ORNL providing a polarized beam with a large field-of-view, which can be further used in combination with optical devices like Wolter optics, focusing guides, or other lenses for the development of microscope arrangement. Such a setup can be of advantage for the existing and future imaging beamlines at the pulsed neutron sources. The first proof-of-concept experiment is performed to study the ferromagnetic phase transition in the Fe3Pt sample. We also demonstrate that the polychromatic neutron beam in combination with in situ 3He cells can be used as the initial step for the rapid measurement and qualitative analysis of radiographs.

The ESS neutrino facility for CP violation discovery

The comparatively large value of the neutrino mixing angle θ13 measured in 2012 by neutrino reactor experiments has opened the possibility to observe for the first time CP violation in the leptonic sector. The measured value of θ13 also privileges the 2nd oscillation maximum for the discovery of CP violation instead of the usually used 1st oscillation maximum. The sensitivity at the 2nd oscillation maximum is about three times higher than at the 1st oscillation maximum implying a significantly lower sensitivity to systematic errors. Measuring at the 2nd oscillation maximum necessitates a very intense neutrino beam with the appropriate energy. The world’s most intense pulsed spallation neutron source, the European Spallation Source, has a proton linac with 5 MW power and 2 GeV energy. This linac also has the potential to become the proton driver of the world’s most intense neutrino beam with very high potential for the discovery of neutrino CP violation. The physics performance of that neutrino Super Beam in conjunction with a megaton Water Cherenkov neutrino detector installed ca 1000 m down in a mine at a distance of about 500 km from ESS has been evaluated. In addition, the use of such a detector will make it possible to extent the physics program to proton decay, atmospheric neutrinos and astrophysics searches. The ESS proton linac upgrade, the accumulator ring needed for proton pulse compression, the target station optimization and the physics potential are described. In addition to the production of neutrinos, this facility will also be a copious source of muons which could be used to feed a low energy nuSTORM facility, a future neutrino factory or a muon collider. The ESS linac, under construction, will reach full operation at 5 MW by 2023 after which the upgrades for the neutrino facility could start.

Development and Experimental Validation of a Correlation Monitor Tool Based on the Endogenous Pulsed Neutron Source Technique

AbstractA correlation measuring tool for an endogenous pulsed neutron source experiment is developed in this work. Paroxysmal pulses generated by a bursts of neutron chains are detected by a 10-kbit embedded shift register with a time resolution of 100 ns. The system is implemented on a single reprogrammable device making it a compact, cost-effective instrument, easily adaptable for any case study. The system was verified experimentally in theEsfahan heavy-water zero power reactor(EHWZPR). The results obtained by the measuring tool are validated by the Feynman-α experiment, and a good agreement is seen within the boundaries of statistical uncertainties. The theory of the methods is briefly initiated in the text. Also, the system structure is described, the experimental results and their uncertainties are discussed, and neutron statistics in EHWZPR is examined experimentally.

On the limit of neutron fluxes in the fission-based pulsed neutron sources

The upper limit of the density of the thermal neutron flux from pulsed sources based on the fission reaction is established. Three types of sources for research on ejected beams are considered: a multiplying target of the proton accelerator (a booster), a booster with the reactivity modulation (a superbooster), and a pulsing reactor. Comparison with other high-flux sources is carried out. The investigation has been performed at the Frank Laboratory of Neutron Physics of JINR.

Characterisation of the incident beam and current diffraction capabilities on the VESUVIO spectrometer

The VESUVIO spectrometer at the ISIS pulsed neutron and muon source is a unique instrument amongst those available at neutron facilities. This is the only inverted-geometry neutron spectrometer accessing values of energy and wavevector transfer above tens of eV and , respectively, and where deep inelastic neutron scattering experiments are routinely performed. As such, the procedure at the base of the technique has been previously described in an article published by this journal (Mayers and Reiter 2012 Meas. Sci. Technol. 23 045902). The instrument has recently witnessed an upsurge of interest due to a new trend to accommodate, within a single experiment, neutron diffraction and transmission measurements in addition to deep inelastic neutron scattering. This work presents a broader description of the instrument following these recent developments. In particular, we assess the absolute intensity and two-dimensional profile of the incident neutron beam and the capabilities of the backscattering diffraction banks. All results are discussed in the light of recent changes to the moderator viewed by the instrument. We find that VESUVIO has to be considered a high-resolution diffractometer as much as other diffractometers at ISIS, with a resolution as high as in backscattering. Also, we describe the extension of the wavelength range of the instrument to include lower neutron energies for diffraction measurements, an upgrade that could be readily applied to other neutron instruments as well.

Materials and Life Science Experimental Facility at the Japan Proton Accelerator Research Complex I: Pulsed Spallation Neutron Source

At the Japan Proton Accelerator Research Complex (J-PARC), a pulsed spallation neutron source provides neutrons with high intensity and narrow pulse width pulse to promote researches on a variety of science in the Materials and Life Science Experimental Facility (MLF). It was designed to be driven by a proton beam with an energy of 3 GeV, a power of 1 MW at a repetition rate of 25 Hz, that is world’s highest power level. It is still on the way towards the goal to accomplish the operation with a 1 MW proton beam. In this review, distinctive features of the target-moderator-reflector system of the pulsed spallation neutron source are presented.

Neutron inelastic scattering measurements on the stable isotopes of titanium

The results of a neutron inelastic scattering experiment performed at the Geel Electron Linear Accelerator pulsed white neutron source of the European Commission Joint Research Centre are reported. The neutrons with energies up to 18 MeV interacted with a $^{\mathrm{nat}}\mathrm{Ti}$ sample and the $\ensuremath{\gamma}$ rays resulting from inelastic scattering reactions on the stable isotopes were detected using the Gamma Array for Inelastic Neutron Scattering (GAINS) spectrometer. We were able to measure the $\ensuremath{\gamma}$-production cross sections for 21 transitions in the five stable Ti isotopes. From these, the level cross sections and the total inelastic cross sections were determined. Our experimental results are compared with theoretical calculations performed using the talys 1.8 code, evaluated nuclear data libraries, and also with previously reported results.

Benchmarks of subcriticality in accelerator-driven system at Kyoto University Critical Assembly

Abstract Basic research on the accelerator-driven system is conducted by combining 235U-fueled and 232Th-loaded cores in the Kyoto University Critical Assembly with the pulsed neutron generator (14 MeV neutrons) and the proton beam accelerator (100 MeV protons with a heavy metal target). The results of experimental subcriticality are presented with a wide range of subcriticality level between near critical and 10,000 pcm, as obtained by the pulsed neutron source method, the Feynman-α method, and the neutron source multiplication method.

Development and Characterization of a High-Energy Neutron Time-of-Flight Imaging System

Los Alamos National Laboratory has developed a prototype of a high-energy neutron time-of-flight imaging system for the nondestructive evaluation of dense, massive, and/or high atomic number objects. High-energy neutrons provide the penetrating power, and thus the high dynamic range necessary to image internal features and defects of such objects. The addition of the time gating capability allows for scatter rejection when paired with a pulsed monoenergetic beam, or neutron energy selection when paired with a pulsed broad-spectrum neutron source. The Time Gating to Reject Scatter and Select Energy system was tested at the Los Alamos Neutron Science Center’s weapons nuclear research facility, a spallation neutron source, to provide proof of concept measurements and to characterize the instrument response. This paper will show results of several objects imaged during this run cycle. In addition, results from system performance metrics, such as the modulation transfer function and the detective quantum efficiency measured as a function of neutron energy, characterize the current system performance and inform the next generation of neutron imaging instrument.

Detection of Combined n/γ Fission Signatures Induced by an Epithermal Neutron Source

In this paper, a method is presented for the detection of special nuclear materials (SNMs) in shielded containers, which is both sensitive and applicable under field conditions. The method uses an external pulsed neutron source to induce fission in SNM and subsequent detection of the fast prompt fission neutrons. The detectors surrounding the container under investigation are liquid scintillation detectors able to distinguish gamma rays from fast neutrons by means of pulse shape discrimination method (PSD). One advantage of these detectors, besides the ability for PSD analysis, is that the analog signal from a detection event is of very short duration (typically few tens of nanoseconds). This allows the use of very short coincidence gates for the detection of the prompt fission neutrons in multiple detectors, while benefiting from a low background coincidence rate, yielding a low detection limit. Another principle advantage of this method derives from the fact that the external neutron source is pulsed. By proper time gating, the interrogation can be conducted by epithermal source neutrons only. These neutrons do not appear in the fast neutron signal following the PSD analysis, thus providing a fundamental method for separating the interrogating source neutrons from the sample response in the form of fast fission neutrons. This paper describes laboratory tests with a configuration of eight detectors in the Pulsed Neutron Interrogation Test Assembly (PUNITA). Both the photon and neutron signature for induced fission is observed, and the methods used to isolate these signatures are described and demonstrated.

Neutron Scattering Measurements of Carbon Dioxide Adsorption in Pores within the Marcellus Shale: Implications for Sequestration.

Shale is an increasingly viable source of natural gas and a potential candidate for geologic CO2 sequestration. Understanding the gas adsorption behavior on shale is necessary for the design of optimal gas recovery and sequestration projects. In the present study neutron diffraction and small-angle neutron scattering measurements of adsorbed CO2 in Marcellus Shale samples were conducted on the Near and InterMediate Range Order Diffractometer (NIMROD) at the ISIS Pulsed Neutron and Muon Source, STFC Rutherford Appleton Laboratory along an adsorption isotherm of 22 °C and pressures of 25 and 40 bar. Additional measurements were conducted at approximately 22 and 60 °C at the same pressures on the General-Purpose Small-Angle Neutron Scattering (GP-SANS) instrument at Oak Ridge National Laboratory. The structures investigated (pores) for CO2 adsorption range in size from Å level to ∼50 nm. The results indicate that, using the conditions investigated densification or condensation effects occurred in all accessible pores. The data suggest that at 22 °C the CO2 has liquid-like properties when confined in pores of around 1 nm radius at pressures as low as 25 bar. Many of the 2.5 nm pores, 70% of 2 nm pores, most of the <1 nm pores, and all pores <0.25 nm, are inaccessible or closed to CO2, suggesting that despite the vast numbers of micropores in shale, the micropores will be unavailable for storage for geologic CO2 sequestration.

An accelerating voltage generator for compact pulsed neutron sources

A multistage generator of high-voltage pulses with a scroll geometry of spark switches, which is produced according to the Marx scheme, is presented. The device is designed for a small pulsed neutron source and makes it possible to obtain accelerating-voltage pulses with amplitudes of up to 450 kV at a stored energy of up to 50 J and a load current of up to 1.5 kA.

SANS method study of surfactant mixture system TX-100+C16TAB in heavy water solutions

The mixture system of two classic surfactants cationic and non-ionic – C16TAB (hexadecyltrimethylammonium bromide)+TX-100(p-(1,1,3,3-tetramethyl) poly(oxyethylene) in heavy water solutions was investigated at temperatures 30o, 50o, 70o for compositions 1:1, 2:1, 3:1 by the small-angle neutron scattering(SANS) method on spectrometer (‘YuMO’) at the IBR-2 pulsed neutron source at FLNP, JINR in Dubna (Russia). Measurements have covered Q range from 7x10-3 to 0.4 Å-1. The SANS measurements of aqueous solutions of nonionic / cationic surfactants have shown that the mixed micelles are formed [1-2]. From the measured dependence of the scattered intensity on the scattering angle, we derived the size, shape of micelles, aggregation number at various compositions and temperatures. The size of mixed micelle is a weak function of the mixing ratio between the two components.

Characterization of a neutron sensitive MCP/Timepix detector for quantitative image analysis at a pulsed neutron source

The uncertainties and the stability of a neutron sensitive MCP/Timepix detector when operating in the event timing mode for quantitative image analysis at a pulsed neutron source were investigated. The dominant component to the uncertainty arises from the counting statistics. The contribution of the overlap correction to the uncertainty was concluded to be negligible from considerations based on the error propagation even if a pixel occupation probability is more than 50%. We, additionally, have taken into account the multiple counting effect in consideration of the counting statistics. Furthermore, the detection efficiency of this detector system changes under relatively high neutron fluxes due to the ageing effects of current Microchannel Plates. Since this efficiency change is position-dependent, it induces a memory image. The memory effect can be significantly reduced with correction procedures using the rate equations describing the permanent gain degradation and the scrubbing effect on the inner surfaces of the MCP pores.

Development of Multi-colored Neutron Talbot–Lau Interferometer with Absorption Grating Fabricated by Imprinting Method of Metallic Glass

For the effective interferometric imaging at pulsed neutron sources, we have developed the Talbot–Lau interferometer which works at several wavelengths, and demonstrated its operation by observing the visibilities of moire fringes in different wavelength conditions. An absorption grating as an analyzer was fabricated by imprinting of metallic glass for the first time, and showed a well-controlled shape. Using such a grating, we have succeeded in interferometric imaging for the samples of metal rods at a wavelength of 5 A.

Experimental benchmarks on kinetic parameters in accelerator-driven system with 100 MeV protons at Kyoto University Critical Assembly

Accelerator-driven system experiments with spallation neutrons (100MeV protons and Pb-Bi target) are carried out in the 235U-fueled and Pb-Bi-zoned core at the Kyoto University Critical Assembly, under a subcritical state ranging between 1160 and 11,556pcm. In these experiments, measurement of the prompt neutron decay constant and the subcriticality is conducted by the pulsed neutron source (PNS) method and the Feynman-α method with the use of optical fiber detectors. The experimental results successfully validate the prompt neutron decay constant and the subcriticality through the deduction of kinetic parameters by both the PNS and the α-fitting methods. The detector position dependency, neutron spectrum and subcriticality measurement methods still remain, however, in these experiments. For onward studies, the experimental benchmarks obtained from these experiments are expected to be involved in the numerical verification of subcriticality on-line monitoring, in the analysis of subcriticality uncertainty and in the deterministic approach to kinetic parameters.

Concentration of the velocity distribution of pulsed neutron beams

The velocity of neutrons from a pulsed neutron source is well-defined as a function of their arrival time. Electromagnetic neutron accelerator/decelerator synchronized with the neutron time-of-flight is capable of selectively changing the neutron velocity and concentrating the velocity distribution. Possible enhancement of the neutron intensity at a specific neutron velocity by orders of magnitude is discussed together with an experimental design.