Laser Properties Research Articles

High quality factor, monodisperse micron-sized random lasers based on porous PLGA spheres

Miniature random lasers with high quality factor are crucial for applications in barcoding, bioimaging, and on-chip technologies. However, achieving monodisperse and size-tunable biocompatible random lasers has been a significant challenge. In this study, we employed poly(lactic-co-glycolic) acid (PLGA), a biocompatible material approved for medical use, as the base material for random lasers. By integrating a dye-doped PLGA solution with a microfluidic system, we successfully fabricated monodisperse and miniature dye-doped PLGA spheres with tunable sizes ranging from 25 to 52 µm. Upon optical pulse excitation, these spheres exhibited strong random lasing emission at 610–640 nm with a threshold of approximately 22 µJ·mm−2. The lasing modes demonstrated a spectral linewidth of 0.2 nm, corresponding to a quality factor of 3100. Fourier transform analysis of the lasing emission revealed fundamental cavity lengths, providing insights into the properties of the random lasers.

Linear and nonlinear optical properties of femtosecond laser inscribed waveguides into GLS glass

Linear and nonlinear optical properties of femtosecond laser inscribed waveguides into GLS glass

A novel method enhanced mechanical properties of a selective laser melted Mar-M247 superalloy by progressive remelting

A novel method has been proposed to avoid the cracks in the Mar-M247 alloy manufactured via selective laser melting (SLM) related to high cooling rate interacted with carbides and eutectics, i.e., progressive remelting used to design the temperature field reducing the thermal stresses in SLM process. The microstructure evolves from a partly fused state to a completely solid block during progressive remelting, and those cracks inhibit effectively. The temperature gradient is gradually reduced in the process of progressive remelting, and eventually 29% lower than that in original SLM process. Quantitative temperature-field analysis signifies a substantial decrease in the cooling rate during manufacturing via progressive remelting, which explains crack inhibition. Compared to the original SLM-built Mar-M247, progressive remelting leads to a 35.1% increase in ultimate tensile strength (UTS) at RT. The UTS and elongation of progressive remelted Mar-M247 exhibit 747.2 MPa and 6.1% at 900 °C, respectively, superior to that of materials fabricated by casting and heat-treatment. This work helps further comprehend the relationship of volumetric energy density - thermal gradient - cooling rate - microstructure - mechanical properties, especially utilizing accumulative input energy to control temperature field, and offers a new opportunity to non-weldable superalloys fabricated in commercially available SLM systems.

Influence of ultrasonic assistance on the microstructure and friction properties of laser cladded Ni60/WC composite coatings

The effects of different ultrasonic vibration powers on the distribution, phase structure, friction and wear properties of WC reinforced particles in laser melted Ni60/WC composite coatings are investigated. The effects of ultrasonic vibration on the microstructure, elemental distribution, crystal orientation, friction and wear properties of the fused coatings are analyzed. The experimental results show that the deposition of WC particles in the lower and middle parts of the coating is significantly improved after the introduction of ultrasonic vibration during the fusion cladding process. In particular, at 600 W ultrasonic power, not only the distribution uniformity of tungsten carbide particles in the coating is optimal, but also the composite coating shows better wear resistance. However, too much ultrasonic power increases the possibility of particle agglomeration. In addition, although the phase pattern of the coating does not change after ultrasonic vibration, the width of the columnar crystalline region of the coating is reduced, and the coating is covered by a homogeneous lamellar nanoscale eutectic structure with the phase compositions of the γ-(Fe, Ni) and M23C6 phases. The ultrasonic vibration improves elemental segregation of the coating, reduces the large number of precipitated phases in the coating, weakens the grain growth orientation, and relieves the local stress concentration in the coating. In addition, the mechanism of the influence of WC particles on the microstructure evolution and wear resistance of the composite coatings is discussed.

Influence of layer thickness and heat treatment on microstructure and properties of selective laser melted maraging stainless steel

As one of the main parameters of selective laser melting (SLM) process, layer thickness has a significant impact on the forming performance and efficiency of printed parts. Based on microstructure analysis and properties testing, the metallurgical mechanism, phase composition and mechanical behavior of SLM-formed Corrax stainless steel with different layer thicknesses were discussed. The influence of heat treatment process on the properties was comparatively investigated. The results indicated that at smaller or larger layer thicknesses, the increase in melt dynamic instability and spheroidisation feature easily induced the formation of unfused pore defects, which in turn led to lower relative density and mechanical properties. At the appropriate layer thickness, the suitable melt flow behaviour promoted the formation of good metallurgical bonding between adjacent melt channels. The maximum tensile strength, yield strength and hardness of the samples prepared at a layer thickness of 60 μm were 1224 MPa, 948 MPa and 39.2 HRC, respectively. The microstructure of the as-built samples was martensite and a small amount of austenite. With increasing layer thickness, the cooling rate of the molten pool decreased and the austenite content increased. After solution treatment, the alloying elements dissolved in the martensitic matrix resulted in lower mechanical properties. After aging and solution aging treatment, the mechanical properties were significantly improved due to precipitation strengthening of NiAl nanoparticles and dislocation strengthening. The corresponding tensile strengths were 1655 MPa and 1796 MPa, the yield strengths were 1328 MPa and 1573 MPa, and the hardnesses were 45.7 HRC and 50.2 HRC, respectively.

Yb:YSAG ceramics: An attractive thin-disk laser material alternative to a single crystal?

The 8.3 at.% Yb-doped yttrium-scandium-aluminum garnet (YSAG) ceramics were fabricated by a modified reverse co-precipitation method followed by uniaxial and cold isostatic pressing, annealing in air and high-temperature sintering in vacuum. Spectroscopic and lasing properties were investigated in dependence on Y/Sc/Al ratio in ceramic composition. Optical transmission of Yb:YSAG ceramics in visible and near-infrared spectral range exceeds 80 % that indicates a high quality of the Yb:YSAG samples. Among all the ceramics, the Y2.35Yb0.25Sc1.00Al4.40O12 composition demonstrates the best lasing performance and the highest slope efficiency up to 75 %.

Joint formation mechanism and mechanical properties of laser brazed Zn coated steel under different defocusing conditions

Laser brazing, producing a class-A joint surface in automotive, relies on the defocus control to manage laser heating mode and braze performance. This work demonstrates that the laser interaction mechanism transitioned from keyhole welding to conduction brazing as defocus distances increased from −20 to ≥18 mm while keeping other parameters consistent. Uniform brazed joints were achieved at defocuses of +22, +25 and + 30 mm. Increased defocus distance resulted in a wider bead, with a larger laser irradiation area and expanded heat affected zone (HAZ), leading to increased steel melting and more Fe-rich precipitates within the Cu braze. The interfacial reaction layers remained Fe(Si) with increasing thickness as defocus changed from +22 to +30 mm, and two distinct Fe(Si) phases were initially identified. The steel Zn coating evaporated upon direct laser irradiation at upper two regions while participated in interfacial reactions at the weld root. At the weld root, a dramatic phase transition from Zn–Cu to Cu was observed, with liquid Zn(Cu) phases particularly forming in joints with a +30 mm defocus, led to solidification cracks that acted as failure initiation sites during tensile testing. Cracks propagated along the interfacial reaction layer/bead interface, or along large Fe-rich precipitates within the bead. A +30 mm defocus produced a lower hardness HAZ than with a +22 mm defocus, due to the higher content of bainite and tempered martensite resulting from a slower cooling rate. This work provides insights into optimizing laser brazing parameters for Zn-coated steel.

Crystal growth, spectra and laser properties of Tm3+ and Ho3+ co-doped GdScO3 crystal

Tm,Ho:GdScO3 single crystal was grown by the Czochralski method. Its quality and effective segregation coefficient of crystal were characterized, and spectral properties of crystal (100) plane were studied. The absorption cross-section of Tm,Ho:GdScO3 at 793 nm is 1.61 × 10−20 cm2 and emission cross-section at 2020 nm is 1.39 × 10−20 cm2. The laser performance of the crystal by 793 nm LD end-pumped was investigated. The maximum output power of 240 mW was obtained with a slope efficiency of 9.1 % in CW(continuous wave) pump mode. In pulse mode, the maximum average output power of 507 mW was achieved. The maximum slope efficiency of 13.7 % was obtained with 100 Hz and 400 μs. The laser wavelength was 2096 nm. The beam quality factors Mx2/My2 were fitted to be 1.81/1.80. These results indicate that Tm,Ho:GdScO3 crystal is a promising candidate medium for near-infrared laser application.

Control of photothermal liquid jets through microbubble Regulation: Fundamental mechanisms and Developing Strategies

Plasmon-induced photoacoustic streaming, considered as a potential application for micro-pumps in microfluidics, currently encounters ongoing debates concerning its fundamental mechanisms. In this study, we investigate the crucial role played by microbubbles in generation of jets in an ethanol aqueous solution. The power density threshold for bubble generation and its dependency on jet initiation are confirmed and the microbubble behavior is well regulated by manipulating the laser and liquid properties. Through simulations coupling fluidic and thermal fields, the significant role of Marangoni effect is validated in jet formation. Specifically, the temperature gradient of microbubbles is determined to be a pivotal factor in the generation of collimated jets. Additionally, factors influencing jetting, such as microbubble size and temperature gradients are studied, and noticeably, a stabilized jet lasting over 4 h is achieved based upon.

Role of processing parameters on relative density, microstructure and mechanical properties of selective laser melted titanium alloy

Role of processing parameters on relative density, microstructure and mechanical properties of selective laser melted titanium alloy

Tailoring the morphological, optical, electrical, and random lasing properties of ZnO nanorods synthesized on metal surfaces for biosensor applications

Laser-based sensors are taking over their counterparts, fluorescence-based sensors, in the field of bioengineering and space communication due to their high amplification, narrow emission beam, low signal-to-noise ratio, and nonlinearity. In this work, we investigated the chemical growth of ZnO nanorods on different metal surfaces (Au, Pt, Ti, and Al) to serve as random laser mediums. Different analytical techniques were used to investigate the optical, electrical, and morphological properties of the fabricated devices. A lasing threshold of 27.68 mJ/cm² with a spectral width of 2.18 nm centered at 385.06 nm is observed when Ti is used as the growth surface. Al surface produces ZnO nanorods with a lasing threshold of 24.21 mJ/cm² and a spectral width of 1.81 nm. Growing ZnO nanorods on metal surfaces using the chemical bath deposition method paves the way for fabricating different random lasing-based biosensors.

Controllable lasing characteristics in Brillouin random fiber lasers by tailoring gain and random feedback fibers

Brillouin random fiber lasers (BRFLs), the combination of stimulated Brillouin scattering (SBS) gain and random distributed feedback, offer narrow linewidth lasing with simplicity and flexibility. However, BRFLs may not gain broad acceptance unless the fundamental lasing mechanisms governing their operation are fully understood and the lasing properties are effectively manipulated. Here, we demonstrate the control of lasing characteristics in BRFLs by tailoring the SBS gain fiber and the scattering pattern of the random feedback fiber. Experimental results show that BRFLs with 5 cm random fiber gratings (RFGs) feedback exhibit lower intensity fluctuation, longer coherence time, and more stable frequency compared to those with 6 km Rayleigh scattering fiber (RSF) feedback thanks to more correlated phase, lower mode density, and weaker dependence on external variations of RFGs. The low-randomness RFG feedback further improves the coherence time and intensity fluctuation attributed to the small period variation of sub-gratings. Moreover, the BRFL based on the high gain fiber and the strong scattering RFG feedback with low loss achieves high lasing efficiency and low threshold. The frequency jitter, intensity noise, and coherence time are also improved by reducing the gain fiber from 20 km to 1 km due to decreased mode hopping from mode competition. These results clarify the impact of gain and random feedback fibers on BRFL performance, offering insights for optimizing complex laser design for applications requiring high frequency stability and long coherence time.

(Cd)SO4 doping on L-Valine crystal for the enhancement of opto-electronic and laser properties

L-Valine is a good molecular platform to induce NLO properties for Laser application and considerable laser properties can be improved by injecting suitable electron administrated substitutional groups. This work is an attempt to make laser properties enhancement by increasing Cd solvent concentration on L-Valine compound. The recorded XRD peaks addressed the significant increment of laser properties of the composite crystal. The results obtained for pure L-Valine was; a=5.221 (Å), b=6.910 (Å) and c=4.994 (Å) and associated indices of refraction was n1=1.511, n2=1.583 and n3=1.599. The results of 2% CdSO4; a=5.580 (Å), b=7.011 (Å) and c=5.091 (Å) and associated indices of refraction was n1=1.561, n2=1.612 and n3=1.633. For 5% CdSO4; a=5.599 (Å), b=7.831 (Å) and c=5.659 (Å) and associated indices of refraction was n1=1.588, n2=1.661 and n3=1.699. For 10 % CdSO4; a=5.592 (Å), b=7.612 (Å) and c=5.822 (Å) and associated indices of refraction was n1=1.661, n2=1.693 and n3=1.593. For 15 % CdSO4; a=5.551 (Å), b=6.332 (Å) and c=4.734 (Å) and associated indices of refraction was n1=1.501, n2=1.599 and n3=1.593. The non linear refractive index was changed from 3.891 X 10-8 cm2/W to 4.231 X 10-8 cm2/W for 2%, 5%, 10% respectively and Third order non linear optical susceptibility (χ(3)) was ranged from 4.621X10‑6 esu to 5.091X10‑6 esu. The restored chemical potential for non linear optical (NLO) and birefringence properties was found to be improved. The scattering capability of homo nuclear and hetero nuclear bonds along with the CdSO4 voids was identified for attaining non linear scattering process.

Enhancing microstructure and mechanical properties of laser directed energy deposited AlSi10Mg alloy by friction stir processing

The low strength-plastic properties of AlSi10Mg alloy prepared by laser directed energy deposition (LDED) have limited its application in aerospace and related fields, prompting researchers to explore friction stir processing (FSP) as a viable post-treatment solution. This study investigated the effects of FSP on the microstructure and mechanical properties of AlSi10Mg alloy formed by LDED, revealing that FSP effectively eliminated pores and refined grains, transforming the coarse and uneven grains in base material (BM) into fine and uniform equiaxed grains. Consequently, the thermal mechanical affected zone presented a microstructure gradient due to the uneven distribution of material flow and frictional heat. Additionally, the yield strength (YS), ultimate tensile strength (UTS), and elongation (EL) of LDEDed specimens were determined to 91.98 MPa, 158.57 MPa, and 4.29 %, respectively. YS and UTS of LDED-FSPed specimens were increased about 20 % and 30 %, and EL was greatly improved approximately 2–3 times compared with LDEDed specimens. Consequently, the grain refinement and porosity elimination caused by FSP improve the mechanical properties and microstructure evolution of LDED-FSPed specimens.

Deep Mouse Brain Two-Photon Near-Infrared Fluorescence Imaging Using a Superconducting Nanowire Single-Photon Detector Array.

Two-photon microscopy (2PM) has become an important tool in biology to study the structure and function of intact tissues in vivo. However, adult mammalian tissues such as the mouse brain are highly scattering, thereby putting fundamental limits on the achievable imaging depth, which typically reside at around 600-800 μm. In principle, shifting both the excitation as well as (fluorescence) emission light to the shortwave near-infrared (SWIR, 1000-1700 nm) region promises substantially deeper imaging in 2PM, yet this shift has proven challenging in the past due to the limited availability of detectors and probes in this wavelength region. To overcome these limitations and fully capitalize on the SWIR region, in this work, we introduce a novel array of superconducting nanowire single-photon detectors (SNSPDs) and associated custom detection electronics for use in near-infrared 2PM. The SNSPD array exhibits high efficiency and dynamic range as well as low dark-count rates over a wide wavelength range. Additionally, the electronics and software permit a seamless integration into typical 2PM systems. Together with an organic fluorescent dye emitting at 1105 nm, we report imaging depth of >1.1 mm in the in vivo mouse brain, limited mostly by available labeling density and laser properties. Our work establishes a promising, and ultimately scalable, new detector technology for SWIR 2PM that facilitates deep tissue biological imaging.

Thickness dependent structural and electrical properties of pulsed laser deposited Y0.95Ca0.05MnO3 thin films and the effect of high energy oxygen ion irradiation

Thickness dependent structural and electrical properties of pulsed laser deposited Y0.95Ca0.05MnO3 thin films and the effect of high energy oxygen ion irradiation

Nondestructive evaluation of microstructure and mechanical property of post-processing annealed selective laser melted 316L stainless steel by laser ultrasonics

By using the laser ultrasonics nondestructive technology, combined with the microstructure and mechanical property of post-processing annealed selective laser melted 316L stainless steel characterized by scanning electron microscopy (SEM), electron backscattering diffraction (EBSD), and mechanical property testing, selective laser melted 316L stainless steel after post-processing annealing was evaluated. The results show that the frequency domain attenuation coefficient of ultrasonic waves is positively correlated with the average grain size; the time domain attenuation coefficient of ultrasonic waves is negatively correlated with the low angle boundary content. The tensile strength has a good correlation with the time domain attenuation coefficient and wave speed, the correlation coefficients R2 are 0.95 and 0.89 respectively; the yield strength correlates with the time domain attenuation coefficient, the correlation coefficient R2 is 0.76; the elongation has a good correlation with the frequency domain attenuation coefficient and wave speed, the correlation coefficient R2 is 0.90 and 0.86 respectively.

Progress in the Study of Quality and Mechanical Properties of Selective Laser Melting Molded Parts

Abstract: Selective laser melting (SLM) is considered to be a widely promising additive manufacturing technology with the advantages of high machining precision, high manufacturing freedom, and short cycle time, which is widely used in aerospace, the integration of medicine, and industry, chemical, and other fields. The research progress on the temperature field, stress field, forming quality, and mechanical properties during the SLM manufacturing process is reviewed. The study aims to systematically analyze how SLM process parameters affect the temperature field, stress field, forming quality, and mechanical properties, and to discuss the importance of the selection of process parameters and performance regulation to achieve high-quality, highperformance metal parts. The effects of SLM process parameters on temperature field, stress field, surface roughness, densification, hardness, strength, and fatigue properties are analyzed and summarized. The importance of process parameters in the SLM forming procedure in the quality of formed components is emphasized, and conducting an in-depth study on the optimization and performance regulation of the process parameters is of great significance in achieving the high quality and performance of metal parts. With the rapid advancement of technology, the potential of SLM technology in terms of molding quality and mechanical performance has become increasingly significant, heralding significant breakthroughs. These potential breakthroughs will greatly promote the widespread application of SLM technology in various industries, thus more efficiently meeting the growing needs and expectations of industries such as petrochemicals, transportation, aerospace, nuclear energy, as well as food and medical sectors.

Influence of Mg Content on Microstructure Coarsening, Molten Pool Size, and Hardness of Laser Remelted Al(-x)-Mg-Sc Alloys.

Investigations leading to high-quality surfaces and optimized properties in laser remelted Al-Mg-Sc alloys remain scarce. Laser surface remelting (LSR) has been used for the final treatment of these alloys processed through additive manufacturing. However, the direct microstructure responses of the treated cast surfaces have not yet been investigated. In the present research, Al-3, 5, and 10 wt %-Mg-0.1 wt %-Sc alloys plates were processed using LSR to study the effects of local melting and rapid solidification. The morphology of the α-Al phase, microstructure coarsening, and hardness were mapped from the bottom to the top of the molten pools, varying with local Mg content and laser heat input (2.5 J/mm, 5 J/mm, and 10 J/mm). This study aimed to create a comprehensive map of the microstructures, hardness, and molten pool sizes under various conditions. The findings may help to optimize these alloys through understanding laser processing parameters. Methods used included CALPHAD computations, optical microscopy, SEM, EDS, image analysis, hardness tests, and heat flow models. The results obtained showed α-Al cell growth with bands in all alloys with hardness changes correlating with cell spacing and heat input. Higher Mg content resulted in more refined cells and a higher fraction of bands. Increased Mg content decreased the thermal diffusivity and enthalpy of melting, enlarging the molten pool size. Hardness increased with decreasing heat input and higher Mg content in the tested alloys, especially in the Al-10 wt %-Mg-0.1 wt %-Sc alloy as the heat input was varied.

Effect of swinging laser on porosity, microstructure, and mechanical properties of laser welded aluminum alloy joints with different lap forms

Oscillating and conventional linear laser welding were conducted to enhance the bonding strength of dissimilar aluminum alloys. The effect of lap joint configuration on porosity, microstructure, and mechanical properties of laser-welded dissimilar aluminum alloy joints was investigated. It was found that the solidification rate of the melt pool was the dominant factor in the difference in porosity for oscillating laser-welded joints with different lap joint configurations. The main precipitated phase in welds with different lap joint configurations was eutectic Si, and the proportion of eutectic Si was higher in oscillating laser welds than in linear laser welds. The elemental distribution in oscillating laser welds was more uniform. The strengthening mechanism for tensile shear strength of oscillating laser welded lap joints was analyzed. The improved tensile shear strength and elongation were attributed to the reduced porosity and solid solution strengthening for the oscillating laser welding. The tensile strengths of the two lap types of oscillating laser welded joints increased by 25.1 MPa and 34.5 MPa, and the elongation increased by 0.7% and 4.5%.