Probe Photon Research Articles

Strong-field vacuum polarisation with high energy lasers

When photons propagate in vacuum they may fluctuate into matter pairs thus allowing the vacuum to be polarised. This linear effect leads to charge screening and renormalisation. When exposed to an intense background field a nonlinear effect can arise when the vacuum is polarised by higher powers of the background. This nonlinearity breaks the superposition principle of classical electrodynamics, allowing for light-by-light scattering of probe and background photons mediated through virtual pairs dressed by the background. Vacuum polarisation is a strong-field effect when all orders of interaction between the virtual pair and the background must be taken into account. In this investigation we show that multiple scattering processes of this type may be observed by utilising high-energy laser pulses with long pulse duration, such as are available at facilities like ELI Beamlines. In combination with appropriate sources of high-energy probe photons, multiple probe-background light-by-light scattering allows for testing the genuine nonlinear regime of strong-field quantum electrodynamics. This provides access to the uncharted non-perturbative regime beyond the weak-field limit.

Remarks on propagating waves in non-linear vacuum electrodynamics

Using the quadratic expansion in the photon fields of Euler–Heisenberg (EH) non-linear electrodynamics (NLED) Lagrangian model we study relevant vacuum properties in a scenario involving the propagation of a photon probe in the presence of a background constant and static magnetic field, mathbf{B_e}. We compute the gauge invariant, symmetric and conserved energy–momentum tensor (EMT) and angular momentum tensor (AMT) for arbitrary magnetic field strength using the Hilbert method under the soft-photon approximation. We discuss how the presence of magneto-electric terms in the EH Lagrangian is a source of anisotropy, induce the non-zero trace in the EMT and leads to differences between EMT calculated by the Hilbert or Noether method. From the Hilbert EMT we analyze some quantities of interest such as the energy density, pressures, Poynting vector, and angular momentum vector, comparing and discussing the differences with respect to the improved Noether method. The magnetized vacuum properties are also studied showing that a photon effective magnetic moment can be defined for different polarization modes. The calculations are done in terms of derivatives of the two scalar invariants of electrodynamics, hence, extension to other NLED Lagrangian is straightforward. We discuss further physical implications and experimental strategies to test magnetization, photon pressure, and effective magnetic moment.

Time-, spin-, and angle-resolved photoemission spectroscopy with a 1-MHz 10.7-eV pulse laser.

We describe a setup of time-, spin-, and angle-resolved photoemission spectroscopy (tr-SARPES) employing a 10.7 eV (λ = 115.6nm) pulse laser at a 1MHz repetition rate as a probe photon source. This equipment effectively combines the technologies of a high-power Yb:fiber laser, ultraviolet-driven harmonic generation in Xe gas, and a SARPES apparatus equipped with very-low-energy-electron-diffraction spin detectors. A high repetition rate (1MHz) of the probe laser allows experiments with the photoemission space-charge effects significantly reduced, despite a high flux of 1013 photons/s on the sample. The relatively high photon energy (10.7eV) also brings the capability of observing a wide momentum range that covers the entire Brillouin zone of many materials while ensuring high momentum resolution. The experimental setup overcomes the low efficiency of spin-resolved measurements, which gets even more severe for the pump-probed unoccupied states, and affords the opportunity to investigate ultrafast electron and spin dynamics of modern quantum materials with energy and time resolutions of 25meV and 360fs, respectively.

Momentum-Space Imaging of Ultra-Thin Electron Liquids in δ-Doped Silicon.

Two-dimensional dopant layers (δ-layers) in semiconductors provide the high-mobility electron liquids (2DELs) needed for nanoscale quantum-electronic devices. Key parameters such as carrier densities, effective masses, and confinement thicknesses for 2DELs have traditionally been extracted from quantum magnetotransport. In principle, the parameters are immediately readable from the one-electron spectral function that can be measured by angle-resolved photoemission spectroscopy (ARPES). Here, buried 2DEL δ-layers in silicon are measured with soft X-ray (SX) ARPES to obtain detailed information about their filled conduction bands and extract device-relevant properties. This study takes advantage of the larger probing depth and photon energy range of SX-ARPES relative to vacuum ultraviolet (VUV) ARPES to accurately measure the δ-layer electronic confinement. The measurements are made on ambient-exposed samples and yield extremely thin (< 1nm) and dense (≈1014 cm-2 ) 2DELs. Critically, this method is used to show that δ-layers of arsenic exhibit better electronic confinement than δ-layers of phosphorus fabricated under identical conditions.

Quantum Induced Coherence Light Detection and Ranging.

Quantum illumination has been proposed and demonstrated to improve the signal-to-noise ratio (SNR) in light detection and ranging (LiDAR). When relying on coincidence detection alone, such a quantum LiDAR is limited by the timing jitter of the detector and suffers from jamming noise. Inspired by the Zou-Wang-Mandel experiment, we design, construct, and validate a quantum induced coherence (QuIC) LiDAR which is inherently immune to ambient and jamming noises. In traditional LiDAR the direct detection of the reflected probe photons suffers from deteriorating SNR for increasing background noise. In QuIC LiDAR we circumvent this obstacle by only detecting the entangled reference photons, whose single-photon interference fringes are used to obtain the distance of the object, while the reflected probe photons are used to erase path information of the reference photons. In consequence, the noise accompanying the reflected probe light has no effect on the detected signal. We demonstrate such noise resilience with both LED and laser light to mimic the background and jamming noise. The proposed method paves a new way of battling noise in precise quantum electromagnetic sensing and ranging.

Direct tracking of ultrafast proton transfer in water dimers.

Upon ionization, water forms a highly acidic radical cation H2O+· that undergoes ultrafast proton transfer (PT)-a pivotal step in water radiation chemistry, initiating the production of reactive H3O+, OH[Formula: see text] radicals, and a (hydrated) electron. Until recently, the time scales, mechanisms, and state-dependent reactivity of ultrafast PT could not be directly traced. Here, we investigate PT in water dimers using time-resolved ion coincidence spectroscopy applying a free-electron laser. An extreme ultraviolet (XUV) pump photon initiates PT, and only dimers that have undergone PT at the instance of the ionizing XUV probe photon result in distinct H3O+ + OH+ pairs. By tracking the delay-dependent yield and kinetic energy release of these ion pairs, we measure a PT time of (55 ± 20) femtoseconds and image the geometrical rearrangement of the dimer cations during and after PT. Our direct measurement shows good agreement with nonadiabatic dynamics simulations for the initial PT and allows us to benchmark nonadiabatic theory.

Implantable photonic neural probes with 3D-printed microfluidics and applications to uncaging.

Advances in chip-scale photonic-electronic integration are enabling a new generation of foundry-manufacturable implantable silicon neural probes incorporating nanophotonic waveguides and microelectrodes for optogenetic stimulation and electrophysiological recording in neuroscience research. Further extending neural probe functionalities with integrated microfluidics is a direct approach to achieve neurochemical injection and sampling capabilities. In this work, we use two-photon polymerization 3D printing to integrate microfluidic channels onto photonic neural probes, which include silicon nitride nanophotonic waveguides and grating emitters. The customizability of 3D printing enables a unique geometry of microfluidics that conforms to the shape of each neural probe, enabling integration of microfluidics with a variety of existing neural probes while avoiding the complexities of monolithic microfluidics integration. We demonstrate the photonic and fluidic functionalities of the neural probes via fluorescein injection in agarose gel and photoloysis of caged fluorescein in solution and in fixed brain tissue.

MXene-Assisted D-Shaped Photonic Crystal Fiber Probe with High Sensitivity for Detection of Tuberculosis

MXene-Assisted D-Shaped Photonic Crystal Fiber Probe with High Sensitivity for Detection of Tuberculosis

Search for dark sector by repurposing the UVX Brazilian synchrotron

We propose the first Search for Dark Sector at the Brazilian Synchrotron Light Laboratory, site of Sirius, a fourth-generation storage ring. We show that UVX, Sirius predecessor, can be a promising dark sector detector, SeDS, with unprecedented sensitivity. The search is based on a 1-3 GeV positron beam impinging on a thick target leading the e^+ e^- rightarrow gamma A' reaction, followed by a missing mass spectrum event reconstruction. We show that SeDS has the potential to probe dark photons with masses up to 55 MeV and kinetic coupling down to epsilon ^2 sim 10^{-12}. Therefore, such experiment would constitute the best dark photon probe worldwide in the 10{-}55 MeV mass range, being able to probe an unexplored region of parameter space.

Enhance high harmonic generation (HHG) efficiency via compact multi-plate continuum post-compression for time-resolved angle-resolved photoemission spectroscopy.

Time-resolved angle-resolved photoemission spectroscopy (Tr-APRES) gives direct insight into electron dynamics by providing temporal-, energy-, and momentum-resolved information in one experiment. A major obstacle to using high harmonic generation (HHG) probe pulses for photoemission spectroscopy is the low conversion efficiency, that is, the low flux of probe photons. We use a Yb-KGW based duo-laser source with an oscillator to pump two separate amplifiers and generate two synchronized pulsed laser sources with average energies of 7.5 and 6W. By using the multiplate continuum method and chirped mirrors, the resulting flux of HHG photons at 33-70eV can be increased 50-fold (up to 1011 photons/s) by using post-compressed 30fs pulses compared with the photon flux generated by the fundamental 190fs pulses. Moreover, pulses from the 6W amplifier are used to pump an optical parametric amplifier that can vary the wavelengths for photoexcitation. The system performance is demonstrated by applying Tr-ARPES to single-crystal graphite. The front tilt broadening is significantly suppressed by the off-plane mounted conical grating, leading to a 184fs temporal resolution that is mainly limited by the pump pulse. The energy resolution is 176meV.

Phase-insensitive amplifier gain estimation at Cramér-Rao bound for two-mode squeezed state of light.

Phase-insensitive amplifiers (PIAs), as a class of important quantum devices, have found significant applications in the subtle manipulation of multiple quantum correlation and multipartite quantum entanglement. Gain is a very important parameter for quantifying the performance of a PIA. Its absolute value can be defined as the ratio of the output light beam power to the input light beam power, while its estimation precision has not been extensively investigated yet. Therefore, in this work, we theoretically study the estimation precision from the vacuum two-mode squeezed state (TMSS), the estimation precision of the coherent state, and the bright TMSS scenario, which has the following two advantages: it has more probe photons than the vacuum TMSS and higher estimation precision than the coherent state. The advantage in terms of estimation precision of the bright TMSS compared with the coherent state is researched. We first simulate the effect of noise from another PIA with gain M on the estimation precision of the bright TMSS, and we find that a scheme in which the PIA is placed in the auxiliary light beam path is more robust than two other schemes. Then, a fictitious beam splitter with transmission T is used to simulate the noise effects of propagation loss and imperfect detection, and the results show that a scheme in which the fictitious beam splitter is placed before the original PIA in the probe light beam path is the most robust. Finally, optimal intensity difference measurement is confirmed to be an accessible experimental technique to saturate estimation precision of the bright TMSS. Therefore, our present study opens a new avenue for quantum metrology based on PIAs.

Highly anisotropic transient optical response of charge density wave order in ZrTe3

Low dimensionality in CDW systems leads to anisotropic optical properties, in both equilibrium and non-equilibrium conditions. Here we perform polarized two-color pump probe measurements on a quasi-1D material ZrTe$_3$, in order to study the anisotropic transient optical response in the CDW state. Profound in-plane anisotropy is observed with respect to polarization of probe photons. Below $T_\mathrm{CDW}$ both the quasi-particle relaxation signal and amplitude mode (AM) oscillation signal are much larger with $\mathbf{E}_\mathrm{pr}$ nearly parallel to $a$ axis ($\mathbf{E}_\mathrm{pr} \parallel a$) than for $\mathbf{E}_\mathrm{pr}$ parallel to $b$ axis ($\mathbf{E}_\mathrm{pr} \parallel b$). This reveals that $\mathbf{E}_\mathrm{pr} \parallel a$ signal is much more sensitive to the variation of the CDW gap. Interestingly, the lifetime of the AM oscillations observed with $\mathbf{E}_\mathrm{pr} \parallel b$ is longer than $\mathbf{E}_\mathrm{pr} \parallel a$. Moreover, at high pump fluence where the electronic order melts and the AM oscillations vanish for $\mathbf{E}_\mathrm{pr} \parallel a$ , the AM oscillatory response still persists for $\mathbf{E}_\mathrm{pr} \parallel b$. We discuss possible origins that lead to such unusual discrepancy between the two polarizations.

Electromagnetic form factors and charge radii of pseudoscalar and scalar mesons: A comprehensive contact interaction analysis

We carry out a comprehensive survey of electromagnetic form factors of all light, heavy and heavy-light ground-state pseudoscalar and scalar mesons. Our analysis is based upon a Schwinger-Dyson equations treatment of a vector $\times$ vector contact interaction. It incorporates confinement and ensures axial vector and vector Ward-Takahashi identities are satisfied along with the corresponding corollaries such as the Goldberger-Treiman relations. The algebraic simplicity of the model allows us to compute the form factors at arbitrarily large virtualities of the probing photon momentum squared with relative ease. Wherever possible and insightful, we compare our results for the electromagnetic form factors and the charge radii with those obtained earlier through Schwinger-Dyson equations, lattice and with experimental observations available. We also comment on the scope and shortcomings of the model.

Strongly Coupled Plasmon and Phonon Polaritons as Seen by Photon and Electron Probes

The ability to control and modify infrared excitations in condensed matter is of both fundamental and applied interest. Here we explore a system supporting low-energy excitations, in particular, mid-infrared localized plasmon modes and phonon polaritons that are tuned to be strongly coupled. We study the coupled modes by using far-field infrared spectroscopy, state-of-the-art monochromated electron energy-loss spectroscopy, numerical simulations, and analytical modeling. We demonstrate that the electron probe facilitates a precise characterization of polaritons constituting the coupled system, and enables an active control over the coupling and the resulting sample response both in frequency and space. Although far-field optical spectra can be substantially different from near-field electron energy-loss spectra, we show that a direct comparison is possible via postprocessing and right positioning of the electron beam. The resulting spectra allow us to evaluate the key parameters of the coupled system, such as the coupling strength, which we demonstrate to be probe independent. Our work establishes a rigorous description of the spectral features observed in light- and localized electron-based spectroscopies, which can be extended to the analysis of analogous optical systems with applications in heat management and electromagnetic field concentration or nanofocusing.

Effects of Pump Photon Energy on Generation and Ultrafast Relaxation of Excitons and Charge Carriers in CdSe Nanoplatelets.

We studied the initial nature and relaxation of photoexcited electronic states in CdSe nanoplatelets (NPLs). Ultrafast transient optical absorption (TA) measurements were combined with the theoretical analysis of the formation and decay of excitons, biexcitons, free charge carriers, and trions. In the latter, photons and excitons were treated as bosons and free charge carriers as fermions. The initial quantum yields of heavy-hole (HH) excitons, light-hole (LH) excitons, and charge carriers vary strongly with photon energy, while thermal relaxation occurs always within 1 ps. After that, the population of LH excitons is negligible due to relaxation to HH excitons or decay into free electrons and holes. Up to the highest average number of about four absorbed photons per NPL in our experiments, we found no signatures of the presence of biexcitons or larger complexes. Biexcitons were only observed due to the interaction of a probe-generated exciton with an exciton produced previously by the pump pulse. For higher pump photon energies, the initial presence of more free charge carriers leads to formation of trions by probe photons. On increasing the number of absorbed pump photons in an NPL, the yield of excitons becomes higher as compared to free charge carriers, since electron-hole recombination becomes more likely. In addition to a TA absorption feature at energy below the HH exciton peak, we also observed a TA signal at the high-energy side of this peak, which we attribute to formation of LH-HH biexcitons or trions consisting of a charge and LH exciton.

Timelike electromagnetic kaon form factor

We compute the electromagnetic charged kaon form factor in the timelike region by employing a Poincar\'e covariant formalism of the Bethe-Salpeter equation to study quark-antiquark bound states in conjunction with the Schwinger-Dyson equation for the quark propagator. Following a recent kindred calculation of the timelike electromagnetic pion form factor, we include the most relevant intermediate composite particles permitted by their quantum numbers in the interaction kernel to allow for a decay mechanism for the resonances involved. This term augments the usual gluon mediated interaction between quarks. For a sufficiently low energy timelike probing photon, the electromagnetic form factor is saturated by the $\ensuremath{\rho}(770)$ and $\ensuremath{\phi}(1020)$ resonances. We assume $SU(2)$ isospin symmetry throughout. Our results for the absolute value squared of the electromagnetic form factor agree qualitatively rather well and quantitatively moderately so with available experimental data.

The Photonic Atom Probe as a Tool for the Analysis of the Effect of Defects on the Luminescence of Nitride Quantum Structures.

By collecting simultaneously optical and chemical/morphological data from nanoscale volumes, the Photonic Atom Probe (PAP) can be applied not only to the study of the relationship between optical and structural properties of quantum emitter but also to evaluate the influence of other factors, such as the presence of point defects, on the photoluminescence. Through the analysis of multiple layers of InGaN/GaN quantum dots (QDs), grown so that the density of structural defects is higher with increasing distance from the substrate, we establish that the light emission is higher in the regions exhibiting a higher presence of structural defects. While the presence of intrinsic point defects with non-radiative recombination properties remains elusive, our result is consistent with the fact that QD layers closer to the substrate behave as traps for non-radiative point defects. This result demonstrates the potential of the PAP as a technique for the study of the optical properties of defects in semiconductors.

Multifunctional one-droplet microfluidic chemosensing of ractopamine in real samples: a user-oriented flexible nano-architecture for on-site food and pharmaceutical analysis using optical sensors.

Illegal use of ractopamine (RAC) in the food industry has dire consequences for health which should be curbed by inexpensive on-site checks. In this study, four advanced nanostructures of AuNPs were examined for this purpose. For the first time, a novel cost-effective colorimetric opto-sensor based on gold nanoparticles in aqueous solution was developed and successfully utilized for the recognition of RAC in real samples. The colorimetric chemosensor based on AuNPs-CysA exhibited a linear range of 0.1 μM to 0.01 M with a limit of detection (LOD) of 0.001 μM. Also, using AuNPs-DDT as a photonic probe two ranges of linearity of 0.01 to 50 μM and 0.005 to 0.01 M were obtained (LOD = 1 nM). The outstanding features of the utilized nanostructures are the simple preparation, the suitable stability of AuNPs-CysA and the excellent selectivity of AuNPs-DDT toward RAC recognition. Finally, the engineered colorimetric systems were combined with a simple and inexpensive optimized microfluidic glass fiber-based device. This work paves the way for devising inexpensive and efficient on-site recognition devices for food safety checks.

Time- and angle-resolved photoemission spectroscopy (TR-ARPES) of TMDC monolayers and bilayers.

Many unique properties in two-dimensional (2D) materials and their heterostructures rely on charge excitation, scattering, transfer, and relaxation dynamics across different points in the momentum space. Understanding these dynamics is crucial in both the fundamental study of 2D physics and their incorporation in optoelectronic and quantum devices. A direct method to probe charge carrier dynamics with momentum resolution is time- and angle-resolved photoemission spectroscopy (TR-ARPES). Such measurements have been challenging, since photoexcited carriers in many 2D monolayers reside at high crystal momenta, requiring probe photon energies in the extreme UV (EUV) regime. These challenges have been recently addressed by development of table-top pulsed EUV sources based on high harmonic generation, and the successful integration into a TR-ARPES and/or time-resolved momentum microscope. Such experiments will allow direct imaging of photoelectrons with superior time, energy, and crystal momentum resolution, with unique advantage over traditional optical measurements. Recently, TR-ARPES experiments of 2D transition metal dichalcogenide (TMDC) monolayers and bilayers have created unprecedented opportunities to reveal many intrinsic dynamics of 2D materials, such as bandgap renormalization, charge carrier scattering, relaxation, and wavefunction localization in moiré patterns. This perspective aims to give a short review of recent discoveries and discuss the challenges and opportunities of such techniques in the future.

Ultrasensitive Optical Rotation Detection With Closed-Loop Suppression of Spin Polarization Error

Optical rotation detection system (ORDS) utilizing quantum nondemolition (QND) measurement methods is widely applied in the field of quantum metrology and quantum information. However, the sensitivity of ORDS is limited by the uncertainty from optical-couple noise during the measurement of the atomic spin ensemble. In this study, we specifically analyze the mechanism of optical-couple noise caused by the fluctuations of probe light’s polarization in the modulated ORDS with a new model established to describe atomic spin precession in this particular condition. It is discovered that transverse electron-spin polarization errors are generated by the residual probe photon spin polarization in the ORDS, which results in extra coupling magnetic noise. In order to suppress this noise, a novel in situ method is proposed that the resultant electron-spin errors are reduced by a specifically designed closed-loop system. The results are verified through the ORDS in a co-magnetometer. After zeroing the extra probe photon spin polarization, an angular sensitivity better than <inline-formula xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink"> <tex-math notation="LaTeX">$1 \times 10 ^{\mathrm {-8}}$ </tex-math></inline-formula> rad/Hz <inline-formula xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink"> <tex-math notation="LaTeX">$^{\mathrm {1/2}}$ </tex-math></inline-formula> is achieved for frequencies higher than 5 Hz, demonstrating a probe background noise of 0.26 fT/Hz <inline-formula xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink"> <tex-math notation="LaTeX">$^{\mathrm {1/2}}$ </tex-math></inline-formula> @14.5 Hz, approaching electronic noise and photon shot noise (PSN). With closed-loop control, the optical rotation bias instability is promoted by 4.2 times (from 107.9 to <inline-formula xmlns:mml="http://www.w3.org/1998/Math/MathML" xmlns:xlink="http://www.w3.org/1999/xlink"> <tex-math notation="LaTeX">$25.7 \mu $ </tex-math></inline-formula> rad/h), and the angular noise of the ORDS is reduced by 2.4 times at 1–100 Hz. The measurement uncertainty of the realized ORDS nears the standard quantum limit, paving the road for long-term ultrasensitive measurements for new physics explorations.