The “charge wave function,” which is the sum of the internal, and semi-internal correlations of the Non-Closed Shell Many-Electron Theory (ncmet) of Sinanoǧlu and co-workers, has been calculated by Sinanoǧlu and Oksuz and more recently by Schaefer and Harris for atomic systems, and for molecules by Das and Wahl, and recently by Schaefer. The results on optical transition probabilities, on hyperfine structures and on molecular pe curves are summarized and the extent of agreement with the initial result of the ncmet theory as given earlier by Sinanoǧlu that the “charge wave function”, a finite ci function, should yield these properties well, and the main features of pe curves, is examined.