Degree Of Polarization Research Articles

Four-dimensional Bell state measurement assisted by polarization and frequency degrees of freedom

Four-dimensional Bell state measurement assisted by polarization and frequency degrees of freedom

Polarized Upconversion of sub-100 nm Single Nanoparticles.

Upconversion nanoparticles are popular as imaging probes due to their advantages in photostability and controllable emission dimensions. However, upconversion polarization remains largely uncharted with previous reports limited to microstructures. In this work, we report the observation of polarized upconversion emissions from β-NaYF4 single nanostructures below 100 nm. At the sub-100 nm scale, nanorods, nanodiscs, and nanoplates exhibit distinctive polarization degrees despite the same doping concentrations of lanthanides. We find this varied polarization degree results from the crystallographic orientation of nanostructure in relation to the light field and can be linked to the distinctive emission spectrum profile with varied Stark splitting transition ratios from Er3+. Our findings provide a comprehensive understanding of the polarization properties of upconversion nanoparticles, revealing a previously unexplored aspect of light emission. This discovery expands our knowledge of upconversion nanoparticles and also opens new possibilities for their use in future imaging and sensing applications, where polarization sensitivity is crucial.

Studying geometry of the ultraluminous X-ray pulsar Swift J0243.6+6124 using X-ray and optical polarimetry

Discovery of pulsations from a number of ultra-luminous X-ray (ULX) sources proved that accretion onto neutron stars can produce luminosities exceeding the Eddington limit by several orders of magnitude. The conditions necessary to achieve such high luminosities as well as the exact geometry of the accretion flow in the neutron star vicinity are, however, a matter of debate. The pulse phase-resolved polarization measurements that became possible with the launch of the Imaging X-ray Polarimetry Explorer (IXPE) can be used to determine the pulsar geometry and its orientation relative to the orbital plane. They provide an avenue to test different theoretical models of ULX pulsars. In this paper we present the results of three IXPE observations of the first Galactic ULX pulsar Swift J0243.6+6124 during its 2023 outburst. We find strong variations in the polarization characteristics with the pulsar phase. The average polarization degree increases from about 5<!PCT!> to 15<!PCT!> as the flux dropped by a factor of three in the course of the outburst. The polarization angle (PA) as a function of the pulsar phase shows two peaks in the first two observations, but changes to a characteristic sawtooth pattern in the remaining data set. This is not consistent with a simple rotating vector model. Assuming the existence of an additional constant polarized component, we were able to fit the three observations with a common rotating vector model and obtain constraints on the pulsar geometry. In particular, we find the pulsar angular momentum inclination with respect to the line of sight of $i_ p the magnetic obliquity of $ p and the pulsar spin position angle of $ p which significantly differs from the constant component PA of about 10 Combining these X-ray measurements with the optical PA, we find evidence for at least a 30 misalignment between the pulsar angular momentum and the binary orbital axis.

Macrophage polarization in human periapical lesions in relation to histopathological diagnosis, clinical features and lesion volume: An exvivo study.

To evaluate M1 and M2 macrophage polarization in radicular cysts and periapical granulomas through an immunohistochemical analysis and the correlation between macrophage polarization and histopathological diagnosis, clinical characteristics and lesion volume using cone-beam computed tomography. Periapical biopsies diagnosed as radicular cysts (n = 52) and periapical granulomas (n = 51) were analysed by immunohistochemical method. Teeth with periapical lesion with no history of root canal treatment (primary lesion) and lesions persistent to root canal treatment (persistent lesions) were included. Pathological diagnosis, patients' age, gender and clinical characteristics were obtained from treatment records. A cone-beam computed tomographic periapical volume index (CBCTPAVI) score was assigned to each periapical lesion based on the volume of the lesion. Immuno-expressions of CD68 and CD163 were quantified. The CD68/CD163 ratio was adopted to represent M1 or M2 macrophage polarization. Mann-Whitney U test was used to determine the different CD68/CD163 ratio between groups of radicular cyst and periapical granuloma. Spearman's correlation test was performed to assess the correlation between the CD68/CD163 ratio and lesion volume and CBCTPAVI score. Radicular cysts and periapical granulomas had CD68/CD163 median of 2.05 (IQR = 1.33) and 1.26 (IQR = 0.81), respectively. A significantly higher CD68/CD163 ratio was observed in radicular cysts (p < .001). In contrast, periapical granulomas had significantly lower median of CD68/CD163 ratio. Larger lesions had a higher median of CD68/CD163 ratio, while smaller lesions had lower median of CD68/CD163 ratio (p = .007, rs = .262). CD68/CD163 ratio was significantly correlated with the CBCTPAVI score in the overall periapical lesions (p = .002, rs = .306). The higher CD68/CD163 ratio in larger lesions indicated a higher degree of M1 polarization compared to smaller lesions. Regarding the pathological diagnosis, there was a significant positive correlation between CBCTPAVI score and CD68/CD163 ratio in periapical granulomas (p < .001, rs = .453), whereas the negative correlation was observed for radicular cysts (p < .001, rs = -.471). Periapical granulomas are characterized by a M2-dominant macrophage polarization, while radicular cysts have significantly higher M1 macrophages. The higher degree of M1 macrophage polarization was significantly correlated with larger volume and higher CBCTPAVI scores of overall periapical lesion and periapical granuloma.

Plasmonic Radiation from Spin-Momentum Locking.

Chiral light emission plays a key role in sensing, tomography, quantum communication, among others. Whereas, achieving highly pure, tunable chirality emission across a broad spectrum currently presents significant challenges. Free-electron radiation emerges as a promising solution to surpass these barriers, especially in hard-to-reach regimes. Here, chiral free-electron radiation is presented by exploiting the spin-momentum locking (SML) property of spoof surface plasmons (SSPs). When the phase velocity of free electrons matches that of the SSPs, the SSPs can be excited. By implementing wavenumber compensation through perturbations, the confined SSPs are transformed into free-space free-electron radiation. Owing to the law of angular momentum conservation, this process converts the transverse spin angular momentum of SSPs into the longitudinal spin angular momentum of free-electron radiation during the process, producing pure, tunable, and chiral free-electron radiation across a broad spectrum. This method achieves an optimal degree of circular polarization approaching -1. The innovative methodology can be adapted to SML-enabled guided states or silicon photonics platforms, offering new avenues for achieving chiral emission.

Silicon-based perovskite plasmonic diode with highly polarized emission

Abstract Here, we propose and develop a silicon (Si)-based perovskite plasmon-emitting diode (PED) with controlled linear polarization in this study. Such polarization originates from the efficient excitation of surface plasmons by excitons in the active layer of the device and the efficient outcoupling by a wedged boundary of a metal electrode. Furthermore, a p-type Si substrate serves as an anode of the diode, and a hole blocking layer of SiO2 is introduced in the PEDOT:PSS/Si heterojunction for carrier injection balance. Pure green emission light has been achieved from devices with varied thicknesses of the emitting layer, and the maximum degree of polarization is measured to be 0.79. The field distribution and polarization of the PED were simulated and measured. Such a low-cost Si-based plasmonic diode provides a promising way to realize simpler and more compact multiple-functional light sources, which are extensively demanded for optoelectronic integration.

Influence of Mixing Valence Band States to the Conduction Band States on Two-Quantum Linear-Circular Dicroism in Semiconductors

A quantitative theory of two-photon linear-circular dichroism caused between the subbands of light and heavy holes of the valence band and conduction band is constructed, which takes into account the admixture of valence band states to the conduction band states and the temperature dependence of the band gap (Eg(T)) in semiconductors of tetrahedral symmetry in the multiband Kane model. It is shown that the type of oscillatory angular dependence or the amplitude values of the probabilities of two-photon optical transitions depend on the state of light polarization. This is due to the fact that, under the influence of linearly polarized light, alignment along the pulse occurs, and under the action of circularly polarized light, the moments of current carriers are oriented. It has been determined that the probability of two-photon optical transitions from the heavy hole subband to the conduction band of semiconductors at a fixed temperature increases with increasing frequency, passes through a maximum, and sharply decreases regardless of the degree of polarization of light, as well as the band gap.

A molecular design strategy to develop all‐organic crosslinked polyetherimide film with high discharged energy density at 150°C

AbstractMiniaturization and lightweight of power systems urgently ask for polymer dielectrics with high discharged energy density at 150°C. Herein, a molecular design strategy is built to prepare new crosslinkable polyetherimide films (PEIDx, x is the molar ratio of dianhydride to amines) through simultaneously improving the polarization degree and reducing the residual polarization. Thermal, mechanical, and dielectric properties of PEIDx improve as x increases. PEID0.92 shows the best integrated performances, especially its discharged energy density (5.46 J cm−3, at 10 Hz and 454 MV m−1) is higher than those of reported polymer dielectrics with discharged energy storage at 150°C, and its charge–discharge efficiency is 80.14%. The outstanding energy storage performance of PEID0.92 is attributed to its unique molecular structure. Specifically, the use of nonplanar and low‐alkaline aliphatic cyclic diamine effectively improves the polarization degree of macromolecules; while the crosslinking of alkynyl groups limits the macromolecular movement, thus ensuring high heat resistance and low residual polarization.

Effect of polarization on spectroscopic characterization of laser produced aluminium plasma

Laser-induced breakdown spectroscopy (LIBS) is a well-established technique widely used in fundamental research and diverse practical fields. Polarization-resolved LIBS, a variant of this technique, aims to improve the sensitivity, which is a critical aspect in numerous scientific domains. In our recent work we demonstrated that the degree of polarization (DOP) in the emission depends on the spatial location and time in a nano second laser generated aluminium plasma1. Present study investigates the effect of polarized emission on the estimation of plasma parameters. The plasma parameters are estimated using the conventional spectroscopic methods such as Boltzmann plot and line intensity ratio for the estimation of electron temperature and Stark broadening for estimating the electron density. The estimated plasma temperature using Boltzmann plot method shows large errors in electron temperature for the locations where DOP is higher. However, the electron density estimated using the Stark width does not show such variation. The observed ambiguity in temperature estimation using the Boltzmann plot method appears to be a consequence of deviation from expected Maxwell Boltzmann distribution of population of the involved energy levels. These findings highlight the need of assessing the DOP of the plasma before selecting the polarization for PRLIBS or temperature estimation using Boltzmann plots in elemental analysis.

Synchrotron polarization with a partially random magnetic field: General approach and application to X-ray polarization from supernova remnants

Context. Diagnostics based on the polarization properties of the synchrotron emission can provide precious information on both the ordered structure and the random level of the magnetic field. While this issue has already been analyzed in the radio band, the polarization data recently obtained by the mission IXPE have shown the need to extend this analysis to the X-ray band. Aims. While our immediate targets are young supernova remnants, the scope of this analysis is wider. Our aim is to extend the analysis to particle energy distributions more complex than a power law, and to investigate a wider range of cases involving a composition of ordered and random magnetic fields. Methods. Since an analytical approach is only possible in a limited number of cases, we devised for this purpose an optimized numerical scheme, and we directly used it to investigate particle energy distributions in the form of a power law with an exponential or super-exponential cutoff. We also considered a general combination of an ordered field plus an anisotropic random component. Results. We show that the previously derived analytic formulae, valid for power-law distributions, may also be good approximations of the polarization degree in the more general case with a cutoff, as typically seen in X-rays. We explicitly analyzed the young supernova remnants SN 1006, Tycho, and Cas A. In particular, for SN 1006 we proved the consistency between the radio and X-ray polarization degrees, favoring the case of a predominantly random field with an anisotropic distribution. In addition, for the power-law case we investigated the effect of a compression on ordered and on random magnetic field components, aimed at describing the mid-age radio supernova remnants. Conclusions. This work allows a more efficient exploitation of radio and X-ray measurements of the synchrotron polarization, and is addressed to present observations with IXPE and to future projects.

A new experimental method to study the flame inhibition performance of low concentration halogenated gas

The minimum fire extinguishing concentration is a key index for the development of next generation chemical clean fire extinguishing gases, which is usually got by the cup-burner. The fire suppression performance of low concentration of chemical gas is hard to be understood by the available methods. In this work, the fundamental acknowledgement of steady flame surface attacking mechanism by halon functional group is newly discussed by conducting a series of bench scale tests with a cylindrical channel under a varied fluorinated gases. The characteristics of flame propagation under differentiated air atmosphere environmental conditions is obtained. The influence of fluorine-containing gas flow rate on flame propagation speed is clarified. A dimensionless relationship including atomic radius, bond length, polarization degree, molar mass and molar volume are proposed to describe the influence of low concentration of fluorine-containing gas on flame propagation speed. It provides an insight for the understanding of the flame inhibition performance of low concentration halogenated gas.

Polarization Study of Swift J151857.0–572147 with IXPE Observation

We present an analysis of the Imaging X-ray Polarimetry Explorer observation from a newly discovered transient source: Swift J151857.0–572147. The obtained polarization degree (PD) and angle are 0.3% ± 0.3% and −24° ± 26° respectively in 2–8 keV within 68% confidence level errors, and polarization results are below MDP99 in all energy bins, with the upper limit on PD of 0.8% in the 2–8 keV energy range. No quasi-periodic oscillations (QPOs) are detected in this observation. The polarization and QPO analyses support the hypothesis that the source was in the high soft state, and the results are consistent with predictions for a thin accretion disk model.

A Multifunctional Nanostructured Hydrogel as a Platform for Deciphering Niche Interactions of Hematopoietic Stem and Progenitor Cells.

For over half a century, hematopoietic stem cells (HSCs) have been used for transplantation therapy to treat severe hematologic diseases. Successful outcomes depend on collecting sufficient donor HSCs as well as ensuring efficient engraftment. These processes are influenced by dynamic interactions of HSCs with the bone marrow niche, which can be revealed by artificial niche models. Here, a multifunctional nanostructured hydrogel is presented as a 2D platform to investigate how the interdependencies of cytokine binding and nanopatterned adhesive ligands influence the behavior of human hematopoietic stem and progenitor cells (HSPCs). The results indicate that the degree of HSPC polarization and motility, observed when cultured on gels presenting the chemokine SDF-1α and a nanoscale-defined density of a cellular (IDSP) or extracellular matrix (LDV) α4β1 integrin binding motif, are differentlyinfluenced on hydrogels functionalized with the different ligand types. Further, SDF-1α promotes cell polarization but not motility. Strikingly, the degree of differentiation correlates negatively with the nanoparticle spacing, which determines ligand density, but only for the cellular-derived IDSP motif. This mechanism potentially offers a means of predictably regulating early HSC fate decisions. Consequently, the innovative multifunctional hydrogel holds promise for deciphering dynamic HSPC-niche interactions and refining transplantation therapy protocols.

GMXPolymer: a generated polymerization algorithm based on GROMACS.

This work introduces a method for generating generalized structures of amorphous polymers using simulated polymerization and molecular dynamics equilibration, with a particular focus on amorphous polymers. The techniques and algorithms used in this method are described in the main text, and example input scripts are provided for the GMXPolymer code, which is based on the GROMACS molecular dynamics package. To demonstrate the efficacy of our method, we apply it to different glassy polymers exhibiting varying degrees of functionality, polarity, and rigidity. The reliability of the method is validated by comparing simulation results with experimental data in various structural and thermal properties, both of which show excellent agreement. This work implements the GMXPolymer simulated polymerization algorithm on the GROMACS program. GMXPolymer code controls the main polymerization loop. The energy minimizations and molecular dynamics simulations use the GROMACS program called by the GMXPolymer code. A new ITP file is generated when a new bond is formed, and the necessary additions to the ITP file are made to include new bonds, angles, and dihedrals. In preparing the ITP file of the monomer, the charge of the reactive atom must be modified before the code runs so that it is a correct value after bonding.

Understanding the multi-wavelength thermal dust polarisation from the Orion molecular cloud in light of the radiative torque paradigm

Dust grains play a key role in various astrophysical processes and serve as indicators of interstellar medium structures, density, and mass. Understanding their physical properties and chemical composition is a crucial goal in astrophysics. Dust polarisation is a valuable tool for studying these properties. The radiative torque (RAT) paradigm, which includes radiative torque alignment (RAT-A) and radiative torque disruption (RAT-D), is essential to interpreting the dust polarisation data and constraining the fundamental properties of dust grains. However, it has been used primarily to interpret observations at a single wavelength. In this study, we analyse the thermal dust polarisation spectrum obtained from observations with SOFIA/HAWC+ and JCMT/POL-2 in the Orion molecular cloud 1 (OMC-1) region and compare the observational data with our numerical results using the RAT paradigm. In general, we show that the dense gas exhibits a positive spectral slope, whereas the warm regions show a negative one. We demonstrate that a one-layer dust (one-phase) model can only reproduce the observed spectra at certain locations and cannot match those with prominent V-shaped spectra (for which the degree of polarisation initially decreases with wavelength from 54 to ~300µm and then increases at longer wavelengths). To address this, we improved our model by incorporating two dust components (warm and cold) along the line of sight, resulting in a two-phase model. This improved model successfully reproduces the V-shaped spectra. The best model corresponds to a mixture composition of silicate and carbonaceous grains in the cold medium. Finally, by assuming the plausible model of grain alignment, we were able to infer the inclination angle of the magnetic fields in OMC-1. This approach is an important step towards a better understanding the physics of grain alignment and constraining 3D magnetic fields using dust polarisation spectra.

Rotation of Polarization Angle in Gamma-Ray Burst Prompt Phase. II. The Influence of the Parameters

In addition to the light curve and energy spectrum, polarization is also important for inferring the physical properties of the gamma-ray burst (GRB). Rotation of the polarization angle (PA) with time will cause depolarization of the time-integrated polarization degree. However, it has rarely been studied before. Here, we use a magnetic reconnection model with a large-scale ordered aligned magnetic field in the emitting region to study the influence of the parameters on the PA rotations in the GRB prompt phase. We find that the half-opening angle of the jet θ j , the observational angle θ V , and the bulk Lorentz factor Γ all have significant impacts on the PA rotations. The PA rotations are affected by the product value of θ j Γ0 (Γ0 is the normalization factor of Γ with Γ(r)=Γ0(r/r0)s ), but are roughly independent of the concrete values of both θ j and Γ0. For the typical parameters, the changes of the PA within T 90 (△PA) would be within (12°, 66°) for slight off-axis observations, where T 90 is the duration of the burst with the accumulated flux density ranging from 5% to 95%. The q range for △PA > 10° becomes smaller with the increase of the product value of θ j Γ0. The most significant PA rotation with △PA ∼ 90° will happen when θ j Γ0 > 50 and 1.0 < q ≤ 1.2.

Polarized luminescence of bound excitons in Cu2O single crystal

Photoluminescence was studied for Cu2O (100) single crystal in the 1.2–1.9 eV spectral range under polarized laser excitation 532 nm at low temperature. Polarized luminescence and negative thermal quenching were detected for the emission bands at 1.34, 1.53 and 1.7 eV, assigned to the bound excitons localized at copper vacancies VCu and oxygen vacancies VO+, VO2+, correspondingly. The complex structure of the most intense emission bands 1.34 and 1.7 eV containing spectrally shifted orthogonally polarized subbands was identified. Luminescence polarization degree, intensity and spectral position of the subbands depend on temperature as well as on the excitation light density and vary from point to point. The origin of the polarized luminescence and negative thermal quenching of the bound excitons in Cu2O crystal is discussed.

X-ray polarization measurement of the gold standard of radio-quiet active galactic nuclei: NGC 1068

Context. NGC 1068 is the most observed radio-quiet active galactic nucleus (AGN) in polarimetry, yet its high-energy polarization has never been probed before due to a lack of dedicated polarimeters. Aims. Using the first X-ray polarimeter sensitive enough to measure the polarization of AGNs, we want to probe the orientation and geometric arrangement of (sub)parsec-scale matter around the X-ray source. Methods. We used the Imaging X-ray Polarimetry Explorer (IXPE) satellite to measure, for the first time, the 2–8 keV polarization of NGC 1068. We pointed IXPE at the target for a net exposure time of 1.15 Ms, in addition to using two Chandra snapshots of ∼10 ks each in order to account for the potential impact of several ultraluminous X-ray sources (ULXs) within IXPE’s field of view. Results. We measured a 2–8 keV polarization degree of 12.4% ± 3.6% and an electric vector polarization angle of 101° ± 8° at a 68% confidence level. If we exclude the spectral region containing bright Fe K lines and other soft X-ray lines where depolarization occurs, the polarization fraction rises to 21.3% ± 6.7% in the 3.5–6.0 keV band, with a similar polarization angle. The observed polarization angle is found to be perpendicular to the parsec-scale radio jet. Using a combined Chandra and IXPE analysis plus multiwavelength constraints, we estimated that the circumnuclear “torus” may sustain a half-opening angle of 50–55° (from the vertical axis of the system). Conclusions. Thanks to IXPE, we have measured the X-ray polarization of NGC 1068 and found comparable results, both in terms of the polarization angle orientation with respect to the radio jet and the torus half-opening angle, to the X-ray polarimetric measurement achieved for the other archetypal Compton-thick AGN: the Circinus galaxy. Probing the geometric arrangement of parsec-scale matter in extragalactic objects is now feasible thanks to X-ray polarimetry.

A robust underwater polarization image recovery based on Angle of Polarization with low-rank and sparse decomposition

Underwater imaging method based on the Angle of Polarization (AoP) is extremely popular due to its ability to remove the backscattered light effectively. However, existing methods overlook a potentially important phenomenon: the AoP contains significant noise in the real world, which leads to inaccurate estimations of key parameters. In this study, we propose a novel robust underwater polarization image recovery method based on AoP with low-rank and sparse decomposition. Based on the analysis of polarization, the AoP of backscattering exhibits low-rank characteristics, whereas the AoP of noise and targets demonstrates sparsity. Considering different sparsity of AoP, we combine Robust Principal Component Analysis and Alternating Direction Multiplier Method (RPCA-ADMM) with an adaptive threshold shrinkage method for low-rank and sparse decomposition, the AoP of the backscattering is obtained. Moreover, according to the low-rank component of the AoP, the Degree of Linear Polarization (DoLP) of backscattering can be effectively and automatically estimated without considering whether the background region exists, relying on a frequency prior strategy. Finally, the degraded image is recovered utilizing underwater polarization imaging model. Extensive experimental results demonstrate that the recovered images from the proposed method have abundant detail, high contrast, and minimal color distortion, which is competitive with most state-of-the-art methods.

Coherent Inverse Compton Scattering in Fast Radio Bursts Revisited

Growing observations of temporal, spectral, and polarization properties of fast radio bursts (FRBs) indicate that the radio emission of the majority of bursts is likely produced inside the magnetosphere of its central engine, likely a magnetar. We revisit the idea that FRBs are generated via coherent inverse Compton scattering (ICS) off low-frequency X-mode electromagnetic waves (fast magnetosonic waves) by bunches at a distance of a few hundred times the magnetar radius. The following findings are revealed: (1) Crustal oscillations during a flaring event would excite kHz Alfvén waves. Fast magnetosonic waves with essentially the same frequency can be generated directly or be converted from Alfvén waves at a large radius, with an amplitude large enough to power FRBs via the ICS process. (2) The cross section increases rapidly with radius and significant ICS can occur at r ≳ 100R ⋆ with emission power much greater than the curvature radiation power but still in the linear scattering regime. (3) The low-frequency fast magnetosonic waves naturally redistribute a fluctuating relativistic plasma in the charge-depleted region to form bunches with the right size to power FRBs. (4) The required bunch net charge density can be sub-Goldreich–Julian, which allows a strong parallel electric field to accelerate the charges, maintain the bunches, and continuously power FRB emission. (5) This model can account for a wide range of observed properties of repeating FRB bursts, including high degrees of linear and circular polarization and narrow spectra as observed in many bursts from repeating FRB sources.