Plasma Filaments Research Articles

Fluorescence and lasing of neutral nitrogen molecules inside femtosecond laser filaments in air: mechanism and applications.

High power femtosecond laser pulses launched in air undergo nonlinear filamentary propagation, featuring a bright and thin plasma channel in air with its length much longer than the Rayleigh length of the laser beam. During this nonlinear propagation process, the laser pulses experience rich and complex spatial and temporal transformations. With its applications ranging from supercontinuum generation, laser pulse compression, remote sensing to triggering of lightning, the underlying physical mechanism of filamentation has been intensively studied. In this review, we will focus on the fluorescence and cavity-free lasing effect of the plasma filaments in air. The different mechanisms underlying the fluorescence of the excited neutral nitrogen molecules will be throughly examined and it is concluded that the electron collision excitation is the dominant channel for the formation of the excited nitrogen molecules. The recently discovered "air lasing" effect, a cavity-free bidirectional lasing emission emitted by the filaments, will be introduced and its main properties will be emphasized. The applications of the fluorescence and lasing effect of the neutral nitrogen molecules will be introduced, with two examples on spectroscopy and detection of electric field. Finally, we discuss the quenching effect of the lasing effect in atmosphere and the mechanisms responsible will be analyzed. An outlook for the achievement of backward lasing in air will be briefly presented.

Unified framework for terahertz radiation from a single- or two-color plasma filament.

The plasma filament induced by photo-ionization in transparent media (e.g., air) is a competitive terahertz (THz) source, whose mechanism has been widely studied in two separate schemes, i.e., the one- or two-color femtosecond laser filamentation. However, the physical commonality of these two schemes is less explored currently, and a common theory is in urgent need. Here, we proposed the traveling-wave antenna (TWA) model applicable to both single- and dual-color laser fields, which successfully reproduced the reported far-field THz angular distribution/dispersion from different filament lengths with either a constant or a varied plasma density. This work paves the way toward a deeper understanding of the important laser-filament-based THz sources within the same theoretical framework.

Local measurement of terahertz field-induced second harmonic generation in plasma filaments

The concept of Terahertz Field-Induced Second Harmonic (TFISH) Generation is revisited to introduce a single-shot detection scheme based on third order nonlinearities. Focused specifically on the further development of THz plasma-based sources, we begin our research by reimagining the TFISH system to serve as a direct plasma diagnostic. In this work, an optical probe beam is used to mix directly with the strong ponderomotive current associated with laser-induced ionization. A four-wave mixing (FWM) process then generates a strong second-harmonic optical wave because of the mixing of the probe beam with the nonlinear current components oscillating at THz frequencies. The observed conversion efficiency is high enough that for the first time, the TFISH signal appears visible to the human eye. We perform spectral, spatial, and temporal analysis on the detected second-harmonic frequency and show its direct relationship to the nonlinear current. Further, a method to detect incoherent and coherent THz inside plasma filaments is devised using spatio-temporal couplings. The single-shot detection configurations are theoretically described using a combination of expanded FWM models with Kostenbauder and Gaussian Q-matrices. We show that the retrieved temporal traces for THz radiation from single- and two-color laser-induced air-plasma sources match theoretical descriptions very well. High temporal resolution is shown with a detection bandwidth limited only by the spatial extent of the probe laser beam. Large detection bandwidth and temporal characterization is shown for THz radiation confined to under-dense plasma filaments induced by < 100 fs lasers below the relativistic intensity limit.Graphical

Weibel-like instability in magnetohydrodynamics

In magnetohydrodynamics (MHD), a density perturbation perpendicular to an electron temperature gradient generates a magnetic field around itself that acts to increase the perturbation, which can lead to instability. An MHD dispersion relation is obtained for perturbations perpendicular to a fixed electron temperature gradient with an initial in-plane magnetic field, including resistivity, viscosity, and the electrothermal coefficient. Instability occurs for sufficiently small electron temperature-gradient scale lengths determined by the ion collisionless skin depth. Both viscosity and resistivity are required to prevent growth at arbitrarily small spatial scales and to give a physical result for the fastest growing mode. The perpendicular electrothermal coefficient is only significant for a narrow range of low electron Hall parameters, causing a modest reduction in magnetic field growth and modifying the criteria for instability in the presence of viscosity. If the definition of the Weibel instability [E. S. Weibel, Phys. Rev. Lett. 2, 83 (1959)] is extended to include all instabilities due to anisotropy in the electron velocity distribution, then this is a Weibel-like instability because an electron temperature gradient implies an anisotropic electron velocity distribution. The implications for the formation of filaments in laser-produced plasmas and for the verification of MHD codes are considered.

Coherence of turbulent structures with varying drive in stellarator edge plasmas

This work investigates the parallel coherence of plasma filaments through numerical simulations using the hot-ion two-fluid hermes-2 model within the BOUT++ framework. Realistic field lines in the scrape-off layer (SOL) of magnetic fusion devices, especially in stellarator configurations possess a highly varying curvature along the magnetic field line. A varying curvature creates a parallel velocity gradient which might tear the filament apart. The main parameters controlling this process are the collisionality and the electron plasma beta. Simulations of realistic curvature variations along field lines in a circular ASDEX Upgrade-like tokamak and Wendelstein 7-X stellarator (W7-X) show the parallel displacement between different filament sections to correlate with the curvature. The rapidly varying W7-X curvature and the low average curvature drive reduce the propagation of the filament to only a few hundred meters per second. The effect of a finite ion temperature on filament propagation in a W7-X field line geometry is found to be a higher diamagnetic current resulting in stronger charge separation. This work supports simulations and experimental findings that filaments in W7-X are comparably slow due to the large major radius of the device. They do not perform ballistic motion and hence do not drive significant turbulence spreading in the SOL.

Statistical analysis of plasma filaments in the island divertor of Wendelstein 7-X

Plasma filaments have been measured with alkali beam emission spectroscopy in the plasma edge, divertor island, and scrape-off layer of Wendelstein 7-X. Due to the high intensity of a 1–2 kHz plasma mode, a new, correlation based conditional averaging algorithm was used to search for filaments in the signals. With that method, effects of different magnetic configurations and density levels on filament properties are observed. In configurations where the islands are small and do not play an important role for the connection length topology, filaments behave similar to tokamaks. In contrast, in configurations with larger magnetic islands and more complex connection length profiles, filaments behave quite differently, for instance they may or may not appear in the inner side of the divertor island depending on the plasma parameters. Coupling between the filaments and lower frequency events are also showed. The role of filaments in the global and local particle transport is briefly discussed.

Hermes-3: Multi-component plasma simulations with BOUT++

A new open source tool for fluid simulation of multi-component plasmas is presented, based on a flexible software design that is applicable to scientific simulations in a wide range of fields. Hermes-3 is built on plasma simulation framework BOUT++, consolidating earlier SD1D and Hermes models into a single code that can be configured at run-time to solve plasma models in 1D, 2D or 3D, either for transport (steady-state) or turbulent (time-evolving) problems, with an arbitrary number of ion and neutral species. We describe the improved numerical algorithms and software design that have been implemented in Hermes-3.To demonstrate the capabilities of this tool, applications relevant to the boundary of tokamak plasmas are presented: 1D simulations of diveror plasmas evolving equations for all charge states of neon and deuterium; 2D transport simulations of tokamak equilibria in single-null X-point geometry with plasma ion and neutral atom species; and simulations of the time-dependent propagation of plasma filaments (blobs).Hermes-3 is publicly available on Github under the GPL-3 open source license. The repository includes documentation and a suite of unit, integrated and convergence tests. Program summaryProgram Title: Hermes-3CPC Library link to program files:https://doi.org/10.17632/rtkvc3r743.1Developer's repository link:https://github.com/bendudson/hermes-3Licensing provisions: GPLv3Programming language: C++14Nature of problem: Simulation of dynamics and steady-state solutions of multiple ion and neutral species in magnetised plasmas using drift-reduced fluid plasma models in 1 to 3 spatial dimensions. Focused on but not restricted to the simulation of turbulence in the boundary of tokamaks.Solution method: Hermes-3 implements a system of flexible software components, that are configured at run-time and coupled by passing a state object between them (the Encapsulate State and Command patterns). Hermes-3 builds on BOUT++ [1], employing the Method of Lines with implicit and explicit time-integration methods in curvilinear coordinates on block-structured meshes, making use of libraries including SUNDIALS, PETSc and Hypre. Hermes-3 implements drift-reduced plasma fluid equations using conservative finite difference methods, and atomic processes that couple plasma and neutral fluids.

Spectral tuning of broadband terahertz radiation from dc-biased laser plasma filaments

Terahertz radiation from laser plasmas exhibits a broadband spectrum, making it a bright prospect for terahertz spectroscopy. In this work, we demonstrate that the continuous redshift of terahertz radiation from a dc-biased plasma filament can be achieved by increasing the length of the plasma filament. A theoretical model concerning a Lorentz distribution of the plasma density along a filament is proposed to interpret this spectral tuning effect. This finding provides not only an approach to spectral tuning but also a gentle way of diagnosing the distribution of the plasma density inside such plasmas.

Non-equilibrium aerodynamics between ionization-wave and shock-wave fronts in millimetre-wave supported detonation

A shock wave driven by discharge plasma propagating in a high-power millimetre-wave beam was investigated both experimentally and numerically. A shadowgraph experiment was used to visualize the shock wave and plasma. The ionization wave front of the plasma preceded the shock wave by 2.0–4.0 mm under conditions of 170 GHz beam frequency, atmospheric pressure, and 1.1 GW m−2 peak power density (power density at the beam axis). Furthermore, a two-dimensional computational fluid dynamics (CFD) simulation considering non-equilibrium temperatures and filamentary plasma structures revealed that an ionization-wave front precedes a shock wave front because the energy relaxation requires a few micro-seconds from vibrational excitation at a plasma front to translational excitation for the shock wave formation. Consequently, the distance between an ionization wave front and shock wave front is 3.8 mm in the two-dimensional CFD simulation, which agreed with the experimental results.

Surface Dielectric Barrier Discharge (sDBD) for Flow Control in Plasma Conversion

Dielectric barrier discharges (DBD) are often used for gas conversion, such as carbon dioxide splitting, volatile organic compound removal or ozone generation. Due to the tiny plasma filaments in DBD discharges, efficient mixing of the gas flow with the plasma is essential. This is studied by using a surface dielectric barrier discharge (sDBD) with an electrode design similar to plasma actuators to optimize plasma-flow interaction. The flow pattern has been measured by Schlieren diagnostics and compared to a fluid dynamic simulation. Gas conversion efficiency has been tested by monitoring the conversion of 0.7% CO2\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$_2$$\\end{document} admixed to an N2\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$_2$$\\end{document} gas stream via infrared spectroscopy in the exhaust. The actuator design of the electrodes induces a significant plasma force on the fluid, which results in the formation of vortices above the electrodes, as reproduced in the simulation. It is shown that the height of the vortices created in the velocity field can characterize the mixing process, which dominates the conversion efficiency of carbon dioxide at different gas flow rates.

How pulse energy affects ignition efficiency of DBD plasma-assisted combustion

This work aims to find how coupled energy per pulse influences the ability of a pulsed dielectric barrier discharge (DBD) plasma to ignite fuel-lean methane–air flow. For that, experiments are performed on a custom-built DBD flow reactor with a variable dielectric thickness and the discharge is operated by bursts of 10 ns duration pulses at 3 kHz repetition rate. With an increase in dielectric thickness, we observe that the coupled energy per pulse decreases even though applied voltage conditions are similar and so more pulses are required to ignite the lean mixture. Interestingly, we observe a significant increase in the minimum ignition energy (MIE) with an increase in the thickness beyond 3 mm. Moreover, the ignition kernel growth rate is much slower in the thicker dielectric cases even though total energy coupling per burst is similar. This phenomenon is investigated further by evaluating plasma parameters using electrical and optical diagnostics. Effective dielectric capacitance, discharge current, and voltage drop across the gas gap are derived from an equivalent circuit analysis, whereas plasma gas temperature and effective reduced electric field ( E/N ) are estimated from optical emission spectroscopy. From these analyses, we conclude that a thicker dielectric limits the discharge current and so the plasma filament temperature. For more than 3 mm thick dielectric cases, the filament heating per pulse is too low to achieve strong enough plasma pulse-to-pulse coupling which eventually leads to higher MIE and slower ignition kernel growth rate or the inability to ignite at all.

A Simulation of Air Lasing Seeded by an External Wave in a Femtosecond Laser Filament.

Air lasers induced by femtosecond laser filaments play an important role in remote sensing applications. Few studies have been dedicated to the spatial distribution of external-seeded air laser radiation in the laser filament based on the numerical simulation method, which can pave the way to understanding the mechanism of the external-seeded air lasing process during filamentation. In this study, numerical simulations of the propagation of an air laser seeded by an external plane wave with a wavelength of 391 nm during femtosecond laser filamentation were performed. The results indicated that the air laser's beam intensity distribution varies from a ring pattern to a donut pattern when the filament length and nitrogen ion density are raised as a result of the defocusing and lasing effects of the filament plasma. Here, the ring pattern is formed by several thin rings, while the donut pattern refers to a notably thicker, ring-like structure. In addition, it has been demonstrated that the air laser's beam power would increase exponentially versus the filament length and the nitrogen ion density. The knowledge about the angular distribution of air lasing could be important for optimizing the detection geometry of the LIDAR setup, including the view angle and the size of the collecting optical component.

Light-guiding-light-based temporal integration of broadband terahertz pulses in air

The next generation of all-optical computation platforms prefers the light-guiding-light (LGL) scheme inside a medium that envisions circuitry-free and rapidly reconfigurable systems powered by dynamic interactions between light beams. Currently, suitable LGL materials and corresponding mechanisms are in urgent need. In this work, we proposed ubiquitous air as a restorable LGL signal manipulation medium with transient air-plasma waveguide circuits. Briefly, by focusing femtosecond laser beams in free space, the created atmospheric plasma filament array via photoionization was able to guide terahertz (THz) pulses along its epsilon-near-zero zone with a 1/f-profile spectral response. Consequently, this achieved a time-domain integration of the THz pulse in broad bandwidth. When the pumping laser was sequentially turned off and on, this air-plasma multi-filament structure was erased and rebuilt within nano- and femto-seconds, respectively, allowing rapid and repeated rearrangements of the all-optical stage. Furthermore, this air-based LGL information processing approach is promising to pave the way toward all-optical calculations during free-space directional transmission of THz waves, in which way the delivered THz signal can be remotely controlled.

Unimodal distribution of terahertz emission from single-color filament plasma

We study the angular distributions of various spectral components of terahertz radiation generated in an air plasma of a single-color filament with a laser wavelength of 930 nm. It is experimentally shown that at a 20-fold excess over the critical power for self-focusing the distribution of terahertz radiation at all studied frequencies is unimodal. The obtained pattern differs significantly from the angular distribution of terahertz radiation observed in the case of filamentation of pulses with a shorter wavelength.

Two-dimensional reconstruction of filament temperatures and densities with the thermal helium beam at ASDEX Upgrade

In the scrape-off layer (SOL) of fusion plasmas, radial particle and energy transport is mainly carried by plasma filaments. The plasma parameters of such filaments can be measured by the thermal helium beam diagnostic (THB). By means of an extended collisional radiative model (CRM) used for the evaluation of the diagnostic data, the light intensity response of neutral helium transitions from filaments is studied, which depends on the parameters of the filament and the background. The electron density of the filament is found to be the dominant parameter impacting the line intensities. By applying a numerical reconstruction algorithm based on the CRM, electron temperatures and densities as well as the sizes of experimentally measured filaments are obtained. This method allows for the first time measurements of the temporal decay rates of filament density and temperature in the co-moving frame of the filament and its radial propagation velocity.

High-speed imaging reveals the dynamics of the initiation and subsequent evolution of a nanosecond discharge propagating along the air–water interface

A nanosecond DBD-like discharge in a coplanar electrode configuration propagating along the water–air interface is an efficient source of reactive species to produce plasma-activated water. In this letter, we report on the mechanism of the discharge onset as well as on further developments over hundreds of nanoseconds. We combined ultrafast optical imaging with electrical characteristics to capture basic morphological imprints of individual discharge phases occurring during a single discharge event with high temporal resolution. We show that during the first nanoseconds, a diffuse bi-directional ionizing avalanche expands over the liquid surface at high speed (>5 105 m s−1). Later, discrete plasma filaments form from the diffuse plasma due to an ionization instability. The filaments, during their subsequent elongation (∼2 105 m s−1), retain the diffuse plasma at both ends. The filaments re-ignite in the same positions on the liquid surface over several successive (mainly capacitive) current pulses (∼1 μs apart), which result from discontinuities in the driving voltage.

Air-laser-based coherent Raman spectroscopy of atmospheric molecules in a filamentary plasma grating.

Coherent Raman spectroscopy (CRS) with air-laser-based hybrid femtosecond/picosecond (fs/ps) pulses has shown promising potential for remote detection and surveillance of atmospheric species with high temporal and frequency resolution. Here, to enhance the sensitivity and extend the detection distance, we generate the CRS spectra of air molecules in situ in a filamentary plasma grating, and show that the grating can efficiently enhance the intensities of the coherent vibrational Raman lines of N2, O2, and N2 + by 2-3 orders of magnitude at an extended distance. By examining the intensities of the Raman lines, fs-pulsed supercontinuum, and ps-pulsed air laser produced under different grating conditions, we reveal that the optimization of the Raman lines is achieved by the dynamic balance between the supercontinuum-induced vibrational coherence and air-laser-induced polarization of the air species.

Terahertz Radiation from Two-Color Laser-Induced Gas Plasma Filament Under a Wide Range of Pressure

Terahertz Radiation from Two-Color Laser-Induced Gas Plasma Filament Under a Wide Range of Pressure

ATP modulation of osmotically activated anionic current in the membrane of Phycomyces blakesleeanus sporangiophore

Ion channels are vital components of filamentous fungi signaling in communication with their environment. We exploited the ability of the apical region of growing sporangiophores of Phycomyces blakesleeanus to form membrane-enveloped cytoplasmic droplets (CDs), to examine ion currents in the filamentous fungi native plasma membrane. In hypoosmotic conditions, the dominant current in the CDs is ORIC, an osmotically activated, anionic, outwardly rectified, fast inactivating instantaneous current that we have previously characterized. Here, we examined the effect of ATP on ORIC. We show that CDs contain active mitochondria, and that respiration inhibition by azide accelerates ORIC inactivation. ATP, added intracellularly, reduced ORIC run-down and shifted the voltage dependence of inactivation toward depolarized potentials, in a manner that did not require hydrolysis. Notably, ATP led to slowing down of ORIC inactivation, as evidenced by an increased time constant of inactivation, τin, and slower decline of τin during prolonged recordings. Flavonoids (genistein and quercetin) had the effect on ORIC opposite to ATP, acting as current inhibitors, possibly by disrupting the stabilizing effect of ATP on ORIC. The integration of osmotic sensing with ATP dependence of the anionic current, typical of vertebrate cells, is described here for the first time in filamentous fungi.

Generation of rf radiation by low-intensity laser pulse trains in air.

In this paper, we analyze and numerically simulate mechanisms for generating directed rf radiation by a low-intensity laser pulse train (LPT) propagating in air. The LPT ionizes the air, forming a plasma filament. The ionization process relies on the background level of radioactivity which plays an important role in initiating a collisional ionization process. In our model a low-intensity LPT photoionizes background negative ions (produced by ambient ionizing radiation) and provides the seed electrons necessary to initiate collisional ionization. The intensity of the LPT is far below tunneling ionization levels. The ponderomotive forces associated with the LPT and self-fields drive plasma oscillations predominately in the radial direction. The driven radial electron currents in turn generate directed rf radiation. As the plasma density builds up on axis, the later portion of the LPT can defocus and limit the interaction length. The spectrum of the rf radiation consists of the fundamental frequency associated with the pulse separation time as well as harmonics. The rf generation mechanism is analyzed using fluid equations which incorporate, among other things, the effects of background radioactivity, photoionization, collisional ionization, ponderomotive and space-charge effects, and electron attachment-recombination processes. As an example, for a specific set of parameters, the rf spectrum and intensity are compared to experimental data.