Photonic Quantum Information Technology Research Articles

Photoluminescence of Monolayer WSe2 Enhanced by the Exciton Funnel Effect and the Interfacial Carrier Tunneling Effect When Integrated with 3D Si Wrinkled Structures

Quantum optics and photonic quantum-information technologies require emitters that have good stability and brightness, coupled with fabrication scalability and on-chip integrability. Most quantized emitters are presently based on 1D and 3D sources. Recently, monolayer transition metal dichalcogenides (TMDCs) hosting spatially localized excitons with narrow linewidths have garnered great interest. Advantages such as large binding energies and long room-temperature lifetimes of intralayer excitons suggest that TMDCs are promising candidates for use in optical devices. Here, we propose an emitter based on a 2D WSe2 semiconductor monolayer integrated with a periodic 3D Si-based wrinkled pattern. Carriers confined within the wrinkled pattern can be electrically and optically pumped, and funneled, to boost emission from the 2D WSe2 layer. This in turn acts as a monochromated quantum light source for the Si or any Si-based quantum optic and photonic information technologies. The brightness of the emission is enhanced by a factor greater than 40 compared with monolayer WSe2 on conventional flat SiGe. Moreover, these monolayer 2D/3D semiconductor composite heterostructures are fully scalable and promisingly efficient chip-integrated emitters.

Theoretical investigation of multiplexed quantum light source in fiber ring cavities with oscillating dispersion

Correlated photon pairs are the core resources for photonic quantum information technology. Multiplexed quantum light sources can appreciably improve the efficiency of quantum information processing. Here, we develop a coupled-mode mean-field model and its corresponding semiclassical theory analysis to investigate the multiple parametric-gain sidebands in dispersion-oscillation fiber-ring cavities. We present a cycle transfer matrix method to give the analytic expressions for parametric gain. From this, we can reach a physical insight, that is additional degree of freedom introduced by the modulation along fiber length is responsible for the multiple parametric-gain sidebands, where the underlying mechanism is the quasi-phase matching of four-wave mixing. Two twin signal and idler photons generated from parametric-gain sidebands are appreciably of frequency and temporal correlation, revealing promising applications in frequency-multiplexed photon pair sources. When we construct an optical cavity with spliced single mode fiber and dispersion shifted fibers, numerous parametric-gain sidebands grow in the vicinity of zero group-velocity-dispersion wavelengths of two fibers, i.e., 1310 nm and 1550 nm, both corresponding to low transmission loss windows of fibers. Therefore, frequency-multiplexed quantum light sources established on dispersion-oscillation fiber-ring cavities have the advantages in economy, remote transmission, scalability and compatibility with fiber communication network. Our work offers inspiration for the development of a multiplexed quantum light source.

Quantum confinement effects on the structural and optical properties of nanostructured tin oxide powder

Nanostructured Tin oxide powders, prepared by chemical precipitation method, exhibit interesting structural and optical properties at nanoscale dimensions. Structural characterization confirmed the formation of pure nanostructured SnO2 powders with average crystalline grain size of 54.4[Formula: see text]nm calculated with relative uncertainty of 1.62%. The optical properties of nanoSnO2 powder performed by using transmittance and photoluminescence measurements reveal high transparency and multi-photon emissions in visible and ultraviolet regions. The different photon emissions are attributed to radiative transitions via oxygen vacancies, Sn interstitials, Sn substitutional and dangling bonds. The lower wavelength value corresponded to the absorption edge peak indicating the good quantum confinement of nanostructured SnO2 powder. The larger optical band gap, calculated through transmittance measurements, confirms the quantum confinement effects. The presence of quantum confinement and native point defects in nanostructured SnO2 powders can contribute to enhancing photon emissions process. This result may offer inherent advantages over conventional materials for photonic quantum information technology. The sustained photon emission at room temperature, indicates that SnO2 nanoparticles could be useful in room temperature quantum computing and can maintain the delicate quantum states required for computation at higher temperatures.

Quantum dots for photonic quantum information technology

The generation, manipulation, storage, and detection of single photons play a central role in emerging photonic quantum information technology. Individual photons serve as flying qubits and transmit the relevant quantum information at high speed and with low losses, for example between individual nodes of quantum networks. Due to the laws of quantum mechanics, the associated quantum communication is fundamentally tap-proof, which explains the enormous interest in this modern information technology. On the other hand, stationary qubits or photonic states in quantum computers can potentially lead to enormous increases in performance through parallel data processing, to outperform classical computers in specific tasks when quantum advantage is achieved. In this review, we discuss in depth the great potential of semiconductor quantum dots in photonic quantum information technology. In this context, quantum dots form a key resource for the implementation of quantum communication networks and photonic quantum computers, because they can generate single photons on demand. Moreover, these solid-state quantum emitters are compatible with the mature semiconductor technology, so that they can be integrated comparatively easily into nanophotonic structures such as resonators and waveguide systems, which form the basis for quantum light sources and integrated photonic quantum circuits. After a thematic introduction, we present modern numerical methods and theoretical approaches to device design and the physical description of quantum dot devices. We then introduce modern methods and technical solutions for the epitaxial growth and for the deterministic nanoprocessing of quantum devices based on semiconductor quantum dots. Furthermore, we highlight the most promising device concepts for quantum light sources and photonic quantum circuits that include single quantum dots as active elements and discuss applications of these novel devices in photonic quantum information technology. We close with an overview of open issues and an outlook on future developments.

Deterministic Quantum Light Arrays from Giant Silica-Shelled Quantum Dots.

Colloidal quantum dots (QDs) are promising candidates for single-photon sources with applications in photonic quantum information technologies. Developing practical photonic quantum devices with colloidal materials, however, requires scalable deterministic placement of stable single QD emitters. In this work, we describe a method to exploit QD size to facilitate deterministic positioning of single QDs into large arrays while maintaining their photostability and single-photon emission properties. CdSe/CdS core/shell QDs were encapsulated in silica to both increase their physical size without perturbing their quantum-confined emission and enhance their photostability. These giant QDs were then precisely positioned into ordered arrays using template-assisted self-assembly with a 75% yield for single QDs. We show that the QDs before and after assembly exhibit antibunching behavior at room temperature and their optical properties are retained after an extended period of time. Together, this bottom-up synthetic approach via silica shelling and the robust template-assisted self-assembly offer a unique strategy to produce scalable quantum photonics platforms using colloidal QDs as single-photon emitters.

Generation of polarization entanglement via the quantum Zeno effect.

The quantum Zeno effect reveals that continuous observation of a quantum system can significantly alter its evolution. Here, we present a method for establishing polarization entanglement between two initially unentangled photons in coupled waveguides via the quantum Zeno effect. We support our analytical investigation with numerical simulations of the underlying Schrodinger equation describing the system. Further, we extend our technique to three coupled waveguides in a planar configuration and determine the parameters required to generate three-qubit W-states. In contrast to existing schemes based on a vacuum and single-photon encoding, the polarization encoding in our approach is compatible with quantum information protocols that remove photon loss through post-selection. Our findings offer a powerful quantum state engineering approach for photonic quantum information technologies.

Temporal shaping of single photons by engineering exciton dynamics in a single quantum dot

The majority of photonic quantum information technologies rely on single photons that have high purity and indistinguishability. Although solid-state quantum emitters can serve such single photons on demand, their asymmetric temporal and spatial mode profiles limit the optimal efficiency and fidelity of quantum interaction. Here, we demonstrate single-photon pulses at a telecom wavelength with a Gaussian-like temporal mode profile from a cavity-coupled single quantum dot. Engineering the exciton dynamics via multi-exciton cascade recombination and cavity detuning enables us to modify the rise and decay dynamics of single excitons. Furthermore, the cascade recombination process temporally retards the single-exciton emission from the background emission, leading to possible purification of single photons at high excitation power. In addition, coupling quantum dots into a low Q cavity mode leads to a Gaussian-like spatial mode profile, which brings a high collection efficiency. This approach paves the way for producing single photons with an optimized temporal and spatial waveform.

Near-field modulation of single photon emitter with a plasmonic probe

Single solid-state quantum dots have significant potential as bright single-photon sources for scalable photonic quantum information technologies. Engineering their radiative relaxation properties is of significant importance for their practical applications. In this study, we demonstrate a cavity-free, broadband approach for modulating and collecting the fluorescence of a single-photon emitter using a fiber taper–silver nanowire plasmonic probe. When the plasmonic probe is located above a single colloidal quantum dot at approximately 20 nm, the photon-emitter interaction increased rapidly and a significant decrease, by an average factor of 3.38, in the lifetime of the quantum dot was observed. The fluorescence signal of the quantum dots was collected by the hybrid probe, with significantly higher efficiency than that of the traditional metal-coated near-field probe. The results of the numerical simulation were in good agreement with the experimental results. The proposed near-field modulation method can be applied to other single-photon sources and proved to be a flexible method for manipulating the luminescence of systems based on single-photon emitters.

Ultra-high-rate nonclassical light source with 50 GHz-repetition-rate mode-locked pump pulses and multiplexed single-photon detectors.

Heralded single photons (HSPs) and entangled photon pairs (EPPs) via spontaneous parametric down-conversion are essential tools for the development of photonic quantum information technologies. In this paper, we report a novel ultra-high-rate nonclassical light source realized by developing 50 GHz-repetition-rate mode-locked pump pulses and multiplexed superconducting nanowire single-photon detectors. The presence of the single-photon state in the heralded photons with our setup was indicated by the second-order intensity correlation below 1/2 at the heralding rate over 20 Mcps. Even at the rate beyond 50 Mcps, the nonclassicality was still observed with the intensity correlation below unity. Moreover, our setup is also applicable to the polarization-EPP experiment, where we obtained the maximum coincidence rate of 1.6 Mcps with the fidelity of 0.881 ± (0.254 × 10-3) to the maximally entangled state. Our versatile source could be a promising tool to explore various large-scale quantum-photonic experiments with low success probability and heavy attenuation.

Silicon-based photonic quantum information technologies

Silicon quantum photonics is a promising platform for the development of advanced quantum information technologies, offering a high level of stability, controllability, scalability and integration density. Silicon quantum photonics has enabled a range of key demonstrations including the development of a versatile toolbox for controlling single-photon’s different degrees of freedom, the generation of multipartite entanglement and high-dimensional entanglement, and realization of large-scale programmable quantum devices. The progress has unlocked the unprecedented power of chip-scale quantum photonic technologies for advanced applications in quantum communication, computing and simulation.

Measuring the refractive index of optical adhesives at cryogenic temperatures

The development of photonic quantum information technologies requires research on the properties of optical adhesives at cryogenic temperatures. In the process of developing microfiber (MF)-coupled superconducting nanowire single-photon detectors (SNSPDs), we invented a cryogenic-temperature refractive index (RI) measurement method based on a kind of MF device. The device was put into the cryostat to observe the variance of MF transmittance with temperature. Then an RI-temperature relationship was established through the correspondence between the confinement conditions of MFs of various diameters in an optical adhesive-${{\rm MgF}_2}$MgF2 environment and transmittance-temperature curves. Using this method, we analyzed the thermal-optical properties of a commercial fluorinated acrylic optical adhesive and obtained the RI values of the adhesive at various temperatures. The results were successfully applied in the development of broadband and high-efficiency MF-coupled SNSPDs.

Quantum interferometric generation of polarization entangled photons

Quantum interference, like Hong-Ou-Mandel interference, has played an important role to test fundamental concepts in quantum physics. We experimentally show that the multiple quantum interference effects enable the generation of high-performance polarization entangled photons. These photons have a high-emission rate, are degenerate, have a broadband distribution, and are postselection free. A quantum interferometric scheme, based on a round-trip configuration of a double-pass polarization Sagnac interferometer, makes it possible to use the large generation efficiency of polarization entangled photons in the process of parametric down-conversion and to separate degenerate photon pairs into different optical modes with no requirement of postselection. We demonstrate experimentally that multiple quantum interference is not only an interesting fundamental quantum optical phenomenon but can be used for novel photonic quantum information technologies.

Photonic quantum information: science and technology

Recent technological progress in the generation, manipulation and detection of individual single photons has opened a new scientific field of photonic quantum information. This progress includes the realization of single photon switches, photonic quantum circuits with specific functions, and the application of novel photonic states to novel optical metrology beyond the limits of standard optics. In this review article, the recent developments and current status of photonic quantum information technology are overviewed based on the author’s past and recent works.

Crystal Phase Quantum Dots in the Ultrathin Core of GaAs-AlGaAs Core-Shell Nanowires.

Semiconductor quantum dots embedded in nanowires (NW-QDs) can be used as efficient sources of nonclassical light with ultrahigh brightness and indistinguishability, needed for photonic quantum information technologies. Although most NW-QDs studied so far focus on heterostructure-type QDs that provide an effective electronic confinement potential using chemically distinct regions with dissimilar electronic structure, homostructure NWs can localize excitons at crystal phase defects in leading to NW-QDs. Here, we optically investigate QD emitters embedded in GaAs-AlGaAs core-shell NWs, where the excitons are confined in an ultrathin-diameter NW core and localized along the axis of the NW core at wurtzite (WZ)/zincblende (ZB) crystal phase defects. Photoluminescence (PL)-excitation measurements performed on the QD-emission reveal sharp resonances arising from excited electronic states of the axial confinement potential. The QD-like nature of the emissive centers are suggested by the observation of a narrow PL line width, as low as ~300 μeV, and confirmed by the observation of clear photon antibunching in autocorrelation measurements. Most interestingly, time-resolved PL measurements reveal a very short radiative lifetime <1 ns, indicative of a transition from a type-II to type-I band alignment of the WZ/ZB crystal interface in GaAs due to the strong quantum confinement in the ultrathin NW core.

Telecom-Wavelength Atomic Quantum Memory in Optical Fiber for Heralded Polarization Qubits

Polarization-encoded photons at telecommunication wavelengths provide a compelling platform for practical realizations of photonic quantum information technologies due to the ease of performing single qubit manipulations, the availability of polarization-entangled photon-pair sources, and the possibility of leveraging existing fiber-optic links for distributing qubits over long distances. An optical quantum memory compatible with this platform could serve as a building block for these technologies. Here we present the first experimental demonstration of an atomic quantum memory that directly allows for reversible mapping of quantum states encoded in the polarization degree of freedom of a telecom-wavelength photon. We show that heralded polarization qubits at a telecom wavelength are stored and retrieved with near-unity fidelity by implementing the atomic frequency comb protocol in an ensemble of erbium atoms doped into an optical fiber. Despite remaining limitations in our proof-of-principle demonstration such as small storage efficiency and storage time, our broadband light-matter interface reveals the potential for use in future quantum information processing.

Single quantum emitters in monolayer semiconductors.

Single quantum emitters (SQEs) are at the heart of quantum optics and photonic quantum-information technologies. To date, all the demonstrated solid-state single-photon sources are confined to one-dimensional (1D; ref. 3) or 3D materials. Here, we report a new class of SQEs based on excitons that are spatially localized by defects in 2D tungsten-diselenide (WSe2) monolayers. The optical emission from these SQEs shows narrow linewidths of ∼130 μeV, about two orders of magnitude smaller than those of delocalized valley excitons. Second-order correlation measurements revealed a strong photon antibunching, which unambiguously established the single-photon nature of the emission. The SQE emission shows two non-degenerate transitions, which are cross-linearly polarized. We assign this fine structure to two excitonic eigenmodes whose degeneracy is lifted by a large ∼0.71 meV coupling, probably because of the electron-hole exchange interaction in the presence of anisotropy. Magneto-optical measurements also reveal an exciton g factor of ∼8.7, several times larger than those of delocalized valley excitons. In addition to their fundamental importance, establishing new SQEs in 2D quantum materials could give rise to practical advantages in quantum-information processing, such as an efficient photon extraction and a high integratability and scalability.

Photonic Quantum Information Technologies Explored by Quantum Optics Research

Photonic Quantum Information Technologies Explored by Quantum Optics Research