Photonic Modes Research Articles

Room‐Temperature Single‐Mode Plasmonic Perovskite Nanolasers with Sub‐Picosecond Pulses

AbstractWith the explosive growth of communication traffic, increasing the modulation bandwidth of semiconductor lasers has attracted significant attention. However, after rapid progress is achieved, further increasing the modulation bandwidth of semiconductor lasers is hampered by the slow charge‐carrier dynamics. Here, a room temperature, single‐mode perovskite nanolaser with sub‐picosecond pulses, enabled by high Purcell enhancement is reported. This enhancement is achieved via transferring an atomically smooth perovskite nanoplatelet onto the surface of an ultra‐smooth SiO2/Ag film. This nanolaser features a low mode volume (V) as low as 0.137 µm3, a high‐quality factor (Q) up to 2180, and a low lasing threshold of 36.65 µJ cm−2. The Q value of the laser is one order of magnitude higher than that of state‐of‐the‐art nanolasers. The smoothness of both the nanoplatelet and the SiO2/Ag film in the laser is critical to achieving a high Purcell enhancement. Polarization analysis reveals that the laser emission consists of a transvere‐magnetic (TM) polarized surface plasmon mode and a transverse‐electric (TE) polarized photonic mode. Furthermore, ultrafast charge‐carrier dynamics indicate the surface plasmon decay time can be as short as 0.6 ± 0.4 ps due to the high Purcell enhancement. This work opens up the possibility of developing nanolasers with high bandwidths and ultra‐small sizes.

Strong coupling spontaneous emission interference near a graphene nanodisk

Abstract In this work, we analyze the spontaneous emission dynamics of a V-type quantum emitter near a graphene nanodisk based on the combination of electromagnetic and quantum dynamical calculations. The presence of the graphene nanodisk gives strong anisotropy to the Purcell factors of the quantum emitter, leading to interference effects in spontaneous emission appearing as coupling between the emitter’s upper levels. This effect is further enhanced by the strong light–matter interaction of the quantum emitter with the modified electromagnetic mode continuum, which induces non-Markovian spontaneous emission dynamics. We have studied the population dynamics of the quantum emitter at a specific distance from the center of the graphene nanodisk for various free-space decay widths and different quantum emitter’s initial conditions and have shown weak coupling results appearing with Markovian decay dynamics, obtained for quantum emitters with small free-space decay widths, and population dynamics that exhibits distinctly non-Markovian features, such as prominent decaying Rabi oscillations in the population evolution of the quantum emitter’s excited states and energy exchange between them during the overall population decay into the photonic mode continuum for largest free-space decay widths. Also, for the largest value of the free-space decay width, we obtain significant population trapping effects in the excited states of the quantum emitter. Furthermore, we find that the population dynamics for specific light–matter interaction strength conditions between the quantum emitter and the graphene nanodisk depend distinctively on the initial state of the quantum emitter, whether it is a single state or a superposition state.

Increase in Modulation Speed of Silicon Photonics Modulator with Quantum-Well Slab Wings: New Insights from a Numerical Study

A Silicon Photonics modulator is a high-speed photonic integrated circuit for optical data transmission in high-capacity optical networks. Silicon Photonics modulators in the configuration of a Mach–Zehnder interferometer, in which a PN-junction rib-waveguide phase shifter is inserted in each arm of the interferometer, are studied in this paper because of their superior performance of high-quality optical data generation in a wide range of spectral bands and their simplicity in fabrication processes suitable to production in foundries. Design, fabrication, and fundamental characteristics of Silicon Photonics Mach–Zehnder modulators are reviewed as an introduction to these high-speed PICs on the Silicon Photonics platform. Modulation speed, or modulation bandwidth, is a key performance item, as well as optical loss, in the application to high-speed optical transmitters. Limiting factors on modulation speed are addressed in equations. Electrical resistance–capacitance coupling, which causes optical modulation bandwidth–optical loss trade-off, is the most challenging limiting factor that limits high-speed modulation. Expansion of modulation bandwidth is not possible without increasing optical loss in the conventional approaches. A new idea including quantum-mechanical effect in the design of Silicon Photonics modulators is proposed and proved in computational analysis to resolve the bandwidth loss trade-off. By adding high-mobility quantum-well overlayers to the side slab wings of the rib-waveguide phase shifter, the modulation bandwidth is doubled without increasing optical loss to achieve a 200 Gbaud modulation rate.

Phase-resolved measurement of entangled states via common-path interferometry

We propose and experimentally demonstrate a method to directly measure the phase of biphoton states using an entangled mode as a collinear reference. The technique is demonstrated with entangled photonic spatial modes in the Laguerre–Gaussian basis, and it is applicable to any pure quantum system containing an exploitable reference state in its entanglement spectrum. As one particularly useful application, we use the new methodology to directly measure the geometric phase accumulation of entangled photons.

Strong coupling-induced frequency shifts of highly detuned photonic modes in multimode cavities.

Strong coupling between light and molecules is a fascinating topic exploring the implications of the hybridization of photonic and molecular states. For example, many recent experiments have explored the possibility that strong coupling of photonic and vibrational modes might modify chemical reaction rates. In these experiments, reactants are introduced into a planar cavity, and the vibrational mode of a chemical bond strongly couples to one of the many photonic modes supported by the cavity. Some experiments quantify reaction rates by tracking the spectral shift of higher-order cavity modes that are highly detuned from the vibrational mode of the reactant. Here, we show that the spectral position of these cavity modes, even though they are highly detuned, can still be influenced by strong coupling. We highlight the need to consider this strong coupling-induced frequency shift of cavity modes if one is to avoid underestimating cavity-induced reaction rate changes. We anticipate that our work will assist in the re-analysis of several high-profile results and has implications for the design of future strong coupling experiments.

Hybrid architectures for terahertz molecular polaritonics

Atoms and their different arrangements into molecules are nature’s building blocks. In a regime of strong coupling, matter hybridizes with light to modify physical and chemical properties, hence creating new building blocks that can be used for avant-garde technologies. However, this regime relies on the strong confinement of the optical field, which is technically challenging to achieve, especially at terahertz frequencies in the far-infrared region. Here we demonstrate several schemes of electromagnetic field confinement aimed at facilitating the collective coupling of a localized terahertz photonic mode to molecular vibrations. We observe an enhanced vacuum Rabi splitting of 200 GHz from a hybrid cavity architecture consisting of a plasmonic metasurface, coupled to glucose, and interfaced with a planar mirror. This enhanced light-matter interaction is found to emerge from the modified intracavity field of the cavity, leading to an enhanced zero-point electric field amplitude. Our study provides key insight into the design of polaritonic platforms with organic molecules to harvest the unique properties of hybrid light-matter states.

TiO2 multi-leg nanotubes for surface-enhanced Raman scattering

Abstract In the recent past, significant research efforts have been put forth to fabricate cost-effective substrates for surface-enhanced Raman scattering (SERS) applications. Here we propose semiconducting TiO2 multi-leg nanotubes and Au nanoparticle-coated TiO2 multi-leg nanotubes (TiO2 MLNTs and Au/TiO2 MLNTs) as SERS substrates. The unique multi-leg architecture of TiO2 nanotubes demonstrated enhanced light-harvesting properties facilitated by an induced photonic absorption edge. Remarkable high SERS sensitivity is observed towards the detection of Methylene blue (MB), up to nM concentration (E.F. ∼104) using TiO2 MLNTs. The same is attributed to the resonantly matched photonic absorption edge of TiO2 MLNTs with the wavelength of incident laser probe light. On the other hand, the Au nanoparticle coating further leveraged the light absorption ability of TiO2 MLNTs with the aid of localized surface plasmon resonance mode. As such, Au/TiO2 MLNTs showed excellent enhancement in SERS sensitivity (E.F. ∼105 , for nM of MB) facilitated by the synergy between the plasmonic modes of Au and the photonic absorption mode of TiO2 MLNTs. UV-Vis diffuse reflectance and Raman spectroscopy measurements are highlighted to elucidate the light absorption and SERS sensitivity of the TiO2 and Au/TiO2 MLNTs.

Topological Photonic Chiral Mode Converters

AbstractTopological photonic states are immune to structural defects and perturbations, which are considered as a promising solution for realizing robust integrated optical devices. As an essential photonic component, the chiral mode converter, which can directionally switch the modes of photonic states, plays a key role in integrated photonics. However, there is no way to realize topological photonic chiral mode converters. Here, a method is proposed to realize topological photonic chiral mode converters by dynamically encircling exceptional points in topological photonic systems. The device can directionally switch modes of topological photonic states and endow the mode converter with topology protection. Chiral dynamic behavior emerges between the two topological states due to the nonadiabatic transitions within the non‐Hermitian topological photonic system. The topological photonic chiral mode converter is robust against random perturbations of coupling strengths. The realization of a topological chiral mode converter endows topology protection into traditional photonic devices and will promote the practical applications of topological photonic states, such as mode multiplexers and optical isolators.

A Multiplexing Optical Temperature Sensing System for Induction Motors Using Few-Mode Fiber Spatial Mode Diversity

Induction motors are widely applied in motor drive systems. Effective temperature monitoring is one of the keys to ensuring the reliability and optimal performance of the motors. Therefore, this paper introduces a multiplexed optical temperature sensing system for induction motors based on few-mode fiber (FMF) spatial mode diversity. By using the spatial mode dimension of FMF, fiber Bragg grating (FBG) carried by different spatial modes of optical paths is embedded in different positions of the motor to realize multipoint synchronous multiplexing temperature monitoring. The paper establishes and demonstrates a photonic lantern-based mode division sensing system for motor temperature monitoring. As a proof of concept, the system demonstrates experiments in multiplexed temperature sensing for motor stators using the fundamental mode LP01 and high-order spatial modes LP11, LP21, and LP02. The FBG sensitivity carried by the above mode is 0.0107 nm/°C, 0.0106 nm/°C, 0.0097 nm/°C, and 0.0116 nm/°C, respectively. The dynamic temperature changes in the stator at different positions of the motor under speeds of 1k rpm, 1.5k rpm, 2k rpm with no load, 3 kg load, and 5 kg load, as well as at three specific speed–load combinations of 1.5k rpm_3 kg, 1k rpm_0kg, 2k rpm_5 kg and so on are measured, and the measured results of different spatial modes are compared and analyzed. The findings indicate that different spatial modes can accurately reflect temperature variations at various positions in motor stator winding.

Multiphysics simulations of a cylindrical waveguide optical switch using phase change materials on silicon

This work presents the design and multiphysics simulation of a cylindrical waveguide-based optical switch using germanium-antimony-tellurium (GST) as an active phase change material. The innovative cylindrical architecture is theoretically analyzed and evaluated at 1550 nm wavelength for telecommunication applications. The dispersion relation is derived analytically for the first time to model the optical switch, while finite element method (FEM) and finite difference time domain (FDTD) techniques are utilized to simulate the optical modes, light propagation, and phase change dynamics. The fundamental TE01 and HE11 modes are studied in detail, enabling switching between low-loss amorphous and high-loss crystalline GST phases. Increasing the GST thickness is found to increase absorption loss in the crystalline state but also slows down phase transition kinetics, reducing switching speeds. A 10 nm GST layer results in competitive performance metrics of 0.79 dB insertion loss, 13.47 dB extinction ratio, 30 nJ average power consumption, and 3.5 Mb/s bit rate. The combined optical, thermal, and electrical simulation provides comprehensive insights towards developing integrated non-volatile photonic switches and modulators utilizing phase change materials.

Universal Approach for Quantum Interfaces with Atomic Arrays

We develop a general framework for the analysis of two-sided quantum interfaces, composed of collections of atoms interacting with paraxial light. Accounting for photon-mediated dipole-dipole interactions, our approach is based on the mapping of collective atom-photon interfaces onto a generic one-dimensional model of light scattering, characterized by a reflectivity parameter r0. This entails two key practical advantages: (i) the efficiency of the quantum interface in performing various quantum tasks, such as quantum memory or entanglement generation, is universally given by r0 and is hence reduced to a measurement or classical calculation of a reflectivity; (ii) the efficiency can be greatly enhanced by a properly designed photon mode that spatially matches a collective-dipole eigenmode of the atoms. We demonstrate our approach for realistic cases of finite-size atomic arrays, partially filled arrays, and circular arrays. This provides a unified approach for treating collective light-matter coupling in various platforms, such as optical lattices and optical tweezers. Published by the American Physical Society 2024

Printable Light-Emitting Metasurfaces with Enhanced Directional Photoluminescence.

Nanoimprint lithography is gaining popularity as a cost-efficient way to reproduce nanostructures in large quantities. Recent advances in nanoimprinting lithography using high-index nanoparticles have demonstrated replication of photonic devices, but it is difficult to confer special properties on nanostructures beyond general metasurfaces. Here, we introduce a novel method for fabricating light-emitting metasurfaces using nanoimprinting lithography. By utilizing quantum dots embedded in resin, we successfully imprint dielectric metasurfaces that function simultaneously as both emitters and resonators. This approach to incorporating quantum dots into metasurfaces demonstrates an improvement in photoluminescence characteristics compared to the situation where quantum dots and metasurfaces are independently incorporated. Design of the metasurface is specifically tailored to support photonic modes within the emission band of quantum dots with a large enhancement of photoluminescence. This study indicates that nanoimprinting lithography has the capability to construct nanostructures using functionalized nanoparticles and could be used in various fields of nanophotonic applications.

Influence of Photonics and Plasmonics Effect on Ultrathin Amorphous Silicon Thin Film Solar Cell

Abstract Our recent surge in silicon derived materials has major demand in thin film photovoltaic (PV) modules and enhancing the significant numbers. The rigorous coupled wave analysis method is a simple and fast method also known as developed to determine the light absorption and cell efficiency. The optics of thin film solar cells (amorphous silicon) garnering crucial role in the photovoltaic market. In this work, an ultrathin thin film amorphous silicon solar cell PV performance investigated by periodically textured surfaces at the nanoscale level. This analysis of periodic textured substrate was deriving optimal surface textures. The nanogratings lead to light scattering mechanism with the higher order diffraction angle and enhanced the light absorption of the incidence spectrum. The influence of grating period and height, the collection of the charge carriers increased at various wavelengths from ultraviolet, visible and infrared spectral regions are discussed with the assistance of photonic and plasmonic modes. Finally, nanoscale engineering mechanism the optimized thin film amorphous silicon solar cell yielded the highest current densities (22.6 and 23.8 mA/cm2) in both polarization modes.

Spatial photoluminescence and lifetime mappings of quasi-2D perovskites coupled with a dielectric metasurface.

Light-matter interaction between quantum emitters and optical cavities plays a vital role in fundamental quantum photonics and the development of optoelectronics. Resonant metasurfaces are proven to be an efficient platform for tailoring the spontaneous emission (SE) of the emitters. In this work, we study the interplay between quasi-2D perovskites and dielectric TiO2 metasurfaces. The metasurface, functioning as an open cavity, enhances electric fields near its plane, thereby influencing the emissions of the perovskite. This is verified through angle-resolved photoluminescence (PL) studies. We also conducted reflectivity measurements and numerical simulations to validate the coupling between the quasi-2D perovskites and photonic modes. Notably, our work introduces a spatial mapping approach to study Purcell enhancement. Using fluorescence lifetime imaging microscopy (FLIM), we directly link the PL and lifetimes of the quasi-2D perovskites in spatial distribution when positioned on the metasurface. This correlation provides unprecedented insights into emitter distribution and emitter-resonator interactions. The methodology opens a new (to the best of our knowledge) approach for studies in quantum optics, optoelectronics, and medical imaging by enabling spatial mapping of both PL intensity and lifetime, differentiating between uncoupled quantum emitters and those coupled with different types of resonators.

Terahertz Magnetic Moiré Grating for Enhanced Chirality Manipulation and Nonreciprocal Spin Isolation

AbstractMagneto‐optical activity is a significant way to achieve asymmetric transmission for spin photons. However, it is severely limited by the weak light‐matter interaction in the terahertz (THz) region. In this work, a magnetic Moiré grating (MMG) is constructed by sandwiching an Yttrium iron garnet (YIG) single crystal in a pair of twisted 2D subwavelength gratings. The twisted angle between two gratings introduces a strong geometric Moiré chirality related to the Moiré pattern. When an external magnetic field is applied to the YIG layer, three different symmetries of spacial mirror image, time reversal, and spin conjugation are broken simultaneously under the chiral coupling between magneto‐optical activity and Moiré chirality, leading to both the enhanced magneto‐optical chiral transmission and the nonreciprocal spin isolation. Under the magnetic field varying from −0.26 to +0.26 T in the experiment, the MMG achieves an active modulation of circular dichroism from 39 to −37.5 dB and optical activity from −35° to 30°. Moreover, the maximum spin isolation over 32.6 dB is also obtained near 0.5 THz. This mechanism provide a new way to realize independent manipulation and active modulation of THz spin photons more flexibly.

Super Bound States in the Continuum on a Photonic Flatband: Concept, Experimental Realization, and Optical Trapping Demonstration.

In this Letter, we theoretically propose and experimentally demonstrate the formation of a super bound state in a continuum (BIC) on a photonic crystal flat band. This unique state simultaneously exhibits an enhanced quality factor and near-zero group velocity across an extended region of the Brillouin zone. It is achieved at the topological transition when a symmetry-protected BIC pinned at k=0 merges with two Friedrich-Wintgen quasi-BICs, which arise from the destructive interference between lossy photonic modes of opposite symmetries. As a proof of concept, we employ the ultraflat super BIC to demonstrate three-dimensional optical trapping of individual particles. Our findings present a novel approach to engineering both the real and imaginary components of photonic states on a subwavelength scale for innovative optoelectronic devices.

Photon-photon correlation of condensed light in a microcavity

The study of temporal coherence in a Bose-Einstein condensate of photons can be challenging, especially in the presence of correlations between the photonic modes. In this work, we use a microscopic, multimode model of photonic condensation inside a dye-filled microcavity and the quantum regression theorem to derive an analytical expression for the equation of motion of the photon-photon correlation function. This allows us to derive the coherence time of the photonic modes and identify a nonmonotonic dependence of the temporal coherence of the condensed light with the cutoff frequency of the microcavity. Published by the American Physical Society 2024

Proton and muon beam tests for ultra-fast MCP-PMT detectors

In collaboration with the North Night Vision Science and Technology (Nanjing) Research Institute Co. Ltd, researchers at the Institute of High Energy of Physics in China have successfully developed the 20-inch micro-channel-plate photomultiplier tube (MCP-PMT) that exhibits high detection efficiency (DE) for use in the Jiangmen Underground Neutrino Observatory (JUNO). Due to the long drift path of electrons from photocathode to MCP, the 20-inch MCP-PMT has a time resolution on the order of nanoseconds. Recently, the team has made advancements in ultra-fast MCP-PMTs (FPMTs), achieving picosecond-level time resolution with both 1-inch and 2-inch types. By now, prototypes featuring single-anode, 2 × 2 anodes, 4 × 4 anodes, and 8 × 8 anodes have been successfully manufactured and tested. The 8 × 8 anode FPMT, in particular, demonstrates a transit time spread (TTS) of 36 ps (Sigma) in single photon mode, thanks to its meticulously engineered structure. To assess the FPMT’s time performance under beam conditions, two beam tests were conducted at Fermi Lab and CERN. In these tests, the 8 × 8 pixel arrays of four distinct radiators, including LYSO, BGO, Pb glass and quartz glass, were paired with the 8 × 8 anodes FPMT. This setup involved the use of two radiator-coupled FPMT detectors for particle detection. The best coincidence time resolution recorded was 64 ps (Sigma) with a 120 GeV proton beam and 56 ps (Sigma) with a 108 GeV muon beam.

A tailor-made fluorescent ionic liquid integrating tetrapropylammonium hydroxide with 1-naphathoic acid to construct a dual-emitting fluoroprobe for sensing hydroquinone in environmental waters

Herein, a dual-emitting fluoroprobe was pioneered for the sensitive and selective detection of hydroquinone (HQ) in environmental waters, which was based on integration of a tailor-made fluorescent ionic liquid ([TBAOH][NA]) with Eu3+ (([TBAOH][NA]/Eu3+). HQ could substantially enhance the 365-nm fluorescence intensity (FI365) of [TBAOH][NA]/Eu3+, whereas no prominent variation ocurred in FI615. After HQ binding with [TBAOH][NA], the electronic structure of S1 was completely pi-pi*, and the orbital overlap of the latter was much higher, thereby promoting photon transitions. After some key factors were optimized using a central-composite-design (CCD) approach, this fluroprobe provided a linear response from 0.5 to 100 μM and detection limit of 0.15 μM for HQ assay, which was comparable to analytical performance by conventional HPLC-DAD analysis. Overall, the prominent advantages of as-developed fluoroprobe lie in two aspects: (1) Employing the ratio of two well-resolved emission and significantly differential responses to HQ greatly enhance sensitivity and accuracy through a self-calibration system; and (2) [TBAOH][NA] has not only the superiority of “green solvent” like conventional ionic liquids, but also possesses strong luminescence signal owing to introducing 1-naphathoic acid as an anion into tetrapropylammonium hydroxide. Consequently, this dual-emitting fluoroprobe is endowed with great potential in on-site and outdoor HQ monitoring.

A neural network model for point defect microcavities of two-dimensional GaAs media background photonic crystals

This paper aims to address the challenge of constructing, training, and optimizing a neural network model for the point defect microcavity of a two-dimensional GaAs media background photonic crystal. The objective is to achieve more accurate predictions and analyses of photon modes, thereby enhancing the performance of the microcavity. Due to the structural complexity and multi-parameter nature of point defect microcavities, traditional analysis methods often fail to capture their optical behavior adequately. Consequently, there is a need for a novel approach to establishing an optical model for point defect microcavities, enabling precise predictions of their optical properties and optimal design. In this study, the MPB computing tool developed by MIT, in conjunction with the programming language Scheme, MATLAB, and the Ubuntu virtual machine platform, was utilized for data acquisition. The neural network model was employed to process the input data of the photonic crystal point defect microcavity, leading to predictions and analyses. This interdisciplinary approach results in a high-precision model of the microcavity. The neural network model is capable of nonlinear mapping and prediction by learning the patterns and features of the data. Additionally, this combination holds the promise of enabling more efficient optical information processing and increased data transfer rates. The relationship between the energy band data and the structure of photonic crystals exhibits a high degree of nonlinearity. The neural network model proposed in this paper can infer the structure of photonic crystals based on the photon energy band (dispersion relation ω-K) of micro-cavity structures with point defects in different photonic crystals. This provides a valuable reference for more accurate predictions and analyses of photon modes in complex photonic crystal micro-cavities, ultimately leading to improved micro-cavity performance.