Reactor Performance Research Articles

Oxygen atom activated ZIF-67/carbon cloth in plasma system for CO2 reduction

ZIF-67 was grown in situ on carbon cloth (CC) using a simple one-step method. The prepared ZIF-67/CC electrodes exhibited excellent CO2 reduction reaction (CO2RR) performance in a dielectric barrier discharge plasma reactor. The highest concentrations of produced formic acid and formaldehyde were 9.16 and 0.068 mmol L−1 at a reaction time of 1 h, respectively. The high performance is related to the unique high aspect ratio structure and pad-like cavity of ZIF-67, which results not only in an increase in the specific surface area for CO2 adsorption but also in the hydrophobicity of the electrode. Unexpectedly, the superoxide radical (·O2−) greatly affects the reduction performance of the electrode. In addition, the ZIF-67/CC electrode maintained good CO2RR performance in the presence of different pollutants, and the production of formic acid and formaldehyde increased to 10.81 and 0.11 mmol L−1 at 1 h with the addition of 10 mg L−1 phenol. This research provides new directions in the field of plasma catalysis.

Superhydrophobic Surface Modification of a Co-Ru/SiO2 Catalyst for Enhanced Fischer-Tropsch Synthesis

Commercial silica support pellets were impregnated and calcined to contain cobalt oxide and ruthenium oxide for Fischer-Tropsch synthesis (FTS). The precatalyst pellets were split evenly into two groups, the control precatalyst (c-precat) and silylated precatalyst (s-precat), which were treated with 1H,1H, 2H, 2H-perfluorooctyltriethoxysilane (PFOS) in toluene. The samples of powderized s-precat were superhydrophobic, as determined by the water droplet contact angle (>150°) and sliding angle (<1°). Thermal analysis revealed the PFOS groups to be thermally stable up to 400 °C and temperature programmed reduction (TPR) studies showed that H2 reduction of the cobalt oxide to cobalt was enhanced at lower temperatures relative to the untreated c-precat. The two active catalysts were examined for their FTS performance in a tubular fixed-bed reactor after in situ reduction at 400 °C for 16 h in flowing H2 to give the active catalysts c-cat and s-cat. The FTS runs were performed under identical conditions (255 °C, 2.1 MPa, H2/CO = 2.0, gas hourly space velocity (GHSV) 510 h–1) for 5 days. Each catalyst was examined in three runs (n = 3) and the mean values with error data are reported. S-cat showed a higher selectivity for C5+ products (64 vs. 54%) and lower selectivity for CH4 (11 vs. 17%), CO2 (2 % vs. 4 %), and olefins (8% vs. 15%) than c-cat. S-cat also showed higher CO conversion, at 37% compared to 26%, leading to a 64% increase in the C5+ productivity measured as g C5+ products per g catalyst per hour. An analysis of the temperature differential between the catalyst bed and external furnace temperature showed that s-cat was substantially more active (DTinitial = 29 °C) and stable over the 5-day run (DTfinal = 22 °C), whereas the attenuated activity of c-cat (DTinitial = 16 °C) decayed steadily over 3 days until it was barely active (DTfinal < 5 °C). A post-run surface analysis of s-cat revealed no change in the water contact angle or sliding angle, indicating that the FTS operation did not degrade the PFOS surface treatment.

Enhanced particle mixing performance of liquid-solid reactor under non-periodic chaotic stirring

This paper introduces the Chebyshev non-periodic chaotic stirring speed based on chaos theory. Additionally, it constructs the DEM-VOF coupled computational model to investigate non-periodic mixing within the reactor system. Numerical calculations are employed to compare and analyze Constant Stirring Speed (CSS) with Chebyshev Non-Periodic Chaotic Stirring Speed and its reverse (CRS, CRS-R). The results indicate that the number of particles deposited at the bottom of end diffusion decreases by 54.3 %. Moreover, it samples particle concentration per unit volume, resulting in a 70.3 % decrease in the Relative Concentration Standard Deviation (RCSD) of particles. Furthermore, it quantifies the mixing effect based on the distribution of distances between particles, leading to a 20.3 % increase in the Unit Block Mixing Index (UBMI). In conclusion, this study improves particle distribution characteristics by utilizing appropriate non-periodic variable speed intervals. Additionally, it provides technical support for production scenarios involving the mixing and dispersion of multiphase non-homogeneous systems.

Carbon monoxide conversion by anaerobic microbiome in a thermophilic trickle bed reactor

Biomethanation offers a promising route for the valorization of synthesis gas, yet significant challenges arise from the limited conversion of carbon monoxide (CO). This study investigated the adaptation of an anaerobic microbiome in a continuous trickle bed reactor (TBR) with CO as the sole carbon and energy source. We evaluated reactor performance and microbial community changes under different CO loading rates and gas retention times (GRT). Optimal performance was achieved at a CO loading rate of 5.16 Nm³ m⁻³ d⁻¹ and a GRT of 60.6 min, resulting in average production rates of 0.99 Nm³ m⁻³ d⁻¹ for CH₄ and 2.55 Nm⁻³ m⁻³ d⁻¹ for CO₂, with an 88 % CO conversion rate. Microbial analysis indicated that the community was dominated by the genus Methanothermobacter, known for its ability to utilize CO as a sole substrate, followed by a co-dominance of syntrophic acetate-oxidizing bacteria Syntrophaceticus. This syntrophic relationship between Methanothermobacter and Syntrophaceticus is expected to be crucial for the efficient CO conversion process. Additionally, the study proposes a two-reactor system for converting synthesis gas to grid-quality methane.

Enhancing fuel breed-burn performance in a sodium-cooled fast reactor using a novel reactivity control method

This study aims to enhance the fuel cycle and fissile breeding performance of a sodium-cooled fast breeder reactor (FBR) by utilizing minor actinides (MAs) as a means of reactivity control alongside partially-inserted control rods. Choosing the PFBR-500 as the reference design, four core models, designated as Cases A, B, C, and D, utilizing various proportions of minor actinides (MAs) were built and simulated using OpenMC. The MA concentrations were optimized to compensate for the withdrawal of control rods and ensure the same initial reactivity for all cores. Burnup analysis over 365 EFPDs revealed a significant increase in cycle length and burnup for the modified cores along with a modest rise in breeding ratio. Notably, Case C, employing 3.45 wt.% MAs in the 88 inner-core fuel subassemblies achieved an extra 62.25 EFPDs cycle length, a 33.74% rise in single-cycle burnup, and a 3.86% increase in breeding gain compared to the reference. Loading MAs into the inner-core region proved to be more effective in enhancing both fertile-to-fissile conversion (thus extending the cycle length and fuel burnup) and transmutation than utilizing MAs throughout the core due to greater neutron flux at the core center. While Case D utilizing 2.2 wt.% MAs both in the inner and outer core fuel subassemblies had the highest overall MA loading, it demonstrated lower increments in cycle length, burnup, and breeding gain compared to Case C. Case C also exhibited the highest overall destruction rate (approximately 24%/y) for Np and Am isotopes, and successfully transmuted around 24.08 kg 237Np, 9.33 kg 241Am and 3.82 kg 243Am over the course of a single year. The addition of MAs also achieved a slight flattening of the axial and radial flux profile and a decrease in the flux peaking factor. However, it slightly lowered the beta-effective, Doppler constant, and control rod assembly worth, and shifted the coolant void reactivity worth to the positive side.

Design and production of a mini-turbo reactor and study of its dual-fuel (gas-hydrogen) operation

The objective of this research was to investigate the effects of hydrogen injection on the performance of a mini turbo reactor. To achieve this, an experimental test bench was constructed, incorporating a specially designed mini turbo reactor capable of operating on various fuel mixtures and a dry cell electrolyzer for on-site hydrogen production. A comprehensive testing campaign was conducted, comparing the mini turbo reactor performance when fueled with pure propane and a propane-hydrogen blend at varying concentrations. Parameters evaluated included power output, thermal efficiency, fuel mass flow rate, flame temperatures, and pollutant emissions (CO, CO2, NOx). The experimental results unequivocally demonstrated that the addition of hydrogen to propane significantly enhances the mini turbo reactor specific power while concurrently reducing CO and CO2 emissions. Furthermore, data analysis revealed an improvement in the thermal efficiency of the cycle, suggesting potential reductions in specific fuel consumption. These findings highlight the promising potential of hydrogen injection as a strategy to enhance the performance and environmental impact of mini turbo reactor.

Different bioaugmentation regimes that mitigate ammonium/salt inhibition in repeated batch anaerobic digestion: Generic converging trend of microbial communities

Bioaugmentation regimes (i.e., dosage, repetition, and timing) in AD must be optimized to ensure their effectiveness. Although previous studies have investigated these aspects, most have focused exclusively on short-term effects, with some reporting conflicting conclusions. Here, AD experiments of three consecutive repeated batches were conducted to determine the effect of bioaugmentation regimes under ammonium/salt inhibition conditions. A positive correlation between reactor performance and inoculum dosage was confirmed in the first batch, which diminished in subsequent batches for both inhibitors. Moreover, a diminishing marginal effect was observed with repeated inoculum introduction. While the bacterial community largely influenced the reactor performance, the archaeal community exhibited only a minor impact. Prediction of the key enzyme abundances suggested an overall decline in different AD steps. Overall, repeated batch experiments revealed that a homogeneous bacterial community deteriorated the AD process during long-term operation. Thus, a balanced bacterial community is key for efficient methane production.

Evaluating and enhancing heat storage in a Ca(OH)2/CaO shell-tube reactor: A numerical study on key factors and performance optimization

Thermochemical energy storage offers a promising solution to addressing the challenges such as the discontinuous operation of concentrating solar power plants. This study develops a comprehensive model to simulate the Ca(OH)2 heat storage process within a shell-tube reactor system by integrating the fluid dynamics, chemical reactions and thermal processes. The influence of operating conditions and geometric characteristics on the reactor's performance is systematically analyzed. Key performance evaluations are evaluated using an orthogonal experimental design. The results reveal that the reactor's reaction time is 11,305 s under baseline conditions. Increasing the HTF temperature from 825 K to 875 K can reduce the reaction time by 47.9 %, while decreasing the reactant porosity from 0.8 to 0.6 leads to an increase of 100 % in energy storage capacity and extends the heat storage duration by 183 %. Additionally, optimizing the tube arrangement by adding 22 tube passes can increase the energy storage efficiency except causing a marginal increase in reaction time. Among the factors analyzed, reactant porosity has the most significant impact on the heat storage time, while the HTF temperature determinates the heat exchange rate and energy storage efficiency.

The Valorization of Fruit and Vegetable Wastes Using an Anaerobic Fixed Biofilm Reactor: A Case of Discarded Tomatoes from a Traditional Market

Tomato waste, characterized by high organic matter and moisture content, offers a promising substrate for anaerobic digestion, though rapid acidification can inhibit methanogenic activity. This study investigated the performance of a 10.25 L anaerobic fixed biofilm reactor for biogas production using liquid tomato waste, processed through grinding and filtration, at high organic loading rates, without external pH control or co-digestion. Four scouring pads were vertically installed as a fixed bed within a fiberglass structure. Reactor performance and buffering capacity were assessed over three stages with progressively increasing organic loading rates (3.2, 4.35, and 6.26 gCOD/L·d). Methane yields of 0.419 LCH4/gCOD and 0.563 LCH4/g VS were achieved during the kinetic study following stabilization. Biogas production rates reached 1586 mL/h, 1804 mL/h, and 4117 mL/h across the three stages, with methane contents of 69%, 65%, and 72.3%, respectively. Partial alkalinity fluctuated, starting above 1500 mg CaCO3/L in Stage 1, dropping below 500 mg CaCO3/L in Stage 2, and surpassing 3000 mg CaCO3/L in Stage 3. Despite periods of forced acidification, the system demonstrated significant resilience and high buffering capacity, maintaining stability through hydraulic retention time adjustments without the need for external pH regulation. The key stability indicators identified include partial alkalinity, effluent chemical oxygen demand, pH, and one-day cumulative biogas. This study highlights the effectiveness of anaerobic fixed biofilm reactors in treating tomato waste and similar fruit and vegetable residues for sustainable biogas production.

Prediction method of adsorption thermal energy storage reactor performances based on reaction wave model

Adsorption thermal energy storage (ATES) is one of the most important ways to achieve efficient utilization of solar energy. The lack of effective prediction methods of reactor performance severely restricts the application of the ATES system. In this paper, the prediction method of reactor performance was proposed based on the adsorption reaction wave model. The expressions between the reactor performances and the design parameters were derived by using the wave parameters of the adsorption rate wave. The mathematical relationships of design parameters-wave parameters and wave parameters-reactor performances were established, respectively. The experiments on adsorption thermal energy storage were performed, in which the zeolite-water vapor was determined as the working pairs. The air temperature and specific humidity at the inlet and outlet of the reactor were measured, and corresponding adsorption amount, thermal energy and stable output power were obtained. A comparison of the predictions for the reactor performances with experiments was carried out. The results indicated that the proposed prediction method was capable of accurately predicting the reactor performances, with a maximum deviation of less than 6.0 %. Moreover, the proposed prediction method is superior to available methods in terms of simplicity and generality.

Characterization of chaotic mixing effects in hydrometallurgical leaching process based on deep learning

Traditional stirring methods in the wet metallurgy leaching process suffer from low efficiency, high consumption, and low output, leading to increased production costs and energy consumption. Therefore, this study evaluates reactor performance using deep learning and introduces variable-speed stirring to enhance laminar mixing and reduce stirring reactor power consumption. An S-Type acceleration and deceleration control algorithm is constructed to ensure that stepper motors do not experience step loss, stalling, or overshoot when the frequency changes abruptly. A deep learning tracking model based on dual cameras is established to dynamically track tracer particles inside the stirring reactor, and a Euclidean distance evaluation method is proposed to characterize and evaluate the mixing performance of the stirring reactor. Experimental results demonstrate that the use of complex function variable-speed stirring and shortening the variable-speed cycle both contribute to improving mixing efficiency. Under a variable-speed cycle of 5 seconds, chaotic speed increases mixing efficiency by 53.1% compared to constant speed. This study provides a theoretical basis for optimizing the wet metallurgy leaching process.

Sulfamethoxazole exposure shifts partial denitrification to complete denitrification: Reactor performance and microbial community

This study elucidated the influence on a partial denitrification (PD) system under 0–1 mg/L sulfamethoxazole (SMX) stress in a sequencing batch reactor. The results showed that the nitrite accumulation rate (NAR) significantly (P ≤ 0.01) decreased from 68.68 ± 9.00% to 49.05 ± 11.68%, while the total nitrogen removal efficiency significantly (P ≤ 0.001) increased from 23.19 ± 4.42% to 31.36 ± 2.73% in presence of SMX. The results indicated that SMX exposure switched the PD process to complete denitrification through the deterioration of the nitrite accumulation and the promotion of further nitrite reduction. The SMX removal loading rate increased from 0.21 ± 0.04 to 5.03 ± 0.77 mg-SMX/(g-MLVSS·d) with the extended reactor operation under SMX stress. Low SMX concentration exposure increased extracellular polymeric substances (EPS) content from 107.69 ± 20.78 mg/g-MLVSS (0.05 mg-SMX/L) to 123.64 ± 9.66 mg/g-MLVSS (0.5 mg-SMX/L), while EPS secretion was inhibited under high SMX concentration exposure (i.e., 1 mg-SMX/L). Moreover, SMX exposure promoted the synthesis of aromatic protein-like compounds and changed the functional groups as revealed by EEM and FTIR analysis. Additionally, SMX exposure significantly shifted the microbial community structures at both phylum and genus levels. Particularly, the abundance of Thauera, i.e., functional bacteria related to PD, considerably decreased from 41.69% to 11.62% after SMX exposure, whereas the abundances of Denitratisoma and SM1A02 significantly rose under different SMX concentrations. These outcomes hinted that the addition of SMX resulted in the shifting of partial denitrification to complete denitrification.

Analyzing Solar Pyrolysis Process of Walnut Shells: Thermal Biomaterial Behavioral Outcomes

This paper presents a new experimental method for the thermal analysis of solar pyrolysis of walnut shells. The method consists of two types of thermal experiments: (A) the pyrolysis of walnut shells, and (B) the heating-cooling of the biochar obtained during experiment A. Nutshells are a waste product from the pecan nut industry. The state of Sonora, Mexico, produces large volumes of walnuts and their residue. Likewise, this region has a considerable solar resource. The motivation of this study is to obtain biochar - a bi-product of high commercial value used for soil enhancement - using solar energy and agro-industrial waste. In this experiment, biomass pyrolysis of 50g of nutshells was carried out inside a stainless-steel reactor heated with concentrated radiation from a solar simulator. Three different heat fluxes were used: 234, 482, and 725 W. The maximum reaction temperatures were: 382, 498, and 674 °C respectively. The composition of the pyrolysis gases (H2, CO, CO2, and CH4) was measured and the biochar obtained was characterized. Finally, the performance of the solar reactor allowed us to identify and differentiate between evaporation, pyrolysis of cellulosic material, and lignin degradation

Mini-Reactor Proliferation-Resistant Fuel with Burnable Gadolinia in Once-Through Operation Cycle Performance Verification

A miniature nuclear reactor is desirable for deployment as a localized nuclear power station in support of a carbon-free power supply. Coupling aspects of proliferation-resistant fuel with natural burnable absorber loading are evaluated for once-through operation cycle performance to minimize the need for refueling and fuel shuffling operations. The incorporation of 0.075 wt.% 237Np provides favorable plutonium isotopic vectors throughout an operational lifetime of 5.5 years. providing 35 MWe. Core performance was assessed using a verification-by-comparison approach for core designs with or without 237Np and/or gadolinia burnable absorber. Burnup Monte Carlo calculations were performed via MCOS coupling of MCNP and ORIGEN to an achievable burnup of ~62.5 GWd/t. The results demonstrate a minimal penalty to reactor performance due to the addition of these materials as compared against the reference design. Coupling of a proliferation-resistant fuel concept with a uniform loading of natural gadolinia burnable absorber for LEU+ fuel (7.5 wt.% 235U/U UO2) provides favorable excess reactivity considerations with minimized concerns for additional residual waste and more uniform distribution of un-depleted 235U in discharged fuel assemblies.

Perturbations to common gardens of anaerobic co-digesters reveal relationships between functional resilience and microbial community composition.

We report the relationship between enrichment of adapted populations and enhancement of community functional resilience in methanogenic bioreactors. Although previous studies have shown the positive effects of acclimation, this work directly investigated the relationships between microbiome dynamics and performance of anaerobic co-digesting reactors in response to different levels of an environmental perturbation (loading of grease interceptor waste [GIW]). Using the methanogenic microbiome from a full-scale digester, we developed eight sets of microbial communities in triplicate using different feed sources. These substrate-specific microbiomes were then exposed to three independent disturbance events of low-, mid- and high-GIW loading rates. This approach allowed us to directly attribute differences in community responses to differences in community composition. Despite identical inocula, environment (digester operation, substrate loading rate, and feeding patterns) and general whole-community function (methane production and effluent quality) during the cultivation period, different substrates led to different microbial community assemblies. Lipid pre-acclimation led to enrichment of a pool of specialized populations, along with thriving of sub-dominant communities. The enrichment of these populations improved functional resilience and process performance when exposed to a low level of lipid-rich perturbation compared with less-acclimated communities. At higher levels of perturbation, the communities were not able to recover methanogenesis, indicating a loading limit to the resilience response. This study extends our current understanding of environmental perturbations, feed-specific adaptation, and functional resilience in methanogenic bioreactors.IMPORTANCEThis study demonstrates, for the first time for GIW co-digestion, how applying similar perturbations to different microbial communities was used to directly identify the causal relationships between microbial community, function, and environment in triplicate anaerobic microbiomes. We evaluated the impact of feed-specific adaptation on methanogenic microbiomes and demonstrated how microbiomes can be influenced to improve their functional (methanogenic) resilience to GIW inhibition. These findings demonstrate how an ecological framework can help improve a biological engineering application, and more specifically, increase the potential of anaerobic co-digestion for converting wastes to energy.

Experimental investigation on cavitation performance of the annular-slit rotational hydrodynamic cavitation reactor

Experimental investigation on cavitation performance of the annular-slit rotational hydrodynamic cavitation reactor

Study on the performance of catalytic reactor for aircraft fuel tank inerting system

The catalytic reactor, which plays a pivotal role in the novel aircraft fuel tank green inerting system, encounters complex and alternating inlet boundary conditions. In this study, a transient theoretical model of the catalytic reactor was established and solved through programming, and its accuracy was verified through self-built experimental setups. The dynamic performance of the catalytic reactor and the impact of operational parameters were investigated. Additionally, a method for determining the operational range of the catalytic reactor was proposed. The results indicate that the bed temperature gradually increases to 370°C along the axial direction as the reaction progresses over time. In addition, the concentrations of fuel vapor and oxygen gradually decrease along the axial direction or with time, while achieving a fuel vapor conversion rate of 70.13% under design conditions. The promotion of catalytic reactions can be achieved by lowering the inlet gas velocity, elevating temperature, or increasing the concentrations of fuel vapor and oxygen. However, the bed's maximum temperature may surpass the self-ignition temperature of fuel vapor by 425°C. A novel indicator for oxygen consumption rate is proposed, which should be comprehensively evaluated in conjunction with the conversion rate to determine the performance of catalytic reactors. Moreover, increasing the reactor diameter can enhance both conversion rate and oxygen consumption rate. Pressure drop is detrimental to the catalytic reaction, therefore, high altitude and low-pressure conditions should be considered as the standard for reactor design. Meanwhile, this paper proposes a theoretical model to determine the operational range of the catalytic reactor based on criteria such as suitable catalytic efficiency and flight temperature. The research findings presented in this study provide a solid theoretical foundation for optimizing catalytic reactor design, thereby significantly promoting the application of green inerting systems.

Analysis of zirconium hydride moderator effect on the micro lead-based reactor

As a crucial parameter for the design of micro reactors, the neutron spectrum directly impacts the keff, the critical size, burnup characteristics, reactivity temperature coefficients and so on. When considering the optimization of the reactor size, designs utilizing thermal neutron spectrum and fast neutron spectrum each present their unique advantages and challenges. To investigate the impact of energy spectrum on the reactor performance, a micro lead-based reactor with annular channel fuel elements is proposed and the study of the influence of varying the volume ratio of moderator and fuel (the M/F ratio) on the keff, the critical size, burnup characteristic and reactivity temperature coefficients by using the Reactor Monte Carlo code (RMC code) is conducted. The results show that for the micro lead-based reactor proposed, when the reactor energy output demand is greater than 350 MWt·years, the design with fast neutron spectrum (without moderator) exhibits the minimum size. While the reactor energy output demand is less than 350 MWt·years, the design with a thermal neutron spectrum (with moderator) achieves the minimum size. Moreover, to ensure the negative reactivity temperature effect, the M/F ratio should be maintained below 3.4. The insights presented in this paper will serve as valuable references for the design of the micro reactor.

Experimental investigations on the thermal destabilization and performance enhancement of ventilation air methane in a reversed flow oxidation reactor

Proper mitigation and utilization of coal mine ventilation air methane (VAM) are important to alleviate resource shortage and environmental issues. This work presents a pilot-scale experimental analysis of heat storage and oxidation performance in a VAM-fuelled reversal flow reactor, aiming at elucidating the thermal destabilization behaviour and providing feasible ways to maintain the system stability. Experimental results show that the system could become unstable under variable conditions. When the methane concentration is varied from 0.74 % to 0.70 %, the temperature is gradually becoming steady after operating the system for 5160 s. However, this balance will be broken, and the combustor is extinguished if the methane concentration is decreased from 0.68 % to 0.64 %. A critical average temperature of 780 °C in the combustion chamber is identified, below which the system starts to become unstable. Further analysis reveals the importance of heat-releasing proportion from the regenerator to the fresh gases in determining the system performance with the methane concentration varied. A sufficiently low proportion implies that the fresh gases cannot be properly preheated when entering the combustion chamber. Finally, increasing ventilation gas flow rate and reducing switching time are shown to be effective in promoting the oxidation process due to the enhanced heat storage.

Effect of partition arrangement of metal hydrides and phase change materials on hydrogen absorption performance in the metal hydride reactor

Metal hydride (MH) suffers from strong thermal effects during hydrogen absorption. To fully utilize the reaction heat during hydrogen absorption, phase change material (PCM) can be used to achieve efficient thermal management in the reactor. A novel MH-PCM reactor with the partition arrangement of MH and PCM was proposed in this paper. Then, the two-dimensional multiphysics coupled model of the reactor was developed, and the effects of the number of partitions n, the mass of PCM and the hydrogen absorption pressure Pa on the hydrogen absorption performance were discussed detailedly. The results indicated that the novel MH-PCM reactor not only increases the heat transfer area and boots the hydrogen absorption rate, but also improves the uniformity of temperature distribution. As the n increases from 2 to 5, the hydrogen absorption time gradually shortens. Compared to the conventional MH-PCM reactor, the time for 90% hydrogen absorption shortens by 67.13%. Furthermore, the hydrogen absorption rate can be enhanced with the increasing mass of PCM and Pa. However, the larger these values are, the weaker the enhancement effect becomes. The results of this paper may provide a new direction for the optimized design and engineering application of MH-PCM reactors.