The albedo of surfaces in urban areas plays an important role in regulating the urban microclimate and needs to be measured. Artificial urban surfaces, e.g., pavements with lower albedo than natural surfaces such as grass or soil, are a key contributor to the Urban Heat Island (UHI) effect. However, widespread measurement of pavement albedo in the field remains challenging due to limited available daylight hours to record the measurements, the need for clear sky conditions, and slow data collection speed. A new portable system called Discrete SPectrAl RefleCtometer (D-SPARC) was developed to overcome these difficulties. D-SPARC was calibrated in the lab using 25 concrete specimens of known albedo and found to be accurate to within ±0.05, which is similar or better than recently developed aerial or satellite methods. The calibrated D-SPARC device was then used to acquire measurements on ten pavement sections during both the day and night and compared to the results from an albedometer. The RMSE during the day was 0.06 and during the night was 0.02. Each measurement with D-SPARC took about 4 min per test location as compared to 15 min with the albedometer. D-SPARC can be used to conveniently and rapidly measure pavement albedo over a road network with reasonable accuracy and minimal traffic disruption.