Paul Scherrer Institut Research Articles

Non-invasive characterization of the manufacturing process of a Nuragic bronze statuette: a Neutron Imaging study

The Nuragic civilization (Sardinia, Italy, XVIII–VIII Cen. B.C) developed a flourishing bronze metallurgy. The production of Nuragic bronze figurines from Sardinia represents a rich historical archive that provides key information about the iconography, the metal production and casting techniques, and on the development of metallurgy in the Mediterranean basin. Since the question about their manufacturing method remains without definitive answer, the understanding of the Sardinian bronze metallurgy is essential to determine which manufacturing techniques were employed to produce complex bronze artefacts. In the frame of a wider research project relating to Nuragic bronzes, four artefacts, three anthropomorphic statuettes (a warrior, a priestess, and an offering figure), and one miniature of a basket, were made available by Museo Nazionale Preistorico “L. Pigorini” (Roma, IT). In this work we present the results of the analyses conducted on a bronze figurine depicting an iconic type of Nuragic figure: the Priestess. The analysis was performed using White Beam Neutron Tomography (NT) and Bragg Edge Neutron Transmission (BENT) at the Paul Scherrer Institut (PSI) (Villigen, CH). Neutron techniques are nowadays the only available approach for revealing, non-destructively and with good spatial resolution, the morphological and microstructural properties within the whole volume of solid cast metallic artefacts such as this bronze statuette. This work presents the result of a non-invasive analytical investigation on an archaeological bronze artefact, providing outstanding results: from a quantitative analysis of the composition to an in-depth morphological and microstructural analysis capable of unveiling details on the ancient casting methods of the statuette.

Anomalous spin precession systematic effects in the search for a muon EDM using the frozen-spin technique

At the Paul Scherrer Institut (PSI), we are developing a high-precision apparatus with the aim of searching for the muon electric dipole moment (EDM) with unprecedented sensitivity. The underpinning principle of this experiment is the frozen-spin technique, a method that suppresses the spin precession due to the anomalous magnetic moment, thereby enhancing the signal-to-noise ratio for EDM signals. This increased sensitivity enables measurements that would be difficult to achieve with conventional g-2\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$g - 2$$\\end{document} muon storage rings. Given the availability of the 125MeV/c\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$${125}\\,{\ extrm{MeV}/\ extit{c}}$$\\end{document} muon beam at PSI, the anticipated statistical sensitivity for the EDM after a year of data collection is 6×10-23e·cm.\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$${6\ imes 10^{-23}}\\,{e\\!\\cdot \\!\ extrm{cm}}.$$\\end{document} To achieve this goal, it is imperative to do a detailed analysis of any potential spurious effects that could mimic EDM signals. In this study, we present a quantitative methodology to evaluate the systematic effects that might arise in the context of the frozen-spin technique utilised within a compact storage ring. Our approach involves the analytical derivation of equations governing the motion of the muon spin in the electromagnetic (EM) fields intrinsic to the experimental setup, validated through numerical simulations. We also illustrate a method to calculate the cumulative geometric (Berry’s) phase. This work complements ongoing experimental efforts to detect a muon EDM at PSI and contributes to a broader understanding of spin-precession systematic effects.

Operation and performance of the MEG II detector

The MEG II experiment, located at the Paul Scherrer Institut (PSI) in Switzerland, is the successor to the MEG experiment, which completed data taking in 2013. MEG II started fully operational data taking in 2021, with the goal of improving the sensitivity of the μ+→e+γ\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$\\upmu ^+ \\rightarrow {\ extrm{e}}^+ \\upgamma $$\\end{document} decay down to ∼6×10-14\\documentclass[12pt]{minimal} \\usepackage{amsmath} \\usepackage{wasysym} \\usepackage{amsfonts} \\usepackage{amssymb} \\usepackage{amsbsy} \\usepackage{mathrsfs} \\usepackage{upgreek} \\setlength{\\oddsidemargin}{-69pt} \\begin{document}$$\\sim 6 \ imes 10^{-14}$$\\end{document} almost an order of magnitude better than the current limit. In this paper, we describe the operation and performance of the experiment and give a new estimate of its sensitivity versus data acquisition time.

A new NEG coating setup with travelling thin solenoids for the SLS 2.0 complex vacuum chambers

The 288 m long Storage Ring of Swiss Light Source 2.0 (SLS 2.0) consists of several vacuum chambers with unique geometries. Complicated features, with many changes in the cross sections, are essential to provide the best impedance matching, and to allow synchrotron light extraction under the tight geometrical constraints. In order to speed up the commissioning time, it was decided to coat most of the vacuum chambers with non-evaporable getter (NEG) material. A new magnetron sputtering setup has been developed in Paul Scherrer Institut (PSI), where the plasma length, defined by thin solenoids, is relatively small. The solenoids are continuously travelling over the entire vacuum chambers more than hundred times per coating process with an average speed of 4 mm/s to assure the best possible thickness uniformity and to limit the cathode heat up. Flexibility provided by this solution allows to coat various vacuum vessels in one assembly. This paper will describe this NEG coating setup and show results on SLS 2.0 vacuum chambers.

First operation of the JUNGFRAU detector in 16-memory cell mode at European XFEL

The JUNGFRAU detector is a well-established hybrid pixel detector developed at the Paul Scherrer Institut (PSI) designed for free-electron laser (FEL) applications. JUNGFRAU features a charge-integrating dynamic gain switching architecture, with three different gain stages and 75 μm pixel pitch. It is widely used at the European X-ray Free-Electron Laser (EuXFEL), a facility which produces high brilliance X-ray pulses at MHz repetition rate in the form of bursts repeating at 10 Hz. In nominal configuration, the detector utilizes only a single memory cell and supports data acquisition up to 2 kHz. This constrains the operation of the detector to a 10 Hz frame rate when combined with the pulsed train structure of the EuXFEL. When configured in so-called burst mode, the JUNGFRAU detector can acquire a series of images into sixteen memory cells at a maximum rate of around 150 kHz. This acquisition scheme is better suited for the time structure of the X-rays as well as the pump laser pulses at the EuXFEL. To ensure confidence in the use of the burst mode at EuXFEL, a wide range of measurements have been performed to characterize the detector, especially to validate the detector alibration procedures. In particular, by analyzing the detector response to varying photon intensity (so called ‘intensity scan’), special attention was given to the characterization of the transitions between gain stages. The detector was operated in both dynamic gain switching and fixed gain modes. Results of these measurements indicate difficulties in the characterization of the detector dynamic gain switching response while operated in burst mode, while no major issues have been found with fixed gain operation. Based on this outcome, fixed gain operation mode with all the memory cells was used during two experiments at EuXFEL, namely in serial femtosecond protein crystallography and Kossel lines measurements. The positive outcome of these two experiments validates the good results previously obtained, and opens the possibility for a wider usage of the detector in burst operation mode, although compromises are needed on the dynamic range.

Development of the scintillating fiber timing detector for the Mu3e experiment

We present the development and discuss the performance of a compact scintillating fiber detector for the Mu3e experiment for accurate time measurements at very high particle rates. Mu3e is a new experiment under preparation at the Paul Scherrer Institut (PSI) to search for charged Lepton Flavor Violation in the neutrinoless muon decay μ+→e+e−e+ with a projected sensitivity of 10−16 using the most intense continuous surface muon beam in the world. A very thin scintillating fiber detector (thickness <0.2% of a radiation length X0) with a time resolution of about 250 ps, efficiency around 97%, and spatial resolution of ∼100μm has been developed. The SciFi detector is read out with multi-channel silicon photomultiplier arrays at both ends to achieve the best timing performance. Different scintillating fiber types have been evaluated and various assembly procedures have been tested to achieve the best performance.

The Cylindrical Drift Chamber of the MEG II experiment

The MEG experiment at the Paul Scherrer Institut (PSI) represents the state of the art in the search for the charged Lepton Flavor Violating μ+→e+γ decay, setting the most stringent upper limit on the BR (μ+→e+γ)≤4.2×10−13 (90% C.L.). An upgrade of MEG, MEG II, was designed, commissioned and recently started the physics data taking. Its goal is to reach a sensitivity level of 6×10−14. In order to reconstruct the positron momentum vector a Cylindrical Drift CHamber (CDCH) with unprecedented peculiarities was built, featuring angular and momentum resolutions at the 6.5 mrad and 100 keV/c level. The CDCH is a 2-meter long, 60 cm in diameter, low-mass, single volume detector with high granularity: 9 layers of 192 drift cells, few mm wide, defined by ∼12000 wires in a stereo configuration for longitudinal hit localization. The filling gas mixture is Helium:Isobutane 90:10. The total radiation length is 1.5×10−3 X0, thus minimizing the Multiple Coulomb Scattering and allowing for a single-hit resolution <120μm. After the assembly at INFN Pisa, the CDCH was transported to PSI and integrated into the MEG II experimental apparatus since 2018. The commissioning phase lasted for the past three years until the operational stability was reached in 2020. The analysis software is continuously developing and the tuning of the reconstruction algorithms is one of the main activities. The latest updates on the positron momentum vector resolutions and tracking efficiency are presented.

Probing the losses for a high power beam

The High Intensity Proton Accelerator (HIPA) cyclotron at the Paul Scherrer Institut (PSI) delivers 590 MeV CW proton beam with a maximum power of 1.42 MW. After extraction, the beam is transferred in a 120 m long channel towards two target stations (TgM and TgE) for surface muon production before depositing its remaining power at the spallation target SINQ for neutron production. As part of the High Intensity Muon Beamline (HIMB) feasibility study, the first of these targets will be replaced with a thicker one thereby increasing the rate of surface muon production. However, a key challenge for HIMB is to maintain the proton beam losses to the lowest possible levels which requires improving our understanding of the distributed losses along the MW-class beamline. To this end, a new approach was developed where the aim is to relate the experimental values of the temperature, beam profile measurements as well as beam current measurements to the combined power deposition calculations and primary beam losses using Monte Carlo simulation tools.

Commissioning and preliminary performance of the MEG II drift chamber

In the quest for Lepton Flavor Violation (LFV) the MEG experiment at the Paul Scherrer Institut (PSI) represents the state of the art in the search for the charged LFV decay μ+→e+γ, setting the most stringent upper limit on the BR(μ+→e+γ)≤4.2×10−13 (90% C.L.). An upgrade of MEG, MEG II, was designed and it recently started the physics data taking, with the aim to reach a sensitivity level of 6×10−14. The Cylindrical Drift CHamber (CDCH) is a key detector in order to improve the e+ angular and momentum resolutions at the 6.5 mrad and 100 keV/c level. The CDCH is a low-mass single volume detector with high granularity: 9 layers of 192 drift cells each, few mm wide, defined by 12000 wires in a stereo configuration for longitudinal hit localization. After the assembly, the CDCH was transported to PSI for the commissioning phase and it has been integrated into the MEG II experimental apparatus since 2018. The operational stability was reached in 2020 and the complete readout electronics was tested for the first time in 2021. A preliminary analysis of 2020–2021 data is presented.

Experimental assessment of thermal radiation effects on containment atmospheres with varying steam content

The thermal-hydraulics phenomena in a containment during an accident will necessarily include radiative heat transfer (i) within the gas mixture due to the high radiative absorption and emission of steam and (ii) between the gas mixture and the surrounding structures. The analysis of some previous PANDA experiments (PSI, Switzerland) demonstrated the importance of the proper modelling of radiation for the benefit of numerical simulations. These results together with dedicated scoping calculations conducted for the present experiments indicated that the radiative heat transfer is considerable, even for a very low amount of steam (≈2%).The H2P2 series conducted in the large-scale PANDA facility at the Paul-Scherrer-Institut (PSI) in the framework of the OECD/NEA HYMERES-2 project is intended to enhance the understanding of thermal radiation phenomena and to provide a benchmark for corresponding numerical simulations. Thus, the test matrix was tailored around the two opposite extremes: either gas compositions with small steam content such that radiative heat transfer phenomena can be neglected. Or gas mixtures containing larger amounts of steam, so that radiative heat transfer is expected to play a dominant role.The H2P2 series consists of 5 experiments designed to isolate the radiation phenomena from convective and diffusive effects as much as possible. One vessel with a diameter of 4 m and a height of 8 m was preconditioned with different mixtures of air / steam at room and elevated temperatures. This was followed by the build-up of a stable helium stratification at constant pressure in the upper part of the vessel. After that, helium was injected from the top into the vessel which leads to an increase of the vessel pressure and a corresponding elevation-dependent and transient rise of the gas temperature. It is shown that even the addition of small amounts of steam in the initial gas atmosphere considerably impacts the radiative heat transport throughout all phases of the experiments and markedly influences i) the monitored gas peak temperature, ii) the temperature history during the compression and iii) the following relaxation phase after the compression was stopped. These PANDA experiments are the first of its kind conducted in a large scale thermal-hydraulic facility.

Improved Search for Neutron to Mirror-Neutron Oscillations in the Presence of Mirror Magnetic Fields with a Dedicated Apparatus at the PSI UCN Source

While the international nEDM collaboration at the Paul Scherrer Institut (PSI) took data in 2017 that covered a considerable fraction of the parameter space of claimed potential signals of hypothetical neutron (n) to mirror-neutron (n′) transitions, it could not test all claimed signal regions at various mirror magnetic fields. Therefore, a new study of n−n′ oscillations using stored ultracold neutrons (UCNs) is underway at PSI, considerably expanding the reach in parameter space of mirror magnetic fields (B′) and oscillation time constants (τnn′). The new apparatus is designed to test for the anomalous loss of stored ultracold neutrons as a function of an applied magnetic field. The experiment is distinguished from its predecessors by its very large storage vessel (1.47 m3), enhancing its statistical sensitivity. In a test experiment in 2020 we have demonstrated the capabilities of our apparatus. However, the full analysis of our recent data is still pending. Based on already demonstrated performance, we will reach sensitivity to oscillation times τnn′/cos(β) well above a hundred seconds, with β being the angle between B′ and the applied magnetic field B. The scan of B will allow the finding or the comprehensive exclusion of potential signals reported in the analysis of previous experiments and suggested to be consistent with neutron to mirror-neutron oscillations.

Towards a New μ→eγ Search with the MEG II Experiment: From Design to Commissioning

The MEG experiment represents the state of the art in the search for the Charged Lepton Flavour Violating μ+→e+γ decay. With its first phase of operations at the Paul Scherrer Institut (PSI), MEG set the most stringent upper limit on the BR (μ+→e+γ)≤4.2×10−13 at 90% confidence level, imposing one of the tightest constraints on models predicting LFV-enhancements through new physics beyond the Standard Model. An upgrade of the MEG experiment, MEG II, was designed and it is presently in the commissioning phase, aiming at a sensitivity level of 6×10−14. The MEG II experiment relies on a series of upgrades, which include an improvement of the photon detector resolutions, brand new detectors on the positron side with better acceptance, efficiency and performances and new and optimized trigger and DAQ electronics to exploit a muon beam intensity twice as high as that of MEG (7×107 μ+/s). This paper presents a complete overview of the MEG II experimental apparatus and the current status of the detector commissioning in view of the physics data taking in the upcoming three years.

The Meson Production Targets in the high energy beamline of HIPA at PSI

Two target stations in the 590 MeV proton beamline of the High Intensity Proton Accelerator (HIPA) at the Paul Scherrer Institut (PSI) produce pions and muons for seven secondary beamlines, leading to several experimental stations. The two target stations are 18 m apart. Target M is a graphite target with an effective thickness of 5 mm, Target E is a graphite wheel with a thickness of 40 mm or 60 mm. Due to the spreading of the beam in the thick target, a high power collimator system is needed to shape the beam for further transport. The beam is then transported to either the SINQ target, a neutron spallation source, or stopped in the beam dump, where about 450 kW beam power is dissipated. Targets, collimators and beam dumps are described.

The search for the neutron electric dipole moment at PSI

The existence of a nonzero permanent electric dipole moment (EDM) of the neutron would reveal a new source of CP violation and shed light on the origin of the matter–antimatter asymmetry of the Universe. The sensitivity of current experiments using stored ultracold neutrons (UCN) probe new physics beyond the TeV scale. Using the UCN source at the Paul Scherrer Institut, the nEDM collaboration has performed the most sensitive measurement of the neutron EDM to date, still compatible with zero (|d_n|&lt;1.8\times 10^{-26} \, e {cm}|dn|&lt;1.8×10−26ecm, C.L.,90%). A new experiment designed to improve the sensitivity by an order of magnitude, n2EDM, is currently under construction.

NEURAP-A Dedicated Neutron-Imaging Facility for Highly Radioactive Samples.

NEURAP is a dedicated set-up at the Swiss neutron spallation source (SINQ) at the Paul Scherrer Institut (PSI), optionally implemented as a special configuration of the neutron-imaging station NEUTRA. It is one of very few instrumentations available worldwide enabling neutron-imaging of highly radioactive samples to be performed routinely, with special precautions and following a specific procedure. Since the relevant objects are strong γ-sources, dedicated techniques are needed to handle the samples and to perform neutron-imaging despite the radiation background. Dysprosium (Dy)-loaded imaging plates, effectively made sensitive to neutrons only, are employed. Neutrons are captured by Dy during neutron irradiation. Then the imaging plate is erased removing gamma detections. A subsequent relatively long self-exposure by the radiation from the intrinsic neutron-activated Dy within the imaging plate yields the neutron-only radiograph that is finally read out. During more than 20 years of NEURAP operation, images have been obtained for two major applications: (a) highly radioactive SINQ target components were investigated after long-term operation life; and (b) spent fuel rods and their cladding from Swiss nuclear power plants were characterized. Quantitative analysis of the image data demonstrated the accumulation of spallation products in the lead filled “Cannelloni” Zircaloy tubes of the SINQ target and the aggregation of hydrogen at specific sites in used fuel pins of power plants and their cladding, respectively. These results continue to help understanding material degradation and optimizing the operational regimes, which might lead to extending the safe lifetimes of these components.

METHODOLOGY FOR HIGH-FIDELITY DETERMINISTIC MODELLING OF SWISS LWR FUEL ASSEMBLIES

The main goal of this work is to perform pin-by-pin calculations of Swiss LWR fuel assemblies with neutron transport deterministic methods. At Paul Scherrer Institut (PSI), LWR calculations are performed with the core management system CMSYS, which is based on the Studsvik suite of codes. CMSYS includes models for all the Swiss reactors validated against a database of experimental information. Moreover, PSI has improved the pin power calculations by developing models of Swiss fuel assemblies for the Monte Carlo code MCNP, with the isotopic compositions obtained from the In-Core Fuel Management data of the Studsvik suite of codes, by using the SNF code. A step forward is to use a neutron code based on fast deterministic neutron transport methods. The method used in this work is based on a planar Method of Characteristics in which the axial coupling is solved by 1D SP3 method. The neutron code used is nTRACER. Thus, the methodology of this work develops nTRACER models of Swiss PWR fuel assemblies, in which the fuel of each pin and axial level is modelled with the isotopic composition obtained from SNF. This methodology was applied to 2D and 3D calculations of a Swiss PWR fuel assembly. However, this method has two main limitations. First, the cross sections libraries of nTRACER lack some of the isotopes obtained by SNF. Fortunately, this work proves that the missing isotopes do not have a strong effect on keff and the power distribution. Second, the 3D models require high computational memory resources, that is, more than 260 Gb. Thus, the nTRACER code was modified, so now it uses only 8 Gb, without any loss of accuracy. Finally, the keff and power results are compared with Monte Carlo calculations obtained by Serpent.

Analysis of the first magnetic results of the PSI APPLE X undulators in elliptical polarisation

The new APPLE X undulators are novel elliptically-polarised undulators, which have a highly symmetric geometry. Theoretically, all the elliptical polarisation states are expected to have the same deflection parameter if the magnetic and geometrical errors are negligible. Nonetheless, the magnetic measurements of the first ten APPLE X undulators performed at Paul Scherrer Institut (PSI) contradicted this simple statement and numerical simulations were required to understand and validate the results. After the valuation of the magnetic-force induced mechanical deformations of the undulator frame, the central role played by the magnetic susceptibility χ was investigated. The simulation results indicate that the impact of different magnet types in the Halbach array, the anisotropic properties, and the choice of shaped field radial magnets are critical for the achieved magnetic field. The numerical results are compared with the measurement data.

A Retrospective of Materials Synthesis at the Paul Scherrer Institut (PSI)

The availability of high-quality and well characterized materials is a key factor for condensed-matter research [...]

Commissioning of the MEG II tracker system

The MEG experiment at the Paul Scherrer Institut (PSI) represents the state of the art in the search for the charged Lepton Flavour Violating (cLFV) μ+→ e+ γ decay. With the phase 1, MEG set the new world best upper limit on the BR(μ+→ e+ γ) < 4.2 × 10−13 (90% C.L.). With the phase 2, MEG II, the experiment aims at reaching a sensitivity enhancement of about one order of magnitude compared to the previous MEG result. The new Cylindrical Drift CHamber (CDCH) is a key detector for MEG II. CDCH is a low-mass single volume detector with high granularity: 9 layers of 192 drift cells, few mm wide, defined by ∼ 12000 wires in a stereo configuration for longitudinal hit localization. The filling gas mixture is Helium:Isobutane (90:10). The total radiation length is 1.5 × 10−3 X0, thus minimizing the Multiple Coulomb Scattering (MCS) contribution and allowing for a single-hit resolution < 120 μm and an angular and momentum resolutions of 6 mrad and 90 keV/c respectively. This article presents the CDCH commissioning activities at PSI after the wiring phase at INFN Lecce and the assembly phase at INFN Pisa. The endcaps preparation, HV tests and conditioning of the chamber are described, aiming at reaching the final stable working point. The integration into the MEG II experimental apparatus is described, in view of the first data taking with cosmic rays and μ^+ beam during the 2018 and 2019 engineering runs. The first gas gain results are also shown. A full engineering run with all the upgraded detectors and the complete DAQ electronics is expected to start in 2020, followed by three years of physics data taking.

Selective Cs-removal from highly acidic spent nuclear fuel solutions

Abstract Thirty liters of highly acidic spent nuclear fuel solutions need to be disposed at the “Hot Laboratory (hotlab)” facility in Paul Scherrer Institut (PSI), Switzerland. In order to significantly reduce the γ dose rate before proper disposal treatment, 137Cs must be removed. In the here presented sub-project, the ion-exchange method was evaluated. Two promising sorbents, CLEVASOL® and AMP (ammonium molybdophosphate), and two derived products AMP_PAN (AMP immobilized in polyacrylonitrile) and AMP/SiO2 (AMP immobilized on silica gel) were tested by the batch method using model solutions of important high-yield fission products (Cs, Eu, Zr, Ru, Pd and Ag), as well as U and Pu. The results showed that AMP, AMP/SiO2 and AMP_PAN have higher selectivity for Cs than CLEVASOL® in 0.1–8 M (mol/L) HNO3 solutions. 4 M HNO3 solution was identified as the most suitable condition for Cs-removal with AMP, AMP_PAN and AMP/SiO2 due to the still sufficiently high separation factor of Cs from other metal ions and an acceptable volume increase factor after dilution. The follow-up kinetic studies on AMP, AMP_PAN and AMP/SiO2 indicated that although Cs exchange on AMP and AMP/SiO2 is faster than on AMP_PAN in the first 5 min, they all nearly reach equilibrium after 30 min of contacting time. The isotherm curves of Cs adsorption on AMP, AMP_PAN and AMP/SiO2 in 4 M HNO3 showed that the maximum sorption capacity of Cs is reached asymptotically. The results from Langmuir isotherm modeling agree with results from other publications.