Advanced Microwave Scanning Radiometer-2 (AMSR2) is a successor of AMSR for Earth-Observation System (AMSR-E), while the third generation of AMSR (AMSR3) will be launched in the near future. The AMSR2 soil moisture product is also an important component of the Soil Moisture Operational Products System (SMOPS) datasets that are operationally produced by National Oceanic and Atmospheric Administration (NOAA). Refinement of the NOAA AMSR2 soil moisture data product can not only benefit the past AMSR-E and the upcoming AMSR3, but also improve the SMOPS data quality. In this second paper of the two-part series, the Extreme Gradient Boosting (XGB) model was trained using the AMSR2 6.925 GHz, 10.65 GHz, 18.7 GHz and 36.5 GHz brightness temperature (Tb) measurements in dual polarizations, ancillary maps and the vegetation index datasets, and in turn used to predict the daily global AMSR2 soil moisture retrievals from 2012 to 2021. Validation results show that the refined AMSR2 soil moisture retrievals (AMSRr) show an overwhelming advantage in data accuracy over the currently operational AMSR2 product (AMSRc). Comapred to the AMSRc, the developed AMSRr presents a significant improvement on data availability. Results also indicate that the refined AMSR2 datasets are comparable with the latest version Soil Moisture Active Passive soil moisture product. Based on this study, higher quality AMSRr soil moisture data product will be operationally produced in the NOAA, and will eventually benefit the NOAA SMOPS blended soil moisture product and its users.