AbstractBroadband terahertz (THz) chirality and wavefront manipulation play important roles in wireless communication, imaging, and radar systems. In this work, by integrating liquid crystal (LC) into a dielectric metasurface, the gradient phase distribution from the Si metasurface and the tunable birefringent phase shift from LC are engineered to perform an active spin‐decoupled beam steering with the strong spin asymmetric transmission. By using geometric symmetry analysis, the relationships between the symmetry breaking and the optical chirality of the metadevice are revealed under different LC orientations, and both the simulations and experiments further verify the dependence of this chirality on spin‐decoupled beam steering with different spin states. The results show that with the orientation changes of the LC by driving the different magnetic fields, the circular dichroism of the device at the 0° deflection angle is ≈100% dynamically modulated and even flipped in the broadband range of 0.8–1.3 THz. With these changes in THz chirality, a tunable spin‐decoupled beam steering occurs in the range of 25°‐45°. This work shows that tunable LC anisotropy leads to more complex symmetry breaking in this structure, and results in more functions than conventional spin‐decoupled wavefront manipulations, which expands the scope of THz chiral metadevice and its applications.