Amplitude Of Order Parameter Research Articles

Periodic external driving of transmission-delay-coupled phase oscillator system: Switching between different twisted states.

We consider the effects of an external periodic forcing on a spatially extended system that consists of identical phase oscillators coupled with transmission delays on a ring. Analyzing the continuum limit N→∞ of the model system along the Ott-Antonsen invariant manifold, we obtain the stability diagram for two regimes, called the forced and drifting entrainments. The former exhibits a spatially homogeneous solution trying to lock onto the drive, of which the stability boundary is rigorously determined. The latter represents a spatially organized group of oscillators that entrain one another at a frequency different from that of the drive. We show that in the drifting entrainment the external driving triggers the occurrence of unusual twisted states, characterized by nonuniform phase gradient as well as by the traveling wave of the order parameter amplitude. Moreover, it is found that by increasing or decreasing the forcing strength one can effectively switch between twisted states with different winding numbers. Our theoretical and numerical results for the reduced system are supported by the direct numerical simulations of the model system.

Floquet engineering Higgs dynamics in time-periodic superconductors

Higgs modes emerge in superconductors as collective excitations of the order-parameter amplitude when periodically driven by electromagnetic radiation. In this work, we develop a Floquet approach to study Higgs modes in superconductors under time-periodic driving, where the dynamics of the order parameter is captured by anomalous Floquet Green's functions. We show that the Floquet description is particularly powerful as it allows one to exploit the time-periodic nature of the driving, thus considerably reducing the complexity of the time-dependent problem. Interestingly, the Floquet approach is also enlightening because it naturally offers a physical explanation for the renormalized steady-state order parameter as a result of photon-assisted transitions between Floquet sidebands. We demonstrate the usefulness of Floquet engineering Higgs modes in time-periodic s-wave superconductors. Published by the American Physical Society 2024

Melting of Unidirectional Charge Density Waves across Twin Domain Boundaries in GdTe3.

Solids undergoing a transition from order to disorder experience a proliferation of topological defects. The melting process generates transient quantum states. However, their dynamic nature with a femtosecond lifetime hinders exploration with atomic precision. Here, we suggest an alternative approach to the dynamic melting process by focusing on the interface created by competing degenerate quantum states. We use a scanning tunneling microscope (STM) to visualize the unidirectional charge density wave (CDW) and its spatial progression ("static melting") across a twin domain boundary (TDB) in the layered material GdTe3. Combining the STM with a spatial lock-in technique, we reveal that the order parameter amplitude attenuates with the formation of dislocations and thus two different unidirectional CDWs coexist near the TDB, reducing the CDW anisotropy. Notably, we discovered a correlation between this anisotropy and the CDW gap. Our study provides valuable insight into the behavior of topological defects and transient quantum states.

Strain modulation effects on the topological properties of a chiral p−wave superconductor

We present a study of strain modulation effects on electronic structures of a two-dimensional single-band chiral $p\text{\ensuremath{-}}\mathrm{wave}$ superconductor within the BCS mean-field scheme. We employ a lattice model and solve the Bogolyubov-de Gennes equations numerically. Implementing strain modulations through spatially varying hopping matrix elements, we observe the appearance of spontaneous supercurrents from the resulting spatial modulation of order parameter amplitudes. Moreover, sufficiently strong strain modulation induces the formation of topologically distinct domains within the system and causes the appearance of chiral edge modes, which is captured by spectral functions and local Chern markers.

Structural origins of the low-temperature orthorhombic to low-temperature tetragonal phase transition in high- Tc cuprates

We undertake a detailed high-resolution diffraction study of a novel plain band insulator, La$_2$MgO$_4$, which may be viewed as a structural surrogate system of the undoped end-member of the high-T$_c$ superconductors, La$_{2-x-y}$A$^{2+}_x$RE$^{3+}_y$CuO$_{4}$ (A = Ba, Sr, RE= Rare Earth). We find that La$_2$MgO$_4$ exhibits the infamous low-temperature orthorhombic (LTO) to low-temperature tetragonal (LTT) phase transition that has been linked to the suppression of superconductivity in a variety of underdoped cuprates, including the well known La$_{2-x}$Ba$_{x}$CuO$_4$ ($x=0.125$). Furthermore, we find that the LTO-to-LTT phase transition in La$_2$MgO$_4$ occurs for an octahedral tilt angle in the 4 $^{\circ}$ to 5 $^{\circ}$ range, similar to that which has previously been identified as a critical tipping point for superconductivity in these systems. We show that this phase transition, occurring in a system lacking spin correlations and competing electronic states such as charge-density waves and superconductivity, can be understood by simply navigating the density-functional theory ground-state energy landscape as a function of the order parameter amplitude. This result calls for a careful re-investigation of the origins of the phase transitions in high-T$_c$ superconductors based on the hole-doped, $n = 1$ Ruddelsden-Popper lanthanum cuprates.

SARS-coronavirus-2 infections: biological instabilities characterized by order parameters

A four-variable virus dynamics TIIV model was considered that involves infected cells in an eclipse phase. The state space description of the model was transferred into an amplitude space description which is the appropriate general, nonlinear physics framework to describe instabilities. In this context, the unstable eigenvector or order parameter of the model was determined. Subsequently, a model-based analysis of viral load data from eight symptomatic COVID-19 patients was conducted. For all patients, it was found that the initial SARS-CoV-2 infection evolved along the respective patient-specific order parameter, as expected by theoretical considerations. The order parameter amplitude that described the initial virus multiplication showed doubling times between 30 min and 3 h. Peak viral loads of patients were linearly related to the amplitudes of the patient order parameters. Finally, it was found that the patient order parameters determined qualitatively and quantitatively the relationships between the increases in virus-producing infected cells and infected cells in the eclipse phase. Overall, the study echoes the 40 years old suggestion by Mackey and Glass to consider diseases as instabilities.

Localization of the Higgs mode at the superfluid–Mott glass transition

The amplitude (Higgs) mode near the two-dimensional superfluid-Mott glass quantum phase transition is studied. We map the Bose-Hubbard Hamiltonian of disordered interacting bosons onto an equivalent classical XY model in (2+1) dimensions and compute the scalar susceptibility of the order parameter amplitude via Monte Carlo simulation. Analytic continuation of the scalar susceptibilities from imaginary to real frequency to obtain the spectral densities is performed by a modified maximum entropy technique. Our results show that the introduction of disorder into the system leads to unconventional dynamical behavior of the Higgs mode that violates naive scaling,despite the underlying thermodynamics of the transition being of conventional power-law type. The computed spectral densities exhibit a broad, non-critical response for all energies, and a momentum-independent dispersion for long-wavelengths, indicating strong evidence for the localization of the Higgs mode for all dilutions.

Higgs-Mediated Optical Amplification in a Nonequilibrium Superconductor

The quest for new functionalities in quantum materials has recently been extended to non-equilibrium states, which are interesting both because they exhibit new physical phenomena and because of their potential for high-speed device applications. Notable advances have been made in the creation of metastable phases and in Floquet engineering under external periodic driving. In the context of non-equilibrium superconductivity, examples have included the generation of transient superconductivity above the thermodynamic transition temperature, the excitation of coherent Higgs mode oscillations, and the optical control of the interlayer phase in cuprates. Here, we propose theoretically a novel non-equilibrium phenomenon, through which a prompt quench from a metal to a transient superconducting state could induce large oscillations of the order parameter amplitude. We argue that this oscillating mode could act as a source of parametric amplification of the incident radiation. We report experimental results on optically driven K$_3$C$_{60}$ that are consistent with these predictions. The effect is found to disappear when the onset of the excitation becomes slower than the Higgs mode period, consistent with the theory proposed here. These results open new possibilities for the use of collective modes in many-body systems to induce non-linear optical effects.

Spin and charge currents driven by the Higgs mode in high-field superconductors

The Higgs mode in superconducting materials describes slowly decaying oscillations of the order parameter amplitude. We demonstrate that in superconductors with a built-in spin-splitting field the Higgs mode is strongly coupled to the spin degrees of freedom, allowing for the generation of time-dependent spin currents. Converting such spin currents to electric signals by spin-filtering elements provides a tool for the second-harmonic generation and the electrical detection of the Higgs mode generated by the external irradiation. The nonadiabatic spin torques generated by these spin currents allow for the magnetic detection of the Higgs mode by measuring the precession of the magnetic moment in the adjacent ferromagnet. We discuss also the reciprocal effect, which is the generation of the Higgs mode by the magnetic precession. Coupling the collective modes in superconductors to light and magnetic dynamics provides an opportunity for the study of superconducting optospintronics.Received 1 July 2019Revised 23 August 2020Accepted 25 August 2020DOI:https://doi.org/10.1103/PhysRevResearch.2.033416Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article's title, journal citation, and DOI.Published by the American Physical SocietyPhysics Subject Headings (PhySH)Research AreasFFLOOptical conductivitySpin currentSuperconducting phase transitionPhysical SystemsFerromagnetic superconductorsHiggs bosonsMultilayer thin filmsTunnel junctionsTechniquesMethods in superconductivityCondensed Matter & Materials Physics

Domain wall mobility and roughening in doped ferroelectric hexagonal manganites

This work demonstrates a relationship between ferroelectric domain wall pinning by dopants and the local order parameter amplitude around the dopants. The authors propose that such pinning can be predicted from the free-energy landscape of polarization switching.

Transient Trapping into Metastable States in Systems with Competing Orders

The quench dynamics of a system involving two competing orders is investigated using a Ginzburg-Landau theory with relaxational dynamics. We consider the scenario where a pump rapidly heats the system to a high temperature, after which the system cools down to its equilibrium temperature. We study the evolution of the order parameter amplitude and fluctuations in the resulting time dependent free energy landscape. Exponentially growing thermal fluctuations dominate the dynamics. The system typically evolves into the phase associated with the faster-relaxing order parameter, even if it is not the global free energy minimum. This theory offers a natural explanation for the widespread experimental observation that metastable states may be induced by laser induced collapse of a dominant equilibrium order parameter.

Self-Consistent Consideration of Fluctuations in Singlet Superconducting Phases with s and d Symmetry

We analyze the behavior of thermal fluctuations of the superconducting order parameter with extended s-wave and $${{d}_{{{{x}^{2}} - {{y}^{2}}}}}$$-wave symmetry. For this purpose, we develop a method of self-consistent consideration of the order parameter fluctuations and charge carrier scatterers by fluctuations of coupled electron pairs using the theory of functional integration. The study is performed based on the quasi-two-dimensional one-band model with attraction between electrons located at neighboring sites. We obtain the distribution functions of the phase fluctuation probabilities depending on temperature, charge carrier concentrations, and model parameters. It is shown that the phase of the order parameter in the superconducting region is coherent, and the density of states has a dip at the Fermi level. In approaching the incoherent region of the phase diagram, the dip in the density of states disappears simultaneously with the loss of phase coherence. At the same time, the order parameter amplitude averaged over fluctuations remains finite at any temperature and concentration of charge carriers. Our results show that the pseudogap state cannot be explained in the frames of this scenario.

Collective modes in pumped unconventional superconductors with competing ground states

Motivated by the recent development of terahertz pump-probe experiments, we investigate the short-time dynamics in superconductors with multiple attractive pairing channels. Studying a single-band square lattice model with spin-spin interaction as an example, we find the signatures of collective excitations of the pairing symmetries (known as Bardasis-Schrieffer modes) as well as the order parameter amplitude (Higgs mode) in the short-time dynamics of the spectral gap and quasiparticle distribution after an excitation by a pump pulse. We show that the polarization and intensity of the pulse can be used to control the symmetry of the non-equilibrium state as well as frequencies and relative intensities of the contributions of different collective modes. We find particularly strong signatures of the Bardasis-Schrieffer mode in the dynamics of the quasiparticle distribution function. Our work shows the potential of modern ultrafast experiments to address the collective excitations in unconventional superconductors and highlights the importance of sub-dominant interactions for the non-equilibrium dynamics in these systems.

Quantum electrodynamics of a superconductor–insulator phase transition

A chain of Josephson junctions implements one of the simplest many-body models undergoing a superconductor-insulator (SI) quantum phase transition between states with zero and infinite resistance. Apart from zero resistance, the superconducting state is necessarily accompanied by a sound-like mode due to collective oscillations of the phase of the complex-valued order parameter. Exciting this phase mode results in transverse photons propagating along the chain. Surprisingly little is known about the fate of this mode upon entering the insulating state, where the order parameter's amplitude remains non-zero, but the phase ordering is "melted" by quantum fluctuations. Here we report momentum-resolved radio-frequency spectroscopy of collective modes in nanofabricated chains of Al/AlOx/Al tunnel junctions. We find that the phase mode survives remarkably far into the insulating regime, such that $\textrm{M}\Omega$-resistance chains carry $\textrm{GHz}$-frequency alternating currents as nearly ideal superconductors. The insulator reveals itself through broadening and random frequency shifts of collective mode resonances, originated from intrinsic interactions. By pushing the chain parameters deeper into the insulating state, we achieved propagation with the speed of light down to $8\times 10^5~\textrm{m/s}$ and the wave impedance up to $23~\textrm{k}\Omega$. The latter quantity exceeds the predicted critical impedance by an order of magnitude, which opens the problem of quantum electrodynamics of a Bose glass insulator for both theory and experiment. Notably, the effective fine structure constant of such a 1D vacuum exceeds a unity, promising transformative applications to quantum science and technology.

Nonlinear electromagnetic response and Higgs-mode excitation in BCS superconductors with impurities

We reveal that due to the presence of disorder oscillations of the order parameter amplitude called the Higgs mode can be effectively excited by the external electromagnetic radiation in usual BCS superconductors. This mechanism works for superconductors with both isotropic s-wave and anisotropic, such as d-wave, pairings. The non-linear response in the presence of impurities is captured by the quasiclassical formalism. We demonstrate that analytical solutions of the Eilenberger equation with impurity collision integral and external field drive coincide with the exact summation of ladder impurity diagrams. Using the developed formalism we show that resonant third-harmonic signal observed in recent experiments is naturally explained by the excitation of Higgs mode mediated by impurity scattering.

Spin texture and spin current in excitonic phases of the two-band Hubbard model

Using the mean-field approximation, we study the $k$-space spin textures and local spin currents emerged in the spin-triplet excitonic insulator states of the two-band Hubbard model defined on the square and triangular lattices. We assume a noninteracting band structure with a direct band gap and introduce $s$-, $p$-, $d$-, and $f$-type cross-hopping integrals, i.e., the hopping of electrons between different orbitals on adjacent sites with four different symmetries. First, we calculate the ground-state phase diagrams in the parameter space of the band filling and interaction strengths, whereby we present the filling dependence of the amplitude and phase of the excitonic order parameters. Then, we demonstrate that the spin textures (or asymmetric band structures) are emerged in the Fermi surfaces by the excitonic symmetry breaking when particular phases of the order parameter are stabilized. Moreover, in case of the $p$-type cross-hopping integrals, we find that the local spin current can be induced spontaneously in the system, which does not contradict the Bloch theorem for the absence of the global spin current. The proofs of the absence of the global spin current and the possible presence of the local spin currents are given on the basis of the Bloch theorem and symmetry arguments.

Charged domain walls in improper ferroelectric hexagonal manganites and gallates

Ferroelectric domain walls are attracting broad attention as atomic-scale switches, diodes and mobile wires for next-generation nanoelectronics. Charged domain walls in improper ferroelectrics are particularly interesting as they offer multifunctional properties and an inherent stability not found in proper ferroelectrics. Here we study the energetics and structure of charged walls in improper ferroelectric YMnO$_3$, InMnO$_3$ and YGaO$_3$ by first principles calculations and phenomenological modeling. Positively and negatively charged walls are asymmetric in terms of local structure and width, reflecting that polarization is not the driving force for domain formation. The wall width scales with the amplitude of the primary structural order parameter and the coupling strength to the polarization. We introduce general rules for how to engineer $n$- and $p$-type domain wall conductivity based on the domain size, polarization and electronic band gap. This opens the possibility of fine-tuning the local transport properties and design $p$-$n$-junctions for domain wall-based nano-circuitry.

NMR Frequency Shifts and Phase Identification in Superfluid $$^3\hbox {He}$$

The pressure dependence of the order parameter in superfluid $^3$He is amazingly simple. In the Ginzburg-Landau regime, i.e. close to $T_c$, the square of the order parameter can be accurately measured by its proportionality to NMR frequency shifts and is strictly linear in pressure. This behavior is replicated for superfluid $^3$He imbibed in isotropic and anisotropic silica aerogels. The proportionality factor is constrained by the symmetry of the superfluid state and is an important signature of the corresponding superfluid phase. For the purpose of identifying various new superfluid states in the $p$-wave manifold, the order parameter amplitude of $^3$He-A is a useful reference, and this simple pressure dependence greatly facilitates identification.

Amplitude mode in the planar triangular antiferromagnet Na0.9MnO2

Amplitude modes arising from symmetry breaking in materials are of broad interest in condensed matter physics. These modes reflect an oscillation in the amplitude of a complex order parameter, yet are typically unstable and decay into oscillations of the order parameter’s phase. This renders stable amplitude modes rare, and exotic effects in quantum antiferromagnets have historically provided a realm for their detection. Here we report an alternate route to realizing amplitude modes in magnetic materials by demonstrating that an antiferromagnet on a two-dimensional anisotropic triangular lattice (α-Na0.9MnO2) exhibits a long-lived, coherent oscillation of its staggered magnetization field. Our results show that geometric frustration of Heisenberg spins with uniaxial single-ion anisotropy can renormalize the interactions of a dense two-dimensional network of moments into largely decoupled, one-dimensional chains that manifest a longitudinally polarized-bound state. This bound state is driven by the Ising-like anisotropy inherent to the Mn3+ ions of this compound.

Interorbital topological superconductivity in spin-orbit coupled superconductors with inversion symmetry breaking

We study the superconducting state of multi-orbital spin-orbit coupled systems in the presence of an orbitally driven inversion asymmetry assuming that the inter-orbital attraction is the dominant pairing channel. Although the inversion symmetry is absent, we show that superconducting states that avoid mixing of spin-triplet and spin-singlet configurations are allowed, and remarkably, spin-triplet states that are topologically nontrivial can be stabilized in a large portion of the phase diagram. The orbital-dependent spin-triplet pairing generally leads to topological superconductivity with point nodes that are protected by a nonvanishing winding number. We demonstrate that the disclosed topological phase can exhibit Lifshitz-type transitions upon different driving mechanisms and interactions, e.g., by tuning the strength of the atomic spin-orbit and inversion asymmetry couplings or by varying the doping and the amplitude of order parameter. Such distinctive signatures of the nodal phase manifest through an extraordinary reconstruction of the low-energy excitation spectra both in the bulk and at the edge of the superconductor.