Optical Effects Research Articles

The Study on the Nonlinear Effects of Soliton in Optical Fibre

Abstract: In optical fibres, the chirps generated by GVD and SPM, which both limit the system's performance when operating independently, balance each other out to produce soliton formation. To comprehend how such a balance is possible, we shall study the nonlinear optical effects and the dispersion-induced pulse broadening. If an optical pulse is not adequately chirped before it propagates inside an optical fibre, the GVD broadens the pulse. More specifically, an early stage of transmission compresses a chirped pulse whenever β2 and the chirp parameter C have opposite signs and β2C is negative. The optical pulse chirps due to SPM, ensuring that C > 0. If β2 < 0, it is easy to meet the criteria β2C < 0. Moreover, because the SPM-induced chirp depends on power, it is possible that in some situations, SPM and GVD could cooperate to the extent that the SPM-induced chirp is precisely the right amount to cancel out the pulse broadening caused by GVD. Here, an optical pulse propagates distortion-free as a soliton [27].

Determining pair distribution functions of thin films using laboratory-based X-ray sources.

This article demonstrates the feasibility of obtaining accurate pair distribution functions of thin amorphous films down to 80 nm, using modern laboratory-based X-ray sources. The pair distribution functions are obtained using a single diffraction scan without the requirement of additional scans of the substrate or of the air. By using a crystalline substrate combined with an oblique scattering geometry, most of the Bragg scattering of the substrate is avoided, rendering the substrate Compton scattering the primary contribution. By utilizing a discriminating energy filter, available in the latest generation of modern detectors, it is demonstrated that the Compton intensity can further be reduced to negligible levels at higher wavevector values. Scattering from the sample holder and the air is minimized by the systematic selection of pixels in the detector image based on the projected detection footprint of the sample and the use of a 3D-printed sample holder. Finally, X-ray optical effects in the absorption factors and the ratios between the Compton intensity of the substrate and film are taken into account by using a theoretical tool that simulates the electric field inside the film and the substrate, which aids in planning both the sample design and the measurement protocol.

Stokes Phenomena in Lensing

As lensing of coherent astrophysical sources, e.g., pulsars, fast radio bursts, and gravitational waves, becomes observationally relevant, the mathematical framework of Picard–Lefschetz theory has recently been introduced to fully account for wave optics effects. Accordingly, the concept of lensing images has been generalized to include complex solutions of the lens equation referred to as “imaginary images,” and more radically, to the Lefschetz thimbles, which are a sum of the steepest descent contours connecting the real and imaginary images in the complex domain. In this wave-optics-based theoretical framework of lensing, we study the “Stokes phenomena” as the change of the topology of the Lefschetz thimbles. Similar to the well-known caustics at which the number of geometric images changes abruptly, the corresponding Stokes lines are the boundaries in the parameter space where the number of effective imaginary images changes. We map the Stokes lines for a few lens models. The resulting Stokes line-caustics network represents a unique feature of the lens models. The observable signature of the Stokes phenomena is the change of interference behavior, in particular the onset of frequency oscillation for some Stokes lines. We also demonstrate high-order Stokes phenomena where the system has a continuous number of effective images but with an abrupt change in the way they are connected to each other by the Lefschetz thimbles. Their full characterization calls for an analogy of the catastrophe theory for caustics.

Dynamically Tunable Circularly Polarized Selectivity in Plasmon-Enhanced Halide Perovskite Nanocrystal Glasses.

Ultrafast spin manipulation for optical spin-logic applications requires material systems with strong spin-selective light-matter interactions. The optical Stark effect can realize spin-selective light-matter interactions by breaking the degeneracy of spin-selective transitions with an external electric field. Halide perovskites have large exciton binding energies, which enable a room-temperature optical Stark effect. However, halide perovskites are prone to degradation when interacting with light and polar solvents, limiting further integration with nanophotonic structures. We demonstrate a hybrid material system consisting of CsPbBr3 nanocrystal glass weakly coupled to resonant plasmonic silver nanoparticles, showing ultrafast tunable spin-based polarization selectivity at room temperature. We performed circularly polarized pump-probe characterizations to investigate the optical Stark effect in this material system, which resulted in a maximum energy shift of ∼3.67 meV (detuning energy of 0.11 eV and pump intensity of 0.62 GW/cm2). We show that halide perovskite nanocrystal glasses have excellent resistance to heat and moisture, which may be favorable for integration with nanophotonic structures for further engineering polarization states, energy tuning, and coherence time.

Design of optical Kerr effect in multilayer hyperbolic metamaterials

Abstract The design of optical materials in nonlinear devices represents a fundamental step for their optimization and miniaturization, that would significantly contribute to the progress of advanced nanophotonics and quantum technologies. In this work, the effect of geometry and composition of multilayer hyperbolic metamaterials on their third-order nonlinear optical properties, i.e. the optical Kerr effect, is investigated. One figure of merit is provided to be used as a predictive tool to design and best exploit the local intensity enhancement in low-loss metamaterials to be used for various applications in nonlinear nanophotonics.

Spin-transport across semi-crystalline polyvinylidene fluoride thin films in Ta/Co/PVDF/NiFe pseudo spin-valve devices

Room temperature magnetoresistance (MR) across semi-crystalline polyvinylidene fluoride (PVDF) thin films in Ta(2 nm)/Co(15 nm)/PVDF/NiFe(28 nm) pseudo-spin-valve devices (PSVs) are systematically investigated by varying PVDF thicknesses from 80 − 230 nm and applied bias voltages up to 100 mV. NiFe, Ta/Co magnetic bottom and top electrodes, and PVDF thin films are deposited by DC magnetron sputtering and spin-coating methods. The structural, microstructural, and magnetic natures have been evaluated using grazing incidence X-ray diffraction, atomic force microscopy, and magneto optic kerr effect systems. Electrical characteristics reveal a maximum MR of ∼0.25 % at 60 mV bias voltage across PVDF-80 nm and ∼0.08 % across PVDF-230 nm & PVDF- 120 nm devices. A constant MR is found across all the devices up to 100 mV applied bias voltages. In addition to the electrical spin injection evaluation, coplanar waveguide ferromagnetic resonance measurements are utilized to validate the spin injection into PVDF layers by estimating the Gilbert damping parameters of NiFe and PVDF/NiFe bilayers. Furthermore, low MR in PSVs is discussed with the parallel spin-dependent conducting channels corresponding to PVDF’s amorphous, alpha, and beta crystalline phases.

Ferroelectric nematic fluids as spontaneous polarization field for enhanced orientational-dependent second-harmonic generation

ABSTRACT Second-order nonlinear optical effects have piqued researchers’ interest in fundamental physics and practical perspectives. The ferroelectric nematic liquid crystals (NF LCs) have recently drawn attention to LC nonlinear optical applications due to their relatively high second-harmonic generation output. Further improving the nonlinear optical properties to get closer to the performance of inorganic nonlinear optical materials is challenging. Here, we take a blending strategy to enhance the nonlinear optical response of a prototype NF LC, DIO. We mixed an organic nonlinear optical crystalline material, 3,5,5-trimethyl (cyclohex-2-enylidene) malononitrile (TCM), with DIO and investigated the effects of TCM doping at various concentrations. We quantitatively determined the second-harmonic generation and spontaneous polarization as functions of temperature and concentration. We found that, compared with the pure DIO, the second-harmonic generation performance increased by about 130% at maximum, 93% in maximum for the nonlinear optical coefficient, and 10% in maximum for spontaneous polarization.

Topological Optical Waveguiding of Exciton‐Polariton Condensates

Abstract1D models with topological non‐trivial band structures are a simple and effective way to study novel and exciting concepts in topological photonics. In this work, the propagation of light‐matter quasi‐particles, so‐called exciton‐polaritons, is studied in waveguide arrays. Specifically, topological states are being investigated at the interface between dimer chains, characterized by a non‐zero winding number. In order to exercise precise control over the polariton propagation, non‐resonant laser excitation, as well as resonant excitation, are studied in transmission geometry. The results highlight a new platform for the study of quantum fluids of light and non‐linear optical propagation effects in coupled semiconductor waveguides.

Utilizing a synergistic strategy that combines electromagnetic and chemical enhancement to analyze the SERS effect of the Fe3O4@GO@Ag on PAHs detection

A comprehensive understanding of the enhancement mechanism of the substrate material is crucial to ensure the repeatability and functionality of SERS detection technology. Therefore, this study introduces a theoretical analysis method that integrates electromagnetic and chemical enhancement to achieve a comprehensive understanding of the SERS effect on the magnetic composite substrate. The visual model is employed in this study to comprehensively analyze and illustrate the electric field enhancement and optical effects of composite substrate materials. The study also elucidated the adsorption and charge transfer between the substrate material and target molecules. Based on this theory, Fe3O4@GO@Ag material was prepared and used to detect hydrophobic organic molecules such as polycyclic aromatic hydrocarbons (PAHs), with a concentration as low as 0.5 nM. This study comprehensively analyzed the SERS enhancement effect of the composite substrate for the first time, and prepared a magnetic composite substrate material for the detection of hydrophobic organic molecules, opening up a new avenue for theoretical guidance and experimental exploration in SERS detection and analysis.

Vector magnetic field characteristics of magneto-shape effect with high figure of merit based on fiber optic vernier effect

The vector magnetic field structures utilizing magnetic fluid (MF) mainly rely on the magneto-refractive index effect (MRI), which has the low spatial resolution due to the long sensitive length. In this article, the vector magnetic field characteristics of the magneto-shape effect (MSE) are simulated and experimentally studied based on the fiber optic vernier effect. The high vector magnetic field sensitivity can be achieved under the condition of Φ128*73 μm in the sensitive area by combine the MSE and vernier effect. The distribution of magnetic field on the concavity of MF varies with magnetic field direction, giving rising to MF concavity different deformations. The magnetic field observation structure based on fiber optic vernier effect are fabricated to verify the vector magnetic field characteristics of MSE. The observation structure is subjected to one-dimensional and two-dimensional magnetic field. The test results demonstrate that the magnetic field sensibility can reach 2.36 nm/Gs, 3.88 nm/Gs and 4.52 nm/Gs under 0–55.0 Gs, 55.0–91.7 Gs and 91.7–119.2 Gs in Y direction field. The magnetic field sensibility is 0.91 nm/Gs in Z direction field. The magnetic field direction sensitivity can reach 1.16 nm/° in XY dimensional field. The structure of the MSE is very compact and the size is very small, which is very helpful for detecting the narrow space and gradient magnetic field.

Giant Kerr nonlinearity of terahertz waves mediated by stimulated phonon polaritons in a microcavity chip

Optical Kerr effect, in which input light intensity linearly alters the refractive index, has enabled the generation of optical solitons, supercontinuum spectra, and frequency combs, playing vital roles in the on-chip devices, fiber communications, and quantum manipulations. Especially, terahertz Kerr effect, featuring fascinating prospects in future high-rate computing, artificial intelligence, and cloud-based technologies, encounters a great challenge due to the rather low power density and feeble Kerr response. Here, we demonstrate a giant terahertz frequency Kerr nonlinearity mediated by stimulated phonon polaritons. Under the influences of the giant Kerr nonlinearity, the power-dependent refractive index change would result in a frequency shift in the microcavity, which was experimentally demonstrated via the measurement of the resonant mode of a chip-scale lithium niobate Fabry-Pérot microcavity. Attributed to the existence of stimulated phonon polaritons, the nonlinear coefficient extracted from the frequency shifts is orders of magnitude larger than that of visible and infrared light, which is also theoretically demonstrated by nonlinear Huang equations. This work opens an avenue for many rich and fruitful terahertz Kerr effect based physical, chemical, and biological systems that have terahertz fingerprints.

Enhancement of nonlinear optic effect of the second harmonic generation in plasmonic waveguide using graphene and pyramid-shape gold nanoparticles

Enhancement of nonlinear optic effect of the second harmonic generation in plasmonic waveguide using graphene and pyramid-shape gold nanoparticles

Nonlinear Responses and Optical Limitation of Copper Nanoparticles by Z-scan Method

Recently, copper particles in nano dimensions have been gaining attention because they have advanced features and potential applications in various fields. This work studies the nonlinear optical performance of copper nanoparticles. We utilized laser ablation to create copper nanoparticles. In this technique, a piece of copper in distilled water is irradiated using the laser beam. Laser ablation was done for 30 min. The optical nonlinearities are measured by means of the Z-scan technology. The open-aperture Z-scan experiments showed that Cu nanoparticles have strong nonlinear absorption. Through a closed aperture Z-scan experiment, we could analyze the nonlinear refraction of sample. We analyze the optical limiting effect of copper nanoparticles. A theoretical model is presented and shows that at high laser light intensity, nonlinear light scattering occurs. By analyzing the experimental data with the presented model, the values of optical nonlinearities of copper particles were found to be n2=0.8×10-19m2w-1 and γ=1.46×10-13m/W, respectively. Our work confirmed that Cu nanoparticles show outstanding nonlinear optical features, which can cause the development of nonlinear optics.

Polarizability inversion suspension for nonlinear optical limiting with a low limiting threshold.

We propose what we believe to be a novel nonlinear optical limiting (NOL) method with a low limiting threshold based on a light intensity-controlled polarizability inversion suspension (PIS). This suspension has negative polarizability under weak light, allowing stable propagation of weak light with a low loss. Nevertheless, the suspension reverses into positive polarizability due to the optical Kerr effect under strong light, resulting in enhanced scattering that rapidly attenuates the intense light. In a proof-of-concept experiment, PS (polystyrene)-CS2-CCl4 suspension is used as the example suspension. We experimentally verify the NOL performance of several samples. Among them, 4 g/L PS-CS2-CCl4 suspension with a volume ratio of 0.15 has the best optical limiting effect, with a high limiting capacity coefficient of 0.48 and a very low limiting threshold of 14.80 kW/cm2, which is an order magnitude lower than that of most common NOL materials. Therefore, the proposed method provides a new promising approach to achieve NOL of continuous wave laser with a low limiting threshold.

A Review on Underwater Wireless Optical Communication and Effect on Information Exchange

A Review on Underwater Wireless Optical Communication and Effect on Information Exchange

Real-time monitoring of fast gas dynamics with a single-molecule resolution by frequency-comb-referenced plasmonic phase spectroscopy

Surface plasmon resonance (SPR) sensors are based on photon-excited surface charge density oscillations confined at metal-dielectric interfaces, which makes them highly sensitive to biological or chemical molecular bindings to functional metallic surfaces. Metal nanostructures further concentrate surface plasmons into a smaller area than the diffraction limit, thus strengthening photon-sample interactions. However, plasmonic sensors based on intensity detection provide limited resolution with long acquisition time owing to their high vulnerability to environmental and instrumental noises. Here, we demonstrate fast and precise detection of noble gas dynamics at single molecular resolution via frequency-comb-referenced plasmonic phase spectroscopy. The photon-sample interaction was enhanced by a factor of 3,852 than the physical sample thickness owing to plasmon resonance and thermophoresis-assisted optical confinement effects. By utilizing a sharp plasmonic phase slope and a high heterodyne information carrier, a small atomic-density modulation was clearly resolved at 5 Hz with a resolution of 0.06 Ar atoms per nano-hole (in 10–11 RIU) in Allan deviation at 0.2 s; a faster motion up to 200 Hz was clearly resolved. This fast and precise sensing technique can enable the in-depth analysis of fast fluid dynamics with the utmost resolution for a better understanding of biomedical, chemical, and physical events and interactions.

The Directional Design of the Quasi‐Phase‐Matching Short‐Wave Ultraviolet Nonlinear Optical Crystal

AbstractSince the study of short‐wave ultraviolet nonlinear optical crystals based on the quasi‐phase‐matching principle will effectively expand the development field of nonlinear optical materials, it is urgent to achieve their directional design. Here, it is proposed and implemented on account of the hexagonal wurtzite structure. Thus, the LiRbSeO4 crystal is obtained with [SeO4] groups as the main tetrahedra and [LiO4] as the separation. It exhibits a wide transparency window (0.22–5.57 µm) and an excellent nonlinear optical effect (≈1.7 × KH2PO4), which originates from the synergy of distorted tetrahedral groups and their uniform arrangement. More importantly, the LiRbSeO4 crystal is confirmed to be a ferroelectric with a typical polarization‐electric field hysteresis loop (a coercive field of 27.71 kV cm−1, a remanent polarization of 8.60 µC cm−2 at 373 K). Its ferroelectricity is further identified by the domain engineering studies, involving piezoelectricity and the chirality. Besides, ferroelectricity is attributed to the ordered arrangement of tetrahedra with the polarization reversal involving atomic displacements. Therefore, the LiRbSeO4 crystal is a promising short‐wave ultraviolet nonlinear optical candidate based on the quasi‐phase‐matching principle. This work also provides a new horizon for the design of nonlinear optical crystals.

Mie-resonant metaphotonics

Mie-resonant metaphotonics is a rapidly developing field that employs the physics of Mie resonances to control light at the nanoscale. Mie resonances are excited in high-refractive-index transparent nanoparticles and voids created in dielectric media, and they can be used to achieve a wide range of optical effects, including enhanced light–matter interaction, nonlinear optical effects, and topological photonics. Here, we review the recent advances in Mie-resonant metaphotonics, with a focus on the physics of Mie resonances and their applications in metaphotonics and metasurfaces. Through a comprehensive multipolar analysis, we demonstrate the complex interplay of electric and magnetic multipoles that govern their interaction with light. Recent advances have unveiled a diverse spectrum of scattering phenomena that can be achieved within precisely engineered structures. Within this framework, we review the underlying mechanics of the first and second Kerker conditions and describe the intricate mechanisms guiding these nanostructures’ light-scattering properties. Moreover, we cover intriguing phenomena such as the anapole and bound or quasi-bound states in the continuum. Of profound interest are the numerous practical applications that result from these revelations. Ultrafast processes, the emergence of nanolasers, and advancements in magneto-optic devices represent just a fraction of the transformative applications.

The nonlinear optical properties of meso-substituted porphyrins using spatial self-phase modulation

Herein, we studied the nonlinear optical properties of four meso-substituted porphyrins (H2MHTPP, H2THTPP, H2DETPP, and H2TETPP) by the spatial self-phase modulation (SSPM) method, using CW lasers with wavelengths of 532 nm and 780 nm. All samples exhibit strong nonlinear response due to the thermal optical nonlinear effect at 532 nm, which corresponds to the strong absorption band. In addition, four porphyrin samples were calculated that have nonlinear refractive index coefficients of the same order of magnitude (10−10 m2/W) at 532 nm. However, four porphyrins exhibited different optical nonlinear responses affected by the type and numbers of peripheral substituents at 780 nm. This work is of significance for reasonably adjusting the structure of compounds and improving their third-order nonlinear optical coefficients.

A four core fiber temperature and strain dual parameter sensor based on T-shaped taper

A four core fiber temperature and strain dual parameter sensor based on T-shaped taper is proposed and prepared. The sensor is composed of single-mode fiber (SMF), multi-mode fiber (MMF), and four core fiber (FCF). Among them, MMF plays a role in beam expansion, and FCF is tapered and fused with SMF to form a T-shaped taper structure, thereby preparing a sensor based on Mach Zehnder interference principle. When the external environmental temperature and strain change, due to thermal effect and elastic optical effect, the refractive index of the FCF cladding and fiber core changes differently, resulting in shift in the interference spectrum. Based on the temperature and strain sensitivity at different interference valleys, the temperature and strain dual parameter matrix equation of the sensor can be obtained. The experimental results indicate that when the temperature rises within the range of 30 ℃ to 90 ℃, the sensor spectrum shows a red shift phenomenon, and the maximum temperature sensitivity can reach 55 pm/ ℃. When the strain increases within the range of 0 με∼ 2000 με, the transmission spectrum of the sensor exhibits a blue shift phenomenon, and the maximum strain sensitivity can reach −2.6 pm/ με. Finally, based on the experimental results, the matrix equation for dual parameter sensing can be obtained. This sensor is easy to manufacture and has high sensitivity. It can measure sensing parameters normally in micro magnetic and micro electric field environments.