When confronting the dual challenges of rapid urbanization and climate change, although extensive research has investigated the factors influencing urban carbon emissions and the practical strategies regarding urban vibrancy, the unclear mutual nexus between them and the development strategy for collaborative optimization requires further in-depth analysis. This study explores the delicate balance between urban vibrancy and low-carbon sustainability within the confines of Beijing’s Fifth Ring Road. By integrating OpenStreetMap, land use, population, and buildings’ carbon emission data, we have developed a reproducible method to estimate total carbon emissions and emission intensity. Furthermore, we have introduced vibrancy index data to distinguish the vibrancy evaluation of residential and non-residential land and applied cross-combinational classification technology to dissect the spatial correlation between urban carbon emissions and urban vibrancy. The results reveal that the four combination typologies show more significant differences and regularity in residential land. Based on the discovery of spatial correlation, this study puts forward corresponding development strategy suggestions for each of these four typologies based on the geographical location and requirements of urban development policies. In conclusion, our study highlights the importance of integrating carbon emissions and urban vibrancy comprehensively in sustainable urban planning and proposes that various land use combinations need targeted development strategies to achieve this goal, which need to consider population, energy, service facilities, and other diverse aspects.