This paper reports the result of an investigation into the nonlinear viscoelastic dynamic characteristics of bi-graphene sheets/piezoelectric (BGP) laminated films subjected to moving particles (gas molecules, lithium ion, catalyst molecules, etc.). Based on the nonlocal elasticity theory and the von Kármán nonlinear geometric relation, and considering a rigorous van der Waals force between any two layers and the viscoelastic behavior of piezoelectric, the nonlinear viscoelastic dynamic equations of BGP laminated films is found by utilizing Hamilton's principles and Galerkin method. A reformulated differential quadrature method (DQM) is used to solve the nonlinear viscoelastic dynamic equation. Results show that the applied voltage and the mass of moving particles appear in larger effect on the nonlinear dynamic characteristics of BGP laminated films; the viscoelastic behavior of piezoelectric layer decreases the nonlinear dynamic amplitude of BGP laminated films only in free vibration part; the difference between linear and nonlinear solutions depends on the speed of moving particles. The obtained new features and interesting results about the nonlinear viscoelastic dynamic responses of bi-graphene/piezoelectric laminated films under moving particles in this paper are helpful for the design of chemical, physical and biomechanical sensors for the possible applications in sensing mass, force and charge, in which graphene/piezoelectric films act as basic elements, and will trigger a wave of research on the graphene/piezoelectric films based electrical elements or devises in the near future.