A method of nonlinear optimization based on the Laplace–Carson transform to determine the parameters of a model of the mechanical behavior of viscous materials is presented. The introduction of time-dependent functional relationships between stresses and strains leads to an analysis of the Volterra integral equation of the second kind. In practice, this equation is successfully used in modeling a wide class of structural materials. One of optimum kernels of the operator in the governing equation for describing the deformation of materials with “memory” is the Rabotnov fractional-exponential function. The search for the optimum values of model parameters is reduced to the problem of minimization of a functional. The results of analytic modeling are compared with experimental data obtained in the creep and quasi-static loading of polymer composites containing various carbon modifications in the form of nanotubes. The essential distinctions in the behavior of the nanocomposites are compared. These distinctions are found to correlate with the results of structural investigations by the atomic-force microscopy, scanning electron microscopy, and micro- and nanoindentation.