Nontrivial Berry Curvature Research Articles

Berry curvature, orbital magnetization, and Nernst effect in biased bilayer WSe2

A valley-contrasting Berry curvature in bilayer transition metal dichalcogenides with spin-orbit coupling can generate valley magnetization when the inversion symmetry is broken, for example, by an electric field, regardless of time-reversal symmetry. A nontrivial Berry curvature can also lead to anomalous transport responses, such as the anomalous Hall effect and the anomalous Nernst effect. Applied to a bilayer $\mathrm{W}{\mathrm{Se}}_{2}$, an electric field can tune the Berry curvature and orbital magnetic moment, which has important consequences for the orbital magnetization and the anomalous Nernst responses. The orbital magnetization and its two contributions, one due to the magnetic moment and one due to the Berry curvature, are calculated and interpreted in terms of opposite circulating currents of the bands in the two layers. The valley anomalous Nernst coefficient and spin Nernst coefficient are also calculated. We find that a finite electric field leads to peaks and dips in the Nernst responses that have the signs of the Berry curvatures of the bands and are proportional to their magnitudes; it also enhances the valley Nernst responses. These experimentally verifiable findings may be promising for caloritronic applications.

Thermal transport for probing quantum materials

Abstract

Controllable inversion symmetry breaking in single layer graphene induced by sub-lattice contrasted charge polarization

It has been revealed that inversion symmetry breaking in graphene could induce non-trivial Berry curvature, which leads to topologically protected valleytronic applications. Here, we propose an active controllable way of realizing the inversion symmetry breaking of single layer graphene, which is induced by the contrasted AB sub-lattice charge polarization. Our theory model indicates the split of in-plane optical phonons (iTO/iLO) at Γ point is the direct result of inversion symmetry breaking in single layer graphene. Density functional theory calculation was used to quantify the sub-lattice charge polarization and the split of iTO/iLO phonons under the external in-plane electric field, which was further confirmed by Raman spectroscopy. We believe that the method of symmetry manipulation by external in-plane electric field advances fundamental comprehension for the inner mechanism of topological phase transition of graphene.

Generalized triple-component fermions: Lattice model, Fermi arcs, and anomalous transport

We generalize the construction of time-reversal symmetry-breaking triple-component semimetals, transforming under the pseudospin-1 representation, to arbitrary (anti-)monopole charge $2 n$, with $n=1,2,3$ in the crystalline environment. The quasiparticle spectra of such systems are composed of two dispersing bands with pseudospin projections $m_s=\pm 1$ and energy dispersions $E_{\bf k}=\pm \sqrt{ \alpha^2_n k^{2n}_\perp +v^2_z k^2_z}$, where $k_\perp=\sqrt{k^2_x+k^2_y}$, and one completely flat band at zero energy with $m_s=0$. We construct simple tight-binding models for such spin-1 excitations on a cubic lattice and address the symmetries of the generalized triple-component Hamiltonian. In accordance to the bulk-boundary correspondence, triple-component semimetals support $2 n$ branches of topological Fermi arc surface states and also accommodate a \emph{large} anomalous Hall conductivity (in the $xy$ plane), given by $\sigma^{\rm 3D}_{xy} \propto 2 n \times$ the separation of the triple-component nodes (in units of $e^2/h$). Furthermore, we compute the longitudinal magnetoconductivity, planar Hall conductivity, and magneto thermal conductivity in these systems, which increase as $B^2$ for sufficiently weak magnetic fields ($B$) due to the nontrivial Berry curvature in the medium. A generalization of our construction to arbitrary integer spin systems is also highlighted.

Origin of planar Hall effect in type-II Weyl semimetal MoTe2

Besides the negative longitudinal magnetoresistance (MR), planar Hall effect (PHE) is a newly emerging experimental tool to test the chiral anomaly or nontrivial Berry curvature in Weyl semimetals (WSMs). However, the origins of PHE in various systems are not fully distinguished and understood. Here we perform a systematic study on the PHE and anisotropic MR (AMR) of Td-MoTe2, a type-II WSM. Although the PHE and AMR curves can be well fitted by the theoretical formulas, we demonstrate that the anisotropic resistivity arises from the orbital MR (OMR), instead of the negative MR as expected in the chiral anomaly effect. In contrast, the positive MR indicates that the large OMR dominates over the chiral anomaly effect. This explains why it is difficult to measure negative MR in type-II WSMs. We argue that the measured PHE can be related with the chiral anomaly only when the negative MR is simultaneously observed.

Quantum transport in topological semimetals under magnetic fields (II)

We review our recent works on the quantum transport, mainly in topological semimetals and also in topological insulators, organized according to the strength of the magnetic field. At weak magnetic fields, we explain the negative magnetoresistance in topological semimetals and topological insulators by using the semiclassical equations of motion with the nontrivial Berry curvature. We show that the negative magnetoresistance can exist without the chiral anomaly. At strong magnetic fields, we establish theories for the quantum oscillations in topological Weyl, Dirac, and nodal-line semimetals. We propose a new mechanism of 3D quantum Hall effect, via the "wormhole" tunneling through the Weyl orbit formed by the Fermi arcs and Weyl nodes in topological semimetals. In the quantum limit at extremely strong magnetic fields, we find that an unexpected Hall resistance reversal can be understood in terms of the Weyl fermion annihilation. Additionally, in parallel magnetic fields, longitudinal resistance dips in the quantum limit can serve as signatures for topological insulators.

Observation of planar Hall effect in topological semimetal ZrSiSe device

Planar Hall effect(PHE) is a newly emerging experimental tool to detect chiral anomaly and nontrivial Berry curvature in topological semimetals, as chiral-anomaly-induced negative magnetoresistance is sensitive to the angle between magnetic field <i>B</i> and current <i>I</i>. Here we demonstrate the PHE in a topological nodal-line semimetal ZrSiSe device by electric transport measurement. According to our analysis, we conclude that the PHE results from the trivial anisotropic magnetoresistance (AMR). We argue that there is no inevitability between PHE and chiral anomaly, and some other mechanisms can induce PHE. This work indicates that PHE cannot be considered as evidence of chiral anomaly and one may seek for non-topological origin in such studies.

Planar Hall effect in the type-II Dirac semimetal VAl3

The study of electronic properties in topological systems is one of the most fascinating topics in condensed matter physics, which has generated enormous interests in recent times. New materials are frequently being proposed and investigated to identify their non-trivial band structure. While sophisticated techniques such as angle-resolved photoemission spectroscopy have become popular to map the energy-momentum relation, the transport experiments lack any direct confirmation of Dirac and Weyl fermions in a system. From band structure calculations, VAl$_{3}$ has been proposed to be a type II topological Dirac semimetal. This material represents a large family of isostructural compounds, all having similar electronic band structure and is an ideal system to explore the rich physics of Lorentz symmetry violating Dirac fermions. In this work, we present a detailed analysis on the magnetotransport properties of VAl$_{3}$. A large, non-saturating magnetoresistance has been observed. Hall resistivity reveals the presence of two types of charge carriers with high mobility. Our measurements show a large planar Hall effect in this material, which is robust and can be easily detectable up to high temperature. This phenomenon originates from the relativistic chiral anomaly and non-trivial Berry curvature, which validates the theoretical prediction of the Dirac semimetal phase in VAl$_{3}$.

Chiral Anomaly as the Origin of the Planar Hall Effect in Weyl Semimetals.

In condensed matter physics, the term "chiral anomaly" implies the violation of the separate number conservation laws of Weyl fermions of different chiralities in the presence of parallel electric and magnetic fields. One effect of the chiral anomaly in the recently discovered Dirac and Weyl semimetals is a positive longitudinal magnetoconductance. Here we show that chiral anomaly and nontrivial Berry curvature effects engender another striking effect in Weyl semimetals, the planar Hall effect (PHE). Remarkably, the PHE manifests itself when the applied current, magnetic field, and the induced transverse "Hall" voltage all lie in the same plane, precisely in a configuration in which the conventional Hall effect vanishes. In this work we treat the PHE quasiclassically, and predict specific experimental signatures for type-I and type-II Weyl semimetals that can be directly checked in experiments.

Zeno Hall Effect.

We show that the quantum Zeno effect gives rise to the Hall effect by tailoring the Hilbert space of a two-dimensional lattice system into a single Bloch band with a nontrivial Berry curvature. Consequently, a wave packet undergoes transverse motion in response to a potential gradient-a phenomenon we call the Zeno Hall effect to highlight its quantum Zeno origin. The Zeno Hall effect leads to retroreflection at the edge of the system due to an interplay between the band flatness and the nontrivial Berry curvature. We propose an experimental implementation of this effect with ultracold atoms in an optical lattice.

Kondo screening in two-dimensional p -type transition-metal dichalcogenides

Systems with strong spin orbit coupling support a number of new phases of matter and novel phenomena. This work focuses on the interplay of spin orbit coupling and interactions in yielding correlated phenomena in two dimensional transition metal dichalcogenides. In particular we explore the physics of Kondo screening resulting from the lack of centro-symmetry, large spin splitting and spin valley locking in hole doped systems. The key ingredients are i) valley dependent spin-momentum locking perpendicular to the two dimensional crystal; ii) single nondegenerate Fermi surface per valley, and iii) nontrivial Berry curvature associated with the low energy bands. The resulting Kondo resonance has a finite triplet component and nontrivial momentum space structure which facilitates new approaches to both probe and manipulate the correlated state. Using a variational wave function and the numerical renormalization group approaches we study the nature of the Kondo resonance both in the absence and presence of circularly polarized light. The latter induces an imbalance in the population of the two valleys leading to novel magnetic phenomena in the correlated state.

Chiral Second-Sound Collective Modes at the Edge of 2D Systems with a Nontrivial Berry Curvature.

We study the thermal transport in two-dimensional systems with a nontrivial Berry curvature texture. The physical realizations are many; for the sake of definiteness, we consider undoped graphene gapped by the presence of an aligned hexagonal-boron-nitride substrate. The same phenomenology applies, i.e., to surface states of 3D topological insulators in the presence of a uniform magnetization. We find that chiral valley-polarized second-sound collective modes propagate along the edges of the system. The localization length of the edge modes has a topological origin stemming from the anomalous velocity term in the quasiparticle current. At low temperature, the single-particle contribution to the transverse thermal conductance is exponentially suppressed, and only second-sound modes carry heat along the boundary. A sharp change in the behavior of the thermal Hall conductance, extracted from nonlocal measurements of the temperature along the edge, marks the onset of ballistic heat transport due to second-sound edge modes.

Berry Fermi liquid theory

We develop an extension of the Landau Fermi liquid theory to systems of interacting fermions with non-trivial Berry curvature. We propose a kinetic equation and a constitutive relation for the electromagnetic current that together encode the linear response of such systems to external electromagnetic perturbations, to leading and next-to-leading orders in the expansion over the frequency and wave number of the perturbations. We analyze the Feynman diagrams in a large class of interacting quantum field theories and show that, after summing up all orders in perturbation theory, the current–current correlator exactly matches with the result obtained from the kinetic theory.

Magnon Spin Nernst Effect in Antiferromagnets.

We predict that a temperature gradient can induce a magnon-mediated spin Hall response in an antiferromagnet with nontrivial magnon Berry curvature. We develop a linear response theory which gives a general condition for a Hall current to be well defined, even when the thermal Hall response is forbidden by symmetry. We apply our theory to a honeycomb lattice antiferromagnet and discuss a role of magnon edge states in a finite geometry.

Spin torque and Nernst effects in Dzyaloshinskii-Moriya ferromagnets

We predict that a temperature gradient can induce a magnon-mediated intrinsic torque and a transverse spin current in systems with non-trivial magnon Berry curvature. With the help of a microscopic linear response theory of nonequilibrium magnon-mediated torques and spin currents we identify the interband and intraband components that manifest in ferromagnets with Dzyaloshinskii-Moriya interactions and magnetic textures. To illustrate and assess the importance of such effects, we apply our theory to the magnon-mediated spin Nernst and torque responses in a kagome lattice ferromagnet.

Nernst and magnetothermal conductivity in a lattice model of Weyl fermions

Weyl semimetals (WSM) are topologically protected three dimensional materials whose low energy excitations are linearly dispersing massless Dirac fermions, possessing a non-trivial Berry curvature. Using semi-classical Boltzmann dynamics in the relaxation time approximation for a lattice model of time reversal (TR) symmetry broken WSM, we compute both magnetic field dependent and anomalous contributions to the Nernst coefficient. In addition to the magnetic field dependent Nernst response, which is present in both Dirac and Weyl semimetals, we show that, contrary to previous reports, the TR-broken WSM also has an anomalous Nernst response due to a non-vanishing Berry curvature. We also compute the thermal conductivities of a WSM in the Nernst (${\nabla T} \perp \mathbf{B}$) and the longitudinal (${\nabla T} \parallel \mathbf{B}$) set-up and confirm from our lattice model that in the parallel set-up, the Wiedemann-Franz law is violated between the longitudinal thermal and electrical conductivities due to chiral anomaly.

Nonlinear optical selection rule based on valley-exciton locking in monolayer ws2

Optical selection rule fundamentally determines the optical transition between energy states in a variety of physical systems from hydrogen atoms to bulk crystals such as GaAs. It is important for optoelectronic applications such as lasers, energy-dispersive X-ray spectroscopy and quantum computation. Recently, single layer transition metal dichalcogenide (TMDC) exhibits valleys in momentum space with nontrivial Berry curvature and excitons with large binding energy. However, it is unclear how the unique valley degree of freedom combined with the strong excitonic effect influences the optical excitation. Here we discover a new set of optical selection rules in monolayer WS2,imposed by valley and exciton angular momentum. We experimentally demonstrated such a principle for second harmonic generation (SHG) and two-photon luminescence (TPL). Moreover, the two-photon induced valley populations yield net circular polarized photoluminescence after a sub-ps interexciton relaxation (2p->1s) and last for 8 ps. The discovery of this new optical selection rule in valleytronic 2D system not only largely extend information degrees but sets a foundation in control of optical transitions that is crucial to valley optoeletronic device applications such as 2D valley-polarized light emitting diodes (LED), optical switches and coherent control for quantum computing.

Optical activity as a test for dynamic chiral magnetic effect of Weyl semimetals

Recent angle resolved photoemission spectroscopy measurements have identified an inversion symmetry breaking Weyl semimetal phase in TaAs and NbAs. In an inversion symmetry breaking Weyl semimetal the left and the right handed Weyl points can occur at different energies and the energy mismatch between the Weyl points of opposite chirality is known as the chiral chemical potential. In the presence of the chiral chemical potential, the nontrivial Berry curvature of the Weyl fermions gives rise to the \emph{dynamic} chiral magnetic effect. This describes how a time dependent magnetic field leads to an electrical current along the applied field direction, which is also proportional to the field strength. We derive a general formula for the dynamic chiral magnetic conductivity of the inversion symmetry breaking Weyl semimetal. We show that the measurement of the natural optical activity or rotary power provides a direct confirmation of the existence of the dynamic chiral magnetic effect in inversion symmetry breaking Weyl semimetals.

Optical gyrotropy in quadrupolar Kondo systems

Recent experiments point to a variety of intermetallic systems which exhibit exotic quadrupolar orders driven by the Kondo coupling between conduction electrons and localized quadrupolar degrees of freedom. Using a Luttinger $k\ifmmode\cdot\else\textperiodcentered\fi{}p$ Hamiltonian for the conduction electrons, we study the impact of such quadrupolar order on their energies and wave functions. We discover that such quadrupolar orders can induce a nontrivial Berry curvature for the conduction electron bands, leading to a nonvanishing optical gyrotropic effect. We estimate the magnitude of the gyrotropic response in a candidate quadrupolar material, ${\mathrm{PrPb}}_{3}$, and discuss the resulting Faraday rotation in thin films.

Spin–orbit coupling and semiclassical electron dynamics in noncentrosymmetric metals

Spin–orbit coupling of electrons with the crystal lattice plays a crucial role in materials without inversion symmetry, lifting spin degeneracy of the Bloch states and endowing the resulting nondegenerate bands with complex spin textures and topologically nontrivial wavefunctions. We present a detailed symmetry-based analysis of the spin–orbit coupling and the band degeneracies in noncentrosymmetric metals. We systematically derive the semiclassical equations of motion for fermionic quasiparticles near the Fermi surface, taking into account both the spin–orbit coupling and the Zeeman interaction with an applied magnetic field. Some of the lowest-order quantum corrections to the equations of motions can be expressed in terms of a fictitious “magnetic field” in the momentum space, which is related to the Berry curvature of the band wavefunctions. The band degeneracy points or lines serve as sources of a topologically nontrivial Berry curvature. We discuss the observable effects of the wavefunction topology, focusing, in particular, on the modifications to the Lifshitz–Onsager semiclassical quantization condition and the de Haas-van Alphen effect in noncentrosymmetric metals.