non-Markovian Quantum Dynamics Research Articles

Dynamical learning of non-Markovian quantum dynamics

We study the non-Markovian dynamics of an open quantum system with machine learning. The observable physical quantities and their evolutions are generated by using the neural network. After the pre-training is completed, we fix the weights in the subsequent processes thus do not need the further gradient feedback. We find that the dynamical properties of physical quantities obtained by the dynamical learning are better than those obtained by the learning of Hamiltonian and time evolution operator. The dynamical learning can be applied to other quantum many-body systems, non-equilibrium statistics and random processes.

Operational applications of the diamond norm and related measures in quantifying the non-physicality of quantum maps

Although quantum channels underlie the dynamics of quantum states, maps which are not physical channels — that is, not completely positive — can often be encountered in settings such as entanglement detection, non-Markovian quantum dynamics, or error mitigation. We introduce an operational approach to the quantitative study of the non-physicality of linear maps based on different ways to approximate a given linear map with quantum channels. Our first measure directly quantifies the cost of simulating a given map using physically implementable quantum channels, shifting the difficulty in simulating unphysical dynamics onto the task of simulating linear combinations of quantum states. Our second measure benchmarks the quantitative advantages that a non-completely-positive map can provide in discrimination-based quantum games. Notably, we show that for any trace-preserving map, the quantities both reduce to a fundamental distance measure: the diamond norm, thus endowing this norm with new operational meanings in the characterisation of linear maps. We discuss applications of our results to structural physical approximations of positive maps, quantification of non-Markovianity, and bounding the cost of error mitigation.

General Non-Markovian Quantum Dynamics.

A general approach to the construction of non-Markovian quantum theory is proposed. Non-Markovian equations for quantum observables and states are suggested by using general fractional calculus. In the proposed approach, the non-locality in time is represented by operator kernels of the Sonin type. A wide class of the exactly solvable models of non-Markovian quantum dynamics is suggested. These models describe open (non-Hamiltonian) quantum systems with general form of nonlocality in time. To describe these systems, the Lindblad equations for quantum observable and states are generalized by taking into account a general form of nonlocality. The non-Markovian quantum dynamics is described by using integro-differential equations with general fractional derivatives and integrals with respect to time. The exact solutions of these equations are derived by using the operational calculus that is proposed by Yu. Luchko for general fractional differential equations. Properties of bi-positivity, complete positivity, dissipativity, and generalized dissipativity in general non-Markovian quantum dynamics are discussed. Examples of a quantum oscillator and two-level quantum system with a general form of nonlocality in time are suggested.

Quantum Field Thermal Machines

Recent years have enjoyed an overwhelming interest in quantum thermodynamics, a field of research aimed at understanding thermodynamic tasks performed in the quantum regime. Further progress, however, seems to be obstructed by the lack of experimental implementations of thermal machines in which quantum effects play a decisive role. In this work, we introduce a blueprint of quantum field machines, which - once experimentally realized - would fill this gap. Even though the concept of the QFM presented here is very general and can be implemented in any many body quantum system that can be described by a quantum field theory. We provide here a detailed proposal how to realize a quantum machine in one-dimensional ultra-cold atomic gases, which consists of a set of modular operations giving rise to a piston. These can then be coupled sequentially to thermal baths, with the innovation that a quantum field takes up the role of the working fluid. In particular, we propose models for compression on the system to use it as a piston, and coupling to a bath that gives rise to a valve controlling heat flow. These models are derived within Bogoliubov theory, which allows us to study the operational primitives numerically in an efficient way. By composing the numerically modelled operational primitives we design complete quantum thermodynamic cycles that are shown to enable cooling and hence giving rise to a quantum field refrigerator. The active cooling achieved in this way can operate in regimes where existing cooling methods become ineffective. We describe the consequences of operating the machine at the quantum level and give an outlook of how this work serves as a road map to explore open questions in quantum information, quantum thermodynamic and the study of non-Markovian quantum dynamics.

Entropic Bounds on Information Backflow.

In the dynamics of open quantum systems, the backflow of information to the reduced system under study has been suggested as the actual physical mechanism inducing memory and thus leading to non-Markovian quantum dynamics. To this aim, the trace-distance revivals between distinct evolved system states have been shown to be subordinated to the establishment of system-environment correlations or changes in the environmental state. We show that this interpretation can be substantiated also for a class of entropic quantifiers. We exploit a suitably regularized version of Umegaki's quantum relative entropy, known as telescopic relative entropy, that is tightly connected to the quantum Jensen-Shannon divergence. In particular, we derive general upper bounds on the telescopic relative entropy revivals conditioned and determined by the formation of correlations and changes in the environment. We illustrate our findings by means of examples, considering in particular the Jaynes-Cummings model and a phase covariant dynamics.

Quantum Maps with Memory from Generalized Lindblad Equation.

In this paper, we proposed the exactly solvable model of non-Markovian dynamics of open quantum systems. This model describes open quantum systems with memory and periodic sequence of kicks by environment. To describe these systems, the Lindblad equation for quantum observable is generalized by taking into account power-law fading memory. Dynamics of open quantum systems with power-law memory are considered. The proposed generalized Lindblad equations describe non-Markovian quantum dynamics. The quantum dynamics with power-law memory are described by using integrations and differentiation of non-integer orders, as well as fractional calculus. An example of a quantum oscillator with linear friction and power-law memory is considered. In this paper, discrete-time quantum maps with memory, which are derived from generalized Lindblad equations without any approximations, are suggested. These maps exactly correspond to the generalized Lindblad equations, which are fractional differential equations with the Caputo derivatives of non-integer orders and periodic sequence of kicks that are represented by the Dirac delta-functions. The solution of these equations for coordinates and momenta are derived. The solutions of the generalized Lindblad equations for coordinate and momentum operators are obtained for open quantum systems with memory and kicks. Using these solutions, linear and nonlinear quantum discrete-time maps are derived.

Non-Markovian quantum dynamics: Extended correlated projection superoperators.

The correlated projection superoperator techniques provide a better understanding about how correlations lead to strong non-Markovian effects in open quantum systems. Their superoperators are independent of initial state, which may not be suitable for some cases. To improve this, we develop another approach, that is extending the composite system before use the correlated projection superoperator techniques. Such an approach allows the choice of different superoperators for different initial states. We apply these techniques to a simple model to illustrate the general approach. The numerical simulations of the full Schrödinger equation of the model reveal the power and efficiency of the method.

Equivalence between non-Markovian dynamics and correlation backflows

The information encoded into an open quantum system that evolves under a Markovian dynamics is always monotonically non-increasing. Nonetheless, for a given quantifier of the information contained in the system, it is in general not clear if for all non-Markovian dynamics it is possible to observe a non-monotonic evolution of this quantity, namely a backflow. We address this problem by considering correlations of finite-dimensional bipartite systems. For this purpose, we consider a class of correlation measures and prove that if the dynamics is non-Markovian there exists at least one element from this class that provides a correlation backflow. Moreover, we provide a set of initial probe states that accomplish this witnessing task. This result provides the first one-to-one relation between non-Markovian quantum dynamics and correlation backflows. Finally, we introduce a measure of non-Markovianity.

Effects of intramolecular vibrations on excitation energy transfer dynamics of the Fenna-Matthews-Olson complex

The role of vibrational coherence in photosynthetic pigment-proteins has been controversial. The present article investigates theoretically how the intramolecular vibrations of bacteriochlorophyll (BChl) influence the excitation energy transfer (EET) dynamics in the Fenna-Matthews-Olson complex (FMO). To this end, we use an exciton model incorporating recent experimental data and treat the vibrations as both coherent and incoherent. We simulate the transfer phenomena numerically with non-Markovian quantum dynamics. Our results at 300 K indicate that incoherent vibrations can moderately improve the efficiency of EET between FMO and a reaction center. With a vibronic model, we show that the coherent vibrations in either strongly or resonantly coupled BChl pairs can generate characteristic oscillations in their electronic populations which persist for several picoseconds even at 300 K. Despite such robust coherences, no significant improvement in the efficiency of EET is observed.

Experimental investigation of the effect of classical noise on quantum non-Markovian dynamics

We provide an experimental study of the relationship between the action of different classical noises on the dephasing dynamics of a two-level system and the non-Markovianity of the quantum dynamics. The two-level system is encoded in the photonic polarization degrees of freedom and the action of the noise is obtained via a spatial light modulator, thus allowing for an easy engineering of different random environments. The quantum non-Markovianity of the dynamics driven by classical Markovian and non-Markovian noise, both Gaussian and non-Gaussian, is studied by means of the trace distance. Our study clearly shows the different nature of the notion of non-Markovian classical process and non-Markovian quantum dynamics.

Non-Markovian quantum dynamics: What is it good for?

Recent developments in practical quantum engineering and control techniques have allowed significant developments for experimental studies of open quantum systems and decoherence engineering. Indeed, it has become possible to test experimentally various theoretical, mathematical, and physical concepts related to non-Markovian quantum dynamics. This includes experimental characterization and quantification of non-Markovian memory effects and proof-of-principle demonstrations how to use them for certain quantum communication and information tasks. We describe here recent experimental advances for open system studies, focussing in particular to non-Markovian dynamics including the applications of memory effects, and discuss the possibilities for ultimate control of decoherence and open system dynamics.

Non-Markovian quantum dynamics: What does it mean?

During the last ten years, the studies on non-Markovian open system dynamics has become increasingly popular and having contributions from diverse sets of research communities. This interest has arisen due to fundamental problematics as to how to define and quantify memory effects in the quantum domain, how to exploit and develop applications based on them, and also due to the following question: what are the ultimate limits for controlling open system dynamics? We give here a simple theoretical introduction to the basic approaches to define and quantify quantum non-Markovianity —also highlighting their connections and differences. In addition to the importance of the development for open quantum systems studies, we also discuss the implications of the progress for other fields including, e.g., formal studies of stochastic processes and quantum information science, and conclude with possible future directions the recent developments open.

Quantum process identification: a method for characterizing non-markovian quantum dynamics

Established methods for characterizing quantum information processes do not capture non-Markovian (history-dependent) behaviors that occur in real systems. These methods model a quantum process as a fixed map on the state space of a predefined system of interest. Such a map averages over the system’s environment, which may retain some effect of its past interactions with the system and thus have a history-dependent influence on the system. Although the theory of non-Markovian quantum dynamics is currently an active area of research, a systematic characterization method based on a general representation of non-Markovian dynamics has been lacking. In this article we present a systematic method for experimentally characterizing the dynamics of open quantum systems. Our method, which we call quantum process identification (QPI), is based on a general theoretical framework which relates the (non-Markovian) evolution of a system over an extended period of time to a time-local (Markovian) process involving the system and an effective environment. In practical terms, QPI uses time-resolved tomographic measurements of a quantum system to construct a dynamical model with as many dynamical variables as are necessary to reproduce the evolution of the system. Through numerical simulations, we demonstrate that QPI can be used to characterize qubit operations with non-Markovian errors arising from realistic dynamics including control drift, coherent leakage, and coherent interaction with material impurities.

Efficient non-Markovian quantum dynamics using time-evolving matrix product operators

In order to model realistic quantum devices it is necessary to simulate quantum systems strongly coupled to their environment. To date, most understanding of open quantum systems is restricted either to weak system–bath couplings or to special cases where specific numerical techniques become effective. Here we present a general and yet exact numerical approach that efficiently describes the time evolution of a quantum system coupled to a non-Markovian harmonic environment. Our method relies on expressing the system state and its propagator as a matrix product state and operator, respectively, and using a singular value decomposition to compress the description of the state as time evolves. We demonstrate the power and flexibility of our approach by numerically identifying the localisation transition of the Ohmic spin-boson model, and considering a model with widely separated environmental timescales arising for a pair of spins embedded in a common environment.

Reconstructing non-Markovian quantum dynamics with limited control

The dynamics of an open quantum system can be fully described and tomographically reconstructed if the experimenter has complete control over the system of interest. Most real-world experiments do not fulfill this assumption, and the amount of control is restricted by the experimental set-up. That is, the set of performable manipulations of the system is limited. For instance, imagine a set-up where unitary operations are easy to make, but only one measurement at the end of the experiment is allowed. In this paper, we provide a general reconstruction scheme that yields operationally well-defined dynamics for any conceivable kind of experimental situation. If one additional operation can be performed, these `restricted' dynamics allow for the construction of witnesses for initial correlations and the presence of memory effects. We demonstrate the applicability of our framework for the the two important cases where the set of performable operations comprises only unitary operations or projective measurements, respectively, and show that it provides a powerful tool for the description of quantum control experiments.

Non-Markovianity-assisted high-fidelity Deutsch\u2013Jozsa algorithm in diamond

The memory effects in non-Markovian quantum dynamics can induce the revival of quantum coherence, which is believed to provide important physical resources for quantum information processing (QIP). However, no real quantum algorithms have been demonstrated with the help of such memory effects. Here, we experimentally implemented a non-Markovianity-assisted high-fidelity refined Deutsch–Jozsa algorithm (RDJA) with a solid spin in diamond. The memory effects can induce pronounced non-monotonic variations in the RDJA results, which were confirmed to follow a non-Markovian quantum process by measuring the non-Markovianity of the spin system. By applying the memory effects as physical resources with the assistance of dynamical decoupling, the probability of success of RDJA was elevated above 97% in the open quantum system. This study not only demonstrates that the non-Markovianity is an important physical resource but also presents a feasible way to employ this physical resource. It will stimulate the application of the memory effects in non-Markovian quantum dynamics to improve the performance of practical QIP.

Dark state with counter-rotating dissipative channels

Dark state as a consequence of interference between different quantum states has great importance in the fields of chip-scale atomic clock and quantum information. For the Λ-type three-level system, this dark state is generally regarded as being dissipation-free because it is a superposition of two lowest states without dipole transition between them. However, previous studies are based on the rotating-wave approximation (RWA) by neglecting the counter-rotating terms in the system-environment interaction. In this work, we study non-Markovian quantum dynamics of the dark state in a Λ-type three-level system coupled to two bosonic baths and reveal the effect of counter-rotating terms on the dark state. In contrast to the dark state within the RWA, leakage of the dark state occurs even at zero temperature, as a result of these counter-rotating terms. Also, we present a method to restore the quantum coherence of the dark state by applying a leakage elimination operator to the system.

Implications of non-Markovian quantum dynamics for the Landauer bound

We study the dynamics of a spin-1/2 particle interacting with a multi-spin environment, modelling the corresponding open system dynamics through a collision-based model. The environmental particles are prepared in individual thermal states, and we investigate the effects of a distribution of temperatures across the spin environment on the evolution of the system, particularly how thermalisation in the long-time limit is affected. We study the phenomenology of the heat exchange between system and environment and consider the information-to-energy conversion process, induced by the system–environment interaction and embodied by the Landauer principle. Furthermore, by considering an interacting-particles environment, we tune the dynamics of the system from an explicit Markovian evolution up to a strongly non-Markovian one, investigating the connections between non-Markovianity, the establishment of system–environment correlations, and the breakdown of the validity of Landauer principle.

Colloquium: Non-Markovian dynamics in open quantum systems

The dynamical behavior of open quantum systems plays a key role in many applications of quantum mechanics, examples ranging from fundamental problems, such as the environment-induced decay of quantum coherence and relaxation in many-body systems, to applications in condensed matter theory, quantum transport, quantum chemistry and quantum information. In close analogy to a classical Markov process, the interaction of an open quantum system with a noisy environment is often modelled by a dynamical semigroup with a generator in Lindblad form, which describes a memoryless dynamics leading to an irreversible loss of characteristic quantum features. However, in many applications open systems exhibit pronounced memory effects and a revival of genuine quantum properties such as quantum coherence and correlations. Here, recent results on the rich non-Markovian quantum dynamics of open systems are discussed, paying particular attention to the rigorous mathematical definition, to the physical interpretation and classification, as well as to the quantification of memory effects. The general theory is illustrated by a series of examples. The analysis reveals that memory effects of the open system dynamics reflect characteristic features of the environment which opens a new perspective for applications, namely to exploit a small open system as a quantum probe signifying nontrivial features of the environment it is interacting with. This article further explores the various physical sources of non-Markovian quantum dynamics, such as structured spectral densities, nonlocal correlations between environmental degrees of freedom and correlations in the initial system-environment state, in addition to developing schemes for their local detection. Recent experiments on the detection, quantification and control of non-Markovian quantum dynamics are also discussed.

Quantum Langevin approach for non-Markovian quantum dynamics of the spin-boson model

One long-standing difficult problem in quantum dissipative dynamics is to solve the spin-boson model in a non-Markovian regime where a tractable systematic master equation does not exist. The spin-boson model is particularly important due to its crucial applications in quantum noise control and manipulation as well as its central role in developing quantum theories of open systems. Here we solve this important model by developing a non-Markovian quantum Langevin approach. By projecting the quantum Langevin equation onto the coherent states of the bath, we can derivie a set of non-Markovian quantum Bloch equations containing no explicit noise variables. This special feature offers a tremendous advantage over the existing stochastic Schr\"odinger equations in numerical simulations. The physical significance and generality of our approach are briefly discussed.