Multiple Dirac Cones Research Articles

Electronic band structure of 4d and 5d transition metal trichalcogenides

Transition metal trichalcogenides (TMTs), a family of van der Waals materials, have gained increasing interests from the discovery of magnetism in few-layer forms. Although TMTs with 3d transition metal elements have been studied extensively, much less is explored for the 4d and 5d cases, where the interesting interplay between electron correlations and the relativistic spin-orbit coupling is expected. Using ab initio calculations, we here investigate the electronic property of TMTs with 4d and 5d transition metal elements. We show that the band structures exhibit multiple node-like features near the Fermi level. These are the remnant of multiple Dirac cones that were recently discovered in the monolayer cases. Our results indicate that the peculiar two-dimensional multiple Dirac cones are concealed even in the layered bulk systems.

First-Principles Prediction of Spin-Polarized Multiple Dirac Rings in Manganese Fluoride.

Spin-polarized materials with Dirac features have sparked great scientific interest due to their potential applications in spintronics. But such a type of structure is very rare and none has been fabricated. Here, we investigate the already experimentally synthesized manganese fluoride (MnF_{3}) as a novel spin-polarized Dirac material by using first-principles calculations. MnF_{3} exhibits multiple Dirac cones in one spin orientation, while it behaves like a large gap semiconductor in the other spin channel. The estimated Fermi velocity for each cone is of the same order of magnitude as that in graphene. The 3D band structure further reveals that MnF_{3} possesses rings of Dirac nodes in the Brillouin zone. Such a spin-polarized multiple Dirac ring feature is reported for the first time in an experimentally realized material. Moreover, similar band dispersions can be also found in other transition metal fluorides (e.g., CoF_{3}, CrF_{3}, and FeF_{3}). Our results highlight a new interesting single-spin Dirac material with promising applications in spintronics and information technologies.

Multiple Dirac cones at the surface of the topological metal LaBi

The rare-earth monopnictide LaBi exhibits exotic magneto-transport properties, including an extremely large and anisotropic magnetoresistance. Experimental evidence for topological surface states is still missing although band inversions have been postulated to induce a topological phase in LaBi. In this work, we have revealed the existence of surface states of LaBi through the observation of three Dirac cones: two coexist at the corners and one appears at the centre of the Brillouin zone, by employing angle-resolved photoemission spectroscopy in conjunction with ab initio calculations. The odd number of surface Dirac cones is a direct consequence of the odd number of band inversions in the bulk band structure, thereby proving that LaBi is a topological, compensated semimetal, which is equivalent to a time-reversal invariant topological insulator. Our findings provide insight into the topological surface states of LaBi’s semi-metallicity and related magneto-transport properties.

Towards large-Chern-number topological phases by periodic quenching

Topological phases with large Chern numbers have important implications. They were previously predicted to exist by considering fabricated long-range interactions or multi-layered materials. Stimulated by recent wide interests in Floquet topological phases, here we propose a scheme to engineer large-Chern-number phases with ease by periodic quenching. Using a two-band system as an example, we theoretically show how a variety of topological phases with widely tunable Chern numbers can be generated by periodic quenching between two simple Hamiltonians that otherwise give low Chern numbers. The obtained large Chern numbers are explained through the emergence of multiple Dirac cones in the Floquet spectra. The transition lines between different topological phases in the two-band model are also explicitly found, thus establishing a class of easily solvable but very rich systems useful for further understandings and applications of topological phases in periodically driven systems.

Hedgehog spin texture and competing orders associated with strains on the surface of a topological crystalline insulator

We have investigated spin reorientation phenomena and interaction driven effects under the presence of applied strains on the (001) surface of Pb$_{1-x}$Sn$_x$(Te, Se) topological crystalline insulators, which host multiple Dirac cones. Our analysis is based on a four-band $k\cdot p$ model, which captures the spin and orbital textures of the surface states at low energies around the $\bar{X}$ and $\bar{Y}$ points, including the Lifshitz transition. Even without breaking the time-reversal symmetry, we find that certain strains which break the mirror symmetry can induce hedgehog-like spin texture associated with gap formation at the Dirac points. The Chern number of the gapped surface ground state is shown to be tunable through the interplay of strains and a perpendicular Zeeman field. We also consider effects of strain in the presence of interactions in driving competing orders, and obtain the associated phase diagram at the mean-field level. Potential applications of our results for low power consuming electronics are discussed.

Tunability of 1/f Noise at Multiple Dirac Cones in hBN Encapsulated Graphene Devices.

The emergence of multiple Dirac cones in hexagonal boron nitride (hBN)-graphene heterostructures is particularly attractive because it offers potentially better landscape for higher and versatile transport properties than the primary Dirac cone. However, the transport coefficients of the cloned Dirac cones is yet not fully characterized and many open questions, including the evolution of charge dynamics and impurity scattering responsible for them, have remained unexplored. Noise measurements, having the potential to address these questions, have not been performed to date in dual-gated hBN-graphene-hBN devices. Here, we present the low-frequency 1/f noise measurements at multiple Dirac cones in hBN encapsulated single and bilayer graphene in dual-gated geometry. Our results reveal that the low-frequency noise in graphene can be tuned by more than two-orders of magnitude by changing carrier concentration as well as by modifying the band structure in bilayer graphene. We find that the noise is surprisingly suppressed at the cloned Dirac cone compared to the primary Dirac cone in single layer graphene device, while it is strongly enhanced for the bilayer graphene with band gap opening. The results are explained with the calculation of dielectric function using tight-binding model. Our results also indicate that the 1/f noise indeed follows the Hooge's empirical formula in hBN-protected devices in dual-gated geometry. We also present for the first time the noise data in bipolar regime of a graphene device.

Multiple Dirac cones in BN co-doped β-graphyne

BN co-doped β-graphyne (β-GY) was investigated using state-of-the-art theoretical calculations.

Electrically tunable multiple Dirac cones in thin films of the (LaO)2(SbSe2)2 family of materials.

Two-dimensional Dirac physics has aroused great interests in condensed matter physics ever since the discovery of graphene and topological insulators. The ability to control the properties of Dirac cones, such as bandgap and Fermi velocity, is essential for various new phenomena and the next-generation electronic devices. On the basis of first-principles calculations and an analytical effective model, we propose a new Dirac system with eight Dirac cones in thin films of the (LaO)2(SbSe2)2 family of materials, which has the advantage in its tunability: the existence of gapless Dirac cones, their positions, Fermi velocities and anisotropy all can be controlled by an experimentally feasible electric field. We identify layer-dependent spin texture induced by spin-orbit coupling as the underlying physical reason for electrical tunability of this system. Furthermore, the electrically tunable quantum anomalous Hall effect with a high Chern number can be realized by introducing magnetization into this system.

Matter waves in two-dimensional arbitrary atomic crystals

We present a general scheme to realize a cold-atom quantum simulator of bidimensional atomic crystals. Our model is based on the use of two independently trapped atomic species: the first one, subject to a strong in-plane confinement, constitutes a two-dimensional matter wave which interacts only with atoms of the second species, deeply trapped around the nodes of a two-dimensional optical lattice. By introducing a general analytic approach we show that the system Green function can be exactly determined, allowing for the investigation of the matter-wave transport properties. We propose some illustrative applications to both Bravais (square, triangular) and non-Bravais (graphene, kagom\'e) lattices, studying both ideal periodic systems and experimental-size and disordered ones. Some remarkable spectral properties of these atomic artificial lattices are pointed out, such as the emergence of single and multiple gaps, flat bands, and Dirac cones. All these features can be manipulated via the interspecies interaction, which proves to be widely tunable due to the interplay between scattering length and confinements.

Mapping the unconventional orbital texture in topological crystalline insulators

The newly discovered topological crystalline insulators (TCIs) harbor a complex band structure involving multiple Dirac cones. These materials are potentially highly tunable by external electric field, temperature or strain and could find future applications in field-effect transistors, photodetectors, and nano-mechanical systems. Theoretically, it has been predicted that different Dirac cones, offset in energy and momentum-space, might harbor vastly different orbital character, a unique property which if experimentally realized, would present an ideal platform for accomplishing new spintronic devices. However, the orbital texture of the Dirac cones, which is of immense importance in determining a variety of materials properties, still remains elusive in TCIs. Here, we unveil the orbital texture in a prototypical TCI Pb$_{1-x}$Sn$_x$Se. By using Fourier-transform (FT) scanning tunneling spectroscopy (STS) we measure the interference patterns produced by the scattering of surface state electrons. We discover that the intensity and energy dependences of FTs show distinct characteristics, which can directly be attributed to orbital effects. Our experiments reveal the complex band topology involving two Lifshitz transitions and establish the orbital nature of the Dirac bands in this new class of topological materials, which could provide a different pathway towards future quantum applications.

Topological states inBi2Se3surfaces created by cleavage within a quintuple layer: Analysis in terms of the Shockley criterion

In topologically trivial materials, the existence of surface states within the bulk band gap depends on the surface condition. A surface state exists if the system is Shockley inverted, and vice versa; furthermore, this surface condition in a superlattice can be tuned from one case to the other by varying the terminating atomic plane within a superlattice period. By contrast, we demonstrate here based on first-principles calculations for ${\text{Bi}}_{2}$${\text{Se}}_{3}$ cleaved at different atomic planes within a quintuple layer that topological surface states always span the bulk band gap in accordance with the topologically nontrivial nature of ${\text{Bi}}_{2}$${\text{Se}}_{3}$. However, the number of surface bands, the band dispersion relations, and the degree of spin polarization are strongly dependent on the cleavage plane. Multiple Dirac cones can exist at the zone center and/or zone boundary, and a massive but topologically nontrivial Dirac cone is observed for a Se-terminated surface. The results confirm the robustness of the topological nature of the system, but the details of the topological surface states themselves can vary substantially within the broad topological constraint. The persistent existence of topological states within the gap is discussed in terms of the Shockley criterion.

Generation of Multiple Dirac Cones in Graphene under Double-Periodic and Quasiperiodic Potentials

We investigate generation of new Dirac cones in graphene under double-periodic and quasiperiodic superlattice potentials. We first show that double-periodic potentials generate the Dirac cones sporadically, following the Diophantine equation, in spite of the fact that double-periodic potentials are also periodic ones, for which previous studies predict consecutive appearance of the cones. The sporadic appearance is due to the fact that the dispersion relation of graphene is linear only up to an energy cutoff. We then show that quasiperiodic potentials generate the new Dirac cones densely with its density depending on the energy. We also extend the above predictions to other materials of Dirac electrons with different energy cutoffs of the linear dispersion.

Driven electronic states at the surface of a topological insulator

Motivated by recent photoemission experiments on the surface of topological insulators we compute the spectrum of driven topological surface excitations in the presence of an external light source. We completely characterize the spectral function of these nonequilibrium electron excitations for both linear and circular polarizations of the incident light. We find that in the latter case, the circularly polarized light gaps out the surface states, whereas linear polarization gives rise to an anisotropic metal with multiple Dirac cones. We compare the sizes of the gaps with recent pump-probe photoemission measurements and find good agreement. We also identify theoretically several new features in the time-dependent spectral function, such as shadow Dirac cones.

Multiple Dirac fermions from a topological insulator and graphene superlattice

Graphene and three-dimensional topological insulators are well-known Dirac materials whose bulk and surface states are governed by Dirac equations. They not only show good transport properties but also carry various quanta related to the geometrical phase such as charge, spin, and valley Hall conductances. Therefore, it is a great challenge to combine the two Dirac materials together, realizing multiple Dirac fermions. By using first-principles density-functional-theory calculations, we demonstrate such a system built from topological insulator-band insulator-graphene superlattice structures. Hexagonal boron nitride is proposed as an ideal band-insulating material in gluing graphene and topological insulators, providing a good substrate for graphene and a sharp interface with a topological insulator. The power factors for $p$-type doping are largely enhanced due to the charge-conducting channels through multiple Dirac cones. The systems characterized by the coexistence of the topologically protected interfacial and graphene Dirac cones can pave the way for developing integrated devices for electronics, spintronics and valleytronics applications.

Manipulation of the Dirac cones and the anomaly in the graphene related quantum Hall effect

The quantum Hall effect in graphene is regarded to be involving half-integer topological numbers associated with the massless Dirac particle, this is usually not apparent due to the doubling of the Dirac cones. Here we theoretically consider two classes of lattice models in which we manipulate the Dirac cones with either (a) two Dirac points that have mutually different energies, or (b) multiple Dirac cones having different Fermi velocities. We have shown, with an explicit calculation of the topological (Chern) number for case (a) and with an adiabatic argument for case (b) that the results are consistent with the picture that a single Dirac fermion contributes the half-odd integer series (… -3/2, -1/2, 1/2, 3/2, …) to the Hall conductivity when the Fermi energy traverses the Landau levels.

Tunable Multiple Layered Dirac Cones in Optical Lattices

We show that multiple layered Dirac cones can emerge in the band structure of properly addressed multicomponent cold fermionic gases in optical lattices. The layered Dirac cones contain multiple copies of massless spin-1/2 Dirac fermions at the same location in momentum space, whose different Fermi velocity can be tuned at will. On-site microwave Raman transitions can further be used to mix the different Dirac species, resulting in either splitting of or preserving the Dirac point (depending on the symmetry of the on-site term). The tunability of the multiple layered Dirac cones allows us to simulate a number of fundamental phenomena in modern physics, such as neutrino oscillations and exotic particle dispersions with E~p(N) for arbitrary integer N.

Photonic analog of graphene model and its extension: Dirac cone, symmetry, and edge states

This paper investigates the topological phase transition in honeycomb lattice photonic crystals with and without time-reversal and space-inversion symmetries through extensive analysis on bulk and edge states. In the system with both the symmetries, there appear multiple Dirac cones in the photonic band structure, and the mass gaps are controllable via symmetry breaking. The zigzag and armchair edges of the photonic crystals can support novel edge states that reflect the symmetries of the photonic crystals. The dispersion relation and the field configuration of the edge states are analyzed in detail in comparison to electronic edge states. Leakage of the edge states to free space, which is inherent in photonic systems, is fully taken into account in the analysis. A topological relation between bulk and edge states, which has been discussed in the context of electronic quantum Hall effect, is also examined in the photonic system with leaky edge states.