A kind of novel general multiband digital predistortion (DPD) model is proposed for the linearization of the multifrequency transmitters. By the theoretical analysis, we extend the existing instantaneous sample indexed magnitude-selective affine (IMSA) function-based model to multidimensional cases, which includes the 2-D-IMSA model and the 3-D-IMSA model for concurrent dual-band and triband scenarios, respectively. The core of the new models is to use the multidimensional IMSA function to replace the complex basis function of the classic multiband model through the method of segmentation and approximation. After segmentation, the proposed models have a simple linear structure in each small area, which greatly reduces the model complexity. Experiments show that the proposed models can give similar normalized mean square error and DPD performance in comparison with existing classic models when a power amplifier is excited by two 20-MHz signals in the concurrent dual-band scenario and by three 20-MHz signals in the concurrent triband scenario.